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Uniaxial pressure effect on the magnetic ordered moment and transition temperatures in BaFe$$_{2-x}$$T$$_{x}$$As$$_{2}$$ ($$T$$ = Co,Ni)

Tam, D. M.*; Song, Y.*; Man, H.*; Cheung, S. C.*; Yin, Z.*; Lu, X.*; Wang, W.*; Frandsen, B. A.*; Liu, L.*; Gong, Z.*; et al.

Physical Review B, 95(6), p.060505_1 - 060505_6, 2017/02

 被引用回数:18 パーセンタイル:75.96(Materials Science, Multidisciplinary)

We use neutron diffraction and muon spin relaxation to study the effect of in-plane uniaxial pressure on the antiferromagnetic (AF) orthorhombic phase in BaFe$$_{2-x}$$T$$_{x}$$As$$_{2}$$ and its Co- and Ni-substituted members near optimal superconductivity. In the low-temperature AF ordered state, uniaxial pressure necessary to detwin the orthorhombic crystals also increases the magnetic ordered moment, reaching an 11% increase under 40 MPa for BaFe$$_{1.9}$$Co$$_{0.1}$$As$$_2$$, and a 15% increase for BaFe$$_{1.915}$$Ni$$_{0.085}$$As$$_2$$. We also observe an increase of the AF ordering temperature ($$T_N$$) of about 0.25 K/MPa in all compounds, consistent with density functional theory calculations that reveal better Fermi surface nesting for itinerant electrons under uniaxial pressure. The doping dependence of the magnetic ordered moment is captured by combining dynamical mean field theory with density functional theory, suggesting that the pressure-induced moment increase near optimal superconductivity is closely related to quantum fluctuations and the nearby electronic nematic phase.


Volume-wise destruction of the antiferromagnetic Mott insulating state through quantum tuning

Frandsen, B. A.*; Liu, L.*; Cheung, S. C.*; Guguchia, Z.*; Khasanov, R.*; Morenzoni, E.*; Munsie, T. J. S.*; Hallas, A. M.*; Wilson, M. N.*; Cai, Y.*; et al.

Nature Communications (Internet), 7, p.12519_1 - 12519_8, 2016/08

 被引用回数:20 パーセンタイル:73.09(Multidisciplinary Sciences)

RENiO$$_3$$ (RE = rare-earth element) and V$$_2$$O$$_3$$ are archetypal Mott insulator systems. When tuned by chemical substitution (RENiO$$_3$$) or pressure (V$$_2$$O$$_3$$), they exhibit a quantum phase transition (QPT) between an antiferromagnetic Mott insulating state and a paramagnetic metallic state. Because novel physics often appears near a Mott QPT, the details of this transition, such as whether it is first or second order, are important. Here, we demonstrate through muon spin relaxation/rotation experiments that the QPT in RENiO$$_3$$ and V$$_2$$O$$_3$$ is first order: the magnetically ordered volume fraction decreases to zero at the QPT, resulting in a broad region of intrinsic phase separation, while the ordered magnetic moment retains its full value until it is suddenly destroyed at the QPT. These findings bring to light a surprising universality of the pressure-driven Mott transition, revealing the importance of phase separation and calling for further investigation into the nature of quantum fluctuations underlying the transition.


Li(Zn,Mn)As as a new generation ferromagnet based on a I-II-V semiconductor

Deng, Z.*; Jin, C. Q.*; Liu, Q. Q.*; Wang, X. C.*; Zhu, J. L.*; Feng, S. M.*; Chen, L. C.*; Yu, R. C.*; Arguello, C.*; 後神 達郎*; et al.

Nature Communications (Internet), 2, p.1425_1 - 1425_5, 2011/08

 被引用回数:137 パーセンタイル:93.89(Multidisciplinary Sciences)



Muon spin rotation measurements of heterogeneous field response in overdoped La$$_{2-x}$$Sr$$_{x}$$CuO$$_{4}$$

MacDougall, G. J.*; Savici, A. T.*; Aczel, A. A.*; Birgeneau, R. J.*; Kim, H.*; Kim, S.-J.*; 伊藤 利充*; Rodriguez, J. A.*; Russo, P. L.*; 植村 泰朋*; et al.

Physical Review B, 81(1), p.014508_1 - 014508_7, 2010/01

 被引用回数:9 パーセンタイル:43.25(Materials Science, Multidisciplinary)

Transverse-field muon spin rotation measurements of overdoped La$$_{2-x}$$Sr$$_{x}$$CuO$$_{4}$$ reveal a large broadening of the local magnetic field distribution in response to applied field, persisting to high temperatures. The field response is approximately Curie-Weiss-like in temperature and is largest for the highest doping investigated. Such behavior is contrary to the canonical Fermi-liquid picture commonly associated with the overdoped cuprates and implies extensive heterogeneity in this region of the phase diagram. A possible explanation for the result lies in regions of staggered magnetization about dopant cations, analogous to what is argued to exist in underdoped systems.


