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論文

Enhanced strength and ductility in an additively manufactured Al10SiMg alloy at cryogenic temperatures

Naeem, M.*; Rehman, A. U.*; Romero Resendiz, L.*; Salamci, E.*; Aydin, H.*; Ansari, P.*; Harjo, S.; Gong, W.; Wang, X.-L.*; 他3名*

Communications Materials (Internet), 6, p.65_1 - 65_13, 2025/04

The need for lightweight materials with mechanical integrity at ultralow temperatures drives the development of advanced alloys for cryogenic use. Additive manufacturing via laser powder bed fusion (LPBF) offers a scalable way to create alloys with tailored properties. Here, we show that LPBF-processed Al10SiMg exhibits a high ultimate tensile strength (395 MPa) and uniform elongation (25%) at 15 K. These enhancements stem from grain refinement, increased geometrically necessary dislocations, and stress partitioning between the Al matrix and the stiffer Si phase, aiding strain accommodation. ${it In-situ}$ neutron diffraction reveals that the Si phase, with its higher yield strength, bears most of the load, while the Al matrix undergoes continuous strain hardening, extending deformation capacity. These results highlight Al10SiMg's promise for cryogenic applications such as hydrogen storage, aerospace, and quantum computing hardware.

論文

Local structure analysis of heavy fermion Ce$$_2$$Pt$$_6$$Ga$$_{15}$$ with a honeycomb structure using extended X-ray absorption fine structure

松本 裕司*; 渡部 悠貴*; Iesari, F.*; 大角 将勝*; 太田 玖吾*; 芳賀 芳範; 畑田 圭介*; 岡島 敏浩*

Metals, 15(4), p.436_1 - 436_13, 2025/04

 被引用回数:0 パーセンタイル:0.00(Materials Science, Multidisciplinary)

A heavy fermion system Ce$$_2$$Pt$$_6$$Ga$$_{15}$$ is studied by the extended X-ray absorption fine structure (EXAFS). The spectra show that cerium is in trivalent state. On the other hand, EXAFS result is well explained by the proposed structure model with the honeycomb arrangement.

論文

Reevaluation of structures in $$^{70}$$Se from combined conversion-electron and $$gamma$$-ray spectroscopy

Smallcombe, J.; Garnsworthy, A. B.*; Korten, W.*; Singh, P.*; Muir, D.*; Pr$'o$chniak, L.*; Ali, F. A.*; Andreoiu, C.*; Ansari, S.*; Ball, G. C.*; et al.

Physical Review C, 110(2), p.024318_1 - 024318_16, 2024/08

 被引用回数:1 パーセンタイル:52.60(Physics, Nuclear)

In the selenium isotopes various shape phenomena are present, in particular the emergence of a dominant oblate deformation in the most neutron-deficient isotopes has been observed. The scenario of shape coexisting oblate and prolate bands has been proposed across the isotopic chain, with the crossing point of such bands being located near $$^{70}$$Se, where no coexistence has yet been identified. To determine the presence or absence of any low-lying $$0^+$$ state in $$^{70}$$Se, confirm the level structure, and interpret the nuclear deformation with theoretical models. A combined internal conversion electron and $$gamma$$-ray spectroscopy study was undertaken with the SPICE and TIGRESS spectrometers at the TRIUMF-ISAC-II facility. Nuclear models were provided by the Generalised Triaxial Rotor Model (GTRM) and the collective Generalised Bohr Hamiltonian (GBH). Despite a comprehensive search, no evidence was found for the existence of a $$0^+$$ state below 2 MeV in $$^{70}$$Se. Significant discrepancies to the previously established positive parity level scheme were found. GBH calculations using UNEDF1 mass parameters were found to reproduce the revised low-lying level structure well. $$^{70}$$Se does not have a well defined axial shape. The 2$$_2^{+}$$ state at 1601 keV resembles a quasi-$$gamma$$ excitation rather than a member of a shape coexisting band; the presence of such a band is all but ruled out.

