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Journal Articles

Improvement of the laboratory calibration experiment method for a borehole extensometer measurement using a straddle-sliding-packer system

Sakuma, Keisuke; Ishii, Eiichi; Aoyagi, Kazuhei; Tamura, Tomonori

Zairyo, 75(3), p.166 - 172, 2026/03

A borehole extensometer using a conventional straddle-sliding-packer system has been developed as a method for evaluating the shear compliance of a fault. In this study, we re-evaluated the laboratory experiment method for determining the compliance of the packer system which is required when applying the borehole extensometer method. The packer compliance measured by the previous method using a single packer was compared with that derived from a method using double packers, where the latter method more reproduces the actual in-situ test conditions. The results showed that the previous method using a single packer may over- or under-estimate the packer compliance, and the difference between those from the methods using a single packer and double packers is greater with smaller packer pressure. We also found that the packer compliance depends on the packer pressure and increases with decreasing packer pressure. Therefore, it is desired to conduct laboratory experiments using double packers at packer pressure close to the in-situ test conditions. The knowledge obtained by this study improves the reliability of the borehole extensometer measurement using a straddle-sliding-packer system.

JAEA Reports

Horonobe Underground Research Laboratory Project Investigation report for the 2024 fiscal year

Nakayama, Masashi; Ishii, Eiichi; Aoyagi, Kazuhei; Hayano, Akira; Murakami, Hiroaki; Ono, Hirokazu; Takeda, Masaki; Fukatsu, Yuta; Mochizuki, Akihito; Ozaki, Yusuke; et al.

JAEA-Review 2025-042, 136 Pages, 2025/12

JAEA-Review-2025-042.pdf:12.95MB

The Horonobe Underground Research Laboratory (URL) Project is being pursued by the Japan Atomic Energy Agency (JAEA) to enhance the reliability of relevant technologies for geological disposal of high-level radioactive waste through investigating the deep geological environment within the host sedimentary rocks at Horonobe-cho in Hokkaido, north Japan. In the fiscal year 2024, we continued R&D on "Study on near-field system performance in geological environment", "Demonstration of repository design options", and "Understanding of buffering behaviour of sedimentary rock to natural perturbations". These are identified as key R&D on challenges to be tackled in the Horonobe underground research plan for the fiscal year 2020 onwards. Specifically, "full-scale engineered barrier system (EBS) performance experiment" and "solute transport experiment with model testing" were carried out as part of "Study on near-field system performance in geological environment". "Demonstration of engineering feasibility of repository technology" and "evaluation of EBS behaviour over 100$$^{circ}$$C" were addressed for "Demonstration of repository design options". The validation of a method for assessing permeability using the Ductility Index and a method for estimating the state of in-situ ground pressure from hydraulic perturbation tests were investigated as part of the study "Understanding of buffering behaviour of sedimentary rock to natural perturbations". In FY2024, we continued construction of the East Access Shaft and the Ventilation Shaft, and construction of these shafts were completed to a depth of 500 m. After the completion of the East Access Shaft, excavation of the West Access Shaft and 500 m gallery has began. As of the end of FY2024, excavation progress is as follows, the East Access Shaft and the Ventilation Shaft were 500 m depth, the West Access Shaft was 472 m depth, 500 m gallery was 112.9 m, respectively. In the Horonobe International Project (HIP), Management Board and Joint Task Meeting was held at the Horonobe URL in June 2024 to review the progress of construction of galleries and preparations of experiments. Task Meetings to review the implementation plan for in-situ testing and analysis were also held. HIP will be implemented in two phases: Phase 1 (from FY2022 to FY2024) and Phase 2 (from FY2025 to FY2028), the research results of Phase 1 were compiled in FY2024.

