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Osawa, Takahito; Nagasawa, Shunsaku*; Ninomiya, Kazuhiko*; Takahashi, Tadayuki*; Nakamura, Tomoki*; Wada, Taiga*; Taniguchi, Akihiro*; Umegaki, Izumi*; Kubo, Kenya*; Terada, Kentaro*; et al.
ACS Earth and Space Chemistry (Internet), 7(4), p.699 - 711, 2023/04
Times Cited Count：7 Percentile：71.80(Chemistry, Multidisciplinary)The concentrations of carbon and other major elements in asteroid samples provide very important information on the birth of life on the Earth and the solar-system evolution. Elemental analysis using muonic X-rays is one of the best analytical methods to determine the elemental composition of solid materials, and notably, is the only method to determine the concentration of light elements in bulk samples in a non-destructive manner. We developed a new analysis system using muonic X-rays to measure the concentrations of carbon and other major elements in precious and expectedly tiny samples recovered from the asteroid Ryugu by spacecraft Hayabusa2. Here we report the development process of the system in 4 stages and their system configurations, The analysis system is composed of a stainless-steel analysis chamber, an acrylic glove box for manipulating asteroid samples in a clean environment, and Ge semiconductor detectors arranged to surround the analysis chamber. The performance of the analysis system, including the background level, which is crucial for the measurement, was greatly improved from the first stage to the later ones. Our feasibility study showed that the latest model of our muonic X-ray analysis system is capable of determining the carbon concentration in Hayabusa2's sample model with an uncertainty of less than 10 percent in a 6-day measurement.
and 
shell gap for Ti and V by the first high-precision multireflection time-of-flight mass measurements at BigRIPS-SLOWRIIimura, Shun*; Rosenbusch, M.*; Takamine, Aiko*; Tsunoda, Yusuke*; Wada, Michiharu*; Chen, S.*; Hou, D. S.*; Xian, W.*; Ishiyama, Hironobu*; Yan, S.*; et al.
Physical Review Letters, 130(1), p.012501_1 - 012501_6, 2023/01
Times Cited Count：15 Percentile：87.12(Physics, Multidisciplinary)Yamamoto, Kazami; Kinsho, Michikazu; Hayashi, Naoki; Saha, P. K.; Tamura, Fumihiko; Yamamoto, Masanobu; Tani, Norio; Takayanagi, Tomohiro; Kamiya, Junichiro; Shobuda, Yoshihiro; et al.
Journal of Nuclear Science and Technology, 59(9), p.1174 - 1205, 2022/09
Times Cited Count：8 Percentile：71.02(Nuclear Science & Technology)In the Japan Proton Accelerator Research Complex, the purpose of the 3 GeV rapid cycling synchrotron (RCS) is to accelerate a 1 MW, high-intensity proton beam. To achieve beam operation at a repetition rate of 25 Hz at high intensities, the RCS was elaborately designed. After starting the RCS operation, we carefully verified the validity of its design and made certain improvements to establish a reliable operation at higher power as possible. Consequently, we demonstrated beam operation at a high power, namely, 1 MW. We then summarized the design, actual performance, and improvements of the RCS to achieve a 1 MW beam.
Sawada, Shinichi*; Kimura, Takehiro*; Nishijima, Haruyuki*; Kodaira, Takahide*; Tanaka, Nobuyuki; Kubo, Shinji; Imabayashi, Shinichiro*; Nomura, Mikihiro*; Yamaki, Tetsuya*
International Journal of Hydrogen Energy, 45(27), p.13814 - 13820, 2020/05
Times Cited Count：3 Percentile：4.71(Chemistry, Physical)An electrochemical membrane Bunsen reaction using a cation exchange membrane (CEM) is a key to achieving an iodine-sulfur (IS) thermochemical water splitting process for mass-production of hydrogen. In this study, we prepared both the radiation-grafted CEM with a high ion exchange capacity (IEC) and the highly-porous Au-electroplated anode, and then used them for the membrane Bunsen reaction to reduce the cell overvoltage. The high-IEC grafted CEM exhibited low resistivity for proton transport, while the porous Au anode had a large effective surface area for anodic SO
oxidation reaction. As a result, the cell overvoltage for the membrane Bunsen reaction was significantly reduced to 0.21 V at 200 mA/cm
, which was only one-third of that of the previous test using the commercial CEM and non-porous anode. From the analysis of the current-voltage characteristics, employment of the grafted CEM was found to be more effective for the overvoltage reduction compared to the porous Au anode.