論文

Quantum critical behavior of the hyperkagome magnet Mn$$_3$$CoSi

山内 宏樹; Sari, D. P.*; 安井 幸夫*; 坂倉 輝俊*; 木村 宏之*; 中尾 朗子*; 大原 高志; 本田 孝志*; 樹神 克明; 井川 直樹; et al.

Physical Review Research (Internet), 6(1), p.013144_1 - 013144_9, 2024/02

$$beta$$-Mn-type family alloys Mn$$_3$$$$TX$$ have three-dimensional antiferromagnetic (AFM) corner-shared triangular network. The antiferromagnet Mn$$_3$$RhSi shows magnetic short-range order (SRO) over a wide temperature range of approximately 500 K above the N$'{e}$el temperature $$T_{rm N}$$ = 190 K. Mn$$_3$$CoSi has the smallest lattice parameter and the lowest $$T_{rm N}$$ in the family compounds. The quantum critical point (QCP) from AFM to the quantum paramagnetic state is expected near a cubic lattice parameter of 6.15 $AA. Although $T_N$$ of Mn$$_3$$CoSi is only 140 K, quantum critical behavior is observed in Mn$$_3$$CoSi as the enhancement of the electronic specific heat coefficient $$gamma$$. We study how the magnetic SRO appears in Mn$$_3$$CoSi by using neutron scattering, $$mu$$SR, and physical property measurements. The experimental results show that the neutron scattering intensity of the magnetic SRO does not change much regardless of the suppressed magnetic moment in the long-range magnetic ordered state compared to those of Mn$$_3$$RhSi. The initial asymmetry drop ratio of $$mu$$SR above $$T_{rm N}$$ becomes small, and the magnetic SRO temperature $$T_{SRO}$$ is suppressed to 240 K. The results suggest that the Mn$$_3$$CoSi is close to the QCP in the Mn$$_3$$$$TX$$ system.

論文

Synthesis, crystal structure, local structure, and magnetic properties of polycrystalline and single-crystalline Ce$$_2$$Pt$$_6$$Al$$_{15}$$

太田 玖吾*; 渡部 悠貴*; 芳賀 芳範; Iesari, F.*; 岡島 敏浩*; 松本 裕司*

Symmetry (Internet), 15(8), p.1488_1 - 1488_13, 2023/07

 被引用回数:2 パーセンタイル:37.80(Multidisciplinary Sciences)

Polycrystalline and single crystalline Ce$$_2$$Pt$$_6$$Al$$_{15}$$ samples were synthesized and characterized using EPMA, XRD, XAS and magnetization measurements. The valence of Ce in this compound is trivalent, in agreement with magnetic susceptibility and XAS spectra. The analysis of EXAFS spectra indicates the formation of a honeycomb lattice rather than the disordered hexagonal structure.

論文

Improved measurement of the $$0_2^+rightarrow0_1^+$$ $$E$$0 transition strength for $$^{72}$$Se using the SPICE spectrometer

Smallcombe, J.; Garnsworthy, A. B.*; Korten, W.*; Singh, P.*; Ali, F. A.*; Andreoiu, C.*; Ansari, S.*; Ball, G. C.*; Barton, C. J.*; Bhattacharjee, S. S.*; et al.

Physical Review C, 106(1), p.014312_1 - 014312_9, 2022/07

 被引用回数:5 パーセンタイル:60.14(Physics, Nuclear)

The selenium isotopes lie at the heart of a tumultuous region of the nuclear chart where shape coexistence effects grapple with neutron-proton pairing correlations, triaxiality, and the impending proton dripline. In this work a study of $$^{72}$$Se by internal conversion electron and $$gamma$$-ray spectroscopy was undertaken with the SPICE and TIGRESS arrays. New measurements of the branching ratio and lifetime of the $$0_2^+$$ state were performed yielding a determination of $$rho^2(E0; 0_2^+{rightarrow}0_1^+)=29(3)$$ milliunits. Two state mixing calculations were performed that highlighted the importance of interpretation of such $$E0$$ strength values in the context of shape-coexistence.

