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Jeong, S. G.*; Kwon, J.*; Kim, E. S.*; Prasad, K.*; Harjo, S.; Gong, W.; 川崎 卓郎; Estrin, Y.*; Bouaziz, O.*; Hong, S. I.*; et al.
Materials Science & Engineering A, 942, p.148712_1 - 148712_11, 2025/10
The cellular structure plays a key role in determining the mechanical properties of metal additive manufacturing (MAM) components. This study presents in situ neutron diffraction and dislocation density-based modeling for a CoCrFeMnNi high-entropy alloy (HEA) made via directed energy deposition (DED). A constitutive model based on the Kocks-Mecking-Estrin framework was used to represent the cellular structure. Parametric analysis showed lower dislocation accumulation and annihilation rates in the as-built sample (with cellular structure) than in the heat-treated one. These differences are linked to dislocation forest networks and local stacking fault energy variations. Dislocation density across cell interiors and walls was also compared with deformation-induced dislocation cells.
ders band-assisted high uniform ductility in ultrastrong ferrous medium-entropy alloy via hierarchical microstructureKwon, H.*; Lee, J. H.*; Zargaran, A.*; Harjo, S.; Gong, W.; Wang, J.*; Gu, G. H.*; Lee, B.-J.*; Bae, J. W.*; Kim, H. S.*
International Journal of Plasticity, 190, p.104378_1 - 104378_18, 2025/07
被引用回数：0 パーセンタイル：79.09(Engineering, Mechanical)In this work, we harness a hierarchical microstructure to simultaneously tailor strengthening and deformation mechanisms in a Co
Cr
Fe
Ni
Mo
(at%) ferrous medium-entropy alloy (MEA). A simple thermomechanical process (cold rolling and 90 s annealing) produces ultrafine recrystallized grains, non-recrystallized grains with substructures, and intragranular nanoprecipitates. This structure, with high dislocation density and fine grains, yields a high strength of 
1.60 GPa but can risk premature fracture. To overcome this, Lders deformation, enabled by ultrafine grain boundaries and stress-induced martensitic transformation at pre-existing nucleation sites, is employed. Stable Lders band propagation delays strain hardening and enables large uniform ductility. As a result, a tensile strength of 1.84 GPa and uniform elongation of 20% are achieved, matching the best tensile properties among reported multi-principal element alloys.
Gu, G. H.*; Jeong, S. G.*; Heo, Y.-U.*; Harjo, S.; Gong, W.; Cho, J.*; Kim, H. S.*; 他4名*
Journal of Materials Science & Technology, 223, p.308 - 324, 2025/07
被引用回数：1 パーセンタイル：85.58(Materials Science, Multidisciplinary)Face-centered cubic (FCC) equi-atomic multi-principal element alloys (MPEAs) exhibit excellent mechanical properties from cryogenic to room temperatures. At room temperature, deformation is dominated by dislocation slip, while at cryogenic temperatures (CTs), reduced stacking fault energy enhances strain hardening with twinning. This study uses in-situ neutron diffraction to analyze the temperature-dependent deformation behavior of Al
(CoNiV)
, a dual-phase (FCC/BCC) medium-entropy alloy (MEA). At liquid nitrogen temperature (LNT), deformation twinning in the FCC matrix leads to additional strain hardening through the dynamic Hall-Petch effect, giving the appearance of improved strengthening at LNT. In contrast, BCC precipitates show dislocation slip at both 77 K and 298 K, with temperature-dependent lattice friction stress playing a significant role in strengthening. The study enhances understanding of deformation behaviors and provides insights for future alloy design.