Nomura, Mikihiro*; Kodaira, Takahide*; Ikeda, Ayumi*; Naka, Yasuhito*; Nishijima, Haruyuki*; Imabayashi, Shinichiro*; Sawada, Shinichi*; Yamaki, Tetsuya*; Tanaka, Nobuyuki; Kubo, Shinji
Journal of Chemical Engineering of Japan, 51(9), p.726 - 731, 2018/09
Times Cited Count：3 Percentile：11.11(Engineering, Chemical)Thermochemical hydrogen production by the iodine-sulfur process decomposes water into hydrogen and oxygen by combining the chemical reactions of iodine and sulfur. Two types of acids are produced through the Bunsen reaction. To improve the performance of this reaction, ion-exchange membranes for the membrane Bunsen reaction should be developed. In the present study, a cation-exchange membrane was prepared by using a radiation-graft polymerization method. It was found that a divinylbenzene crosslinking procedure was very effective in reducing water permeation through the membrane, and the membrane Bunsen reaction was successfully carried out by using the developed crosslinked membrane. Therefore, the developed crosslinked membrane is a potential candidate for cation-exchange membranes for the membrane Bunsen reaction.
Hidaka, Akihide; Nakano, Yoshihiro; Watanabe, Yoko; Arai, Nobuyoshi; Sawada, Makoto; Kanaizuka, Seiichi*; Katogi, Aki; Shimada, Mayuka*; Ishikawa, Tomomi*; Ebine, Masako*; et al.
JAEA-Review 2016-011, 208 Pages, 2016/07
JAEA-Review-2016-011-01.pdf:33.85MBJAEA-Review-2016-011-02.pdf:27.68MB
JAEA has been conducting the Instructor Training Program (ITP) since 1996 under the auspices of MEXT to contribute to human resource development in currently 11 Asian countries in the field of radiation utilization for seeking peaceful use of nuclear energy. ITP consists of Instructor Training Course (ITC), Follow-up Training Course (FTC) and Nuclear Technology Seminars. In the ITP, trainings or seminars relating to technology for nuclear utilization are held in Japan by inviting nuclear related people from Asian countries to Japan and after that, the past trainees are supported during FTC by dispatching Japanese specialists to Asian countries. News Letter is also prepared to provide the broad range of information obtained through the trainings for local people near NPPs in Japan. The present report describes the activities of FY2014 ITP and future challenges for improving ITP more effectively.
Nakajima, Kyo*; Teramoto, Takahiro*; Akagi, Hiroshi; Fujikawa, Takashi*; Majima, Takuya*; Minemoto, Shinichiro*; Ogawa, Kanade*; Sakai, Hirofumi*; Togashi, Tadashi*; Tono, Kensuke*; et al.
Scientific Reports (Internet), 5, p.14065_1 - 14065_11, 2015/09
Times Cited Count：38 Percentile：81.49(Multidisciplinary Sciences)We report on the measurement of deep inner-shell 2p X-ray photoelectron diffraction (XPD) patterns from laser-aligned I molecules using X-ray free-electron laser (XFEL) pulses. The XPD patterns of the I molecules, aligned parallel to the polarization vector of the XFEL, were well matched with our theoretical calculations. Further, we propose a criterion for applying our molecular-structure-determination methodology to the experimental XPD data. In turn, we have demonstrated that this approach is a significant step toward the time-resolved imaging of molecular structures.