JAEA Reports

Horonobe Underground Research Laboratory Project; Investigation program for the fiscal year 2025

Nakayama, Masashi; Ishii, Eiichi; Hayano, Akira; Aoyagi, Kazuhei; Murakami, Hiroaki; Ono, Hirokazu; Takeda, Masaki; Mochizuki, Akihito; Ozaki, Yusuke; Kimura, Shun; et al.

JAEA-Review 2025-027, 80 Pages, 2025/09

JAEA-Review-2025-027.pdf:6.22MB

The Horonobe Underground Research Laboratory Project is being pursued by the Japan Atomic Energy Agency to enhance the reliability of relevant technologies for geological disposal of high-level radioactive waste through investigating the deep geological environment within the host sedimentary rocks at Horonobe Town in Hokkaido, north Japan. In the fiscal year 2025, we continue R&D on "Study on near-field system performance in geological environment" and "Demonstration of repository design options". These are identified as key R&D challenges to be tackled in the Horonobe underground research plan for the fiscal year 2020 onwards. In the "Study on near-field system performance in geological environment", we continue to obtain data from the full-scale engineered barrier system performance experiment, and work on the specifics of the full-scale engineered barrier system dismantling experiment. As for "Demonstration of repository design options", the investigation, design, and evaluation techniques are to be systemized at various scales, from the tunnel to the pit, by means of an organized set of evaluation methodologies for confinement performance at these respective scales. Preliminary borehole investigations will be conducted within a 500 m gallery, with the objectives of obtaining rock strength and rock permeability data, as well as surveying the extent of the excavation damaged zone surrounding the test tunnel via tomographic analysis. A planning study for the in-situ construction test will be conducted to investigate the construction of backfill material and watertight plugs. The volume of water inflow associated with the excavation of the 500 m gallery will be observed, and its magnitude will be compared with the range of water inflow predicted in the analysis. The test plan to determine the extent of the excavation damaged zone around the pit, which is planned to be constructed in the 500 m gallery, will be studied to determine the in-situ excavation damaged zone. In addition, the investigation and evaluation methods for the amount of water inflow from fractures and the extent of the excavation damaged zone around the pit will be organized. Concerning the construction and maintenance of the subsurface facilities, excavation of the West Access Shaft and the 500 m gallery will continue. It is anticipated that the construction of the facilities will be completed by the end of the fiscal year 2025. In addition, we continue R&D on the following three tasks in the Horonobe International Project; Task A: Solute transport experiment with model testing, Task B: Systematic integration of repository technology options, and Task C: Full-scale engineered barrier system dismantling experiment.

Journal Articles

Development of a test system for evaluating poroelastic parameters of rocks using circumferential strain control

Morita, Mana*; Kiyama, Tamotsu*; Fukuda, Daisuke*; Aoyagi, Kazuhei; Tamura, Tomonori; Yagi, Keisuke*; Kodama, Junichi*

Shigen, Sozai Koenshu (Internet), 12(2), 5 Pages, 2025/09

no abstracts in English

Journal Articles

Observational evidence of elastic shear displacement along a minor fault in soft siliceous mudstone

Tamura, Tomonori; Ishii, Eiichi; Aoyagi, Kazuhei; Yagi, Keisuke*

Rock Mechanics and Rock Engineering, 9 Pages, 2025/00

 Times Cited Count:0 Percentile:0.00(Engineering, Geological)

Journal Articles

Degradation of a lithium cobalt oxide cathode under high voltage operation at an interface with an oxide solid electrolyte

Ito, Kotaro*; Tamura, Kazuhisa; Shimizu, Keisuke*; Yamada, Norifumi*; Watanabe, Kenta*; Suzuki, Kota*; Kanno, Ryoji*; Hirayama, Masaaki*