magnetic orderings in a triangular lattice; Implications for multi- orderings in general two-dimensional latticesPark, P.*; Cho, W.*; Kim, C.*; An, Y.*; 飯田 一樹*; 梶本 亮一; Matin, S.*; Zhang, S.-S.*; Batista, C. D.*; Park, J.-G.*
Physical Review X, 15(3), p.031032_1 - 031032_29, 2025/07
Multi- magnetic structures on two-dimensional (2D) lattices provide a key route to realizing topological physics in 2D magnetism. A major experimental challenge is to unambiguously confirm their formation by excluding the possibility of topologically trivial multi-domain single- or double- magnetic orders, which cannot be distinguished using conventional diffraction techniques. Here, we propose that long-wavelength spin dynamics offers a universal diagnostic for triangular lattices: triple- orders that preserve rotational symmetry and single- or double- orders that break it exhibit qualitatively distinct anisotropies in their Goldstone mode velocities, stemming from fundamental differences in their underlying spin configurations. We validate this concept using the metallic triangular-lattice antiferromagnet Co
TaS
, which hosts both a stripe-type single- state and a triple- tetrahedral ordering at different temperatures. Using inelastic neutron-scattering and spin dynamics simulations, we first refine the spin Hamiltonian by fitting the paramagnetic excitation spectra, allowing us to develop an unbiased model independent of magnetic ordering. We then show that the observed velocity profiles of the Goldstone modes agree with the high-temperature model's predictions: markedly anisotropic for the single- phase and near isotropic for the triple- phase. Importantly, this contrast persists across various exchange parameters, highlighting its model-independent nature and suggesting potential applicability to other 2D lattice systems. Beyond the long-wavelength regime, we present a substantial discrepancy between the measured and simulated magnon spectra exclusively in the triple- phase. We attribute this discrepancy to magnon energy renormalization arising from order-of-magnitude-enhanced magnon-magnon interactions in the triple- phase, due to its noncollinear configuration. This work provides universal insight into the dynamical properties of topological multi- magnetic orderings in 2D lattice structures, offering a broadly applicable diagnostic to distinguishing them from topologically trivial single- or double- counterparts. The unequivocal confirmation of the triple- structure in CoTaS further establishes it as a prominent material platform for exploring topological spin textures in the genuine 2D limit.
Cho, S. H.*; Cho, S. W.*; Lv, Z.*; 関根 由莉奈; Liu, S.*; Zhou, M.*; Nuxoll, R. F.*; Kanatzidis, E. E.*; Ghaffari, R.*; Kim, D.*; et al.
Lab on a Chip, 25(7), p.1647 - 1655, 2025/04
被引用回数：1 パーセンタイル：97.42(Biochemical Research Methods)アミノ酸は体内のタンパク質合成と代謝プロセスに不可欠な物質である。本研究では、運動中の汗からのアミノ酸損失について定量的に調べることを目的とした。汗中のアミノ酸含有量をリアルタイムで分析するため、測定のための技術基盤としてウェアラブルなマイクロ流体システムを構築した。定量分析を実現するため、ウェアラブルデバイスに蛍光アッセイを組み込み、さらにスマートフォンベースの画像化技術を統合させたシステムを開発した。
浪江 将成; 斉藤 淳一; 岡 涼太郎*; Kim, J.-H.*
Vacuum, 234, p.114038_1 - 114038_9, 2025/04
被引用回数：0 パーセンタイル：0.00(Materials Science, Multidisciplinary)Wettability of titanium (Ti) and surface-modified (Oxidized or Fluorinated) Ti with liquid sodium (Na) were investigated via experiments and theoretical calculations. From the experimental results, a sliding angle of Na droplet on oxidized Ti was smaller than that on untreated Ti, indicating the worsening of wettability by oxidation. In contrast, the sliding angle of Na droplet on fluoridated Ti was larger than that on untreated Ti, indicating an improvement in wettability by fluorination. Additionally, the cluster models for the interface between Na droplets and treated or untreated Ti were constructed for theoretical calculations of electronic states at the interface, covalent and ionic bonds at the interface were evaluated from the calculation results. The sliding angles obtained in the wettability tests and the strength of covalent bonding at the interface showed no correlation, but good correlation was observed between the sliding angles and ionic bonding at the interface. Thus, the wettability of surface-modified Ti with liquid Na can be theoretically understood based on the atomic interactions at the interface.
Kim, M.*; Lee, C.*; 杉田 裕; Kim, J.-S.*; Jeon, M.-K.*
Geomechanics for Energy and the Environment, 41, p.100628_1 - 100628_9, 2025/03
被引用回数：1 パーセンタイル：61.45(Energy & Fuels)この研究では、DECOVALEX-2023プロジェクトの一環として幌延の地下研究施設で実施された実規模大の人工バリア試験の数値解析を使用して、非等温二相流のモデリングに対する主要変数の選択の影響を調査した。検証済みの数値モデルを使用して、人工バリアシステム内の不均質多孔質媒体の熱-水連成挙動を解析した。支配方程式を離散化する際の2つの異なる主要変数スキームを比較したところ、結果に大きな違いがあることが明らかになった。
Chung, J.-H.*; Kwangwoo, S.*; Yokoo, Tetsuya R.; 植田 大地*; 今井 正樹; Kim, H.-S.; Kiem, D. H.; Han, M. J.*; 社本 真一
Scientific Reports (Internet), 15, p.5978_1 - 5978_10, 2025/02
被引用回数：0 パーセンタイル：61.64(Multidisciplinary Sciences)Two dimensional honeycomb ferromagnets host massless Dirac magnons which are a bosonic analogue of Dirac fermions in graphene. The Dirac magnons may become massive and topological when the time-reversal symmetry breaks and an energy gap opens up at the Dirac point, which was experimentally observed in Cr
-based van der Waals magnets. Here, we investigate the spin wave excitations in the 
magnetic oxide FeTiO with Fe
electrons (
). Using inelastic neutron scattering, we observe two magnon bands separated by a 1.2-meV gap at the Dirac points indicating that its Dirac magnons are massive. Using the linear spin-wave and density functional theory calculations, we find that the spin-orbit-coupled antisymmetric Dzyaloshinskii-Moriya exchanges can best account for the observed Dirac gap opening. The associated Berry curvature and Chern number (
) indicate that FeTiO hosts topological spin excitations via time-reversal symmetry breaking of Dirac magnons.
