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Status of neutron spectrometers at J-PARC

梶本 亮一; 横尾 哲也*; 中村 充孝; 川北 至信; 松浦 直人*; 遠藤 仁*; 瀬戸 秀紀*; 伊藤 晋一*; 中島 健次; 河村 聖子

Physica B; Condensed Matter, 562, p.148 - 154, 2019/06

Seven time-of-flight quasielastic/inelastic neutron scattering instruments are installed on six beamlines in the Materials and Life Science Experimental Facility (MLF) at the Japan Proton Accelerator Research Complex (JPARC). Four of these instruments are chopper-type direct-geometry spectrometers, one is a near-backscattering indirect-geometry spectrometer, and the other two are spin-echo-type spectrometers. This paper reviews the characteristic features, recent scientific outcomes, and progress in development of MLF spectrometers.


Phase-transition kinetics of magnetic skyrmions investigated by stroboscopic small-angle neutron scattering

中島 多朗*; 稲村 泰弘; 伊藤 崇芳*; 大石 一城*; 大池 広志*; 賀川 史敬*; 吉川 明子*; 田口 康二郎*; 加倉井 和久*; 十倉 好紀*; et al.

Physical Review B, 98(1), p.014424_1 - 014424_5, 2018/07

 被引用回数:1 パーセンタイル:59.26(Materials Science, Multidisciplinary)



Proceedings of the MLF User Group Meeting on Direct Geometry Spectrometers (DIRECTION 2017); October 16-17, 2017, Ibaraki Quantum Beam Research Center (Tokai, Ibaraki, Japan)

梶本 亮一; 横尾 哲也*; 蒲沢 和也*; 中村 充孝; 河村 聖子; 伊藤 晋一*; 中島 健次

JAEA-Review 2017-031, 107 Pages, 2018/02


平成29年10月16日$$sim$$17日の2日間にわたり、いばらき量子ビーム研究センターにおいて、J-PARC物質・生命科学実験施設(MLF)の4台の直接配置型(チョッパー型)中性子分光器合同のユーザーミーティング「DIRECTION 2017」が開催された。4台の装置とは4SEASONS (BL01), HRC (BL12), AMATERAS (BL14), POLANO (BL23)であり、本ミーティングはこれらの装置におけるユーザー利用の活性化に向けて、J-PARC MLF, 高エネルギー加速器研究機構物質構造科学研究所, 総合科学研究機構の共催で開催されたものである。本ミーティングでは各装置、試料環境、ソフトウェアの最新状況に加え、各装置における最近の実験およびデータ解析の例が幅広い研究分野にわたって紹介された。本報告書はこのミーティングの講演要旨および講演で使用された発表資料を収録したものである。


Neutron scattering study of yttrium iron garnet

社本 真一; 伊藤 孝; 大西 弘明; 山内 宏樹; 稲村 泰弘; 松浦 直人*; 赤津 光洋*; 樹神 克明; 中尾 朗子*; 茂吉 武人*; et al.

Physical Review B, 97(5), p.054429_1 - 054429_9, 2018/02

 被引用回数:1 パーセンタイル:100(Materials Science, Multidisciplinary)



Materials and Life Science Experimental Facility (MLF) at the Japan Proton Accelerator Research Complex, 2; Neutron scattering instruments

中島 健次; 川北 至信; 伊藤 晋一*; 阿部 淳*; 相澤 一也; 青木 裕之; 遠藤 仁*; 藤田 全基*; 舟越 賢一*; Gong, W.*; et al.

Quantum Beam Science (Internet), 1(3), p.9_1 - 9_59, 2017/12



New precise measurement of muonium hyperfine structure interval at J-PARC

上野 恭裕*; 青木 正治*; 深尾 祥紀*; 東 芳隆*; 樋口 嵩*; 飯沼 裕美*; 池戸 豊*; 石田 啓一*; 伊藤 孝; 岩崎 雅彦*; et al.

Hyperfine Interactions, 238(1), p.14_1 - 14_6, 2017/11

 被引用回数:1 パーセンタイル:17.79

MuSEUM is an international collaboration aiming at a new precise measurement of the muonium hyperfine structure at J-PARC (Japan Proton Accelerator Research Complex). Utilizing its intense pulsed muon beam, we expect a ten-fold improvement for both measurements at high magnetic field and zero magnetic field. We have developed a sophisticated monitoring system, including a beam profile monitor to measure the 3D distribution of muonium atoms to suppress the systematic uncertainty.


