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論文

Eustatic change modulates exhumation in the Japanese Alps

King, G. E.*; Ahadi, F.*; 末岡 茂; Herman, F.*; Anderson, L.*; Gautheron, C.*; 塚本 すみ子*; Stalder, N.*; Biswas, R.*; Fox, M.*; et al.

Geology, 51(2), p.131 - 135, 2023/02

The exhumation of bedrock is controlled by the interplay between tectonics, surface processes, and climate. The highest exhumation rates of centimeters per year are recorded in zones of highly active tectonic convergence such as the Southern Alps of New Zealand or the Himalayan syntaxes, where high rock uplift rates combine with very active surface processes. Using a combination of different thermochronometric systems including trapped-charge thermochronometry, we show that such rates also occur in the Hida Mountain Range, Japanese Alps. Our results imply that centimeter per year rates of exhumation are more common than previously thought. Our thermochronometry data allow the development of time series of exhumation rate changes at the time scale of glacial-interglacial cycles, which show a fourfold increase in baseline rates to rates of $$sim$$10 mm/yr within the past $$sim$$65 k.y. This increase in exhumation rate is likely explained by knickpoint propagation due to a combination of very high precipitation rates, climatic change, sea-level fall, range-front faulting, and moderate rock uplift. Our data resolve centimeter-scale sub-Quaternary exhumation rate changes, which show that in regions with horizontal convergence, coupling between climate, surface processes, and tectonics can exert a significant and rapid effect on rates of exhumation.

論文

Results of the Collaborative International Evaluated Library Organisation (CIELO) Project

Fleming, M.*; Chadwick, M.*; Brown, D.*; Capote, R.*; Ge, Z.*; Herman, M.*; Ignatyuk, A.*; Ivanova, T.*; 岩本 修; Koning, A.*; et al.

EPJ Web of Conferences, 239, p.15003_1 - 15003_5, 2020/09

 被引用回数:4 パーセンタイル:95.3(Nuclear Science & Technology)

The Sub- and Expert Groups of the WPEC typically focus on specific technical topics, while the Collaborative International Evaluated Library Organisation Pilot Project (CIELO) was established to generate complete evaluations for a selection of the most important isotopes for criticality in nuclear technologies: $$^{235,238}$$U, $$^{239}$$Pu, $$^{56}$$Fe, $$^{16}$$O and $$^{1}$$H. The outcomes of these evaluations include significant harmonisation of discrepancies between the independent programmes, improvement in the performance for international standard nuclear criticality and neutron transmission benchmarks, complete uncertainties for nearly all parameters and the utilisation of modern data storage technologies. This work has leveraged the considerable, parallel experimental work in collecting improved experimental measurements to support nuclear data and highlighted high-priority areas for further study. A productive and durable framework for international evaluation has been established which will build upon the lessons learned. These will continue through new WPEC groups and a new IAEA evaluation network, which has been initiated in response to the success of the CIELO project. This talk will summarize some performance feedback on the CIELO evaluations, including recent results, and will describe ongoing and future, planned CIELO-related collaborations to further advance our understanding.

論文

Overview of the OECD-NEA Working Party on International Nuclear Data Evaluation Cooperation (WPEC)

Fleming, M.*; Bernard, D.*; Brown, D.*; Chadwick, M. B.*; De Saint Jean, C.*; Dupont, E.*; Ge, Z.*; 原田 秀郎; Hawari, A.*; Herman, M.*; et al.

EPJ Web of Conferences, 239, p.15002_1 - 15002_4, 2020/09

 被引用回数:0 パーセンタイル:0.1(Nuclear Science & Technology)

The OECD Nuclear Energy Agency (NEA) Working Party on International Nuclear Data Evaluation Cooperation (WPEC) was established in 1989 to facilitate collaboration in nuclear data activities. Over its thirty year history, fifty different subgroups have been created to address topics in nearly every aspect of nuclear data, including: experimental measurements, evaluation, validation, model development, quality assurance of databases and the development of software tools. After three decades we will review the status of WPEC, how it integrates other collections and activities organised by the NEA and how it dovetails with the initiatives of the IAEA and other bodies to effectively coordinate international activities in nuclear data.