signatures in two-dimensional cone beam interferometrySarenac, D.*; Gorbet, G.*; Clark, C. W.*; Cory, D. G.*; Ekinci, H.*; Henderson, M. E.*; Huber, M. G.*; Hussey, D. S.*; Kapahi, C.*; Kienzle, P. A.*; et al.
Physical Review Research (Internet), 6(3), p.L032054_1 - L032054_8, 2024/09
Neutron interferometry has played a distinctive role in fundamental science and characterization of materials. Moir neutron interferometers are candidate next-generation instruments: they offer microscopy-like magnification of the signal, enabling direct camera recording of interference patterns across the full neutron wavelength spectrum. Here we demonstrate the extension of phase-grating moir interferometry to two-dimensional geometries. Our measurements of phase topologies and gravitationally induced phase shifts are in good agreement with theory.
浪江 将成; 斉藤 淳一; 池田 明日香; 岡 涼太郎*; Kim, J.-H.*
Surfaces (Internet), 7(3), p.550 - 559, 2024/09
The iron (Fe) specimens selected as the substrate metal for this study were surface-treated using fluorine gas, and their wettability with liquid sodium (Na) was evaluated using the sliding angle. Additionally, the surface morphology and binding state were analyzed, and the applicability of wettability control with liquid sodium by fluorination was discussed using the analysis results. Fluorination formed a fluoride layer comprising FeF and FeF
bonds on the iron surface. The composition of the fluoride layer varied, depending on the treatment conditions. The surface of the specimen that contains a lot of FeF bonds had a small sliding angle for the liquid sodium droplet and was harder to wet than the untreated specimen. In contrast, the surface of the specimen that contains a lot of FeF bonds had a large sliding angle for the liquid sodium droplet and was easier to wet than the untreated specimen. These results indicate that fluorination is an effective surface modification technique that can be applied to control the wettability of iron with liquid sodium.
Nguyen, T.-D.*; Singh, C.*; Kim, Y. S.*; Han, J. H.*; Lee, D.-H.*; Lee, K.*; Harjo, S.; Lee, S. Y.*
Journal of Materials Research and Technology, 31, p.1547 - 1556, 2024/07
被引用回数：6 パーセンタイル：74.94(Materials Science, Multidisciplinary)This study investigates the mechanical properties of a friction-stir-welded (FSW) AA6061-T6 aluminum alloy at ultra-low temperature (ULT) of 20 K. In-situ neutron diffraction and orientation imaging microscopy were employed to compare the tensile deformation behavior of the base metal (BM) and heat-affected zone (HAZ) in the FSW aluminum plate. The results demonstrate that compared to room-temperature (RT), ULT induces a significant improvement in tensile strength and ductility in both the BM and HAZ. The enhanced mechanical properties in BM at ULT result from a more homogeneous deformation than occurs at RT. On the other hand, HAZ at ULT exhibits an even lower yield strength than at RT, but the strain hardening rate (SHR) is the most significant among the alloys, leading to a tensile strength of 346 MPa and the highest ductility of 46.8%. The lowest yield strength corresponds to the lowest-hardness zones in HAZ, caused by dissolved/coarsened precipitates during the FSW process.