論文

Bayesian sparse modeling of extended X-ray absorption fine structure to determine interstitial oxygen positions in yttrium oxyhydride epitaxial thin film

熊添 博之*; 五十嵐 康彦*; Iesari, F.*; 清水 亮太*; 小松 遊矢*; 一杉 太郎*; 松村 大樹; 齋藤 寛之*; 岩満 一功*; 岡島 敏浩*; et al.

AIP Advances (Internet), 11(12), p.125013_1 - 125013_5, 2021/12

 被引用回数:4 パーセンタイル:23.69(Nanoscience & Nanotechnology)

This letter presents a Bayesian sparse modeling method to analyze extended X-ray absorption fine structure (EXAFS) data with basis functions built on two-body signals. This method allows us to evaluate regression coefficients proportional to the radial distribution functions of the respective elements and their errors and is very effective for analysis of EXAFS with weak absorption intensity and severe signal-to-noise ratio. As an application example, we used it to analyze EXAFS of an yttrium oxyhydride (YO$$_{x}$$H$$_{y}$$) epitaxial thin film. This EXAFS data shows weak absorption intensity due to the small amount of X-ray absorption in the thin film sample. However, this approach revealed that the radial distance ratio of the second neighbor yttrium to the first neighbor oxygen coincides with that of a tetrahedral configuration. This result demonstrates that the interstitial oxygen position is tetrahedral in the YO$$_{x}$$H$$_{y}$$ thin film.

論文

Optimization of a 9 MeV electron accelerator bremsstrahlung flux for photofission-based assay techniques using PHITS and MCNP6 Monte Carlo codes

Meleshenkovskii, I.*; 小川 達彦; Sari, A.*; Carrel, F.*; Boudergui, K.*

Nuclear Instruments and Methods in Physics Research B, 483, p.5 - 14, 2020/11

 被引用回数:10 パーセンタイル:68.22(Instruments & Instrumentation)

核分裂性物質の検知を目的として、制動放射線を検知対象に照射して光核分裂反応を発生させ、放出される中性子線を観測する技術が注目されている。この技術で制動放射線を発生させるための電子加速器は、同等の性能を発揮する中性子源と比べて放射化や即発線量が低く、装置の小型化が容易という利点がある。一方、光核分裂反応は中性子誘導核分裂反応より断面積が低いため、電子線ターゲットや制動放射線の取り出し口、照射野などを最適化することが検知効率の向上に必要となる。本研究では、汎用モンテカルロ放射線輸送計算コードMCNPとPHITSを用いて、最適化に必要な要素を明らかにした。その結果、ターゲットでの制動放射線の生成は原子番号の高い元素の方が有利であるが、発生した光子がターゲット周辺で($$gamma$$,n)二次反応を起こし、中性子を生成するため、光子によって起こる早い光核分裂反応と、中性子による遅い核分裂が混在し、最終的な検出対象である核分裂の発生時間が広がる問題が明らかとなった。また、中性子を生じる二次反応は電子線ターゲットだけではなく、ターゲット周辺の遮蔽材でも発生するため、中性子放出スレッショルドが高い元素を遮蔽材として選択するなどの工夫が必要であることが明らかになった。

論文

Competition between allowed and first-forbidden $$beta$$ decay; The Case of $$^{208}$$Hg $$rightarrow$$ $$^{208}$$Tl

Carroll, R. J.*; Podoly$'a$k, Zs.*; Berry, T.*; Grawe, H.*; Alexander, T.*; Andreyev, A. N.; Ansari, S.*; Borge, M. J. G.*; Brunet, M.*; Creswell, J. R.*; et al.