論文

CIELO collaboration summary results; International evaluations of neutron reactions on uranium, plutonium, iron, oxygen and hydrogen

Chadwick, M. B.*; Capote, R.*; Trkov, A.*; Herman, M. W.*; Brown, D. A.*; Hale, G. M.*; Kahler, A. C.*; Talou, P.*; Plompen, A. J.*; Schillebeeckx, P.*; et al.

Nuclear Data Sheets, 148, p.189 - 213, 2018/02

 被引用回数:66 パーセンタイル:98.06(Physics, Nuclear)

CIELO国際協力では、原子力施設の臨界性に大きな影響を与える重要核種($$^{235}$$U, $$^{238}$$U, $$^{239}$$Pu, $$^{56}$$Fe, $$^{16}$$O, $$^{1}$$H)の中性子断面積データの精度を改善し、これまで矛盾していると考えられた点を解消することを目的として研究が行われた。多くの研究機関が参加したこのパイロットプロジェクトは、IAEAの支援も受けて、OECD/NEAの評価国際協力ワーキングパーティ(WPEC)のSubgroup 40として組織された。本CIELOプロジェクトは、新たな実験研究や理論研究を行う動機付けとなり、測定データを正確に反映し臨界性の積分テストに優れた新たな一連の評価済みライブラリとして結実した。本報告書は、これまでの研究成果と、本国際協力の次の段階の計画概要をまとめたものである。

論文

The CIELO collaboration; Progress in international evaluations of neutron reactions on Oxygen, Iron, Uranium and Plutonium

Chadwick, M. B.*; Capote, R.*; Trkov, A.*; Kahler, A. C.*; Herman, M. W.*; Brown, D. A.*; Hale, G. M.*; Pigni, M.*; Dunn, M.*; Leal, L.*; et al.

EPJ Web of Conferences, 146, p.02001_1 - 02001_9, 2017/09

 被引用回数:6 パーセンタイル:95.25(Nuclear Science & Technology)

CIELO共同研究では中性子断面積データの改善及びこれまでの評価で見られた断面積の不一致を解決することを目的として、原子力の臨界性に大きな影響を与える5核種($$^{16}$$O, $$^{56}$$Fe, $$^{235,238}$$U, $$^{239}$$Pu)の中性子断面積を評価している。この国際パイロットプロジェクトでは、経済協力開発機構・原子力機関・核データ評価国際協力ワーキングパーティに設置されたサブグループ40の下でIAEAからのサポートを受けて、実験並びに理論的な研究を活発に実施している。これらの研究を通じて測定データを精度よく反映し、さらに臨界性に関する積分テストで良い結果を示す新しい評価済ライブラリを開発している。

論文

The CIELO Collaboration; Neutron reactions on $$^1$$H, $$^{16}$$O, $$^{56}$$Fe, $$^{235,238}$$U, and $$^{239}$$Pu

Chadwick, M. B.*; Dupont, E.*; Bauge, E.*; Blokhin, A.*; Bouland, O.*; Brown, D. A.*; Capote, R.*; Carlson, A. D.*; Danon, Y.*; De Saint Jean, C.*; et al.

Nuclear Data Sheets, 118, p.1 - 25, 2014/04

 被引用回数:107 パーセンタイル:98.48(Physics, Nuclear)

CIELO(Collaborative International Evaluated Library Organization)は核反応データの評価作業を国際協力により実施するためのワーキンググループである。CIELOでは国際的な核データコミュニティから専門家を集め、既存の評価済ライブラリや測定データ、モデル計算の間にある矛盾を明らかにし、その原因を取り除き、より信頼性の高いデータを開発することを目的としている。最初の取り組みとして、最重要核種である$$^{1}$$H, $$^{16}$$O, $$^{56}$$Fe, $$^{235,238}$$U, $$^{239}$$Puを対象とする予定である。この論文ではこれらの最重要核種の評価済データ及び積分結果をレビューし、評価間の矛盾を調査する。また、この枠組みで実施する核データ評価に関する作業計画をまとめている。

論文

Meeting nuclear data needs for advanced reactor systems

原田 秀郎; 柴田 恵一; 西尾 勝久; 井頭 政之*; Plompen, A.*; Hambsch, F.-J.*; Schillebeeckx, P.*; Gunsing, F.*; Ledoux, X.*; Palmiotti, G.*; et al.