RSC Applied Interfaces (Internet), 1(4), p.790 - 799, 2024/04

LiCoO$$_{2}$$ is widely used as a cathode material in lithium-ion batteries. However, the reversible capacity of LiCoO$$_{2}$$ at high voltage is not well known because of the oxidative degradation of the electrolyte. In this study, a thin-film all-solid-state battery was fabricated with epitaxially grown LiCoO$$_{2}$$ cathode and Li$$_{3}$$PO$$_{4}$$ solid electrolyte as a model battery that operates stably at high voltages, ranging up to 4.6 V, without drastic degradation. However, the charge-discharge capacities of the battery decreased with cycling at 4.7 V. ${it In situ}$ synchrotron X-ray diffraction studies revealed that LiCoO$$_{2}$$ was deactivated via a change in its crystal structure to O1 type, with narrow interlayer distances, at 4.7 V. The reduced distance between the interlayers in the O1 structure possibly prevents the re-intercalation of Li ions, leading to irreversibility.

Journal Articles

Intercalative and non-intercalative photo-recharge using all-solid-state cells for solar energy conversion and storage

Yoshimoto, Masataka*; Tamura, Kazuhisa; Watanabe, Kenta*; Shimizu, Keisuke*; Horisawa, Yuhei*; Kobayashi, Takeshi*; Tsurita, Hanae*; Suzuki, Kota*; Kanno, Ryoji*; Hirayama, Masaaki*

Sustainable Energy & Fuels (Internet), 8(6), p.1236 - 1244, 2024/03

 Times Cited Count:2 Percentile:18.03(Chemistry, Physical)

Photo-rechargeable systems, which can efficiently convert and store solar energy into chemical energy within single devices, are essential to harness sunlight effectively. Photo-(de)intercalation plays a pivotal role in the functionality of photorechargeable systems. Nevertheless, the photo-(de)intercalation process has not been conclusively confirmed owing to potential interference from side reactions, such as the decomposition of liquid electrolytes and the elution of electrode materials. In this study, we successfully demonstrated photo-responsive Li$$^{+}$$-deintercalation using an all-solid-state thin-film battery comprised of epitaxially-grown anatase TiO$$_{2}$$ doped with Nb (a-TiO$$_{2}$$:Nb) as the cathode. Under light irradiation, Li$$^{+}$$-deintercalation occurred and was subsequently reversibly intercalated into a-TiO$$_{2}$$:Nb during discharge.

Journal Articles

Investigation of niobium surface roughness and hydrogen content with different polishing conditions for performance recovery of superconducting QWRs in JAEA Tokai-Tandem Accelerator

Kamiya, Junichiro; Nii, Keisuke*; Kabumoto, Hiroshi; Kondo, Yasuhiro; Tamura, Jun; Harada, Hiroyuki; Matsui, Yutaka; Matsuda, Makoto; Moriya, Katsuhiro; Ida, Yoshiaki*; et al.

e-Journal of Surface Science and Nanotechnology (Internet), 21(4), p.344 - 349, 2023/05

no abstracts in English

Journal Articles

Reports of electro-polishing implementation for quarter-wave resonators, 2

Nii, Keisuke*; Ida, Yoshiaki*; Ueda, Hideki*; Yamaguchi, Takanori*; Kabumoto, Hiroshi; Kamiya, Junichiro; Kondo, Yasuhiro; Tamura, Jun; Harada, Hiroyuki; Matsui, Yutaka; et al.

Proceedings of 19th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.601 - 604, 2023/01

no abstracts in English

Journal Articles

Reports of electropolishing implementation for quarter-wave resonators

Nii, Keisuke*; Ida, Yoshiaki*; Ueda, Hideki*; Yamaguchi, Takanori*; Kabumoto, Hiroshi; Kamiya, Junichiro; Kondo, Yasuhiro; Tamura, Jun; Harada, Hiroyuki; Matsui, Yutaka; et al.

