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Suzuki, Kenji*; Miura, Yasufumi*; Toyokawa, Hidenori*; Shiro, Ayumi*; Shobu, Takahisa; Morooka, Satoshi; Shibayama, Yuki
Quantum Beam Science (Internet), 9(2), p.15_1 - 15_15, 2025/06
-rays from slow neutron-induced fission of
U with STEFFWright, T.*; Harada, Hideo; Kimura, Atsushi; 121 of others*
European Physical Journal A, 60(3), p.70_1 - 70_11, 2024/03
Times Cited Count:0 Percentile:0.00(Physics, Nuclear)
,
, and X-rays (Contract research); FY2022 Nuclear Energy Science & Technology and Human Resource Development ProjectCollaborative Laboratories for Advanced Decommissioning Science; Japan Chemical Analysis Center*
JAEA-Review 2023-022, 93 Pages, 2023/12
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2022. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2020, this report summarizes the research results of the "Development of rapid and sensitive radionuclide analysis method by simultaneous analysis of
,
, and X-rays" conducted from FY2020 to FY2022. The present study aims to enable rapid analysis of radionuclides in fuel debris and waste, we have established the latest measurement system, such as the multiple
-ray detection methods, and the Spectral Determination Method (hereinafter referred to as "SDM") was developed. In the research in 2022, we developed a code that handles measurement data of LSC, singles Ge, and 2D spectra (multiple
). In addition, to develop an integrated database, spectral data of 40 nuclides were obtained by actual measurements and simulation calculations.
Iyota, Muneyoshi*; Matsuda, Tomoki*; Sano, Tomokazu*; Shigeta, Masaya*; Shobu, Takahisa; Yumoto, Hirokatsu*; Koyama, Takahisa*; Yamazaki, Hiroshi*; Semba, Yasunori*; Ohashi, Haruhiko*; et al.
Journal of Manufacturing Processes, 94, p.424 - 434, 2023/05
Times Cited Count:8 Percentile:64.94(Engineering, Manufacturing)
/
/
-rays radiolysis (Contract research); FY2021 Nuclear Energy Science & Technology and Human Resource Development ProjectCollaborative Laboratories for Advanced Decommissioning Science; Tohoku University*
JAEA-Review 2022-069, 114 Pages, 2023/03
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2021. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station (1F), Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2020, this report summarizes the research results of the "Development of a new corrosion mitigation technology using nanobubbles toward corrosion mitigation in PCV system under the influence of
/
/
-rays radiolysis" conducted in FY2021. In this work, in order to ensure the long-term reliability of steel structures that ensure important confinement functions in the debris removal process, such as existing PCVs and newly constructed negative pressure maintenance systems and piping, corrosion phenomena in wet environments where
- and
-ray emitting nuclides come into contact with steel are clarified for the first time.
,
, and X-rays (Contract research); FY2021 Nuclear Energy Science & Technology and Human Resource Development ProjectCollaborative Laboratories for Advanced Decommissioning Science; Japan Chemical Analysis Center*
JAEA-Review 2022-037, 118 Pages, 2023/01
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2021. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2020, this report summarizes the research results of the "Development of rapid and sensitive radionuclide analysis method by simultaneous analysis of
,
, and X-rays" conducted in FY2021. The present study aims to enable rapid analysis of radionuclides in fuel debris and waste, we have established the latest measurement system, such as the multiple
-ray detection methods, and the Spectral Determination Method (hereafter referred to "SDM") was developed. In the study, the
-ray measuring device was installed, and the measurement system consisting of the Ge detector, CeBr
detector, and NaI detector was completed in FY2021. In the SDM development, standard spectra of
-ray singles, multiple
-ray measurements, …
/
/
-rays radiolysis (Contract research); FY2020 Nuclear Energy Science & Technology and Human Resource Development ProjectCollaborative Laboratories for Advanced Decommissioning Science; Tohoku University*
JAEA-Review 2022-002, 85 Pages, 2022/06
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2020. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2020, this report summarizes the research results of the "Development of a new corrosion mitigation technology using nanobubbles toward corrosion mitigation in PCV system under the influence of
/
/
-rays radiolysis" conducted in FY2020. In this work, in order to ensure the long-term reliability of steel structures that ensure important confinement functions in the debris removal process, such as existing PCVs and newly constructed negative pressure maintenance systems and piping, corrosion phenomena in wet environments where
- and
-ray emitting nuclides come into contact with steel are clarified for the first time.