NEA/NSC/WPEC/DOC(2014)446, 111 Pages, 2014/02

This report includes investigations performed by the OECD/NEA/NSC Working Party on International Nuclear Data Evaluation Co-operation (WPEC) Subgroup 31, whose mission was to utilise the collective knowledge of the international nuclear data measurement community to consider the appropriate resources to address and meet the data needs quantified by WPEC Subgroup 26 for Advanced Reactor Systems. The members of Subgroup 31 performed reviews of uncertainty evaluations by evaluators, of state-of-art experimental techniques, of current experimental situations, and summarised an appropriate path to meet the requirements.

論文

ENDF/B-VII.1 nuclear data for science and technology; Cross sections, covariances, fission product yields and decay data

Chadwick, M. B.*; Herman, M.*; Oblo$v{z}$insk$'y$, P.*; Dunn, M. E.*; Danon, Y.*; Kahler, A. C.*; Smith, D. L.*; Pritychenko, B.*; Arbanas, G.*; Arcilla, R.*; et al.

Nuclear Data Sheets, 112(12), p.2887 - 2996, 2011/12

 被引用回数:2036 パーセンタイル:100(Physics, Nuclear)

原子力科学・技術の利用分野ための評価済み核データライブラリーENDF/B-VII.1を公開した。米国核データ評価委員会が中心となって評価・整備したこの最新ライブラリーは、前バージョン(ENDF/B-VII.0)公開以後に得られた原子核理論や実験に関する知見を反映した中性子断面積,共分散,核分裂収率や崩壊データ等を格納している。ライブラリーの主な更新内容は、核種数の拡大、共分散データの拡充、R行列理論に基づく軽核の共鳴パラメータ評価、中重核やアクチノイドデータの改訂等である。核外輸送コードMCNPによるベンチマーク解析を行った結果、臨界予測性能等のパフォーマンスが向上した。

論文

Neutron cross-section evaluations for $$^{70,72,73,74,76}$$Ge

岩本 修; Herman, M.*; Mughabghab, S. F.*; Oblozinsk$'y$, P.*; Trkov, A.*

AIP Conference Proceedings 769, p.434 - 437, 2005/05

ゲルマニウム同位体に対する新たな評価を、熱エネルギーから20eVの中性子に対して行った。光子の生成に特に注目した。共鳴領域で以前の評価と比較し、大きな改善が行われた。高速中性子領域の評価に計算コードEMPIRE-2.19を使用した。鉄及びニオブに対する計算を通じて、光子生成の妥当性の検証を行った。また、同位体の評価値から天然元素データを構成し、天然ゲルマニウムの実験データと比較を行った。光子生成に関するさまざまな量を示し、中性子入射エネルギーに対する強い依存性について議論を行う。

論文

Review of neutron cross-section evaluations for fission products

Oblozinsk$'y$, P.*; Herman, M.*; Mughabghab, S. F.*; Sirakov, I.*; Chang, J.*; 中川 庸雄; 柴田 恵一; 川合 將義*; Ignatyuk, A. V.*; Pronyaev, V. G.*; et al.

