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Numerical simulation of the solid particle sedimentation and bed formation behaviors using a hybrid method

Sheikh, M. A. R.*; Liu, X.*; 松元 達也*; 守田 幸路*; Guo, L.*; 鈴木 徹*; 神山 健司

Energies (Internet), 13(19), p.5018_1 - 5018_15, 2020/10


In the safety analysis of sodium-cooled fast reactors, numerical simulations of various thermal-hydraulic phenomena with multicomponent and multiphase flows in core disruptive accidents (CDAs) are regarded as particularly difficult. In the material relocation phase of CDAs, core debris settle down on a core support structure and/or an in-vessel retention device and form a debris bed. The bed's shape is crucial for the subsequent relocation of the molten core and heat removal capability as well as re-criticality. In this study, a hybrid numerical simulation method, coupling the multi-fluid model of the three-dimensional fast reactor safety analysis code SIMMER-IV with the discrete element method (DEM), was applied to analyze the sedimentation and bed formation behaviors of core debris. Three-dimensional simulations were performed and compared with results obtained in a series of particle sedimentation experiments. The present simulation predicts the sedimentation behavior of mixed particles with different properties as well as homogeneous particles. The simulation results on bed shapes and particle distribution in the bed agree well with experimental measurements. They demonstrate the practicality of the present hybrid method to solid particle sedimentation and bed formation behaviors of mixed as well as homogeneous particles.


Spectroscopic and first-principles investigations of iodine species incorporation into ettringite; Implications for iodine migration in cement waste forms

Guo, B.*; Xiong, Y.*; Chen, W.*; Saslow, S. A.*; 香西 直文; 大貫 敏彦*; Dabo, I.*; 笹木 恵子*

Journal of Hazardous Materials, 389, p.121880_1 - 121880_11, 2020/05

To elucidate retention mechanism of cement waste form for radioactive iodine, this paper investigated interaction mechanism between iodine and ettringite, which is a component mineral of cement and has anion exchange ability. We revealed that ettringite has a high capacity for accommodating IO$$_{3}$$$$^{-}$$ via anion substitution for SO$$_{4}$$$$^{2-}$$. The combined iodine K-edge extended X-ray absorption fine structure spectra and first-principles calculations using density functional theory suggested that IO$$_{3}$$$$^{-}$$ was stabilized in ettringite by hydrogen bonding and electrostatic forces. The bonding charge density analysis of the substituted IO$$_{3}$$$$^{-}$$ into the ettringite structure revealed the interaction between intercalated IO$$_{3}$$$$^{-}$$ with the structural water molecules. These results provided valuable insight into the long-term stabilization of anionic iodine species and their migration in cementitious nuclear waste repository or alkaline environments.


Effects of the nuclear structure of fission fragments on the high-energy prompt fission $$gamma$$-ray spectrum in $$^{235}$$U($$n_{rm th},f$$)

牧井 宏之; 西尾 勝久; 廣瀬 健太郎; Orlandi, R.; L$'e$guillon, R.; 小川 達彦; Soldner, T.*; K$"o$ster, U.*; Pollitt, A.*; Hambsch, F.-J.*; et al.

Physical Review C, 100(4), p.044610_1 - 044610_7, 2019/10

 被引用回数:2 パーセンタイル:63.02(Physics, Nuclear)

The prompt fission $$gamma$$-ray energy spectrum for cold-neutron induced fission of $$^{235}$$U was measured in the energy range $$E_{rm gamma}$$ = 0.8 - 20,MeV, by gaining a factor of about 10$$^{5}$$ in statistics compared to the measurements performed so far. The spectrum exhibits local bump structures at $$E_{rm gamma}approx$$4,MeV and $$approx$$6,MeV, and also a broad one at $$approx$$15,MeV. In order to understand the origins of these bumps, the $$gamma$$-ray spectra were calculated using a statistical Hauser-Feshbach model, taking into account the de-excitation of all the possible primary fission fragments. It is shown that the bump at $$approx$$4,MeV is created by the transitions between the discrete levels in the fragments around $$^{132}$$Sn, and the bump at $$approx$$6,MeV mostly comes from the complementary light fragments. It is also indicated that a limited number of nuclides, which have high-spin states at low excitation energies, can contribute to the bump structure around $$E_{rm gamma}approx$$15,MeV, induced by the transition feeding into the low-lying high-spin states.