Kim, J.*; Thompson, B. R.*; 富永 大輝*; 大澤 崇人; 江上 毅*; F
rster, S.*; Ohl, M.*; Senses, E.*; Faraone, A.*; Wagner, N. J.*
ACS Macro Letters (Internet), 13(6), p.720 - 725, 2024/06
被引用回数：2 パーセンタイル：23.55(Polymer Science)準弾性中性子散乱(QENS)を用いて、モデルナノ複合材料であるポリエチレンオキシド(PEO)/シリカナノ粒子(NPs)中のポリマー鎖のラウスダイナミクスを調べた。ポリマー鎖の見かけのラウス速度は粒子負荷が増加するにつれて減少した。しかし、数十psの時間スケールでは、不動なセグメント集団の証拠はない。ダイナミクスの鈍化は、NP相間領域における鎖の修正ラウスモデルの観点から解釈される。こうして、バルクのような鎖集団とラウスモードの抑制を特徴とする鎖集団の2つが同定された。相間領域の空間的な広がりは、吸着層の厚さの約2倍、約2nmと見積もられた。これらの結果は、NPs表面における連鎖ダイナミクスの抑制を詳細に説明するものである。これらの結果は、表面効果と閉じ込めに関する関連した洞察であり、十分に分散したNPを有するポリマーナノコンポジット(PNC)のレオロジー特性を理解するための基礎を提供するものである。
Kim, Y. S.*; Chae, H.*; Lee, D.-Y.*; Han, J. H.*; Hong, S.-K.*; Na, Y. S.*; Harjo, S.; 川崎 卓郎; Woo, W.*; Lee, S.-Y.*
Materials Science & Engineering A, 899, p.146453_1 - 146453_7, 2024/05
被引用回数：7 パーセンタイル：79.07(Nanoscience & Nanotechnology)This work focused on the mechanical properties and serration-involved deformation behavior of advanced alloys at 15 K. Evolution of stacking faults and 
-martensite improved the mechanical performance of CoCrNi alloys, and significant strain-induced martensite transformation of DED-SS316L led to superior strength and strain hardening. A magnitude in stress drop was governed by dislocation density, phase type, and lattice defects, irrespective of processing method. FCC {200} notably was influenced recovery behavior after stress drop, and the contribution of strain energy density by serration on tensile toughness was the greatest for HR-CoCrNi.
Linh, B. D.*; Corsi, A.*; Gillibert, A.*; Obertelli, A.*; Doornenbal, P.*; Barbieri, C.*; Duguet, T.*; G
mez-Ramos, M.*; Holt, J. D.*; Hu, B. S.*; et al.
Physical Review C, 109(3), p.034312_1 - 034312_15, 2024/03
被引用回数：3 パーセンタイル：67.20(Physics, Nuclear)理化学研究所RIビームファクトリーにて中性子過剰核
Arビームからの1中性子ノックアウト反応実験を行い、
Arのエネルギー準位および分光学的因子を導出した。特に、第一励起状態の
への分光学的因子が大きいことから、始状態のArの基底状態において中性子が
軌道を多く占めていることがわかった。これは、中性子数32がよい魔法数として知られる
Caとは異なった性質であり、カルシウムからアルゴンへと陽子が2個減ることで閉殻構造が大きく崩れることが明らかになった。
TaSPark, P.*; Cho, W.*; Kim, C.*; An, Y.*; Avdeev, M.*; 飯田 一樹*; 梶本 亮一; Park, J.-G.*
Physical Review B, 109(6), p.L060403_1 - L060403_7, 2024/02
被引用回数：8 パーセンタイル：87.36(Materials Science, Multidisciplinary)Spontaneous Hall conductivity has recently been reported in the triangular lattice antiferromagnet CoTaS under a zero magnetic field. This phenomenon originates from the distinctive noncoplanar triple- magnetic ground state, possessing uniform real-space Berry curvature characterized by scalar spin chirality. We investigated the physical properties of CoTaS by judiciously controlling the composition, revealing a drastic change in its bulk properties, even by slight variations in cobalt composition, despite the same crystal structure. For 
, Co
TaS keeps all the characteristics of the ground state consistent with the previous studies - two antiferromagnetic phase transitions at 
and 
(
), a large spontaneous Hall conductivity [
], and a weak ferromagnetic moment along the 
axis. However, samples with 
exhibit distinct bulk properties, including the absence of both and the weak ferromagnetic moment. Our neutron diffraction data reveal that CoTaS with develops coplanar helical magnetic order with 
. This is entirely different from what has been seen in 
, explaining the observed composition dependence.
TaSPark, P.*; Cho, W.*; Kim, C.*; An, Y.*; Kang, Y.-G.*; Avdeev, M.*; Sibille, R.*; 飯田 一樹*; 梶本 亮一; Lee, K. H.*; et al.