Kishida, Kiyoshi*; Hosoda, Takashi*; Sawada, Atsushi; Sato, Hisashi; Nakashima, Shinichiro*; Yasuhara, Hideaki*
Harmonising Rock Engineering and the Environment, p.1327 - 1330, 2011/10
Although it is generally known that a natural rock fracture indicates a complex aperture distribution, the fracture is an ideal representation of the parallel plate model. The cubic law is applied to evaluate the hydraulic properties of fractured rock. From several previous research works, it is known that the cubic law can be applied when the Reynolds number is less than 1.0 and that the advection term can basically be ignored in such fracture flows. In this research work, two-dimensional seepage flow analyses, using the authors' proposed 2D model which is considered with the advection term, are carried out for single fracture hydro-conductivity experiments under conditions which allow for the application of the cubic law. From the numerical results, the validity of the 2D model is discussed along with the local Reynolds number and the application of the cubic law.
Sakanaka, Shogo*; Akemoto, Mitsuo*; Aoto, Tomohiro*; Arakawa, Dai*; Asaoka, Seiji*; Enomoto, Atsushi*; Fukuda, Shigeki*; Furukawa, Kazuro*; Furuya, Takaaki*; Haga, Kaiichi*; et al.
Proceedings of 1st International Particle Accelerator Conference (IPAC '10) (Internet), p.2338 - 2340, 2010/05
Future synchrotron light source using a 5-GeV energy recovery linac (ERL) is under proposal by our Japanese collaboration team, and we are conducting R&D efforts for that. We are developing high-brightness DC photocathode guns, two types of cryomodules for both injector and main superconducting (SC) linacs, and 1.3 GHz high CW-power RF sources. We are also constructing the Compact ERL (cERL) for demonstrating the recirculation of low-emittance, high-current beams using above-mentioned critical technologies.
Kishida, Kiyoshi*; Sawada, Atsushi; Sato, Hisashi; Onda, Shinichiro*; Hosoda, Takashi*
Dai-39-Kai Gamban Rikigaku Ni Kansuru Shimpojiumu Koen Rombunshu (CD-ROM), p.287 - 292, 2010/01
no abstracts in English
Sakanaka, Shogo*; Ago, Tomonori*; Enomoto, Atsushi*; Fukuda, Shigeki*; Furukawa, Kazuro*; Furuya, Takaaki*; Haga, Kaiichi*; Harada, Kentaro*; Hiramatsu, Shigenori*; Honda, Toru*; et al.
Proceedings of 11th European Particle Accelerator Conference (EPAC '08) (CD-ROM), p.205 - 207, 2008/06
Future synchrotron light sources based on the energy-recovery linacs (ERLs) are expected to be capable of producing super-brilliant and/or ultra-short pulses of synchrotron radiation. Our Japanese collaboration team is making efforts for realizing an ERL-based hard X-ray source. We report recent progress in our R&D efforts.
-Fe and Ca-Mn exchange selectivity of kaolinite, montmorillonite, and illiteSaeki, Kazutoshi*; Wada, Shinichiro*; Shibata, Masahiro
Soil Science, 169(2), p.125 - 132, 2004/02
Times Cited Count：11 Percentile：26.54(Soil Science)The Gains-Thomas ion exchange selectivity coefficients, KGT of Fe and Mn on three types of Ca-saturated clay minerals (kaolinite, montmorillonite, and illite) were determined in an oxygen-free condition (O 
0.0001 %) in order to understand better the behaviors of these ions in anaerobic soils. The results indicate that KGT values for Ca-Fe, Ca-Mn exchange reactions on kaolinite and montmorillonite are close to unity. The KGT value for Ca-Fe exchange on illite were markedly higher than those for on the other clay minerals. The organic carbon contained in the illite specimen may have affected the results. The present study showed that Fe and Mn are adsorbed on the surface of layered silicate clay minerals, with selectivity similar to Ca. Thus, Fe and Mn behave like alkaline-earth cations such as Ca in soils, sediments and aquifers dominated by layered silicate clay minerals.
Nakano, Tomohide; Fujimoto, Takashi*; Goto, Motoshi*; Hatayama, Akiyoshi*; Kado, Shinichiro*; Kato, Takako*; Kimura, Mineo*; Kubo, Hirotaka; Murakami, Izumi*; Ono, Noriyasu*; et al.