Passive sweat collection and colorimetric analysis of biomarkers relevant to kidney disorders using a soft microfluidic system

Zhang, Y.*; Guo, H.*; Kim, S. B.*; Wu, Y.*; Ostojich, D.*; Park, S. H.*; Wang, X.*; Weng, Z.*; Li, R.*; Bandodkar, A. J.*; et al.

Lab on a Chip, 19(9), p.1545 - 1555, 2019/05

 被引用回数:20 パーセンタイル:1.78(Biochemical Research Methods)



A New detector system for the measurement of high-energy prompt $$gamma$$-rays for low-energy neutron induced fission

牧井 宏之; 西尾 勝久; 廣瀬 健太郎; Orlandi, R.; L$'e$guillon, R.*; 小川 達彦; Soldner, T.*; Hambsch, F.-J.*; A$"i$che, M.*; Astier, A.*; et al.

Nuclear Instruments and Methods in Physics Research A, 906, p.88 - 96, 2018/10

 被引用回数:3 パーセンタイル:40.19(Instruments & Instrumentation)



Numerical simulation on self-leveling behavior of mixed particle beds using multi-fluid model coupled with DEM

Phan, L. H. S.*; 大原 陽平*; 河田 凌*; Liu, X.*; Liu, W.*; 守田 幸路*; Guo, L.*; 神山 健司; 田上 浩孝

Proceedings of 12th International Topical Meeting on Nuclear Reactor Thermal-Hydraulics, Operation and Safety (NUTHOS-12) (USB Flash Drive), 12 Pages, 2018/10



The $$^{95}$$Zr($$n, gamma$$)$$^{96}$$Zr cross section from the surrogate ratio method and its effect on $$s$$-process nucleosynthesis

Yan, S. Q.*; Li, Z. H.*; Wang, Y. B.*; 西尾 勝久; Lugaro, M.*; Karakas, A. I.*; 牧井 宏之; Mohr, P.*; Su, J.*; Li, Y. J.*; et al.

Astrophysical Journal, 848(2), p.98_1 - 98_8, 2017/10

 被引用回数:0 パーセンタイル:100(Astronomy & Astrophysics)

The $$^{95}$$Zr($$n, gamma$$)$$^{96}$$Zr reaction cross section is crucial in the modelling of $$s$$-process nucleosynthesis in asymptotic giant branch stars because it controls the operation of the branching point at the unstable $$^{95}$$Zr and the subsequent production of $$^{96}$$Zr. We have carried out the measurement of the $$^{90}$$Zr($$^{18}$$O,$$^{16}$$O) and $$^{94}$$Zr($$^{18}$$O,$$^{16}$$O) reactions and obtained the $$gamma$$-decay probability ratio of $$^{92}$$Zr$$^{*}$$ and $$^{96}$$Zr$$^{*}$$ to determine the $$^{95}$$Zr($$n, gamma$$)$$^{96}$$Zr reaction cross sections with the surrogate ratio method. We tested our deduced maxwellian-averaged cross section in stellar models with masses between 2 and 6 $$M_{odot}$$ and metallicities 0.014 and 0.03. The largest changes - up 80 % variations in $$^{96}$$Zr - are seen in the models of 3-4 $$M_{odot}$$, where the $$^{22}$$Ne neutron source is mildly activated. The new rate can still provide a match to data from meteoritic stardust silicon carbide grains, provided the maximum mass of the parent stars is below 4 $$M_{odot}$$, for a metallicity of 0.03.


Measurement of high-energy prompt $$gamma$$-rays from neutron induced fission of U-235

牧井 宏之; 西尾 勝久; 廣瀬 健太郎; Orlandi, R.; L$'e$guillon, R.; 小川 達彦; Soldner, T.*; Hambsch, F.-J.*; Astier, A.*; Pollitt, A.*; et al.