Nature Communications (Internet), 14, p.8346_1 - 8346_9, 2023/12
被引用回数：28 パーセンタイル：90.63(Multidisciplinary Sciences)The triangular lattice antiferromagnet (TLAF) has been the standard paradigm of frustrated magnetism for several decades. The most common magnetic ordering in insulating TLAFs is the 120
structure. However, a new triple- chiral ordering can emerge in metallic TLAFs, representing the short wavelength limit of magnetic skyrmion crystals. We report the metallic TLAF CoTaS as the first example of tetrahedral triple- magnetic ordering with the associated topological Hall effect (non-zero 
). We also present a theoretical framework that describes the emergence of this magnetic ground state, which is further supported by the electronic structure measured by angle-resolved photoemission spectroscopy. Additionally, our measurements of the inelastic neutron scattering cross section are consistent with the calculated dynamical structure factor of the tetrahedral triple- state.
Liao, L.*; Puebla, J.*; 山本 慧; Kim, J.*; 前川 禎通*; Hwang, Y.*; Ba, Y.*; 大谷 義近*
Physical Review Letters, 131(17), p.176701_1 - 176701_6, 2023/10
被引用回数：9 パーセンタイル：77.31(Physics, Multidisciplinary)Phonons and magnons are engineered by periodic potential landscapes in phononic and magnonic crystals, and their combined studies may enable valley phonon transport tunable by the magnetic field. Through nonreciprocal surface acoustic wave transmission, we demonstrate valley-selective phonon-magnon scattering in magnetoelastic superlattices. The lattice symmetry and the out-of-plane magnetization component control the sign of nonreciprocity. The phonons in the valleys play a crucial role in generating nonreciprocal transmission by inducing helical strains that couple with the magnons. The transmission spectra show a nonreciprocity peak near a transmission gap, matching the phononic band structure. Our results open the way for manipulating valley phonon transport through periodically varying magnon-phonon coupling.
Yang, D. S.*; Wu, Y.*; Kanatzidis, E. E.*; Avila, R.*; Zhou, M.*; Bai, Y.*; Chen, S.*; 関根 由莉奈; Kim, J.*; Deng, Y.*; et al.
Materials Horizons, 10(11), p.4992 - 5003, 2023/09
被引用回数：21 パーセンタイル：85.14(Chemistry, Multidisciplinary)本論文では、ハード及びソフトハイブリッド材料システムでの3Dプリントによって形成されたマイクロ流体ネットワーク、統合バルブ、およびマイクロスケール光学キュベットにより、汗成分に対してその場で分光および蛍光分析した成果を紹介する。一連の試験により、これらのマイクロキュベットシステムが汗中の銅、塩化物、グルコースの濃度と汗のpHを実験室レベルの精度と感度で評価できることが実証された。
O近藤 洋介*; Achouri, N. L.*; Al Falou, H.*; Atar, L.*; Aumann, T.*; 馬場 秀忠*; Boretzky, K.*; Caesar, C.*; Calvet, D.*; Chae, H.*; et al.
Nature, 620(7976), p.965 - 970, 2023/08
被引用回数：32 パーセンタイル：95.20(Multidisciplinary Sciences)非常に中性子が過剰な原子核Oは、陽子、中性子ともに魔法数であることから古くからその性質に興味が持たれていたが、酸素の最後の束縛核
Oよりも中性子が4個も多いため、これまで観測されてこなかった。この論文では、理化学研究所RIBFにて
Fからの1陽子ノックアウト反応によってOを生成し、そこから放出される中性子を測定することによって初めてその観測に成功した。核構造の観点からは、Oでは二重閉殻が保たれているか興味が持たれていたが、実験で得られた分光学的因子が殻模型計算で予言されて程度の大きいことから、閉殻構造をもたない可能性が高いことがわかった。
Ca cast doubt on a doubly magic 
CaChen, S.*; Browne, F.*; Doornenbal, P.*; Lee, J.*; Obertelli, A.*; 角田 佑介*; 大塚 孝治*; 茶園 亮樹*; Hagen, G.*; Holt, J. D.*; et al.
Physics Letters B, 843, p.138025_1 - 138025_7, 2023/08
被引用回数：9 パーセンタイル：82.79(Astronomy & Astrophysics)
Scからの1陽子ノックアウト反応を用いて、
Caと
Caのガンマ崩壊を観測した。Caでは1456(12)keVの
線遷移が、Caでは1115(34)keVの遷移が観測された。どちらの遷移も暫定的に
と割り当てられた。有効核子間相互作用をわずかに修正した広い模型空間での殻模型計算では、
準位エネルギー、2中性子分離エネルギー、反応断面積が実験とよく一致し、N=34閉殻の上に新しい殻が形成されていることを裏付けた。その構成要素である
と
軌道はほぼ縮退しており、これはCaが二重魔法核である可能性を排除し、Ca同位体のドリップラインを
Caあるいはそれ以上にまで広げる可能性がある。