Turbulent transport reduction induced by transition on radial electric field shear and curvature through amplitude and cross-phase in torus plasma

小林 達哉*; 伊藤 公孝*; 井戸 毅*; 神谷 健作*; 伊藤 早苗*; 三浦 幸俊; 永島 芳彦*; 藤澤 彰英*; 稲垣 滋*; 居田 克巳*

Scientific Reports (Internet), 7(1), p.14971_1 - 14971_8, 2017/11

 被引用回数:4 パーセンタイル:27.2(Multidisciplinary Sciences)

Spatiotemporal evolutions of radial electric field and turbulence are measured simultaneously in the H-mode transition, which is a prototypical example of turbulence structure formation in high-temperature plasmas. In the dynamical phase where transport barrier is established abruptly, the time-space-frequency-resolved turbulent particle flux is obtained. Here we report the validation of the mechanism of transport barrier formation quantitatively. It is found that the particle flux is suppressed predominantly by reducing density fluctuation amplitude and cross phase between density fluctuation and potential fluctuation. Both radial electric field shear and curvature are responsible for the amplitude suppression as was predicted by theory. Turbulence amplitude reduction immediately responds to the growth of the radial electric field non-uniformity and saturates, while cross phase continuously approaches zero.


Reduction and resource recycling of high-level radioactive wastes through nuclear transmutation; Isolation techniques of Pd, Zr, Se and Cs in simulated high level radioactive waste using solvent extraction

佐々木 祐二; 森田 圭介; 伊藤 圭祐; 鈴木 伸一; 塩飽 秀啓; 高橋 優也*; 金子 昌章*; 大森 孝*; 浅野 和仁*

Proceedings of International Nuclear Fuel Cycle Conference (GLOBAL 2017) (USB Flash Drive), 4 Pages, 2017/09

高レベル廃液中のPd, Zr, Se, Csは長半減期核種のPd-107, Zr-93, Se-79, Cs-135を有している。高レベル廃液から除去し、核変換により処分することで、環境負荷低減に役立てることができる。これら元素について、PdはMIDOA, NTAアミド、Csはクラウンエーテル、ZrはTODGA, HDEHP, Seはフェニレンジアミンで抽出可能である。それぞれ元素の回収条件について検討した成果について述べる。


Materials and Life Science Experimental Facility at the Japan Proton Accelerator Research Complex, 3; Neutron devices and computational and sample environments

坂佐井 馨; 佐藤 節夫*; 瀬谷 智洋*; 中村 龍也; 藤 健太郎; 山岸 秀志*; 曽山 和彦; 山崎 大; 丸山 龍治; 奥 隆之; et al.

Quantum Beam Science (Internet), 1(2), p.10_1 - 10_35, 2017/09



Spin wave dispersion just above the magnetic order-order transition in the metallic antiferromagnet Mn$$_{3}$$Pt

井深 壮史*; 横尾 哲也*; 伊藤 晋一*; 蒲沢 和也*; 中村 充孝; 今井 基晴*

Journal of Physics; Conference Series, 868(1), p.012017_1 - 012017_6, 2017/07



Fine dispersion of Pt$$_{4-5}$$ subnanoclusters and Pt single atoms over porous carbon supports and their structural analyses with X-ray absorption spectroscopy

糸井 弘行*; 西原 洋知*; 小林 俊介*; Ittisanronnachai, S.*; 石井 孝文*; Berenguer, R.*; 伊藤 仁*; 松村 大樹; 京谷 隆*

Journal of Physical Chemistry C, 121(14), p.7892 - 7902, 2017/04

 被引用回数:9 パーセンタイル:23.94(Chemistry, Physical)

We demonstrate the fine dispersion of Pt$$_{4-5}$$ subnanoclusters or Pt single atoms on two types of porous carbon supports, Ketjen black (KB) and zeolite-templated carbon (ZTC). For the fine dispersion of Pt subnanoclusters, simply filling an organoplatinum complex, (COD)PtMe$$_{2}$$, as a Pt precursor into the micropores is found to be crucial to prevent agglomeration or sintering of Pt subnanoclusters. Moreover, it is possible to disperse Pt single atoms on ZTC, simply by decreasing the Pt loading amount down to ca. 0.9 wt%, owing to some stabilization effect by oxygen-containing functional groups. Extended X-ray absorption fine structure (EXAFS) analysis for Pt subnanoclusters reveals that the Pt-Pt bond is contracting to a large extent ($$sim$$2.8%) relative to balk values, and upon hydrogen chemisorption, the bond elongates more than the reported values for the 1.0 nm sized Pt nanoparticles.


