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論文

Decay modes of the 9/2$$^-$$ isomeric state in $$^{183}$$Tl

Venhart, M.*; Andreyev, A. N.; Cubiss, J. G.*; Wood, J. L.*; Barzakh, A. E.*; Van Beveren, C.*; Cocolios, T. E.*; de Groote, R. P.*; 他19名*

Physical Review C, 105(3), p.034338_1 - 034338_9, 2022/03

 被引用回数:1 パーセンタイル:34.54(Physics, Nuclear)

The neutron-deficient region of isotopes around $$Z$$=82 is the best studied example of low-energy shape coexistence in nuclei. In this work, the internal transition decay and $$alpha$$ decay of the 53.3-ms isomeric state in $$^{183}$$Tl were studied at ISOLDE, CERN. The branching for the internal decay was measured to be 98.5(4)%, while the much weaker $$alpha$$decay branching is only about 1.4(4)%. The new results include the first identification of an $$E3$$ transition feeding the 3/2$$^+$$ excited state in $$^{183}$$Tl. Three $$alpha$$ decays from the $$^{183m}$$Tl isomer were also oserved, and revealed the population of a candidate 9/2$$^-$$ state in $$^{179}$$Au which has been linked to shape coexistence in the Au nuclei. It is expected that similarly weak $$alpha$$ decays from isomeric states may be found also in neighbouring Tl isotopes.

論文

Producing gold at ISOLDE-CERN

Barzakh, A. E.*; Andreyev, A. N.; Atanasov, D.*; Cubiss, J. G.*; Harding, R. D.*; Al Monthery, M.*; Althubiti, N. A.*; Andel, B.*; 他38名*

Nuclear Instruments and Methods in Physics Research B, 513, p.26 - 32, 2022/02

 被引用回数:0 パーセンタイル:0.02(Instruments & Instrumentation)

The yield of 18 beams of radioactive gold nuclei produced by irradiating the ISOLDE uranium target with 1.4-GeV protons was measured. The production-efficiency dependence on the half-life was derived using the in-target production calculations. Three release models were tested to describe the results. Irregularities in the efficiency curve for 3 long-lived high-spin gold isomers ($$^{187,191,193}$$Au$$^m$$) were found, which require further investigation.

論文

Large shape staggering in neutron-deficient Bi isotopes

Barzakh, A.*; Andreyev, A. N.; Raison, C.*; Cubiss, J. G.*; 他53名*

Physical Review Letters, 127(19), p.192501_1 - 192501_7, 2021/11

 被引用回数:18 パーセンタイル:89.05(Physics, Multidisciplinary)

The changes in the mean-square charge radius (relative to $$^{209}$$Bi, magnetic moments and quadrupole moments of the neutron-deficient bismuth isotopes $$^{187,188,189,190}$$Bi were measured at ISOLDE (CERN). In the experiment, the in-source resonance-ionization spectroscopy technique was employed, which permits to study isotopes produced with rates as low as 0.1/sec. The radii of $$^{187.188.189}$$Bi manifest a large staggering, corresponding to a sudden increase of the radius of $$^{188}$$Bi relative to its $$^{187,189}$$Bi neighbors. This staggering effect occurs at neutron number $$N$$=105, where shape staggering was also observed in the mercury isotopes. Experimental results were compared with state-of-the-art mean-field calculations, which permit to identify the quasiparticle configurations compatible with the observed spin, parity and magnetic moment of the newly observed states.

論文

Solving the puzzles of the decay of the heaviest known proton-emitting nucleus $$^{185}$$Bi

Doherty, D. T.*; Andreyev, A. N.; Seweryniak, D.*; Woods, P. J.*; Carpenter, M. P.*; Auranen, K.*; Ayangeakaa, A. D.*; Back, B. B.*; Bottoni, S.*; Canete, L.*; et al.

Physical Review Letters, 127(20), p.202501_1 - 202501_6, 2021/11

 被引用回数:4 パーセンタイル:66.91(Physics, Multidisciplinary)

$$^{185}$$Bi is the heaviest known proton emitting isotope. Its decay had been observed, but the assumed ground-state lifetime ($$sim$$$$60~mu$$s) was incorrect, leading to unexplained hindrance. With two new experiments at Argonne National Laboratory, two states were clearly identified. One is the proton-emitting ground-state (spin 1/2$$^+$$, half-life: 2.8$$^{+2.3}_{-1.0}$$ $$mu$$s), the second is a 58(2) $$mu$$s $$gamma$$-decaying isomer. The new data show the inversion of the ground and isomeric states compared to neighboring Bi isotopes. This is the only known example of a ground-state proton decay to a daughter nucleus ($$^{184}$$Pb) with a major shell closure.

