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Nozomu, Tsuchiya*; Ikemori, Fumikazu*; Kawasaki, Kazuo*; Yamada, Rena*; Hata, Mitsuhiko*; Furuuchi, Masami*; Iwamoto, Yoko*; Kaneyasu, Naoki*; Sadanaga, Yasuhiro*; Watanabe, Takahiro; et al.
Environmental Science & Technology, 59(21), p.10400 - 10410, 2025/05
Times Cited Count:0 Percentile:0.00(Engineering, Environmental)Black carbon (BC) is a typical primary aerosol emitted from combustion. While its co-existence with iron oxides (FeO) has recently been reported, the extent of bias caused by FeO
mixing to the BC observations is largely unknown. To identify the dominant FeO
emission sources and associated overestimation of BC, magnetics properties of PM
collected at a remote site in East Asia was investigated in combination with detailed isotopic and chemical analyses. Consequently, biomass burning events did not enhance aerosol magnetism as they did for the mass concentration of BC, whereas coal burning events coincided with periods of high magnetization. Therefore, magnetization/BC ratio is proposed as a highly selective indicator for identifying combustion sources (i.e. coal, oil or biomass burning).
Thennakoon, A.*; Yokokura, Ryoga*; Yang, Y.*; Kajimoto, Ryoichi; Nakamura, Mitsutaka; Hayashi, Masahiro*; Michioka, Chishiro*; Chern, G.-W.*; Broholm, C.*; Ueda, Hiroaki*; et al.
Nature Communications (Internet), 16, p.3939_1 - 3939_13, 2025/04
Times Cited Count:0 Percentile:0.00(Multidisciplinary Sciences)Sakurai, Junya*; Torigata, Keisuke*; Matsunaga, Manabu*; Takanashi, Naoto*; Hibino, Shinya*; Kizu, Kenichi*; Morita, Akira*; Inomoto, Masahiro*; Shimohata, Nobuaki*; Toyota, Kodai; et al.
Tetsu To Hagane, 111(5), p.246 - 262, 2025/04
Rajeev, H. S.*; Hu, X.*; Chen, W.-L.*; Zhang, D.*; Chen, T.*; Kofu, Maiko*; Kajimoto, Ryoichi; Nakamura, Mitsutaka; Chen, A. Z.*; Johnson, G. C.*; et al.
Journal of the Physical Society of Japan, 94(3), p.034602_1 - 034602_14, 2025/03
Times Cited Count:0 Percentile:0.00(Physics, Multidisciplinary)Adachi, Tadashi*; Ogawa, Taiki*; Komiyama, Yota*; Sumura, Takuya*; Saito-Tsuboi, Yuki*; Takeuchi, Takaaki*; Mano, Kohei*; Manabe, Kaoru*; Kawabata, Koki*; Imazu, Tsuyoshi*; et al.
Physical Review B, 111(10), p.L100508_1 - L100508_6, 2025/03
Times Cited Count:0 Percentile:0.00(Materials Science, Multidisciplinary)Tanigawa, Masafumi; Seya, Kazuhito*; Asakawa, Naoya*; Hayashi, Hiroyuki*; Horigome, Kazushi; Mukai, Yasunobu; Kitao, Takahiko; Nakamura, Hironobu; Henzlova, D.*; Swinhoe, M. T.*; et al.
JAEA-Technology 2024-014, 63 Pages, 2025/02
The liquid waste treatment process generated sludge items at the plutonium conversion development facility. They are highly heterogeneous and contain large amounts of impurities (Na, Fe, Ni etc.). Therefore, the sludge items have very large sampling uncertainty and so the total measurement uncertainty is very large (approximately 24%). The plutonium scrap multiplicity counter (PSMC) measurement technique for sludge items was developed by joint research between the Japan Atomic Energy Agency (JAEA) and Los Alamos National Laboratory (LANL). The technical validity for sludge items using the PSMC was evaluated using various types of sample measurements and Monte Carlo N-Particle transport code calculations. The PSMC measurement parameters were found to be valid for use with sludge items and the validity of multiplicity analysis was confirmed and demonstrated through comparisons with standard MOX powder and a standard sludge. As a result, the PSMC measurement values were shown to be consistent and reasonable and the large amount of impurity (Fe, Ni etc.) did not impact the results. Therefore, the measurement uncertainty of the improved nuclear material accountancy (NMA) procedure by combined PSMC and high-resolution gamma spectrometry was shown to be 6.5%. In addition, an acceptance test was conducted using PSMC/HRGS and IAEA benchmark equipment. Measured Pu mass by both equipment agrees within the measurement uncertainty of each method, and so the validity for Pu mass measurement by PSMC/HRGS was confirmed. The above results confirm the applicability of PSMC/HRGS as an additional NMA method for sludge and a newly designed NDA procedure based on this study is applied to sludge for NMA in PCDF.