Proceedings of 18th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.334 - 337, 2021/10

no abstracts in English

Journal Articles

Reactions of the Li$$_{2}$$MnO$$_{3}$$ cathode in an all-solid-state thin-film battery during cycling

Hikima, Kazuhiro*; Hinuma, Yoyo*; Shimizu, Keisuke*; Suzuki, Kota*; Taminato, So*; Hirayama, Masaaki*; Masuda, Takuya*; Tamura, Kazuhisa; Kanno, Ryoji*

ACS Applied Materials & Interfaces, 13(6), p.7650 - 7663, 2021/02

 Times Cited Count:23 Percentile:67.50(Nanoscience & Nanotechnology)

We evaluated the structural change of the cathode material Li$$_{2}$$MnO$$_{3}$$ that was deposited as an epitaxial film with an (001) orientation in an all-solid-state battery. In case of the electrode with LiPO$$_{4}$$ coating. Experiments revealed a structural change to a high-capacity (activated) phase that proceeded gradually and continuously with cycling. The activated phase barely showed any capacity fading. We propose a mechanism of structural change with cycling: charging to a high voltage at a sufficiently low Li concentration typically induces irreversible transition to a phase detrimental to cycling that could, but not necessarily, be accompanied by the dissolution of Mn and/or the release of O into the electrolyte, while a gradual irreversible transition to an activated phase happens at a similar Li concentration under a lower voltage.

Journal Articles

Current status of electrostatic accelerator at TIARA

Usui, Aya; Chiba, Atsuya; Yamada, Keisuke; Yokoyama, Akihito; Kitano, Toshihiko*; Takayama, Terumitsu*; Orimo, Takao*; Kanai, Shinji*; Aoki, Yuki*; Hashizume, Masashi*; et al.

Dai-28-Kai Tandemu Kasokuki Oyobi Sono Shuhen Gijutsu No Kenkyukai Hokokushu, p.117 - 119, 2015/12

no abstracts in English

Journal Articles

Present status of TIARA at JAEA

Yuyama, Takahiro; Ishibori, Ikuo; Kurashima, Satoshi; Yoshida, Kenichi; Ishizaka, Tomohisa; Chiba, Atsuya; Yamada, Keisuke; Yokoyama, Akihito; Usui, Aya; Miyawaki, Nobumasa; et al.

Proceedings of 12th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.302 - 304, 2015/09

no abstracts in English

JAEA Reports

Enhancement of the methodology of repository design and post-closure performance assessment for preliminary investigation stage, 3; Progress report on NUMO-JAEA collaborative research in FY2013 (Joint research)

Shibata, Masahiro; Sawada, Atsushi; Tachi, Yukio; Makino, Hitoshi; Wakasugi, Keiichiro; Mitsui, Seiichiro; Kitamura, Akira; Yoshikawa, Hideki; Oda, Chie; Ishidera, Takamitsu; et al.

JAEA-Research 2014-030, 457 Pages, 2015/03

JAEA-Research-2014-030.pdf:199.23MB

JAEA and NUMO have conducted a collaborative research work which is designed to enhance the methodology of repository design and post-closure performance assessment in preliminary investigation stage. With regard to (1) study on rock suitability in terms of hydrology, based on some examples of developing method of hydro-geological structure model, acquired knowledge are arranged using the tree diagram, and model uncertainty and its influence on the evaluation items were discussed. With regard to (2) study on scenario development, the developed approach for "defining conditions" has been reevaluated and improved from practical viewpoints. In addition, the uncertainty evaluation for the effect of use of cementitious material, as well as glass dissolution model, was conducted with analytical evaluation. With regard to (3) study on setting radionuclide migration parameters, based on survey of precedent procedures, multiple-approach for distribution coefficient of rocks was established, and the adequacy of the approach was confirmed though its application to sedimentary rock and granitic rock. Besides, an approach for solubility setting was developed including the procedure of selection of solubility limiting solid phase. The adequacy of the approach was confirmed though its application to key radionuclides.