論文

Laser-assisted nuclear decay spectroscopy of $$^{176,177,179}$$Au

Harding, R. D.*; Andreyev, A. N.; Barzakh, A. E.*; Cubiss, J. G.*; Van Duppen, P.*; Al Monthery, M.*; Althubiti, N. A.*; Andel, B.*; 他26名*

Physical Review C, 104(2), p.024326_1 - 024326_16, 2021/08

 被引用回数:3 パーセンタイル:48.27(Physics, Nuclear)

A detailed nuclear spectroscopy study of $$^{176,177,179}$$Au was performed at ISOLDE, CERN. This work provides new insights into the low-lying levels in the daughter nuclei $$^{172,173,175}$$Ir. For $$^{176}$$Au, the nuclear magnetic moments of a high spin and low spin state were determined and used to predict the most likely configuration of each level. Their $$alpha$$-decay branching ratios were also extracted: a 58(5)% branching for the low-spin state, and 29(5)% for the high-spin state.

論文

Competition between allowed and first-forbidden $$beta$$ decays of $$^{208}$$At and expansion of the $$^{208}$$Po level scheme

Brunet, M.*; Podoly$'a$k, Zs.*; Berry, T. A.*; Brown, B. A.*; Carroll, R. J.*; Lica, R.*; Sotty, Ch.*; Andreyev, A. N.; Borge, M. J. G.*; Cubiss, J. G.*; et al.

Physical Review C, 103(5), p.054327_1 - 054327_13, 2021/05

 被引用回数:2 パーセンタイル:58.42(Physics, Nuclear)

The structure of $$^{208}$$Po populated through the EC/$$beta^{+}$$ decay of $$^{208}$$At is investigated using $$gamma$$-ray spectroscopy at the ISOLDE Decay Station. The presented level scheme contains 27 new excited states and 43 new transitions, as well as a further 50 previously observed $$gamma$$ rays which have been (re)assigned a position. Through the analysis using the shell model calculations approximately half of the $$beta$$-decay strength of $$^{208}$$At is found to proceed via allowed decay and half via first-forbidden decay. The first-forbidden transitions predominantly populate core excited states at high excitation energies, which is qualitatively understood using shell model considerations.

論文

Laser-assisted decay spectroscopy and mass spectrometry of $$^{178}$$Au

Cubiss, J. G.*; Andreyev, A. N.; Barzakh, A. E.*; Manea, V.*; Al Monthery, M.*; Althubiti, N. A.*; Andel, B.*; Antalic, S.*; 他39名*

Physical Review C, 102(4), p.044332_1 - 044332_12, 2020/10

 被引用回数:5 パーセンタイル:53.56(Physics, Nuclear)

A comprehensive study of the isotope $$^{178}$$Au has been made at the CERN-ISOLDE facility, using resonance laser ionization. Two long-lived states in $$^{178}$$Au were identified - a low-spin ground state and a high-spin isomer - each of which were produced as pure beams. Using the ISOLTRAP precision Penning trap, the excitation energy of the isomeric state in $$^{178}$$Au was determined to be $$E^{*} = $$ 189(14) keV. The $$alpha$$-decay fine structure patterns of the two states were studied using the Windmill decay station, providing information on the low-lying states in the daughter nucleus $$^{174}$$Ir. Nuclear spin assignments of $$I(^{178}$$Au$$^{g}) = (2,3)$$ and $$I(^{178}$$Au$$^{m}) = (7,8)$$ are made based on the observed $$beta$$-decay feeding and hyperfine structure intensity patterns.