Absence of broken time-reversal symmetry in the pseudogap state of the high temperature La$$_{2-x}$$Sr$$_{x}$$CuO$$_{4}$$ superconductor from muon-spin-relaxation measurements

MacDougall, G. J.*; Aczel, A. A.*; Carlo, J. P.*; 伊藤 利充*; Rodriguez, J.*; Russo, P. L.*; 植村 泰朋*; 脇本 秀一; Luke, G. M.*

Physical Review Letters, 101(1), p.017001_1 - 017001_4, 2008/07

 被引用回数:60 パーセンタイル:89.38(Physics, Multidisciplinary)



Muon spin rotation study of field-induced magnetism in heavily overdoped La$$_{2-x}$$Sr$$_{x}$$CuO$$_{4}$$

MacDougall, G. J.*; Birgeneau, R. J.*; Kim, H.*; Kim, S.-J.*; Rodriguez, J.*; Russo, P. L.*; Savici, A. T.*; 植村 泰朋*; 脇本 秀一; Wiebe, C. R.*; et al.

Physica B; Condensed Matter, 374-375, p.211 - 214, 2006/03

 被引用回数:4 パーセンタイル:23.8(Physics, Condensed Matter)

高温超伝導体の研究において、単結晶試料育成や化学的ドーピングの困難から、過剰ドープ領域の研究はほとんどなされていなかった。本研究では、世界初となる過剰ドープしたLa$$_{2-x}$$Sr$$_{x}$$CuO$$_{4}$$単結晶の$$mu$$SR実験の結果を報告する。縦磁場$$mu$$SRの結果から、relaxation rateの温度依存性がCurie-Weiss則に従い、そのCurie constantが磁場の関数として$$Cproptoalpha H$$と書かれることが見いだされた。この現象は、内部磁場分布の異常が磁場により誘起されていることを示している。磁場誘起の度合を表す$$alpha$$$$x=0.12$$から既に現れ、過剰ドープ領域の$$x=0.30$$まで単調増加し、ドープ量に依存することがわかった。この磁場誘起による異常な内部磁場分布の原因の解明は、今後の重要な課題である。



大石 一城; Heffner, R. H.; MacDougall, G. J.*; 伊藤 孝; 髭本 亘; Luke, G. M.*; Amato, A.*; Nieuwenhuys, G.*; Spehling, J.*; Klauss, H. H.*; et al.

no journal, , 

最近、CeCoIn$$_5$$のInサイトをCdで置換することにより、$$T_c$$が減少し反強磁性秩序が出現することが報告された。NMR実験によると、Cd置換量10%の試料では磁気秩序と超伝導秩序の共存が示唆され、さらにこの磁性は置換したCd近傍で出現していることが示された。一方、同じ組成の試料による中性子実験では、$$T_N$$以下で$$Q_{AF}$$=(1/2, 1/2, 1/2)の反強磁性秩序を形成することが示された。われわれは本系の磁性に関する微視的知見、特に磁気成分の体積分率を調べるため、Cd置換量3%, 10%及び15%の単結晶試料を用いて零磁場中でミュオンスピン緩和測定を行った。その結果、10%及び15%Cd置換した試料において、$$T_N$$以下で磁気秩序形成に伴うミュオンスピン回転を観測し、磁性成分の体積分率はほぼ100%であることを観測した。また10%の試料では、$$T_c$$の前後で回転周波数の温度依存性に大きな変化はなかった。一方、超伝導のみを示す3%Cd置換試料では、核双極子磁場による緩和以外は観測されず、時間反転対称性が破れていないことを示した。


Magnetism and superconductivity in CeCo(In,Cd)$$_5$$ probed by $$mu$$SR

大石 一城; Heffner, R. H.; Spehling, J.*; MacDougall, G. J.*; 伊藤 孝; 髭本 亘; Amato, A.*; Nieuwenhuys, G.*; Klauss, H. H.*; Luke, G. M.*; et al.

no journal, , 

The heavy fermion superconductor CeCoIn$$_5$$ has the highest critical temperature ($$T_c$$ = 2.3 K) of the Ce-based 115 materials. Recently, it has been found that Cd substitution on the In site drives the system towards antiferromagnetism (AFM). Recent NMR studies suggest that the magnetism develops locally in the vicinity of the Cd atoms. Neutron scattering experiments on a sample with a nominal Cd concentration of 10% showed the coexistence of superconductivity and AFM. The AFM order develops below $$T_N$$ with the commensurate wave vector $$Q_{AF}$$ = (1/2, 1/2, 1/2) and the magnetic intensity did not increase below $$T_c$$. We have performed $$mu$$SR measurements on single crystalline samples of Cd-doped CeCoIn$$_5$$ at nominal Cd concentrations of 3%, 10% and 15% in order to further elucidate the magnetic and superconducting properties of CeCo(In,Cd)$$_5$$. The crystallographic $$c$$ axis was aligned along the initial muon spin for both zero and in applied fields. In contrast to neutron scattering, $$mu$$SR can independently measure both the magnitude of the local field and the magnetic volume fraction. Muon spin precession signal was observed below $$T_N$$ in both the 10% and 15% Cd-doped samples, with different fractions of precession asymmetry. No magnetic signal in zero applied field was observed for the 3% sample.

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