Annual Report of National Institute for Fusion Science; April 2003 - March 2004, P. 414, 2003/10
no abstracts in English
Saeki, Kazutoshi*; Nakagawa, Kei*; Wada, Shinichiro*; Shibata, Masahiro; Horoshiro, Yoshinari*; Jinno, Kenji*
Nendo Kagaku, 42(1), p.1 - 5, 2002/08
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Konno, Azusa; Oba, Yojiro; Tominaga, Aki; Morooka, Satoshi; Ono, Naoko*; Hashimoto, Naoyuki*; Ukai, Shigeharu; Owada, Kenji*; Motokawa, Ryuhei; Kumada, Takayuki; et al.
no journal, ,
An ODS alloy is one of the promising candidate materials applicable to the fusion reactor because of its high-temperature creep strength and irradiation resistance. However, the ODS ferritic stainless steel with high Cr content sometimes suffers from the embrittlement related to phase separation below 748 K for a long term using in the reactor. It is, therefore, an important issue to understand embrittlement phenomena from not only macrostructural viewpoint but also microstructural one. Anomalous Small Angle X-ray Scattering (A-SAXS) is a unique and potential evaluation method that can analyze complex microstructure. This method can extract the signal only from an element of interest to implant the X-ray of the wavelength near orbit electron of the element. In this study, we performed both the A-SAXS analysis and TEM observation for high Cr-ODS alloy in order to assess the applicability of the A-SAXS technique as a microstructure determination and compared the A-SAXS signal with the TEM micrograph. The specimen of the commercial MA956 (Fe-20Cr-4.8Al-0.4Ti-0.02C-0.4YO
(mass%)) were thermally-aged at 748 K for 1, 10, 100 and 1000 hrs, and measured using the A-SAXS diffractometer at BL22XU in SPring-8 and a TEM. The A-SAXS data reveal that the average size of Cr precipitations increases with increasing the aging time. Also, using the A-SAXS profiles, it was estimated that there were two cases; one is the case that the microstructure does have a distinct interface between the matrix and Cr precipitate. The other case is the microstructure does not have the distinct interface. On the other hand, in TEM observation, the periodic modulated structure was observed for 10 hrs thermally-aged sample, and the sphere precipitation was confirmed for 100 hrs thermally-aged sample. It was suggested that there would be a crucial phase separation mode from spinodal decomposition to nucleation-growth between 10 and 100 hrs.
Sudo, Tomoyuki; Ishikawa, Hiroyasu; Uesaka, Takahiro*; Sonoda, Takashi; Ishikawa, Nobuyuki*; Niizato, Tadafumi; Mikake, Shinichiro; Aoki, Isao; Ishizaki, Nobuhiro; Imamura, Hiroaki; et al.
no journal, ,
JAEA is working the decontamination activity for the environmental remediation of Fukushima. In this activity, I support the decontamination activity for local governments to devise a decontamination plan and actually decontaminate. In this report, 1 introduce the technical knowhow for the decontamination activity of a house.
Nakashima, Yosuke*; Ichimura, Kazuya*; Takeda, Hisahito*; Iwamoto, Miki*; Hosoda, Yasunari*; Shimizu, Keita*; Oki, Kensuke*; Sakamoto, Mizuki*; Ono, Noriyasu*; Kado, Shinichiro*; et al.
no journal, ,
no abstracts in English
Sakurai, Takeshi; Yabuuchi, Yukiko; Arai, Nobuyoshi; Sawada, Makoto; Yamashita, Kiyonobu; Sato, Nobuyuki; Torata, Shinichiro; Kanaizuka, Seiichi; Nakamura, Kazuyuki
no journal, ,
Outline of the Instructor Training Program, which is contracted with MEXT, for ten countries in Asia, and status of the Follow-up Training Course, which is one of the three major courses and conducted in Asian countries, will be reported.
Sumiya, Masato; Ikeda, Koki; Sonoda, Takashi; Niizato, Tadafumi; Mikake, Shinichiro; Abe, Hironobu; Inoue, Makoto; Eguchi, Kazutoshi; Kozawa, Masachiyo; Terunuma, Akihiro; et al.
no journal, ,
no abstracts in English