JAEA Reports

Enhancement of the methodology of repository design and post-closure performance assessment for preliminary investigation stage, 2; Progress report on NUMO-JAEA collaborative research in FY2012 (Joint research)

Shibata, Masahiro; Sawada, Atsushi; Tachi, Yukio; Hayano, Akira; Makino, Hitoshi; Wakasugi, Keiichiro; Mitsui, Seiichiro; Oda, Chie; Kitamura, Akira; Osawa, Hideaki; et al.

JAEA-Research 2013-037, 455 Pages, 2013/12

JAEA-Research-2013-037.pdf:42.0MB

Following FY2011, JAEA and NUMO have conducted a collaborative research work which is designed to enhance the methodology of repository design and performance assessment in preliminary investigation stage. With regard to (1) study on rock suitability in terms of hydrology, the tree diagram of methodology of groundwater travel time has been extended for crystalline rock, in addition, tree diagram for sedimentary rock newly has been organized. With regard to (2) study on scenario development, the existing approach has been improved in terms of a practical task, and applied and tested for near field focusing on the buffer. In addition, the uncertainty of some important processes and its impact on safety functions are discussed though analysis. With regard to (3) study on setting radionuclide migration parameters, the approaches for parameter setting have been developed for sorption for rocks and solubility, and applied and tested through parameter setting exercises for key radionuclides.

Journal Articles

Development of a model to predict a radionuclide distribution based on soil migration after Fukushima Dai-ichi Nuclear Power Plant accident

Yamaguchi, Masaaki; Maekawa, Keisuke; Takeuchi, Shinji*; Kitamura, Akihiro; Onishi, Yasuo*

Genshiryoku Bakkuendo Kenkyu (CD-ROM), 20(2), p.53 - 69, 2013/12

We developed a simple novel and fast simulation model to predict a long-term distribution of $$^{137}$$Cs deposited on the land surface of Fukushima due to the Fukushima Dai-ichi Nuclear Power Plant accident triggered by a magnitude 9.0 earthquake and resulting tsunami on 11 March 2011. The model utilizes the Geographical Information System (GIS) to integrate online open data provided by individual institutes, and simulate mechanisms of soil erosion, transport and sedimentation. A preliminary calculation shows the significant deposition of sediments in lakes and reservoirs and eroded silt and clay tend to be transported downstream to river mouths than eroded sand. These results were found to be qualitatively consistent with existing data.

Journal Articles

Sorption of Eu(III) on granite; EPMA, LA-ICP-MS, batch and modeling studies

Fukushi, Keisuke*; Hasegawa, Yusuke*; Maeda, Koshi*; Aoi, Yusuke*; Tamura, Akihiro*; Arai, Shoji*; Yamamoto, Yuhei*; Aosai, Daisuke*; Mizuno, Takashi

Environmental Science & Technology, 47(22), p.12811 - 12818, 2013/11

 Times Cited Count:41 Percentile:68.82(Engineering, Environmental)

Eu(III) sorption on granite was examined by the combined microscopic and macroscopic approaches. Polished thin sections of the granite were reacted with solutions containing 10 $$mu$$M of Eu(III) and analyzed using EPMA and LA-ICP-MS. The Eu enrichment up to 6 wt.% was observed on most of the biotite grains. The Eu-enriched parts commonly lose K, which is the interlayer cation of biotite, indicating that the sorption mode is cation exchange in the interlayer. Batch Eu(III) sorption experiments on granite and biotite powders were conducted. The macroscopic sorption behavior of biotite was consistent with that of granite. The obtained sorption edges can be reproduced reasonably by the modeling considering single-site cation exchange reactions. Granite is complex mineral assemblages. However, the combined microscopic and macroscopic approaches revealed that elementary reactions by single phase can be representative for the bulk sorption reaction in complex mineral assemblages.