Physical Review Letters, 125(19), p.192501_1 - 192501_6, 2020/11

 被引用回数:12 パーセンタイル:62.27(Physics, Multidisciplinary)

The $$beta$$ decay of $$^{208}$$Hg into the one-proton hole, one neutron-particle $$^{208}_{81}$$Tl$$_{127}$$ nucleus was investigated at CERN-ISOLDE. Shell-model calculations describe well the level scheme deduced, validating the proton-neutron interactions used, with implications for the whole of the $$N > 126$$, $$Z < 82$$ quadrant of neutron-rich nuclei. While both negative and positive parity states with spin 0 and 1 are expected within the $$Q_{beta}$$ window, only three negative parity states are populated directly in the $$beta$$ decay. The data provide a unique test of the competition between allowed Gamow-Teller and Fermi, and first-forbidden $$beta$$ decays, essential for the understanding of the nucleosynthesis of heavy nuclei in the rapid neutron capture process. Furthermore, the observation of the parity changing $$0^{+} rightarrow 0^{-} beta$$ decay where the daughter state is core excited is unique, and can provide information on mesonic corrections of effective operators.

論文

High-temperature short-range order in Mn$$_3$$RhSi

山内 宏樹; Sari, D. P.*; 渡邊 功雄*; 安井 幸夫*; Chang, L.-J.*; 近藤 啓悦; 伊藤 孝; 石角 元志*; 萩原 雅人*; Frontzek, M. D.*; et al.

Communications Materials (Internet), 1, p.43_1 - 43_6, 2020/07

中性子とミュオンの相補利用により、720Kまでの高温での短距離磁気秩序現象をMn$$_3$$RhSiで発見した。

論文

Investigation of the $$Delta$$$$n$$ = 0 selection rule in Gamow-Teller transitions; The $$beta$$-decay of $$^{207}$$Hg

Berry, T. A.*; Podoly$'a$k, Zs.*; Carroll, R. J.*; Lic$u{a}$, R.*; Grawe, H.*; Timofeyuk, N. K.*; Alexander, T.*; Andreyev, A. N.; Ansari, S.*; Borge, M. J. G.*; et al.

Physics Letters B, 793, p.271 - 275, 2019/06

 被引用回数:6 パーセンタイル:46.80(Astronomy & Astrophysics)

Gamow-Teller $$beta$$ decay is forbidden if the number of nodes in the radial wave functions of the initial and final states is different. This $$Delta$$$$n$$ = 0 requirement plays a major role in the $$beta$$ decay of heavy neutron-rich nuclei, affecting the nucleosynthesis through the increased half-lives of nuclei on the astrophysical $$r$$-process pathway below both $$Z$$ = 50 (for $$N >$$ 82) and $$Z$$ = 82 (for $$N >$$ 126). The level of forbiddenness of the $$Delta$$$$n$$ = 1 $$nu$$1$$g_{9/2} rightarrow pi$$0$$g_{7/2}$$ transition has been investigated from the $$beta^{-}$$ decay of the ground state of $$^{207}$$Hg into the single-proton-hole nucleus $$^{207}$$Tl in an experiment at the ISOLDE Decay Station. From statistical observational limits on possible $$gamma$$-ray transitions depopulating the $$pi$$0$$g^{-1}_{7/2}$$ state in $$^{207}$$Tl, an upper limit of 3.9$$times$$10$$^{-3}$$ % was obtained for the probability of this decay, corresponding to log$$ft >$$ 8.8 within a 95% confidence limit. This is the most stringent test of the $$Delta$$$$n$$ = 0 selection rule to date.

論文

Magnetic properties of one-dimensional quantum spin system Rb$$_2$$Cu$$_2$$Mo$$_3$$O$$_{12}$$ studied by muon spin relaxation

河村 聖子; 富安 啓輔*; 幸田 章宏*; Sari, D. P.*; Asih, R.*; Yoon, S.*; 渡邊 功雄*; 中島 健次

JPS Conference Proceedings (Internet), 21, p.011007_1 - 011007_5, 2018/03

Rb$$_2$$Cu$$_2$$Mo$$_3$$O$$_{12}$$は、スピンフラストレートしたS=1/2ジグザグ鎖をもつ量子スピン系である。この系の磁気基底状態は、非整合なスピン1重項であることが、理論研究から予想されている。また最近では、磁場中でこの系が強誘電性を示すことも報告されている。我々は、この系の磁気的性質を調べるため、ミュオンスピン緩和法を用いた実験を行った。測定した温度領域0.06K$$sim$$250Kにわたり、核双極子場による遅いミュオンスピン緩和が観測された。この結果は、この系の基底状態が非磁性であることを明確に示している。さらに、内部磁場の分布が、10K以下でわずかに増加していることがわかった。この温度変化は、磁場中の電気分極の振る舞いに似ていることから、局所的な磁気状態の変化あるいは分極が、零磁場中でも生じている可能性を示唆している。

