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論文

Sharp surface tension model with pressure discontinuity and refined curvature for multiphase particle methods

Wang, Z.; 松本 俊慶; 柴本 泰照; Duan, G.*

Journal of Computational Physics, 537, p.114072_1 - 114072_29, 2025/09

In this study, we develop a novel sharp surface tension (SST) model for multiphase particle methods. Our approach integrates surface tension directly into pressure computation, enabling precise representation of pressure discontinuities across interfaces and effectively mitigating parasitic currents. In addition, to improve curvature accuracy, particularly in scenarios involving topological changes, a co-directional scheme is proposed to faithfully consider interfacial normal vectors. Furthermore, we reconstruct the interfacial particle shifting scheme to separately address tangential, normal, and repulsive components, effectively suppressing the common problem of interface particle mixing in multiphase particle methods. The effectiveness and reliability are rigorously validated through a series of numerical tests, including the Rayleigh-Taylor instability, curvature verification, droplet deformation and coalescence, as well as bubble rising and coalescence. The results demonstrate the superior accuracy and robustness of the proposed method, marking a significant advancement in simulations of multiphase flow with surface tension.

論文

Unique deformation behavior of ultrafine-grained 304 stainless steel at 20 K

Mao, W.*; Gong, W.; 川崎 卓郎; Gao, S.*; 伊東 達矢; 山下 享介*; Harjo, S.; Zhao, L.*; Wang, Q.*

Scripta Materialia, 264, p.116726_1 - 116726_6, 2025/07

 被引用回数:0

An ultrafine-grained 304 austenitic stainless steel exhibited pronounced serrated Luders deformation at 20 K, with stress and temperature oscillations reaching 200 MPa and 20 K. ${it In-situ}$ neutron diffraction and digital image correlation revealed discontinuous Luders band propagation and burst martensite formation. During deformation, austenite phase stress remained lower than at upper yielding, indicating elastic behavior. Notably, martensite phase stress stayed lower than austenite until fracture, likely due to stress relaxation from burst martensitic transformation at 20 K. The low martensite stress delayed brittle fracture until austenite plastically yielded during uniform deformation.

論文

Enhanced strength and ductility in an additively manufactured Al10SiMg alloy at cryogenic temperatures

Naeem, M.*; Rehman, A. U.*; Romero Resendiz, L.*; Salamci, E.*; Aydin, H.*; Ansari, P.*; Harjo, S.; Gong, W.; Wang, X.-L.*; 他3名*

Communications Materials (Internet), 6, p.65_1 - 65_13, 2025/04

The need for lightweight materials with mechanical integrity at ultralow temperatures drives the development of advanced alloys for cryogenic use. Additive manufacturing via laser powder bed fusion (LPBF) offers a scalable way to create alloys with tailored properties. Here, we show that LPBF-processed Al10SiMg exhibits a high ultimate tensile strength (395 MPa) and uniform elongation (25%) at 15 K. These enhancements stem from grain refinement, increased geometrically necessary dislocations, and stress partitioning between the Al matrix and the stiffer Si phase, aiding strain accommodation. ${it In-situ}$ neutron diffraction reveals that the Si phase, with its higher yield strength, bears most of the load, while the Al matrix undergoes continuous strain hardening, extending deformation capacity. These results highlight Al10SiMg's promise for cryogenic applications such as hydrogen storage, aerospace, and quantum computing hardware.

論文

Robustness of ferromagnetism in van der Waals magnet Fe$$_3$$GeTe$$_2$$ to hydrostatic pressure

Wang, Y.*; Zeng, X.-T.*; Li, B.*; Su, C.*; 服部 高典; Sheng, X.-L.*; Jin, W.*

Chinese Physics B, 34(4), p.046203_1 - 046203_6, 2025/03

 被引用回数:0 パーセンタイル:0.00(Physics, Multidisciplinary)

二次元ファンデルワールス強磁性体Fe$$_3$$GeTe$$_2$$(FGT)は、その高いキュリー温度、容易な調整性、空気中での優れた構造安定性から、スピントロニクスデバイスへの応用に大きな可能性を秘めている。理論的研究により、外部パラメータとしての圧力が強磁性特性に大きく影響することが示されている。本研究では、5GPaまでの高圧中性子粉末回折(NPD)実験を行い、FGTの静水圧による構造及び磁気特性の変化を調べた。NPDデータは、静水圧による見かけ上の抑制にもかかわらず、FGTにおける強磁性の頑健性を明らかにした。圧力が0から5GPaまで増加すると、キュリー温度は225(5)Kから175(5)Kまで単調減少し、Feの秩序モーメントが劇的に抑制されることがわかった。圧力による構造相転移は5GPaまで観測されなかったが、結合長と結合角の変化を定量的に解析した結果、交換相互作用が大きく変化していることがわかった。

論文

Unusual low-temperature ductility increase mediated by dislocations alone

Naeem, M.*; Ma, Y.*; Tian, J.*; Kong, H.*; Romero-Resendiz, L.*; Fan, Z.*; Jiang, F.*; Gong, W.; Harjo, S.; Wu, Z.*; et al.