EPJ Web of Conferences, 146, p.04036_1 - 04036_4, 2017/09

 被引用回数:2 パーセンタイル:10.14



Numerical simulation of solid-particle sedimentation behavior using a multi-fluid model coupled with DEM

河田 凌*; 大原 陽平*; Sheikh, Md. A. R.*; Liu, X.*; 松元 達也*; 守田 幸路*; Guo, L.*; 神山 健司; 鈴木 徹

Proceedings of 17th International Topical Meeting on Nuclear Reactor Thermal Hydraulics (NURETH-17) (USB Flash Drive), 14 Pages, 2017/09

Numerical simulations of various thermal-hydraulic phenomena with multiphase and multicomponent flows in postulated core disruptive accidents (CDAs) are regarded as particular difficulties in the safety analysis of liquid-metal cooled reactors. In a material relocation phase of CDAs, core debris may settle on the core-support structure and/or in the lower inlet plenum of the reactor vessel and then form the debris bed. In particular, the shape of debris bed is crucial for the relocation of molten core and heat-removal capability of the debris bed as well as re-criticality. In the present study, a hybrid numerical simulation method, which couples the multi-fluid model of the 3D fast reactor safety analysis code SIMMER-IV with the discrete element method (DEM), was applied to analyze sedimentation and bed formation behaviors of core debris. In the present study, 3D simulations were performed for a series of particle sedimentation experiments with gravity driven discharge of solid particles into a quiescent cylindrical water pool. The present simulation predicts the sedimentation behavior of mixed particles with different density or particle size as well as homogeneous particles. The simulation results on bed shapes and particle distribution in the bed agree well with the experimental ones. They demonstrate the fundamental applicability of the present hybrid method to solid-particle sedimentation and bed formation simulations.


Uniaxial pressure effect on the magnetic ordered moment and transition temperatures in BaFe$$_{2-x}$$T$$_{x}$$As$$_{2}$$ ($$T$$ = Co,Ni)

Tam, D. M.*; Song, Y.*; Man, H.*; Cheung, S. C.*; Yin, Z.*; Lu, X.*; Wang, W.*; Frandsen, B. A.*; Liu, L.*; Gong, Z.*; et al.

Physical Review B, 95(6), p.060505_1 - 060505_6, 2017/02

 被引用回数:15 パーセンタイル:23.77(Materials Science, Multidisciplinary)

We use neutron diffraction and muon spin relaxation to study the effect of in-plane uniaxial pressure on the antiferromagnetic (AF) orthorhombic phase in BaFe$$_{2-x}$$T$$_{x}$$As$$_{2}$$ and its Co- and Ni-substituted members near optimal superconductivity. In the low-temperature AF ordered state, uniaxial pressure necessary to detwin the orthorhombic crystals also increases the magnetic ordered moment, reaching an 11% increase under 40 MPa for BaFe$$_{1.9}$$Co$$_{0.1}$$As$$_2$$, and a 15% increase for BaFe$$_{1.915}$$Ni$$_{0.085}$$As$$_2$$. We also observe an increase of the AF ordering temperature ($$T_N$$) of about 0.25 K/MPa in all compounds, consistent with density functional theory calculations that reveal better Fermi surface nesting for itinerant electrons under uniaxial pressure. The doping dependence of the magnetic ordered moment is captured by combining dynamical mean field theory with density functional theory, suggesting that the pressure-induced moment increase near optimal superconductivity is closely related to quantum fluctuations and the nearby electronic nematic phase.


Volume-wise destruction of the antiferromagnetic Mott insulating state through quantum tuning

Frandsen, B. A.*; Liu, L.*; Cheung, S. C.*; Guguchia, Z.*; Khasanov, R.*; Morenzoni, E.*; Munsie, T. J. S.*; Hallas, A. M.*; Wilson, M. N.*; Cai, Y.*; et al.