論文

Radiation-induced grafting of acrylonitrile monomer onto cellulose nonwoven fabric

佐伯 誠一; Puspitasari, T.*; 瀬古 典明

JAEA-Review 2011-043, JAEA Takasaki Annual Report 2010, P. 44, 2012/01

液相における放射線グラフト重合法では、環境・人体に悪影響を及ぼす懸念のある有機溶媒を多用する場合が多いため、有機溶媒使用量の低減が望まれている。本研究では、有機溶媒の代替としてモノマーを水に分散させるo/wエマルジョン溶液を用いて放射線グラフト重合を試みた。重合モノマーにアクリロニトリル、基材にセルロース製不織布、界面活性剤にTween80を用いてエマルジョン溶液を調液してグラフト実験を行った結果、ジメチルスルホキシド等の有機溶媒を使用した場合に比較して、著しくグラフト率が増加することがわかった。また、グラフト率は界面活性剤濃度にあまり依存せず、アクリロニトリル濃度に大きく依存することがわかった。以上より、アクリロニトリルを用いた放射線エマルジョングラフト重合は、有機溶媒の使用量の低減に加え、高効率にグラフト反応を促進することが示された。

論文

Radiation-induced grafting of acrylonitrile monomer onto cellulose nonwoven fabric

佐伯 誠一; Puspitasari, T.*; 瀬古 典明

Proceedings of 12th International Conference on Radiation Curing in Asia (RadTech Asia 2011) (Internet), p.124 - 125, 2011/06

Cellulose has been studied as trunk polymer of radiation-induced grafting as well as synthetic polymers. However, cellulose is easy to be degraded and be brittle by irradiation. In this topic, to lower the dose for radiation-induced grafting on cellulose, radiation-induced grafting with o/w emulsion which has ever succeeded to achieve high degree of grafting on synthetic polymer with lower dose was studied using acrylonitrile monomer as a model of typical vinyl monomer. As a result, degree of grafting in the case of emulsion system increased remarkably compared to organic solvent system. And, from 10% to 20% of acrylonitrile monomer concentration, micelle size and degree of grafting increased with increment of acrylonitrile monomer concentration respectively. It is assumed that larger micelles accelerate grafting reaction. As a whole, the effectiveness of radiation emulsion grafting were elucidated even in the case of cellulose as well as trunk polymer.

口頭

アクリロニトリルを用いた放射線エマルジョングラフト重合の検討

佐伯 誠一; Puspitasari, T.*; 瀬古 典明

no journal, , 

従来の放射線グラフト重合では溶媒としてジメチルスルホキシド等の有機溶媒を使用することから、その使用量の低減が検討されている。本研究では、有機溶媒の代替としてo/wエマルジョンを用いて、アクリロニトリルの不織布への放射線グラフト重合を試みた。結果、ジメチルスルホキシド等の有機溶媒を使用した場合と比較して、著しいグラフト率の増加を確認し、効率的にモノマーを消費できることが示された。また、グラフト率は界面活性剤濃度にあまり依存せず、アクリロニトリル濃度に大きく依存した。以上より、アクリロニトリルを用いた放射線エマルジョングラフト重合は、有機溶媒使用量を低減しながらも、高効率にグラフト反応を促進することが示された。

口頭

Study of $$^{70,72}$$Se nuclear shapes with SPICE and TIGRESS

Smallcombe, J.; Garnsworthy, A. B.*; Korten, W.*; Singh, P.*; Ali, F. A.*; Andreoiu, C.*; Ansari, S.*; Ball, G. C.*; Barton, C. J.*; Bhattacharjee, S. S.*; et al.