Development of prototype reactor maintenance, 1; Application to piping system of sodium-cooled reactor prototype

小竹 庄司*; 近澤 佳隆; 高屋 茂; 大高 雅彦; 久保 重信; 荒井 眞伸; 桾木 孝介; 伊藤 隆哉*; 山口 彰*

Proceedings of 2017 International Congress on Advances in Nuclear Power Plants (ICAPP 2017) (CD-ROM), 6 Pages, 2017/04



Development of prototype reactor maintenance, 2; Application to piping support of sodium-cooled reactor prototype

荒井 眞伸; 桾木 孝介; 相澤 康介; 近澤 佳隆; 高屋 茂; 久保 重信; 小竹 庄司*; 伊藤 隆哉*; 山口 彰*

Proceedings of 2017 International Congress on Advances in Nuclear Power Plants (ICAPP 2017) (CD-ROM), 6 Pages, 2017/04




佐藤 稔紀; 笹本 広; 石井 英一; 松岡 稔幸; 早野 明; 宮川 和也; 藤田 朝雄*; 棚井 憲治; 中山 雅; 武田 匡樹; et al.

JAEA-Research 2016-025, 313 Pages, 2017/03




Uniaxial pressure effect on the magnetic ordered moment and transition temperatures in BaFe$$_{2-x}$$T$$_{x}$$As$$_{2}$$ ($$T$$ = Co,Ni)

Tam, D. M.*; Song, Y.*; Man, H.*; Cheung, S. C.*; Yin, Z.*; Lu, X.*; Wang, W.*; Frandsen, B. A.*; Liu, L.*; Gong, Z.*; et al.

Physical Review B, 95(6), p.060505_1 - 060505_6, 2017/02

 被引用回数:8 パーセンタイル:25.41(Materials Science, Multidisciplinary)

We use neutron diffraction and muon spin relaxation to study the effect of in-plane uniaxial pressure on the antiferromagnetic (AF) orthorhombic phase in BaFe$$_{2-x}$$T$$_{x}$$As$$_{2}$$ and its Co- and Ni-substituted members near optimal superconductivity. In the low-temperature AF ordered state, uniaxial pressure necessary to detwin the orthorhombic crystals also increases the magnetic ordered moment, reaching an 11% increase under 40 MPa for BaFe$$_{1.9}$$Co$$_{0.1}$$As$$_2$$, and a 15% increase for BaFe$$_{1.915}$$Ni$$_{0.085}$$As$$_2$$. We also observe an increase of the AF ordering temperature ($$T_N$$) of about 0.25 K/MPa in all compounds, consistent with density functional theory calculations that reveal better Fermi surface nesting for itinerant electrons under uniaxial pressure. The doping dependence of the magnetic ordered moment is captured by combining dynamical mean field theory with density functional theory, suggesting that the pressure-induced moment increase near optimal superconductivity is closely related to quantum fluctuations and the nearby electronic nematic phase.


Inelastic and quasi-elastic neutron scattering spectrometers in J-PARC

瀬戸 秀紀; 伊藤 晋一; 横尾 哲也*; 遠藤 仁*; 中島 健次; 柴田 薫; 梶本 亮一; 河村 聖子; 中村 充孝; 川北 至信; et al.

Biochimica et Biophysica Acta; General Subjects, 1861(1), p.3651 - 3660, 2017/01

 被引用回数:12 パーセンタイル:10.37(Biochemistry & Molecular Biology)



Excited configurations of hydrogen in the BaTiO$$_{3-x}$$H$$_x$$ perovskite lattice associated with hydrogen exchange and transport

伊藤 孝; 幸田 章宏*; 下村 浩一郎*; 髭本 亘; 松崎 禎市郎*; 小林 洋治*; 陰山 洋*

Physical Review B, 95(2), p.020301_1 - 020301_5, 2017/01

 被引用回数:2 パーセンタイル:66.33(Materials Science, Multidisciplinary)