論文

Laser-assisted decay spectroscopy for the ground states of $$^{180,182}$$Au

Harding, R. D.*; Andreyev, A. N.; Barzakh, A. E.*; Atanasov, D.*; Cubiss, J. G.*; Van Duppen, P.*; 他40名*

Physical Review C, 102(2), p.024312_1 - 024312_16, 2020/08

 被引用回数:9 パーセンタイル:74.44(Physics, Nuclear)

A detailed nuclear spectroscopy study of $$^{180}$$Au was performed. An $$alpha$$-decay branching ratio of $$0.58(10)$$% and a half-life of $$7.2(5)$$s have been derived. The first measurement of the hyper fine structure for atomic transitions has been also performed, from which the magnetic dipole moment has been extracted. A spin assignment of $$(1^+)$$ is proposed for the ground state of $$^{180}$$Au, with a $$(pi3/2^-$$[532]$$timesnu5/2^-$$[512]$$)$$ configuration.

論文

Decay studies of the long-lived states in $$^{186}$$Tl

Stryjczyk, M.*; Andel, B.*; Andreyev, A. N.; Cubiss, J.*; Pakarinen, J.*; 他43名*

Physical Review C, 102(2), p.024322_1 - 024322_9, 2020/08

 被引用回数:3 パーセンタイル:46.04(Physics, Nuclear)

Decay spectroscopy of the long-lived states in $$^{186}$$Tl has been performed at ISOLDE, CERN. The $$alpha$$ decay from the low-spin (2$$^{-}$$) state in $$^{186}$$Tl was observed for the first time and a half-life was determined. Based on the $$alpha$$-decay energy, the relative positions of the long-lived states were fixed, with the (2$$^{-}$$) state as the ground state, the 7$$^{(+)}$$ state at 77(56) keV, and the 10$$^{(-)}$$ state at 451(56) keV. The level scheme of the internal decay of the $$^{186}$$Tl(10$$^{(-)}$$) state, which was known to decay solely through emission of 374-keV $$gamma$$-ray transition, was extended and a lower limit for the $$beta$$-decay branching b$$_{beta}$$ $$>$$ 5.9(3)% was determined. The extracted retardation factors for the $$gamma$$ decay of the 10$$^{(-)}$$ state were compared to the available data in neighboring odd-odd thallium isotopes indicating the importance of the $$pi$$d$$_{3/2}$$ shell in the isomeric decay and significant structure differences between $$^{184}$$Tl and $$^{186}$$Tl.

論文

In-source laser spectroscopy of dysprosium isotopes at the ISOLDE-RILIS

Chrysalidis, K.*; Barzakh, A. E.*; Ahmed, R.*; Andreyev, A. N.; Ballof, J.*; Cubiss, J. G.*; Fedorov, D. V.*; Fedosseev, V. N.*; Fraile, L. M.*; Harding, R. D.*; et al.

Nuclear Instruments and Methods in Physics Research B, 463, p.472 - 475, 2020/01

 被引用回数:3 パーセンタイル:36.99(Instruments & Instrumentation)

放射壊変によって生成された多数のジスプロシウム同位体について、ISOLDEのレーザー共鳴イオン源(RILIS)を用いてイオン源内レーザー分光法によって研究した。$$^{152}$$Dyに対する相対的な同位体シフトを$$4f^{10}6s^{2}~^{5}I_{8}$$ (gs) $$rightarrow$$ $$4f^{10}6s6p~(8,1)^{o}_{8}$$共鳴遷移を用いて測定した。電子的因子Fとマスシフト因子Mを導出し、それらを使って$$^{rm 145m}$$Dyと$$^{rm 147m}$$Dyの平均自乗荷電半径の変化を初めて決定した。

論文

$$alpha$$-decay branching ratio of $$^{180}$$Pt

Cubiss, J. G.*; Harding, R. D.*; Andreyev, A. N.; Althubiti, N.*; Andel, B.*; Antalic, S.*; Barzakh, A. E.*; Cocolios, T. E.*; Day Goodacre, T.*; Farooq-Smith, G. J.*; et al.

Physical Review C, 101(1), p.014314_1 - 014314_4, 2020/01

 被引用回数:5 パーセンタイル:53.56(Physics, Nuclear)

$$^{180}$$Ptの基底状態から娘核$$^{176}$$Osの基底状態への$$alpha$$崩壊分岐比を0.52(5)%と、過去の値と比較してより高精度で再決定した。$$^{180}$$PtはCERN-ISOLDE実験施設において$$^{180}$$Hgを単離し、その$$beta$$崩壊孫核種として生成した。今回の結果を用いて導出した$$alpha$$崩壊の換算崩壊幅は、中性子欠損Pt同位体の$$alpha$$崩壊幅の系統性について新しい描像を与えることとなった。

論文

$$alpha$$-decay properties of $$^{200,202}$$Fr

Ghys, L.*; Andreyev, A. N.; Huyse, M.*; Van Duppen, P.*; Antalic, S.*; Barzakh, A.*; Capponi, L.*; Cocolios, T. E.*; Cubiss, J.*; Derkx, X.*; et al.