AIP Conference Proceedings 769, p.438 - 441, 2005/05

5つの主要評価済核データライブラリーに入っている核分裂生成物核種の断面積データをレビューした。本件は、評価国際協力ワーキングパーティ(WPEC)のサブグループ21の作業として行ったもので、原子番号31から68の範囲の核種に対する最善の評価済データを推奨することを目的としている。全部で、既に存在している211核種のデータを調査し、さらに新たな7核種のデータを加え、218核種に対する推奨値を決定した。

報告書

Hydrogen isotope separation study with the TSTA cryogenic distillation system; Two-column experiment with H-D-T

山西 敏彦; 吉田 浩; 福井 裕*; 内藤 大靖*; 平田 慎吾*; Sherman, R. H.*; K.M.Gruetzmacher*; Bartlit, J. R.*; Anderson, J. L.*

JAERI-M 88-254, 30 Pages, 1988/12

JAERI-M-88-254.pdf:0.6MB

深冷蒸留カスケードの実験が、TSTA同位体分離システムにおける2本の塔を用いてH-D-Tにより行われた。充填部の内容、高さが異なる両塔共に、総括のHETPが約5cmであり、また塔内においてほぼ均一であることが認められた。カスケードの動的挙動もまた考察され、基本的な制御手法が提示された。

口頭

Using a 3-D heat transport model (PeCUBE) to invert OSL- and ESR-derived rock cooling histories into erosion rate changes in the Hida Range of Japan

Anderson, L.*; Bartz, M.*; King, G.*; Fox, M.*; Herman, F.*; Stalder, N.*; Biswas, R.*; 末岡 茂; 塚本 すみ子*; Ahadi, F.*; et al.

no journal, , 

Optically stimulated luminescence (OSL) and electron spin resonance (ESR) thermochronometry have the potential to resolve continuous erosion histories from rapidly eroding settings. These thermochronometers are viable over the past few hundred thousand to a million years. These time periods are defined by persistent oscillations between warm and cold states. During the Quaternary, fundamental questions about the relationship between climate and erosion remain unanswered. With further development, the OSL and ESR thermochronometers could answer these questions. To realize this potential new strategies are required to invert low-temperature thermal histories for erosion rates. Here, we explore the use of PeCUBE (Braun, 2003), a three-dimensional finite-element model that simulates heat conduction and advection in the upper crust. As a training dataset we use cooling histories derived from eight samples from the Tateyama region in the Hida Mountains of Japan. The flexibility of PeCUBE allows us to quantify the role of time varying surface temperatures between glacial and interglacial periods. In high-relief settings the three-dimensionality of the topography, for example between valleys and ridges, can substantially perturb rock temperatures. PeCUBE allows us to quantify and remove these confounding topographic effects. We additionally explore the role of changing topographic relief on time varying thermal fields and erosion rates. Lastly, we explore a generous range of model parameters to quantify the sensitivity and robustness of our inversions.

口頭

Unravelling rock cooling histories of the Japanese Alps using ESR thermochronometry

Bartz, M.*; King, G.*; Anderson, L.*; Herman, F.*; 末岡 茂; 塚本 すみ子*; Ahadi, F.*; Gautheron, C.*; Delpech, G.*; Schwarz, S.*; et al.

no journal, , 

Electron spin resonance (ESR) thermochronometry has the potential to resolve continuous erosion histories from rapidly eroding settings over 10$$^{6}$$ time scales. These time periods are defined by persistent oscillations between warm and cold states. However, questions about the relationship between climate and erosion remain unanswered. We further develop ESR thermochronometry of quartz (Al and Ti centres) to answer these questions in the Tateyama region in the Hida Mountains of Japan. In the result, the Al and Ti centres in quartz can successfully be inverted to unravel rock cooling histories. As future work, all ESR signals will be converted together with OSL data, providing further constraints on their thermal histories.