Materials Science & Engineering A, 924, p.147819_1 - 147819_10, 2025/02

 被引用回数:0 パーセンタイル:0.00(Nanoscience & Nanotechnology)

Face-centered cubic (fcc) medium-/high-entropy alloys (M/HEAs) typically enhance strength and ductility at cryogenic temperatures via stacking faults, twinning, or martensitic transformation. However, in-situ neutron diffraction on VCoNi MEA at 15 K reveals that strain hardening is driven solely by rapid dislocation accumulation, without these mechanisms. This results in increased yield strength, strain hardening, and fracture strain. The behavior, explained by the Orowan equation, challenges conventional views on cryogenic strengthening in fcc M/HEAs and highlights the role of dislocation-mediated plasticity at low temperatures.

論文

High-pressure polymerization of phenol toward degree-4 carbon nanothread

Yang, X.*; Che, G.*; Wang, Y.*; Zhang, P.*; Tang, X.*; Lang, P.*; Gao, D.*; Wang, X.*; Wang, Y.*; 服部 高典; et al.

Nano Letters, 25(3), p.1028 - 1035, 2025/01

 被引用回数:1 パーセンタイル:0.00(Chemistry, Multidisciplinary)

飽和sp$$^3$$-カーボンナノスレッド(CNTh)は、その高いヤング率と熱伝導率が予測され、大きな関心を集めている。中心環へのヘテロ原子の導入がCNThの形成に影響を与え、化学的に均質な生成物が得られることが示されているが、ペンダント基が重合プロセスに与える影響については、まだ未解明である。本研究では、フェノールの圧力誘起重合を調べ、0.5GPaと4GPa以下で起こる2つの相転移を明らかにした。20GPa以上では、フェノールは水酸基とカルボニル基を持つ重合度4のCNTに重合する。ヒドロキシル基の水素移動は、重合度6のナノスレッドの形成を妨げることがわかった。この発見は、さらなるカラム内重合を阻止する水酸基の重要な役割を浮き彫りにし、今後のメカニズム研究やナノ材料合成に貴重な示唆を与えるものである。

論文

Pressure-induced polymerization of 1,4-difluorobenzene towards fluorinated diamond nanothreads

Che, G.*; Fei, Y.*; Tang, X.*; Zhao, Z.*; 服部 高典; 阿部 淳*; Wang, X.*; Ju, J.*; Dong, X.*; Wang, Y.*; et al.

Physical Chemistry Chemical Physics, 27(2), p.1112 - 1118, 2025/01

 被引用回数:3 パーセンタイル:65.57(Chemistry, Physical)

芳香族分子の圧力誘起重合(PIP)は、様々な炭素系材料を合成するための効果的な方法として浮上してきた。目的とする構造や機能を得るためには、適切な官能基化された分子前駆体の選択が極めて重要である。本研究では、1,4-ジフルオロベンゼン(1,4-DFB)をPIPの構成要素として選択した。1,4-DFBをその場高圧で調べた結果、約12.0GPaで相転移が起こり、18.7GPaで不可逆的な化学反応が起こることがわかった。生成物の構造解析と反応のカイネティクスから、直線的な成長を伴う擬六方晶積層フッ素ダイヤモンドナノスレッドの形成が明らかになった。高圧下のベンゼンの結晶構造と比較して、1,4-DFBは[001]軸に沿って高い圧縮を示す。この異方的な圧縮は、[01$$overline{1}$$]軸に沿ったより強いH$$cdot cdot cdot pi$$相互作用と、[100]軸と[010]軸に沿った潜在的な圧縮阻害H$$cdot cdot cdot$$F相互作用に起因し、[01$$overline{1}$$]軸に沿った可能な反応経路を促進する。この研究は、分子スタッキングを調節し、反応経路に影響を与える官能基化の重要な役割を強調している。

論文

Solid-state Alder-ene reaction of 1-hexene under high pressure

Xu, J.*; Lang, P.*; Liang, S.*; Zhang, J.*; Fei, Y.*; Wang, Y.*; Gao, D.*; 服部 高典; 阿部 淳*; Dong, X.*; et al.