no journal, , 

The phenomenon of shape coexistence is prevalent in the Z$$sim$$34 region, with isotopes of neutron-deficient even Ge, Se and Kr each exhibiting the characteristic low-lying coexisting 0+ bands which display quadrupole deformation different to that of the ground states. In the selenium isotopes, $$^{72-78}$$Se seem to show a prolate ground structure with shape coexisting oblate excitation, while in $$^{68}$$Se the oblate structure appears to have become the ground state. The exact nature of the low-lying structure $$^{70}$$Se and any shape coexistence remains uncertain. Combining the Spectrometer for Internal Conversion Electrons (SPICE) with the TIGRESS HPGe Array, a full electron and gamma-ray experimental study of $$^{70}$$Se, $$^{72}$$Se was undertaken at the TRIUMF ISAC-II facility to unveil the low-lying structure of these nuclei. Details of the device and experiment will be presented, alongside the experimental results and possible structural interpretations for both isotopes.

口頭

スピン液体状態と反強磁性秩序が共存した新規磁性体Ba$$_{3}$$Zn$$_{1-x}$$Ca$$_{x}$$Ru$$_{2}$$O$$_{9}$$の磁気特性

貞松 龍介*; 井川 直樹; Sari, D. P.*; 渡邊 功雄*; 寺崎 一郎*; 安井 幸夫*

no journal, , 

Ba$$_{3}$$MRu$$_{2}$$O$$_{9}$$ (M= Ca, Zn, Co等)は、2つのRu$$^{5+}$$イオンが近接した二量体構造を含む結晶構造をもつ。この系ではMサイトの元素の違いにより多様な磁性を示す。本研究では、Ba$$_{3}$$Zn$$_{1-x}$$Ca$$_{x}$$Ru$$_{2}$$O$$_{9}$$ (0 $$leqq$$ x $$leqq$$ 1)について、磁化率と磁気比熱を測定し、また、中性子回折によって磁気構造を解析した。磁化率はxの増加に従って連続的に減少していき、x=1では$$Trightarrow 0$$$$chi$$$$rightarrow 0$$に近づく振る舞いを見せた。一方、比熱測定では、低温でとびが見られたことから反強磁性転移を示すことが分かった。本講演では、これらの結果や中性子回折パターンに単純なcollinear構造を仮定して解析した磁気構造の詳細について報告する。

口頭

スピン液体候補物質Ba$$_{3}$$Zn(Ru$$_{1-x}$$Nb$$_{x}$$)$$_{2}$$O$$_{9}$$の中性子回折および$$mu$$SR実験

安井 幸夫*; 貞松 龍介*; 井川 直樹; Sari, D. P.*; 渡邊 功雄*; 寺崎 一郎*

no journal, , 

Ba$$_{3}$$ZnRu$$_{2}$$O$$_{9}$$は磁化率の温度依存性にCurie tailが見られず低温で一定の磁化率を示すことから、新しいタイプの量子スピン液体の可能性が指摘されている。一方、Ru$$^{5+}$$の一部を非磁性のNb$$^{5+}$$で置換した物質の磁化率の温度依存性では、80K付近から強磁性成分が現れる。この特異な磁気的性質は、Ruダイマー内相互作用とダイマー間相互作用の競合が起源と考えられる。また、理論的研究から、これら相互作用パラメータを変えることで、反強磁性秩序、スピン液体とみなせる状態、これらの共存状態、非磁性、強磁性秩序など多彩な磁気状態が現れ得ることも報告されている。そこで、本物質系の微視的磁性を知るためにBa$$_{3}$$Zn(Ru$$_{1-x}$$Nb$$_{x}$$)$$_{2}$$O$$_{9}$$の粉末中性回折および$$mu$$SR実験を行った。それらの結果、x=0の物質では、反強磁性秩序とスピン液体の共存状態と見なせる状態であると考えられる。本講演ではNb置換系も含めて詳しい実験結果を報告する。

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