Nature Communications (Internet), 7, p.12519_1 - 12519_8, 2016/08

 被引用回数:13 パーセンタイル:33.61(Multidisciplinary Sciences)

RENiO$$_3$$ (RE = rare-earth element) and V$$_2$$O$$_3$$ are archetypal Mott insulator systems. When tuned by chemical substitution (RENiO$$_3$$) or pressure (V$$_2$$O$$_3$$), they exhibit a quantum phase transition (QPT) between an antiferromagnetic Mott insulating state and a paramagnetic metallic state. Because novel physics often appears near a Mott QPT, the details of this transition, such as whether it is first or second order, are important. Here, we demonstrate through muon spin relaxation/rotation experiments that the QPT in RENiO$$_3$$ and V$$_2$$O$$_3$$ is first order: the magnetically ordered volume fraction decreases to zero at the QPT, resulting in a broad region of intrinsic phase separation, while the ordered magnetic moment retains its full value until it is suddenly destroyed at the QPT. These findings bring to light a surprising universality of the pressure-driven Mott transition, revealing the importance of phase separation and calling for further investigation into the nature of quantum fluctuations underlying the transition.


Examination of the surrogate ratio method for the determination of the $$^{93}$$Zr(n,$$gamma$$)$$^{94}$$Zr cross section with $$^{90,92}$$Zr($$^{18}$$O,$$^{16}$$O)$$^{92,94}$$Zr reactions

Yan, S. Q.*; Li, Z. H.*; Wang, Y. B.*; 西尾 勝久; 牧井 宏之; Su, J.*; Li, Y. J.*; 西中 一朗; 廣瀬 健太郎; Han, Y. L.*; et al.

Physical Review C, 94(1), p.015804_1 - 015804_5, 2016/07

 被引用回数:3 パーセンタイル:63.27(Physics, Nuclear)

The relative $$gamma$$-decay probability ratios of the neutron resonance states in $$^{94}$$Zr and $$^{92}$$Zr populated via two neutron transfer reactions, $$^{92}$$Zr($$^{18}$$O,$$^{16}$$O)$$^{94}$$Zr and $$^{90}$$Zr($$^{18}$$O,$$^{16}$$O)$$^{92}$$Zr, have been measured to test the validity of the surrogate ratio method (SRM) in determining the (n,$$gamma$$) reaction cross section. The cross sections of the $$^{93}$$Zr(n,$$gamma$$)$$^{94}$$Zr reaction are derived from the experimentally obtained ratios and the cross sections of the $$^{91}$$Zr(n,$$gamma$$)$$^{92}$$Zr reaction in the equivalent neutron energy range of $$E_{rm n}$$ = 0 - 8 MeV. The deduced cross sections of $$^{93}$$Zr(n,$$gamma$$)$$^{94}$$Zr reaction agree with the directly measured ones in the low-energy region, and with the evaluated ENDF/B-VII.1 data at higher energies of $$E_{rm n} >$$ 3 MeV. The agreement supports the concept of the SRM method to indirectly determine the (n,$$gamma$$) reaction cross sections.


The Martian surface radiation environment; A Comparison of models and MSL/RAD measurements

Matthi$"a$, D.*; Ehresmann, B.*; Lohf, H.*; K$"o$hler, J.*; Zeitlin, C.*; Appel, J.*; 佐藤 達彦; Slaba, T. C.*; Martin, C.*; Berger, T.*; et al.

Journal of Space Weather and Space Climate (Internet), 6, p.A13_1 - A13_17, 2016/03

 被引用回数:40 パーセンタイル:4.98(Astronomy & Astrophysics)

2012年8月6日以降、Mars Science Laboratory (MSL)に搭載された複合型放射線検出器(RAD)を用いて火星表面による放射線環境の測定が続けられている。本研究では、GEANT4, PHITS, HZETRN/OLTARISなど様々なコードを用いて火星表面における放射線環境を推定し、その結果とRADによる測定値を比較した。その結果、計算結果は測定値と概ねよい一致を示すものの、場合によっては大きく解離することが分かった。また、RADのデータは放射線輸送計算について、最適なインプットパラメータや物理モデルの最適な選択に役立つことも確認された。今回の解析結果は、今後、有人火星ミッションを計画する際、その被ばく線量評価や宇宙機遮へい設計などに活用することができる。


Origin of the spin Seebeck effect in compensated ferrimagnets

Gepr$"a$gs, S.*; Kehlberger, A.*; Coletta, F.*; Qiu, Z.*; Guo, E.-J.*; Schulz, T.*; Mix, C.*; Meyer, S.*; Kamra, A.*; Althammer, M.*; et al.