Nakamura, Satoshi; Ishii, Sho*; Kato, Hitoshi*; Ban, Yasutoshi; Hiruta, Kenta; Yoshida, Takuya; Uehara, Hiroyuki; Obata, Hiroki; Kimura, Yasuhiko; Takano, Masahide
Journal of Nuclear Science and Technology, 62(1), p.56 - 64, 2025/01
Times Cited Count:1 Percentile:51.66(Nuclear Science & Technology)A dissolution method for analyzing the elemental composition of fuel debris using the sodium peroxide (NaO
) fusion technique has been developed. Herein, two different types of simulated debris materials (such as solid solution of (Zr,RE)O
and molten core-concrete interaction products (MCCI)) were taken. At various temperatures, these debris materials were subsequently fused with Na
O
in crucibles, which are made of different materials, such as Ni, Al
O
, Fe, and Zr. Then, the fused samples are dissolved in nitric acid. Furthermore, the effects of the experimental conditions on the elemental composition analysis were evaluated using inductively coupled plasma-atomic emission spectroscopy (ICP-AES), which suggested the use of a Ni crucible at 923 K as an optimum testing condition. The optimum testing condition was then applied to the demonstration tests with Three Mile Island unit-2 (TMI-2) debris in a shielded concrete cell, thereby achieving complete dissolution of the debris. The elemental composition of TMI-2 debris revealed by the proposed dissolution method has good reproducibility and has an insignificant contradiction in the mass balance of the sample. Therefore, this newly developed reproducible dissolution method can be effectively utilized in practical applications by dissolving fuel debris and estimating its elemental composition.
Fujihara, Masayoshi; Hagihara, Masato; Koda, Akihiro*; Nakamura, Jumpei*; Matsuo, Akira*; Kindo, Koichi*; Ishikado, Motoyuki*
Physical Review Materials (Internet), 9(1), p.014406_1 - 014406_9, 2025/01
Times Cited Count:1 Percentile:82.77(Materials Science, Multidisciplinary)Tsutsui, Satoshi; Ito, Takashi; Nakamura, Jin*; Yoshida, Mio*; Kobayashi, Yoshio*; Yoda, Yoshitaka*; Nakamura, Jumpei*; Koda, Akihiro*; Higashinaka, Ryuji*; Aoki, Dai*; et al.
Interactions (Internet), 245(1), p.55_1 - 55_9, 2024/12
Tsutsui, Satoshi; Higashinaka, Ryuji*; Mizumaki, Masaichiro*; Kobayashi, Yoshio*; Nakamura, Jin*; Ito, Takashi; Yoda, Yoshitaka*; Matsuda, Tatsuma*; Aoki, Yuji*; Sato, Hideyuki*
Interactions (Internet), 245(1), p.9_1 - 9_10, 2024/12
Ito, Takashi; Higemoto, Wataru; Koda, Akihiro*; Nakamura, Jumpei*; Shimomura, Koichiro*
Interactions (Internet), 245(1), p.25_1 - 25_7, 2024/12
Shimomura, Koichiro*; Koda, Akihiro*; Pant, A. D.*; Sunagawa, Hikaru*; Fujimori, Hiroshi*; Umegaki, Izumi*; Nakamura, Jumpei*; Fujihara, Masayoshi; Tampo, Motonobu*; Kawamura, Naritoshi*; et al.