口頭

Unravelling rock cooling histories of the Japanese Alps using trapped-charge thermochronometry

Bartz, M.*; King, G.*; Anderson, L.*; Herman, F.*; 末岡 茂; 塚本 すみ子*; 田上 高広*

no journal, , 

捕獲電子を用いた熱年代手法に基づいて、日本アルプス飛騨山脈の岩石試料を対象に冷却史の解明を試みた。

口頭

Rates of erosion in the Japanese Alps during the Quaternary; Insights from trapped charge thermochronometry

Bartz, M.*; King, G. E.*; Anderson, L.*; Herman, F.*; 末岡 茂; 塚本 すみ子*; 田上 高広*

no journal, , 

The Japanese Alps uplifted throughout the Quaternary and reached elevations of up to 3,000 m. However, understanding the interaction between rates of Earth surface processes, tectonics and climate is challenging, partly due to the difficulties of measuring changes in the rates of Earth surface processes at the timescale of glacial-interglacial cycles. In particular, the youth of the Japanese Alps has made measurement of their exhumation histories complicated. Here we investigate the potential of ultra-low temperature thermochronometers based on the luminescence and electron spin resonance (ESR) of feldspar and quartz minerals respectively for understanding changes in exhumation rates. We focus on Tateyama (Hida range), which was glaciated during the late Quaternary period. In total, eight samples were analysed by luminescence and ESR thermochronometry. While most luminescence signals have already reached their upper dating limit, ESR signals give insights into Pleistocene exhumation rates. We measured the ESR dose response and thermal decay properties of all samples, specifically targeting the Al and Ti centres. In general, thermal stability is higher for the Ti signals, resulting in ESR ages of between 0.5-0.9 Ma, although some signals are close to or above the upper dating limit of the Ti centre. In contrast, the Al signal still grows with time and is suitable for determining finite exhumation rates. Initial inversions reveal rock cooling rates on the order of 80 deg. C/Ma, which can be inverted to preliminarily rates of rock exhumation of <3 mm/a within the past 1 Ma. In the next step, we will relate these rates to the climatic (glacial) and tectonic history of the Tateyama region.

口頭

Eustatic change modulates exhumation in the Japanese Alps

King, G. E.*; Ahadi, F.*; 末岡 茂; Herman, F.*; Anderson, L.*; Gautheron, C.*; 塚本 すみ子*; Stalder, N.*; Biswas, R.*; Fox, M.*; et al.

no journal, , 

The exhumation of bedrock is controlled by the interplay between tectonics, surface processes and climate. The highest exhumation rates of cm/yr are recorded in zones of highly active tectonic convergence. Here, we use a combination of different thermochronometric systems, and notably trapped-charge thermochronometery, to show that such rates also occur in the Hida Range, Japanese Alps. Our results imply that cm/yr rates of exhumation may be more common than previously thought. The Hida Range is the most northern and most extensive of the Japanese Alps, and reaches elevations of up to 3000 m a.s.l. The Hida Range is thought to have uplifted in the last 3 Myr in response to E-W compression and magmatism. Our study focuses on samples from the Kurobe gorge, which is one of the steepest gorges in Japan. Previous work has shown that exhumation rates in this region are exceptionally high, as documented by the exposure of the ~0.8 Ma Kurobe granite in the gorge. We combined 12 new zircon (U-Th/He) ages and 11 new OSL-thermochronometry ages together with existing thermochronometric data to investigate the late Pleistocene exhumation of this region. We found that exhumation rates increased to ~10 mm/yr within the past 300 kyr, likely in response to river base-level fall that increased channel steepness due to climatically controlled eustatic changes. Our data allow the development of time-series of exhumation rate changes at the timescale of glacial-interglacial cycles and show a four-fold increase in baseline rates over the past ~65 kyr. This increase in exhumation rate is likely explained by knickpoint propagation due to a combination of very high precipitation rates, climatic change, sea-level fall, range-front faulting and moderate rock uplift. Our data show that in regions with horizontal convergence, coupling between climate, surface processes and tectonics can exert a significant effect on rates of exhumation.