Journal Articles

Behavior of the energy of vibration failure experiment by using a 2-mass system model

Seki, Hajime*; Fujita, Satoshi*; Minagawa, Keisuke*; Kitamura, Seiji; Watakabe, Tomoyoshi

Dynamics and Design Conference 2013 (D&D 2013) Koen Rombunshu (USB Flash Drive), 8 Pages, 2013/08

When we study the behavior of the pipes during an earthquake, the most important damage doesn't come from the maximal load by itself, but from the accumulation of the fatigue damage caused by the repetition of the cyclic load. Therefore, from the point of view of seismic design evaluation methods, techniques that can quantitatively assess the probability of fatigue failure of mechanical structures are needed. The relationship between failure and energy is evaluated, and examined by focusing on the Energy Balance Method said to be effective as an earthquake response analysis technique in the present. This study carries out failure experiments using 2-mass system model based on Energy Balance Method. Furthermore, we focus on the strain from the vicinity of broken point as local response.

JAEA Reports

Enhancement of the methodology of repository design and post-closure performance assessment for preliminary investigation stage; Progress report on NUMO-JAEA collaborative research in FY2011 (Joint research)

Shibata, Masahiro; Sawada, Atsushi; Tachi, Yukio; Makino, Hitoshi; Hayano, Akira; Mitsui, Seiichiro; Taniguchi, Naoki; Oda, Chie; Kitamura, Akira; Osawa, Hideaki; et al.

JAEA-Research 2012-032, 298 Pages, 2012/09

JAEA-Research-2012-032.pdf:33.68MB

JAEA and NUMO have conducted a collaborative research work which is designed to enhance the methodology of repository design and performance assessment in preliminary investigation phase. The topics and the conducted research are follows; (1) Study on selection of host rock: in terms of hydraulic properties, items for assessing rock property, and assessment methodology of groundwater travel time has been organized with interaction from site investigation. (2) Study on development of scenario: the existing approach has been embodied, in addition, the phenomenological understanding regarding dissolution of and nuclide release from vitrified waste, corrosion of the overpack, long-term performance of the buffer are summarized. (3) Study on setting nuclide migration parameters: the approach for parameter setting has been improved for sorption and diffusion coefficient of buffer/rock, and applied and tested for parameter setting of key radionuclides. (4) Study on ensuring quality of knowledge: framework for ensuring quality of knowledge has been studied and examined aimed at the likely disposal facility condition.

Journal Articles

Role of cerium oxide in the enhancement of activity for the oxygen reduction reaction at Pt-CeO$$_{x}$$ nanocomposite electrocatalyst; An in situ electrochemical X-ray absorption fine structure study

Masuda, Takuya*; Fukumitsu, Hitoshi*; Fugane, Keisuke*; Togasaki, Hirotaka*; Matsumura, Daiju; Tamura, Kazuhisa; Nishihata, Yasuo; Yoshikawa, Hideki*; Kobayashi, Keisuke*; Mori, Toshiyuki*; et al.

Journal of Physical Chemistry C, 116(18), p.10098 - 10102, 2012/05

 Times Cited Count:134 Percentile:93.70(Chemistry, Physical)

In situ electrochemical X-ray absorption fine structure (XAFS) measurements were performed at the Pt L$$_{3}$$ and Ce L$$_{3}$$ edges of the Pt-CeO$$_{x}$$/C catalyst, which was prepared by a combined process of precipitation and coimpregnation methods, as well as at the Pt L$$_{3}$$ edge of the conventional Pt/C catalyst in oxygen-saturated H$$_{2}$$SO$$_{4}$$ solution to clarify the role of CeO$$_{x}$$ in the reduction of the overpotential for the oxygen reduction reaction (ORR) at the Pt-CeO$$_{x}$$ nanocomposite compared with the conventional Pt/C catalyst. XAFS measurements clearly show that the enhancement of ORR activity is attributed to the inhibition of Pt oxide formation by the CeO$$_{x}$$ layer, of which Ce$$^{3+}$$ was oxidized to Ce$$^{4+}$$ instead of Pt at the Pt oxide formation potential.

47 (Records 1-20 displayed on this page)