Physical Review C, 100(5), p.054310_1 - 054310_13, 2019/11

 被引用回数:11 パーセンタイル:77.66(Physics, Nuclear)

The aim of this work was to investigate the $$alpha$$-decay properties of $$^{200,202}$$Fr and daughter products. Neutron-deficient francium nuclei are produced at ISOLDE-CERN bombarding a UCx target with 1.4 GeV protons. Due to the very high statistics and the high beam purity, improved decay data for $$^{202}$$Fr and its daughters were obtained. The observation of crossover transitions positioned the isomeric high-spin level of $$^{198}$$At at an excitation energy of 265(3) keV. Half-life values of 4.47(5) s and 1.28(10) s were extracted for the ground state and isomeric state of $$^{198}$$At and 52(3) ms for the ground-state decay of $$^{200}$$Fr.

論文

Identification of a 6.6$$mu$$s isomeric state in $$^{175}$$Ir

Gillespie, S. A.*; Andreyev, A. N.; Al Monthery, M.*; Barton, C. J.*; Antalic, S.*; Auranen, K.*; Badran, H.*; Cox, D.*; Cubiss, J. G.*; O'Donnell, D.*; et al.

Physical Review C, 99(6), p.064310_1 - 064310_6, 2019/06

 被引用回数:3 パーセンタイル:33.05(Physics, Nuclear)

An experiment has been performed to study excited states in the neutron-deficient nucleus $$^{175}$$Ir via the use of the JUROGAM II high-purity germanium detector array and the RITU gas-filled separator at JYFL, Jyv$"a$skyl$"a$. By using isomer tagging, an isomeric state with a half-life of 6.58(15) $$mu$$s has been observed in $$^{175}$$Ir for the first time. It has been established that the isomer decays via a 45.2 ($$E1$$) - 26.1 ($$M1$$) keV cascade to new states below the previously reported ground state in $$^{175}$$Ir with $$I^{pi} = (5/2^{-})$$. We now reassign this $$(5/2^{-})$$ state to the isomeric state discovered in this study.

論文

Fine structure in the $$alpha$$ decay of $$^{218}$$At

Cubiss, J. G.*; Andreyev, A. N.; Barzakh, A. E.*; Andel, B.*; Antalic, S.*; Cocolios, T. E.*; Day Goodacre, T.*; Fedorov, D. V.*; Fedosseev, V. N.*; Ferrer, R.*; et al.

Physical Review C, 99(6), p.064317_1 - 064317_6, 2019/06

 被引用回数:6 パーセンタイル:54.59(Physics, Nuclear)

$$^{218}$$Atの$$alpha$$崩壊について、CERN-ISOLDE施設においてレーザーイオン化法を使うことで研究した。$$alpha$$-$$gamma$$同時計数データを初めて取得し、より精度の良い半減期の値として1.27(6)秒を得た。$$alpha$$崩壊の微細構造を基に新しい$$alpha$$崩壊図式を構築した。それらの結果から、$$^{218}$$Atの基底状態のスピン・パリティは(3$$^{-}$$)がより確からしいことが解ったが、(2)$$^{-}$$の可能性も完全には否定しきれない。

論文

Inverse odd-even staggering in nuclear charge radii and possible octupole collectivity in $$^{217,218,219}$$At revealed by in-source laser spectroscopy

Barzakh, A. E.*; Cubiss, J. G.*; Andreyev, A. N.; Seliverstov, M. D.*; Andel, B.*; Antalic, S.*; Ascher, P.*; Atanasov, D.*; Beck, D.*; Biero$'n$, J.*; et al.