Journal of Physical Chemistry Letters (Internet), p.2445 - 2451, 2025/00

 被引用回数:0 パーセンタイル:0.00(Chemistry, Physical)

アルダー-エン反応は、アルケンとアリル水素との化学反応であり、C-C結合を構築する効率的な方法である。従来、この反応には触媒、高温、あるいは光触媒が必要であった。本研究では、触媒を用いずに室温下で加圧することで成功した1-ヘキセンのアルダー-エン反応を報告する。1-ヘキセンは4.3GPaで結晶化し、18GPaで重合してオレフィンを形成する。ガスクロマトグラフィー-質量分析法により、1-ヘキセンが高圧下でのアルダー-エン反応により二量体を生成することを発見した。その場中性子回折から、この反応過程はトポケミカル則に従わないことがわかった。理論計算により、1つのC-H $$sigma$$結合と2つのアルケン$$pi$$結合を含む6員環遷移状態が示され、そのエネルギーは20GPaまで圧縮すると明らかに減少した。本研究は、触媒を用いずに室温でアルダー-エン反応を実現する新規かつ有望な方法を提供し、この重要な反応の応用を拡大するものである。

論文

Strong low-energy rattling modes enabled liquid-like ultralow thermal conductivity in a well-ordered solid

Liu, P.-F.*; Li, X.*; Li, J.*; Zhu, J.*; Tong, Z.*; 古府 麻衣子*; 楡井 真実; Xu, J.*; Yin, W.*; Wang, F.*; et al.

National Science Review, 11(12), p.nwae216_1 - nwae216_10, 2024/12

 被引用回数:12 パーセンタイル:91.22(Multidisciplinary Sciences)

Crystalline solids exhibiting inherently low lattice thermal conductivity ($$kappa_{rm L}$$) are of great importance in applications such as thermoelectrics and thermal barrier coatings. However, $$kappa_{rm L}$$ cannot be arbitrarily low and is limited by the minimum thermal conductivity related to phonon dispersions. In this work, we report the liquid-like thermal transport in a well-ordered crystalline CsAg$$_5$$Te$$_3$$, which exhibits an extremely low $$kappa_{rm L}$$ value of $$sim$$ 0.18 Wm$$^{-1}$$K$$^{-1}$$. On the basis of first-principles calculations and inelastic neutron scattering measurements, we find that there are lots of low-lying optical phonon modes at $$sim$$ 3.1 meV hosting the avoided-crossing behavior with acoustic phonons. These strongly localized modes are accompanied by weakly bound rattling Ag atoms with thermally induced large amplitudes of vibrations. Using the two-channel model, we demonstrate that coupling of the particle-like phonon modes and the heat-carrying wave-like phonons is essential for understanding the low $$kappa_{rm L}$$, which is heavily deviated from the $$1/T$$ temperature dependence of the standard Peierls theory. In addition, our analysis indicates that the soft structural framework with liquid-like motions of the fluctuating Ag atoms is the underlying cause that leads to the suppression of the heat conduction in CsAg$$_5$$Te$$_3$$. These factors synergistically account for the ultralow $$kappa_{rm L}$$ value. Our results demonstrate that the liquid-like heat transfer could indeed exist in a well-ordered crystal.

論文

Enhanced cryogenic mechanical properties of heterostructured CrCoNi multicomponent alloy; Insights from ${it in situ}$ neutron diffraction

Naeem, M.*; Ma, Y.*; Knowles, A. J.*; Gong, W.; Harjo, S.; Wang, X.-L.*; Romero Resendiz, L.*; 他6名*

Materials Science & Engineering A, 916, p.147374_1 - 147374_8, 2024/11

 被引用回数:2 パーセンタイル:63.37(Nanoscience & Nanotechnology)

Heterostructured materials (HSMs) improve the strength-ductility trade-off of alloys, but their cryogenic performance under real-time deformation is unclear. We studied heterostructured CrCoNi medium-entropy alloy via ${it in situ}$ neutron diffraction at 77 K and 293 K. A significant mechanical mismatch between fine and coarse grains led to an exceptional yield strength of 918 MPa at 293 K, increasing to 1244 MPa at 77 K with a uniform elongation of 34%. This strength-ductility synergy at 77 K is attributed to high dislocation pile-up density, increased planar faults, and martensitic transformation. Compared to homogeneous alloys, HSMs show promise for enhancing cryogenic mechanical performance in medium-/high-entropy alloys.