,
, and X-rays (Contract research); FY2020 Nuclear Energy Science & Technology and Human Resource Development ProjectCollaborative Laboratories for Advanced Decommissioning Science; Japan Chemical Analysis Center*
JAEA-Review 2021-060, 105 Pages, 2022/03
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2020. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2020, this report summarizes the research results of the "Development of rapid and sensitive radionuclide analysis method by simultaneous analysis of
,
, and X-rays" conducted in FY2020. The present study aims to enable rapid analysis of radionuclides in fuel debris and waste, and develops the measurement system such as multiple
-ray detection method. We develop a spectral determination method (SDM method) for integrated analysis by constructing a spectral database for nuclides including
-rays and X-rays by measurement using this system and radiation simulation calculation. This method enables simultaneous quantification of multiple nuclides and reduces the chemical separation process.
spectrometry of terrestrial gamma rays using portable germanium detectors in area of 80 km radius around the Fukushima Daiichi Nuclear Power PlantMikami, Satoshi; Tanaka, Hiroyuki*; Okuda, Naotoshi*; Sakamoto, Ryuichi*; Ochi, Kotaro; Uno, Kiichiro*; Matsuda, Norihiro; Saito, Kimiaki
Nihon Genshiryoku Gakkai Wabun Rombunshi, 20(4), p.159 - 178, 2021/12
In order to know the background radiation level where the area affected by the Fukushima Daiichi Nuclear Power Plant accident in 2011, terrestrial gamma rays had been measured by using portable germanium detectors repeatedly from 2013 through 2019, at 370 locations within 80 km radius area centered on the Fukushima Daiichi Nuclear Power Plant. Radioactive concentrations of Uranium 238, Thorium 232, Potassium 40 and kerma rates in air due to terrestrial gamma rays were obtained at those locations based on the method of ICRU report 53. Averaged concentrations of
U,
Th and
K were 18.8, 22.7, 428 Bq/kg, respectively, and kerma rate in air over the area was found to be 0.0402
Gy/h. The obtained kerma rates in air were compared to those reported in literatures. It was confirmed that the data were correlated with each other, and were agreed within the range of their uncertainty. This is because the kerma rate in air due to terrestrial gamma rays is depend on geology. The similar trend to previous findings was observed that the kerma rate in air at locations geologically classified as Mesozoic era, Granite and Rhyolite were statistically significantly higher than the others.
Nakamura, Keisuke; Morishita, Yuki; Takasaki, Koji; Maehata, Keisuke*; Sugimoto, Tetsuya*; Kiguchi, Yu*; Iyomoto, Naoko*; Mitsuda, Kazuhisa*
Journal of Low Temperature Physics, 193(3-4), p.314 - 320, 2018/11
Times Cited Count:0 Percentile:0.00(Physics, Applied)
Se(
, n) cross section and uncertainty evaluation of the
Se(n,
) cross sectionKitatani, Fumito; Harada, Hideo; Goko, Shinji*; Iwamoto, Nobuyuki; Utsunomiya, Hiroaki*; Akimune, Hidetoshi*; Toyokawa, Hiroyuki*; Yamada, Kawakatsu*; Igashira, Masayuki*
Journal of Nuclear Science and Technology, 53(4), p.475 - 485, 2016/04
Times Cited Count:5 Percentile:39.05(Nuclear Science & Technology)Sato, Shigeo*; Shobu, Takahisa; Sato, Kozue*; Ogawa, Hiromi*; Wagatsuma, Kazuaki*; Kumagai, Masayoshi*; Imafuku, Muneyuki*; Tashiro, Hitoshi*; Suzuki, Shigeru*
ISIJ International, 55(7), p.1432 - 1438, 2015/07
Times Cited Count:14 Percentile:51.86(Metallurgy & Metallurgical Engineering)To characterize the distribution and anisotropy of dislocations in cold-drawn pearlitic steel wires, X-ray diffraction line-profile analysis was performed using synchrotron radiation micro-beams. The plastic shear strain was generally more severe near the surface than the center of the wire, whereas the dislocation density distribution was almost constant from the center to the surface. On the other hand, the dislocation rearrangement, which evolves the dislocation cell structure, progressed closer to the surface. It was also revealed that a difference between the hardness in axial and transverse wire directions could be explained by anisotropic dislocation density. Line-profile analysis based on diffraction data at elevated temperatures was performed. Whereas the cementite recovery progressed at a constant rate, the ferrite phase recovery rate was temperature-dependent, suggesting that the ferrite phase recovery was less related to that of the cementite phase.