Interactions (Internet), 245(1), p.31_1 - 31_6, 2024/12
Kotegawa, Hisashi*; Nakamura, Akira*; Huyen, V. T. N.*; Arai, Yuki*; To, Hideki*; Sugawara, Hitoshi*; Hayashi, Junichi*; Takeda, Keiki*; Tabata, Chihiro; Kaneko, Koji; et al.
Physical Review B, 110(21), p.214417_1 - 214417_8, 2024/12
Times Cited Count:0 Percentile:0.00(Materials Science, Multidisciplinary)Ishikawa, Akihisa; Tanaka, Hiroki*; Nakamura, Satoshi*; Kumada, Hiroaki*; Sakurai, Yoshinori*; Watanabe, Kenichi*; Yoshihashi, Sachiko*; Tanagami, Yuki*; Uritani, Akira*; Kiyanagi, Yoshiaki*
Journal of Radiation Research (Internet), 65(6), p.765 - 775, 2024/11
Times Cited Count:0 Percentile:0.00(Biology)Koda, Yuya; Nakamura, Yasuyuki; Iguchi, Yukihiro*; Yanagihara, Satoshi*
Proceedings of 31st International Conference on Nuclear Engineering (ICONE31) (Internet), 10 Pages, 2024/11
"Fugen" has been proceeding with decommissioning work since receiving approval for the decommissioning plan in 2008, and is currently in the second step of dismantling the reactor peripheral equipment. In decommissioning, project management is important to select strategies and optimize processes, waste, safety, costs, etc. In Japan, it is expected that decommissioning work for nuclear facilities will become more serious in the future, and the knowledge and project management data obtained from the decommissioning work carried out at "Fugen" to date will be useful for planning. Since the dismantling and removal of the main turbine equipment and the peripheral equipment in preparation for the reactors have been completed so far, the actual data has been organized and analyzed and compiled into unit work coefficients. The project management data, collected during the decommissioning work carried out at "Fugen" is organized and calculated as a unit work coefficient.
Sugiura, Ayumu*; Takito, Kiyotaka; Furuya, Osamu*; Nakamura, Izumi*; Okuda, Yukihiko
Proceedings of 31st International Conference on Nuclear Engineering (ICONE31) (Internet), 8 Pages, 2024/11
Nakamura, Hiroki; Machida, Masahiko
Proceedings of 31st International Conference on Nuclear Engineering (ICONE31) (Internet), 5 Pages, 2024/11
Efficiency and safety improvements in nuclear fuel development demand a comprehensive understanding of the thermal properties of PuO. Because of difficulty of experiments at high temperatures, they have been supplemented by numerical simulations, such as density functional theory (DFT). While DFT struggles to replicate the nonmagnetic insulating ground state of PuO
, DFT+U can reproduce nonmagnetic insulating state. However, the obtained state remains less stable than magnetic states and is not the ground state. Adiabatic connection fluctuation-dissipation theory (ACFDT) is expected to be a promising solution, addressing higher-order correlations and exact exchange energies. In this study, we evaluate the ground state energy using ACFDT and find that the nonmagnetic state can be the ground state. This result successfully reproduces the observed nonmagnetic ground state of PuO
and has the potential to improve predictions of the thermal properties of nuclear fuel materials.
Yoshida, Go*; Matsumura, Hiroshi*; Nakamura, Hajime*; Miura, Taichi*; Toyoda, Akihiro*; Masumoto, Kazuyoshi*; Nakabayashi, Takayuki*; Matsuda, Makoto
Journal of Nuclear Science and Technology, 61(10), p.1298 - 1307, 2024/10
Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)Sugiura, Ayumu*; Furuya, Osamu*; Takito, Kiyotaka; Okuda, Yukihiko; Nakamura, Izumi*
Dynamics and Design Conference 2024 (D&D 2024) Koen Rombunshu, 11 Pages, 2024/09
no abstracts in English
Nakajima, Taro*; Saito, Hiraku*; Kobayashi, Naoki*; Kawasaki, Takuro; Nakamura, Tatsuya; Furukawa, Hazuki*; Asai, Shinichiro*; Masuda, Takatsugu*
Journal of the Physical Society of Japan, 93(9), p.091002_1 - 091002_5, 2024/09
Times Cited Count:2 Percentile:64.46(Physics, Multidisciplinary)