Nature Communications (Internet), 7, p.10452_1 - 10452_6, 2016/02

 被引用回数:80 パーセンタイル:2.93(Multidisciplinary Sciences)

Magnons are the elementary excitations of a magnetically ordered system. Here, we show that the spin Seebeck effect is sensitive to the complexities of the magnon spectrum. The spin Seebeck effect is caused by a thermally excited spin dynamics that is converted to a voltage by the inverse spin Hall effect at the interface to a heavy metal contact. By investigating the temperature dependence of the spin Seebeck effect in the ferrimagnet gadlinium iron garnet, with a magnetic compensation point near room temperature, we demonstrate that high-energy exchange magnons play a key role in the spin Seebeck effect.


Development of assessment method for a self-leveling behavior of debris bed and analyses of experiments

田上 浩孝; Cheng, S.; 飛田 吉春; Guo, L.*; Zhang, B.*; 守田 幸路*

Proceedings of 22nd International Conference on Nuclear Engineering (ICONE-22) (DVD-ROM), 8 Pages, 2014/07



In-beam $$gamma$$ spectroscopy of the even-even nucleus $$^{190}$$Pt

Li, G. S.*; Liu, M. L.*; Zhou, X. H.*; Zhang, Y. H.*; Liu, Y. X.*; Zhang, N. T.*; Hua, W.*; Zheng, Y. D.*; Fang, Y. D.*; Guo, S.*; et al.

Physical Review C, 89(5), p.054303_1 - 054303_9, 2014/05

 被引用回数:3 パーセンタイル:68.06(Physics, Nuclear)

タンデム加速器で88MeVにまで加速された$$^{18}$$Oビームを用いて$$^{176}$$Yb($$^{18}$$O, 4$$n$$)反応を起こし、$$^{190}$$Ptの高スピン準位を調べた。その結果、$$nu$$ $$i^{-2}_{13/2}$$ $$nu$$ $$h^{-1}_{9/2}$$ $$nu$$ $$j^{-1}$$1(ここで$$nu j$$$$nu p_{3/2}$$もしくは$$nu f_{5/2}$$)配位による正パリティバンドを大幅に拡張するとともに新しく負パリティバンドを同定し、$$nu$$ $$i^{-3}_{13/2}$$ $$nu$$ $$j^{-1}$$配位を持つことを明らかにした。また、イラスト準位においてスピンの増加に伴い振動から回転へと構造変化を起こしている可能性について議論した。さらにバンド特性を明らかにするためにTotal Routhian surface計算を行った。


Development of a GEM-TPC for H-dibaryon search experiment at J-PARC

佐甲 博之; Ahn, J. K.*; Baek, K. H.*; Bassalleck, B.*; Fujioka, H.*; Guo, L.*; 長谷川 勝一; Hicks, K.*; Honda, R.*; Hwang, S. H.*; et al.

Journal of Instrumentation (Internet), 9(4), p.C04009_1 - C04009_10, 2014/04

 被引用回数:3 パーセンタイル:79.22(Instruments & Instrumentation)