論文

Brightening triplet excitons enable high-performance white-light emission in organic small molecules via integrating n-$$pi^*/pi$$-$$pi^*$$ transitions

Yang, Q.*; Yang, X.*; Wang, Y.*; Fei, Y.*; Li, F.*; Zheng, H.*; Li, K.*; Han, Y.*; 服部 高典; Zhu, P.*; et al.

Nature Communications (Internet), 15, p.7778_1 - 7778_9, 2024/09

 被引用回数:9 パーセンタイル:88.46(Multidisciplinary Sciences)

明るい一重項励起子と三重項励起子を同時に発現する発光材料は、オプトエレクトロニクス、サイネージ、情報暗号化において大きな可能性を秘めている。しかしながら、高性能の白色発光を実現するためには、蛍光と燐光の寄与が不均衡であることが大きな障害となっている。ここでは、水素結合の協同効果による圧力処理エンジニアリングによって、n-$$pi^*/pi$$-$$pi^*$$遷移の混合を実現し、イソフタル酸(IPA)中で三重項状態の発光を7%から40%に高めることで、この課題に対処した。加圧処理したIPAでは、蛍光と燐光のハイブリッドに基づく優れた白色発光が得られ、フォトルミネッセンス量子収率は当初の19%(青色発光)から75%に増加した。その場での高圧IRスペクトル、X線回折、中性子回折から、圧力の上昇に伴い水素結合が連続的に強化されることが明らかになった。さらに、この強化された水素結合は、圧力処理後も常圧条件下まで保持され、バランスの取れた一重項/三重項励起子集団のための効率的な系間交差を目的としたIPAに与え、効率的な白色発光をもたらした。この研究は、有機低分子の三重項状態を明るくするルートを提案するだけでなく、一重項励起子と三重項励起子の比率を調節して、高性能の白色発光を構築するものである。

論文

Antiferromagnetism and phase stability of CrMnFeCoNi high-entropy alloy

Zhu, L.*; He, H.*; Naeem, M.*; Sun, X.*; Qi, J.*; Liu, P.*; Harjo, S.; 中島 健次; Li, B.*; Wang, X.-L.*

Physical Review Letters, 133(12), p.126701_1 - 126701_6, 2024/09

 被引用回数:1 パーセンタイル:48.32(Physics, Multidisciplinary)

It has long been suspected that magnetism could play a vital role in the phase stability of multi- component high-entropy alloys. However, the nature of the magnetic order, if any, has remained elusive. Here, by using elastic and inelastic neutron scattering, we demonstrate evidence of antiferromagnetic order below $$sim$$80 K and strong spin fluctuations persisting to room temperature in a single-phase face-centered cubic (fcc) CrMnFeCoNi high-entropy alloy. Despite the chemical complexity, the magnetic structure in CrMnFeCoNi can be described as $$gamma$$-Mn-like, with the magnetic moments confined in alternating (001) planes and pointing toward the $$langle$$111$$rangle$$ direction. Combined with first-principles calculation results, it is shown that the antiferromagnetic order and spin fluctuations help stabilized the fcc phase in CrMnFeCoNi high-entropy alloy.

論文

Anomalous dislocation response to deformation strain in CrFeCoNiPd high-entropy alloys with nanoscale chemical fluctuations

Ying, H.*; Yang, X.*; He, H.*; Yan, A.*; An, K.*; Ke, Y.*; Wu, Z.*; Tang, S.*; Zhang, Z.*; Dong, H.*; et al.

Scripta Materialia, 250, p.116181_1 - 116181_7, 2024/09

 被引用回数:1 パーセンタイル:41.92(Nanoscience & Nanotechnology)

Nanoscale chemical fluctuations and their effect on the deformation behavior of CrFeCoNi-based high-entropy alloys (HEAs) were investigated using small-angle scattering and in situ neutron diffraction measurements. Small-angle scattering results demonstrated the presence of nano ($$>$$10 nm) chemical fluctuations in the as-prepared CrFeCoNiPd HEAs, which was attributed to the negative mixing of enthalpy and the significant atomic radius difference between Pd and the constituent elements in the CrFeCoNi-based alloys. Subsequent tensile tests demonstrated that the yield and tensile strengths of the as-prepared CrFeCoNiPd HEA surpass those of the as-prepared CrMnFeCoNi HEA. Neutron diffraction data analysis revealed an anomalous response of dislocation evolution with the strain.