Yokoseki, Takashi; Abe, Hiroshi; Makino, Takahiro; Onoda, Shinobu; Tanaka, Yuki*; Kandori, Mikio*; Yoshie, Toru*; Hijikata, Yasuto*; Oshima, Takeshi
Materials Science Forum, 821-823, p.705 - 708, 2015/07
Shibano, Junichi*; Kajiwara, Kentaro*; Tsukamoto, Takuya*; Kawai, Hirokazu*; Miura, Setsuo*; Zhang, S.*; Shobu, Takahisa; Kobayashi, Michiaki*
Materials Science Forum, 777, p.176 - 181, 2014/02
Times Cited Count:2 Percentile:50.61(Materials Science, Multidisciplinary)Yokoya, Akinari; Fujii, Kentaro; Ushigome, Takeshi; Shikazono, Naoya; Urushibara, Ayumi; Watanabe, Ritsuko
Radiation Protection Dosimetry, 122(1-4), p.86 - 88, 2006/12
Times Cited Count:13 Percentile:64.33(Environmental Sciences)We have studied yields of DNA damages induced by soft X-rays obtained from a conventional soft X-ray machine in a LET region between
-rays and ultrasoft X-rays. Practically soft X-rays with a broad energy spectrum emitted from a target of heavy metal, such as tungsten, have been widely used not only for radiobiological experiments but also for medical application such as mammography. Radiation weighting factors for these soft X-rays have been assigned to be 1 by ICRP. However, the fraction of a large number of low energy photons in the spectrum (below several tens keV) provided by bremsstrahlung is expected to be more effective for DNA damage induction than
-rays since low energy photo- and Auger electrons predominantly ejected in consequence of a photoelectric effect can produce dense clusters of ionization/excitation on DNA molecules. We have examined the yield of DNA strand breaks induced by white soft X-rays (150 kVp, tungsten target). Yields of base lesions revealed by base excision repair enzymes will be also presented.
(Ce) scintillation detector applications for environmental
-ray measurements of low to high dose ratesTsutsumi, Masahiro; Tanimura, Yoshihiko
Nuclear Instruments and Methods in Physics Research A, 557(2), p.554 - 560, 2006/02
Times Cited Count:16 Percentile:71.14(Instruments & Instrumentation)A new cerium-doped LaCl
(Ce) scintillator is evaluated with respect to the application in environmental
-ray dosimetry and spectrometry. The scintillator is very attractive for
-ray spectrometry in the case of high count rate, because it has excellent energy resolution and fast decay time. The performance characteristics of a scintillator with a 25.4 mm
25.4 mm LaCl
(Ce) crystal are studied and compared to those of a NaI(Tl) scintillator with the same size crystal. Acquired pulse-height spectra are converted to dose rates by using the G(E) function method. Though the LaCl
(Ce) crystal itself produces a rather high background in the crystal itself, the scintillator provides good energy information and dose-rate readings from low to high-level (several mGy/h) by subtracting the self-background. The properties of LaCl
(Ce) scintillator suggest that the scintillator could be a promising candidate for monitoring at high-dose levels as in emergencies, as well as at ordinary levels of background radiation.