口頭

Working towards a robust thermochronometer based on the ESR of quartz minerals

King, G.*; Bartz, M.*; Bossin, L.*; Wen, X.*; 塚本 すみ子*; Herman, F.*; 小形 学; 末岡 茂

no journal, , 

Electron spin resonance dating of quartz minerals offers a significant advantage over luminescence dating because of its later signal saturation. We are seeking to exploit this to build upon earlier studies in the development of a thermochronometry system capable of resolving rock cooling rates throughout the Quaternary. In order to determine a rock cooling history, it is necessary to constrain both signal accumulation and signal thermal loss robustly within the laboratory. We have collated a series of geological samples including rocks from boreholes that have known isothermal histories to investigate the potential of this technique. Our objective is to use the latter rocks to confirm the validity of our laboratory measurements and data-fitting/numerical models. Specifically, we have investigated known-thermal history samples from the MIZ1 borehole (Japan) and the KTB borehole (Germany). Preliminary data reveal that the ESR dose response and thermal decay of different quartz samples is highly variable.

口頭

Will ESR thermochronometry reveal the timing of Rh$^o$ne valley incision?

King, G. E.*; Wen, X.*; Bartz, M.*; Anderson, L.*; Bossin, L.*; 塚本 すみ子*; Li, Y.*; Herman, F.*; 小形 学; 末岡 茂

no journal, , 

To determine a rock cooling history using ESR thermochronometry, signal accumulation and signal thermal loss must be robustly determined within the laboratory. We have collected a series of geological samples including rocks from boreholes that have known isothermal histories to investigate the potential of this technique. Our objective is to use the latter rocks to confirm the validity of our laboratory measurements and data-fitting/numerical models. Specifically, we have investigated known-thermal history samples from the MIZ1 borehole (Japan) and the KTB borehole (Germany) as well as samples from Sion in the Western European Alps. Preliminary data reveal that the ESR dose response and thermal decay of different quartz samples is highly variable. Whereas the Al-centre of some samples exhibits linear dose response to laboratory irradiation up to 15 kGy, the Al-centre of other samples exhibits exponential, or double exponential growth and saturates at doses of 3-4 kGy. The Ti-centre of most samples is well described by a single saturating exponential function, however samples from the MIZ1 borehole exhibit pronounced sub-linearity in the low-dose response region. Furthermore, whereas for some samples the Al-centre is less thermally stable than the Ti-centre, for other samples the inverse is observed. These observations suggest that a uniform measurement protocol and data-fitting approach may not be appropriate for quartz ESR data. Inversion of two KTB samples yielded temperatures within uncertainty of borehole temperature, however results for the MIZ1 borehole are more variable and can only recover temperature at best within c.a. 10%. Investigations into the cause of the poor results for the MIZ1 borehole are ongoing (i.e. measurement protocol, data-fitting/numerical model) and will be discussed. Preliminary data from Sion are promising and reveal consistent cooling rates.

口頭

High-relief exhumation history in the Japanese Alps within the past 1 Ma inferred from trapped charge thermochronometry

Bartz, M.*; King, G. E.*; Herman, F.*; Anderson, L.*; 末岡 茂; 塚本 すみ子*; 田上 高広*

no journal, , 

The interaction between rates of Earth surface processes, climate and tectonics determines the landscape in mountain regions. The Japanese Alps uplifted throughout the Quaternary and now reach elevations of up to 3,000 m. However, quantifying relief changes in response to tectonic activity, magmatism and Late Quaternary glaciation is challenging due to the young age of the Japanese Alps and the difficulty of measuring surface processes at the timescale of glacial-interglacial cycles. Here, we use ultra-low temperature thermochronometers based on the luminescence of feldspar minerals and the electron spin resonance (ESR) of quartz minerals, in combination with inverse modelling to derive rock cooling rates and time series of exhumation rates at 10$$^{4}$$-10$$^{6}$$ years timescales. We focus on the Tateyama region in the Hida range of the Japanese Alps, which was glaciated during the late Quaternary period. In total, 19 new samples were analyzed by luminescence and ESR thermochronometry. While most luminescence signals have already reached their upper dating limit, ESR signals (Al and Ti centres) yielded ESR ages of between 0.5-0.9 Ma. In general, thermal stability is lower for the Al centre compared to that of the Ti centre, but both centres constrain similar exhumation rates. Inversions reveal rock cooling rates on the order of 30-80 deg. C/Ma, which can be inverted to exhumation rates of less than 1 mm/a within the past 1 Ma. In the next step, we will relate the exhumation rates to the glacial and tectonic history of the Tateyama region.

