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論文

Fission of $$^{180,182,183}$$Hg* and $$^{178}$$Pt* nuclei at intermediate excitation energies

Kozulin, E. M.*; Knyazheva, G. N.*; Itkis, I. M.*; Itkis, M. G.*; Mukhamejanov, Y. S.*; Bogachev, A. A.*; Novikov, K. V.*; Kirakosyan, V. V.*; Kumar, D.*; Banerjee, T.*; et al.

Physical Review C, 105(1), p.014607_1 - 014607_12, 2022/01

 被引用回数:18 パーセンタイル:95.49(Physics, Nuclear)

Asymmetric fission in the neutron-deficient Hg region was first observed about 10 years ago at ISOLDE, and caused a revision of the current understanding of fission in this region. In this work, the fission of $$^{180,182,183}$$Hg and $$^{178}$$Pd were studied using the time-of-flight spectrometer CORSET at the Flerov Laboratory in Dubna. The observed fission fragments mass distributions of the different isotopes suggest the presence of four concurrent fission modes, one symmetric and three asymmetric fission modes. The asymmetric modes differ in the total kinetic energies and fragment mass splits. These results point out the existence of a well deformed proton shell at $$Z$$=36 and a less deformed proton shell at $$Z$$=46.

論文

Evolution of Fe 3$$d$$ impurity band state as the origin of high Curie temperature in the $$p$$-type ferromagnetic semiconductor (Ga,Fe)Sb

武田 崇仁*; 坂本 祥哉*; 荒木 恒星*; 藤澤 唯太*; Anh, L. D.*; Tu, N. T.*; 竹田 幸治; 藤森 伸一; 藤森 淳*; 田中 雅明*; et al.

Physical Review B, 102(24), p.245203_1 - 245203_8, 2020/12

 被引用回数:7 パーセンタイル:38.96(Materials Science, Multidisciplinary)

(Ga$$_{1-x}$$,Fe$$_x$$)Sb is one of the promising ferromagnetic semiconductors for spintronic device applications because its Curie temperature (Tc) is above 300 K when the Fe concentration $$x$$ is equal to or higher than 0.20. However, the origin of the high Tc in (Ga,Fe)Sb remains to be elucidated. To address this issue, we use resonant photoemission spectroscopy (RPES) and first-principles calculations to investigate the x dependence of the Fe 3$$d$$ states in (Ga$$_{1-x}$$,Fe$$_x$$)Sb ($$x$$ = 0.05, 0.15, and 0.25) thin films. The observed Fe 2$$p$$-3$$d$$ RPES spectra reveal that the Fe-3$$d$$ impurity band (IB) crossing the Fermi level becomes broader with increasing $$x$$, which is qualitatively consistent with the picture of double-exchange interaction. Comparison between the obtained Fe-3$$d$$ partial density of states and the first-principles calculations suggests that the Fe-3$$d$$ IB originates from the minority-spin ($$downarrow$$) $$e$$ states. The results indicate that enhancement of the double-exchange interaction between $$e_{downarrow}$$ electrons with increasing $$x$$ is the origin of the high Tc in (Ga,Fe)Sb.

論文

Electronic structure of the high-$$T_{rm C}$$ ferromagnetic semiconductor (Ga,Fe)Sb; X-ray magnetic circular dichroism and resonance photoemission spectroscopy studies

坂本 祥哉*; Tu, N. T.*; 竹田 幸治; 藤森 伸一; Hai, P. N.*; Anh, L. D.*; 若林 勇希*; 芝田 悟朗*; 堀尾 眞史*; 池田 啓祐*; et al.

Physical Review B, 100(3), p.035204_1 - 035204_8, 2019/07

 被引用回数:16 パーセンタイル:62.18(Materials Science, Multidisciplinary)

The electronic structure and the magnetism of the ferromagnetic semiconductor (Ga,Fe)Sb, whose Curie temperature $$T_{rm C}$$ can exceed room temperature, were investigated by means of X-ray absorption spectroscopy (XAS), X-ray magnetic circular dichroism (XMCD), and resonance photoemission spectroscopy (RPES). The line-shape analyses of the XAS and XMCD spectra suggest that the ferromagnetism is of intrinsic origin. The orbital magnetic moments deduced using XMCD sum rules were found to be large, indicating that there is a considerable 3$$d^{6}$$ contribution to the ground state of Fe. From RPES, we observed a strong dispersive Auger peak and nondispersive resonantly enhanced peaks in the valence-band spectra. The latter is a fingerprint of the correlated nature of Fe 3$$d$$ electrons, whereas the former indicates their itinerant nature. It was also found that the Fe 3$$d$$ states have a finite contribution to the density of states at the Fermi energy. These states would be responsible for the ferromagnetic order in this material.

論文

Electronic structure of the high-$$T_{rm C}$$ ferromagnetic semiconductor (Ga,Fe)Sb; X-ray magnetic circular dichroism and resonance photoemission spectroscopy studies

坂本 祥哉*; Tu, N. T.*; 竹田 幸治; 藤森 伸一; Hai, P. N.*; Anh, L. D.*; 若林 勇希*; 芝田 悟朗*; 堀尾 眞史*; 池田 啓祐*; et al.

Physical Review B, 100(3), p.035204_1 - 035204_8, 2019/07

The electronic structure and the magnetism of the ferromagnetic semiconductor (Ga,Fe)Sb, whose Curie temperature $$T_{rm C}$$ can exceed room temperature, were investigated by means of X-ray absorption spectroscopy (XAS), X-ray magnetic circular dichroism (XMCD), and resonance photoemission spectroscopy (RPES). The line-shape analyses of the XAS and XMCD spectra suggest that the ferromagnetism is of intrinsic origin. The orbital magnetic moments deduced using XMCD sum rules were found to be large, indicating that there is a considerable 3$$d^{6}$$ contribution to the ground state of Fe. From RPES, we observed a strong dispersive Auger peak and nondispersive resonantly enhanced peaks in the valence-band spectra. The latter is a fingerprint of the correlated nature of Fe 3$$d$$ electrons, whereas the former indicates their itinerant nature. It was also found that the Fe 3$$d$$ states have a finite contribution to the density of states at the Fermi energy. These states, presumably consisting of majority-spin $$p$$-$$d$$ hybridized states or minority-spin e states, would be responsible for the ferromagnetic order in this material.

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