Excited configurations of hydrogen in the oxyhydride BaTiO$$_{3-x}$$H$$_x$$ ($$x=0.1-0.5$$), which are considered to be involved in its hydrogen transport and exchange processes, were investigated by $$mu^+$$SR spectroscopy using muonium (Mu) as a pseudoisotope of hydrogen. Muons implanted into BaTiO$$_{3-x}$$H$$_x$$ were mainly found in two metastable states. One was assigned to a highly mobile interstitial protonic state, which is commonly observed in perovskite oxides. The other was found to form an entangled two spin-$$frac{1}{2}$$ system with the nuclear spin of an H$$^-$$ ion at the anion site. The structure of the (H,Mu) complex agrees well with that of a neutralized center containing two H$$^-$$ ions at a doubly charged oxygen vacancy, which was predicted to form in SrTiO$$_{3-delta}$$ by a computational study. Above 100 K, interstitial Mu$$^+$$ diffusion and retrapping to a deep defect were observed, which could be a rate-limiting step of macroscopic Mu/H transport in BaTiO$$_{3-x}$$H$$_x$$.


New muonium HFS measurements at J-PARC/MUSE

Strasser, P.*; 青木 正治*; 深尾 祥紀*; 東 芳隆*; 樋口 嵩*; 飯沼 裕美*; 池戸 豊*; 石田 啓一*; 伊藤 孝; 岩崎 雅彦*; et al.

Hyperfine Interactions, 237(1), p.124_1 - 124_9, 2016/12

 被引用回数:3 パーセンタイル:10.17

At the Muon Science Facility (MUSE) of J-PARC (Japan Proton Accelerator Research Complex), the MuSEUM collaboration is planning new measurements of the ground state hyperfine structure (HFS) of muonium both at zero field and at high magnetic field. The previous measurements were performed both at LAMPF (Los Alamos Meson Physics Facility) with experimental uncertainties mostly dominated by statistical errors. The new high intensity muon beam that will soon be available at MUSE H-Line will provide an opportunity to improve the precision of these measurements by one order of magnitude. An overview of the different aspects of these new muonium HFS measurements, the current status of the preparation, and the results of a first commissioning test experiment at zero field are presented.


Statistical analysis using the Bayesian nonparametric method for irradiation embrittlement of reactor pressure vessels

高見澤 悠; 伊藤 裕人; 西山 裕孝

Journal of Nuclear Materials, 479, p.533 - 541, 2016/10

 パーセンタイル:100(Materials Science, Multidisciplinary)

高中性子照射量領域における照射脆化に関して、ノンパラメトリックベイズ法を用いて日本国内の監視試験データや試験炉照射データに対して統計解析を実施した。ノンパラメトリックベイズ法は実測データを正規分布の和で表す解析手法であり、正規分布の数と平均値や分散は実測データの複雑さに応じて決定される。本研究では、照射脆化の主因として考えられている溶質原子クラスタを構成する元素(Cu, Ni, Mn, Si, P)や照射条件を入力パラメータとして、照射脆化との関係を評価した。解析の結果、中性子照射量が異なるデータであっても同じ材料のデータは同じ正規分布に分類されており、中性子照射量に依存した脆化メカニズムが顕在化していないことが示唆された。


Electronic structure of hydrogen donors in semiconductors and insulators probed by muon spin rotation

下村 浩一郎*; 伊藤 孝

Journal of the Physical Society of Japan, 85(9), p.091013_1 - 091013_5, 2016/09

 パーセンタイル:100(Physics, Multidisciplinary)

Hydrogen in semiconductors and insulators plays a crucial role in their electric conductivity. Substantial experimental and theoretical efforts have been made to establish this hypothesis in the last decade, and the muon spin rotation technique has played a pioneering role. Positive muons implanted into such low-carrier systems often form a muonium (a hydrogen analogue). Although its dynamical aspect may be different from the heavier hydrogen, the electronic structure of the muonium is expected to be identical to that of hydrogen after a small correction of the reduced mass. Since the discovery of a shallow muonium in CdS, its properties have been intensively studied in many semiconductors and insulators, and then it was interpreted as a possible origin of $$n$$-type conductivity under the context of a classical shallow donor model. In this article, we will describe the principle of muonium experiments and survey recent achievements in this field.

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