論文

Dual nanoprecipitation and nanoscale chemical heterogeneity in a secondary hardening steel for ultrahigh strength and large uniform elongation

Wang, S.*; Wang, J.*; Zhang, S.*; Wei, D.*; Chen, Y.*; Rong, X.*; Gong, W.; Harjo, S.; Liu, X.*; Jiao, Z.*; et al.

Journal of Materials Science & Technology, 185, p.245 - 258, 2024/06

 被引用回数:15 パーセンタイル:97.90(Materials Science, Multidisciplinary)

Nanoprecipitates and nanoscale retained austenite (RA) with suitable stability play crucial roles in determining the yield strength (YS) and ductility of ultrahigh strength steels (UHSSs). However, owing to the kinetics incompatibility between nanoprecipitation and austenite reversion, it is highly challenging to simultaneously introduce high-density nanoprecipitates and optimized RA in UHSSs. In this work, through the combination of austenite reversion treatment (ART) and subsequent flash austenitizing (FA), nanoscale chemical heterogeneity was successfully introduced into a low-cost UHSS prior to the aging process. This chemical heterogeneity involved the enrichment of Mn and Ni in the austenite phase. The resulting UHSS exhibited dual-nanoprecipitation of Ni(Al,Mn) and (Mo,Cr)$$_{2}$$ C and nanoscale austenite stabilized via Mn and Ni enrichment. The hard martensitic matrix strengthened by high-density dual-nanoprecipitates constrains the plastic deformation of soft RA with a relatively low fraction, and the presence of relatively stable nanoscale RA with adequate Mn and Ni enrichment leads to a marginal loss in YS but keeps a persistent transformation-induced plasticity (TRIP) effect. As a result, the newly-developed UHSS exhibits an ultrahigh YS of 1.7 GPa, an ultimate tensile strength (UTS) of 1.8 GPa, a large uniform elongation (UE) of 8.5 percent, and a total elongation (TE) of 13 percent. The strategy of presetting chemical heterogeneity to introduce proper metastable phases before aging can be extended to other UHSSs and precipitation-hardened alloys.

論文

Microscopic insights of the extraordinary work-hardening due to phase transformation

Ma, Y.*; Naeem, M.*; Zhu, L.*; He, H.*; Sun, X.*; Yang, Z.*; He, F.*; Harjo, S.; 川崎 卓郎; Wang, X.-L.*

Acta Materialia, 270, p.119822_1 - 119822_13, 2024/05

 被引用回数:9 パーセンタイル:95.42(Materials Science, Multidisciplinary)

We report an in situ neutron diffraction study of 316 L that reveals an extraordinary work-hardening rate (WHR) of $$sim$$7 GPa at 15 K. Detailed analyses show that the major contribution to the excellent strength and ductility comes from the transformation-induced plasticity (TRIP) effect, introduced by the austenite-to-martensite ($$gamma$$-to-$$alpha$$') phase transition. A dramatic increase in the WHR is observed along with the transformation; the WHR declined when the austenite phase is exhausted. During plastic deformation, the volume-fraction weighted phase stress and stress contribution from the $$alpha$$'-martensite increase significantly. The neutron diffraction data further suggest that the $$gamma$$-to-$$alpha$$' phase transformation was mediated by the $$varepsilon$$-martensite, as evidenced by the concurrent decline of the $$varepsilon$$ phase with the $$gamma$$ phase.

論文

Characteristics of temporal variability of long-duration bursts of high-energy radiation associated with thunderclouds on the Tibetan plateau

土屋 晴文; 日比野 欣也*; 川田 和正*; 大西 宗博*; 瀧田 正人*; 宗像 一起*; 加藤 千尋*; 霜田 進*; Shi, Q.*; Wang, S.*; et al.

Progress of Earth and Planetary Science (Internet), 11, p.26_1 - 26_14, 2024/05

 被引用回数:0 パーセンタイル:0.00(Geosciences, Multidisciplinary)

From 1998 to 2017, neutron monitors located at an altitude of 4300 m on the Tibetan plateau detected 127 long-duration bursts of high-energy radiation in association with thunderclouds. These bursts typically lasted for 10-40 min, and 89% of them occurred between 10:00 and 24:00 local time. They were also found to be more likely to occur at night, especially during 18:00-06:00 local time period. The observed diurnal and seasonal variations in burst frequency were consistent with the frequencies of lightning and precipitation on the Tibetan plateau. Based on 19 years of data, the present study suggests that an annual variation in burst frequency has a periodicity of $$sim$$16 years and a lag of $$sim$$3 years relative to solar activity.