口頭

Unravelling rock cooling histories of the Japanese Alps within the past 1 Ma using ESR and OSL thermochronometry

Bartz, M.*; King, G. E.*; Herman, F.*; Anderson, L.*; 末岡 茂; 塚本 すみ子*; 田上 高広*

no journal, , 

To resolve exhumation histories of the Japanese Alps throughout the Quaternary, we investigate the potential of ultra-low temperature thermochronometers based on the luminescence of feldspar minerals and electron spin resonance (ESR) of quartz minerals, in combination with inverse modelling to derive rock cooling rates and exhumation rates histories at 10$$^{4}$$-10$$^{6}$$ years timescales. We focus on the Tateyama region in the Hida range of the Japanese Alps. In total, 19 new samples were analyzed by luminescence and ESR thermochronometry. While most luminescence signals have already reached saturation, ESR signals (Al and Ti centres) still grow with dose and are suitable for determining finite exhumation rates in the Tateyama region. We used the ESR single aliquot regenerative additive (SARA) dose protocol for dose evaluation including protocol optimization (i.e., preheat-plateau test). We checked for sensitivity changes due to the high-temperature annealing step within the SARA procedure using SARA vs. single aliquot additive dose response, repeated dose points (i.e., recycling ratio) and dose recovery of an artificially zeroed sample. Thermal stabilities of the ESR signals were analysed by using isothermal decay experiments and simulations of the isothermal decay using the experimentally constrained kinetic parameters. Our experiments showed insignificant sensitivity changes during measurements, resulting in Al and Ti ages of between 0.3-0.9 Ma and 0.5-1.1 Ma, respectively. In general, thermal stability is lower for the Al centre compared to that of the Ti centre but simulations yielded valuable thermal stability over Quaternary timescales for both ESR centres. Inversions reveal rock cooling rates on the order of 30-80 deg. C/Ma, much lower than those of the luminescence thermochronometry technique, which helps to resolve erosion rates histories on the order of few mm/a. Thus, preliminary erosion rates of $$<$$1 mm/a within the past 1 Ma could be inverted.

口頭

Borehole calibration of ESR thermochronometry

King, G. E.*; Wen, X.*; Bartz, M.*; Bossin, L.*; 塚本 すみ子*; Li, Y.*; Herman, F.*; 小形 学; 末岡 茂

no journal, , 

Whereas the luminescence thermochronometry system is limited to areas experiencing very rapid rock cooling (exhumation) of 10s of mm/yr, our data indicate that ESR thermochronometry can resolve rates of $$<$$1 mm/yr over Quaternary timescales. To determine a rock cooling history using ESR thermochronometry, signal accumulation and signal thermal loss must be robustly determined within the laboratory. We have collected a series of borehole samples with known isothermal histories to investigate the potential of this technique. Our objective is to use the latter rocks to confirm the validity of our laboratory measurements and data-fitting/numerical models by using the ESR-thermochronometry method to recover their known in-situ temperatures. Specifically, we have investigated known-thermal history samples from the MIZ1 borehole (Japan) and the KTB borehole (Germany). Preliminary data reveal that the ESR dose response and thermal decay of different quartz samples is highly variable. Whereas the Al-centre of some samples exhibits linear dose response to laboratory irradiation up to 15 kGy, the Al-centre of other samples exhibits exponential, or double-exponential growth and saturates at doses of 3-4 kGy. The Ti-centre of most samples is well described by a single saturating exponential function, however samples from the MIZ1 borehole exhibit pronounced sublinearity in the low-dose response region. Furthermore, whereas for some samples the Al-centre is less thermally stable than the Ti-centre, for other samples the inverse is observed. These observations suggest that a uniform measurement protocol and data-fitting approach may not be appropriate for quartz ESR data.

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