Physical Review C, 99(5), p.054317_1 - 054317_9, 2019/05

 被引用回数:12 パーセンタイル:77.66(Physics, Nuclear)

Hyperfine-structure parameters and isotope shifts for the 795-nm atomic transitions in $$^{217,218,219}$$At have been measured at CERN-ISOLDE, using the in-source resonance-ionization spectroscopy technique. Magnetic dipole and electric quadrupole moments, and changes in the nuclear mean-square charge radii, have been deduced. A large inverse odd-even staggering in radii, which may be associated with the presence of octupole collectivity, has been observed. Namely, the radius of the odd-odd isotope $$^{218}$$At has been found to be larger than the average.

論文

Change in structure between the $$I$$=1/2 states in $$^{181}$$Tl and $$^{177,179}$$Au

Cubiss, J. G.*; Barzakh, A. E.*; Andreyev, A. N.; 他57名*

Physics Letters B, 786, p.355 - 363, 2018/11

 被引用回数:19 パーセンタイル:83.92(Astronomy & Astrophysics)

The first accurate measurements of the $$alpha$$-decay branching ratio and half-life of the I$$^pi$$=1/2$$^{+}$$ ground state in $$^{181}$$Tl have been made, along with the first determination of the magnetic moments and I=1/2 spin assignments of the ground states in $$^{177,179}$$Au. The results are discussed within the complementary systematics of the reduced $$alpha$$-decay widths and nuclear g factors of low-lying, I$$^pi$$=1/2$$^{+}$$states in the neutron-deficient lead region. The findings shed light on the unexpected hindrance of the 1/2$$^{+}$$ $$rightarrow$$ 1/2$$^{+}$$, $$^{181}$$Tl$$^{g}$$ $$rightarrow$$ $$^{177}$$Au$$^{g}$$ $$alpha$$decay, which is explained by a mixing of $$pi$$3s$$_{1/2}$$and $$pi$$2d$$_{3/2}$$ configurations in $$^{177}$$Au$$^{g}$$, whilst $$^{181}$$Tl$$^{g}$$ remains a near-pure $$pi$$3s$$^{1/2}$$. This conclusion is inferred from the g factor of $$^{177}$$Au$$^{g}$$ which has an intermediate value between those of $$pi$$3s$$_{1/2}$$ and $$pi$$2d$$_{3/2}$$ states. A similar mixed configuration is proposed for the I$$^pi$$=1/2$$^{+}$$ ground state of $$^{179}$$Au. This mixing may provide evidence for triaxial shapes in the ground states in these nuclei.

論文

Charge radii and electromagnetic moments of $$^{195-211}$$At

Cubiss, J.*; Andreyev, A. N.; 光岡 真一*; 永目 諭一郎; 西尾 勝久; 太田 周也*; 若林 泰生*; 他60名*

Physical Review C, 97(5), p.054327_1 - 054327_19, 2018/05

 被引用回数:30 パーセンタイル:92.76(Physics, Nuclear)

Hyperfine-structure parameters and isotope shifts of $$^{195-211}$$At have been measured for the first time at CERN-ISOLDE, using the in-source resonance-ionization spectroscopy method. The hyperfine structures of isotopes were recorded using a triad of experimental techniques for monitoring the photo-ion current. The Multi-Reflection Time-of-Flight Mass Spectrometer, in connection with a high-resolution electron multiplier, was used as an ion-counting setup for isotopes that either were affected by strong isobaric contamination or possessed a long half-life; the ISOLDE Faraday cups were used for cases with high-intensity beams; and the Windmill decay station was used for short-lived, predominantly $$alpha$$-decaying nuclei. The electromagnetic moments and changes in the mean-square charge radii of the astatine nuclei have been extracted from the measured hyperfine-structure constants and isotope shifts. This was only made possible by dedicated state-of-the-art large-scale atomic computations of the electronic factors and the specific mass shift of atomic transitions in astatine that are needed for these extractions. By comparison with systematics, it was possible to assess the reliability of the results of these calculations and their ascribed uncertainties. A strong deviation in the ground-state mean-square charge radii of the lightest astatine isotopes, from the trend of the (spherical) lead isotopes, is interpreted as the result of an onset of deformation. This behavior bears a resemblance to the deviation observed in the isotonic polonium isotopes. Cases for shape coexistence have been identified in $$^{197,199}$$At, for which a significant difference in the charge radii for ground (9/2$$^{-}$$) and isomeric (1/2$$^{+}$$) states has been observed.

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