($$K^+$$,$$K^-$$)反応によるHダイバリオン探索実験(J-PARC E42)のためのTPCの開発を行っている。TPCにおいてHが2個の$$pi^{-}$$と2個の$$p$$に崩壊する事象を測定する。TPCのドリフト体積は50cm直径、55cmドリフト長を持つ8角柱構造をしておりAr-CH$$_4$$ガスを使用する。増幅部には3層のGEMを使用する。荷電粒子の運動量測定のためTPCにはドリフト電場と平行に鉛直方向の1Tの双極磁場を超伝導ヘルムホルツ型磁石によりかける。H崩壊のアクセプタンスを最大にするためダイアモンド標的がTPC内部の筒状の穴に設置される。さらに、超高レートの$$K^-$$ビームをTPCに直接照射するため陽イオンフィードバックを極力抑制必要がある。このためTPCにGEMとgating gridを採用した。


Rotational band properties of $$^{173}$$W

Wang, H. X.*; Zhang, Y. H.*; Zhou, X. H.*; Liu, M. L.*; Ding, B.*; Li, G. S.*; Hua, W.*; Zhou, H. B.*; Guo, S.*; Qiang, Y. H.*; et al.

Physical Review C, 86(4), p.044305_1 - 044305_11, 2012/10


 被引用回数:4 パーセンタイル:67.56(Physics, Nuclear)

High-spin states in $$^{173}$$W have been studied using the $$^{150}$$Nd($$^{28}$$Si,5$$n$$)$$^{173}$$W reaction at beam energies of 135 and 140 MeV. The previously known bands associated with the 7/2$$^+$$[633], 5/2$$^-$$[512], and 1/2$$^-$$[521] configurations are extended significantly, and the unfavored signature branch of the 1/2$$^-$$[521] band is established for the first time. The band properties, such as level spacings, band-crossing frequencies, alignment gains, and signature splittings, are discussed with an emphasis on the low-spin signature inversion observed in the 5/2$$^-$$[512] band. By comparing the experimental $$B$$($$M$$1)/$$B$$($$E$$2) ratios with the theoretical values, we conclude that the configuration of the 5/2$$^-$$[512] band is quite pure at low spins without appreciable admixture of the 5/2$$^-$$[523] orbit, in conflict with the particle rotor model calculated results.


High-j proton alignments in $$^{101}$$Pd

Zhou, H. B.*; Zhou, X. H.*; Zhang, Y. H.*; Zheng, Y.*; Liu, M. L.*; Zhang, N. T.*; Chen, L.*; Wang, S. T.*; Li, G. S.*; Wang, H. X.*; et al.

European Physical Journal A, 47(9), p.107_1 - 107_7, 2011/09

 被引用回数:4 パーセンタイル:63.94(Physics, Nuclear)

$$^{101}$$Pd原子核の高スピン状態を、タンデム加速器及び多重$$gamma$$線検出装置GEMINI-IIを用いて、インビーム$$gamma$$線核分光法で調べた。既知の$$d$$$$_{5/2}$$バンド, 1/2$$^-$$[550]バンドをより高スピン状態まで拡張した。発見されたバンド交差は$$g$$$$_{9/2}$$陽子の整列によるものであると解釈した。$$^{101}$$Pdの回転バンドの性質を周辺の核、及びcranked shell modelと比較・議論した。


Identification of a new band and its signature inversion in $$^{174}$$Re

Zhang, Y. H.*; Guo, S.*; Zhou, X. H.*; Ma, L.*; Guo, W. T.*; 大島 真澄; 藤 暢輔; 小泉 光生; 長 明彦; 木村 敦; et al.

Chinese Physics Letters, 24(5), p.1203 - 1206, 2007/05

タンデム加速器からの重イオン($$^{27}$$Al)ビームを用い、多重$$gamma$$線検出装置GEMINI-IIにより、重イオン核反応後の即発$$gamma$$線を測定し、$$^{174}$$Reの高励起状態の準位構造を調べた。$$gamma - gamma$$同時計数データを解析した。既知の$$pi 1/2^-[541] bigotimes nu 1/2^-[521]$$回転バンドとの結合関係から、新しい回転バンドが同定された。近傍核の系統性から、このバンドは$$pi 1/2^-[541] bigotimes nu 5/2^-[512]$$配位の上に立つ基底状態回転バンドであることを提唱した。新しいバンドは低スピン指標逆転現象を示し、新たな理論解析の必要性を示唆する結果となった。

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