Taguchi, Mitsumasa; Kojima, Takuji
JAEA-Review 2005-001, TIARA Annual Report 2004, p.181 - 182, 2006/01
The yields of OH radicals in water containing phenol have been investigated for several ten MeV/n C ion and Ne ion having the same LET value, as a function of the residual ion energy at the specific depth in water. In this study, beside such energy dependence, the dependence of reaction time of OH radical yield was examined by changing the concentration of phenol as solute. The defferential G'-values of OH radicals, those G-values per kinetic energy of ions increase with specific energy of Ne ions. The G'-value just after irradiation(1.5ns) is relatively high but become lower with reaction time to be the value (2.7) obtained for
Co
-rays. It suggests the diffusion behavior of OH radicals locally induced in water.
-nonylphenols in water and elimination of their estrogen activities by
Co
-ray irradiationKimura, Atsushi; Taguchi, Mitsumasa; Otani, Yoshimi*; Takigami, Machiko; Shimada, Yoshitaka*; Kojima, Takuji; Hiratsuka, Hiroshi*; Namba, Hideki
Radiation Physics and Chemistry, 75(1), p.61 - 69, 2006/01
Times Cited Count:13 Percentile:64.33(Chemistry, Physical)Decomposition of
-Nonylphenols (NPs) in water at 1
mol dm
was decreased exponentially with absorbed dose when NPs were irradiated by
Co
-rays. Two products having molecular weight of 236, presumably OH adducts of NPs, were detected by LC-MS analyses. The elimination of estrogen activity of aqueous NPs solution including such irradiation products at 5000 Gy (J kg
) was confirmed by the yeast two hybrid assay. These results should expand the application of ionizing radiation to the treatment of NPs.
Shibata, Yasushi*; Yamamoto, Kazuyoshi; Matsumura, Akira*; Yamamoto, Tetsuya*; Hori, Naohiko; Kishi, Toshiaki; Kumada, Hiroaki; Akutsu, Hiroyoshi*; Yasuda, Susumu*; Nakai, Kei*; et al.
JAERI-Research 2005-009, 41 Pages, 2005/03
The measurement of neutron flux and boron concentration in the blood during medical irradiation is indispensable in order to evaluate the radiation in boron neutron capture therapy. It is, however, difficult to measure the blood boron concentration during neutron irradiation because access to the patient is limited. Therefore we prospectively investigated the predictability of blood boron concentrations using the data obtained at the first craniotomy after infusion of a low dosage of BSH. When the test could not be carried out, the blood boron concentration during irradiation was also predicted by using the 2-compartment model. If the final boron concentration after the end of the infusion is within 95% confidence interval of the prediction, direct prediction from biexponential fit will reduce the error of blood boron concentrations during irradiation to around 6%. If the final boron concentration at 6 or 9 hours after the end of infusion is out of 95% confidence interval of the prediction, proportional adjustment will reduce error and expected error after adjustment to around 12%.
Solomon, H. M.*; Kojima, Takuji
Nucleus, 33, p.16 - 20, 2005/00
Low-dose dosimeters were developed based on the mixture films of polyvinyl butyral (PVB) and the acid-sensitive dye leucomalachite green (LMG). Chloral hydrate (RX) was added to the mixture for enhancement of the radiation sensitivity of the film dosimeters. Different film dosimeter materials were prepared using 9.07
10
mole LMG per one gram PVB with various RX:LMG molar concentration ratio. The dosimeter response, which is expressed in terms of change in absorbance at 628 nm per unit thickness, increased linearly with dose and RX concentration. The PVB-LMG dosimeter system, in which the ratio of RX concentration to that of LMG is higher than 10, show measurable dose range of 1-100 Gy for
Co
-rays.