論文

Crystal-liquid duality driven ultralow two-channel thermal conductivity in $$alpha$$-MgAgSb

Li, J.*; Li, X.*; Zhang, Y.*; Zhu, J.*; Zhao, E.*; 古府 麻衣子; 中島 健次; Avdeev, M.*; Liu, P.-F.*; Sui, J.*; et al.

Applied Physics Reviews (Internet), 11(1), p.011406_1 - 011406_8, 2024/03

 被引用回数:7 パーセンタイル:91.57(Physics, Applied)

The desire for intrinsically low lattice thermal conductivity ($$kappa_L$$) in thermoelectrics motivates numerous efforts on understanding the microscopic mechanisms of heat transport in solids. Here, based on theoretical calculations, we demonstrate that $$alpha$$-MgAgSb hosts low-energy localized phonon bands and avoided crossing of the rattler modes, which coincides with the inelastic neutron scattering result. Using the two-channel lattice dynamical approach, we find, besides the conventional contribution ($$sim$$70% at 300 K) from particlelike phonons propagating, the coherence contribution dominated by the wavelike tunneling of phonons accounts for $$sim$$30% of total $$kappa_L$$ at 300 K. By considering dual contributions, our calculated room-temperature $$kappa_L$$ of 0.64 Wm$$^{-1}$$K$$^{-1}$$ well agrees with the experimental value of 0.63 Wm$$^{-1}$$K$$^{-1}$$. More importantly, our computations give a nonstandard $$kappa_L propto T^{-0.61}$$ dependence, perfectly explaining the abnormal temperature-trend of $$sim T^{-0.57}$$ in experiment for $$alpha$$-MgAgSb. By molecular dynamics simulation, we reveal that the structure simultaneously has soft crystalline sublattices with the metavalent bonding and fluctuating liquid-like sublattices with thermally induced large amplitude vibrations. These diverse forms of chemical bonding arouse mixed part-crystal part-liquid state, scatter strongly heat-carrying phonons, and finally produce extremely low $$kappa_L$$. The fundamental research from this study will accelerate the design of ultralow-$$kappa_L$$ materials for energy-conversion applications.

論文

Development of wide range photon detection system for muonic X-ray spectroscopy

水野 るり恵*; 新倉 潤*; 齋藤 岳志*; 松崎 禎市郎*; 櫻井 博儀*; Amato, A.*; 浅利 駿介*; Biswas, S.*; Chiu, I.-H.; Gianluca, J.*; et al.

Nuclear Instruments and Methods in Physics Research A, 1060, p.169029_1 - 169029_14, 2024/03

 被引用回数:2 パーセンタイル:46.61(Instruments & Instrumentation)

We have developed a photon detection system for muonic X-ray spectroscopy. The detector system consists of high-purity germanium detectors with BGO Compton suppressors. The signals from the detectors are readout with a digital acquisition system. The absolute energy accuracy, energy and timing resolutions, photo-peak efficiency, the performance of the Compton suppressor, and high count rate durability are studied with standard $$gamma$$-ray sources and in-beam experiment using $$^{27}$$Al($$p,gamma$$)$$^{28}$$Si resonance reaction. The detection system was demonstrated at Paul Scherrer Institute. A calibration method for a photon detector at a muon facility using muonic X-rays of $$^{197}$$Au and $$^{209}$$Bi is proposed.

論文

Onset of collectivity for argon isotopes close to $$N=32$$

Linh, B. D.*; Corsi, A.*; Gillibert, A.*; Obertelli, A.*; Doornenbal, P.*; Barbieri, C.*; Duguet, T.*; G$'o$mez-Ramos, M.*; Holt, J. D.*; Hu, B. S.*; et al.

Physical Review C, 109(3), p.034312_1 - 034312_15, 2024/03

 被引用回数:2 パーセンタイル:58.81(Physics, Nuclear)

理化学研究所RIビームファクトリーにて中性子過剰核$$^{50}$$Arビームからの1中性子ノックアウト反応実験を行い、$$^{49}$$Arのエネルギー準位および分光学的因子を導出した。特に、第一励起状態の$$1/2^-$$への分光学的因子が大きいことから、始状態の$$^{50}$$Arの基底状態において中性子が$$p_{1/2}$$軌道を多く占めていることがわかった。これは、中性子数32がよい魔法数として知られる$$^{52}$$Caとは異なった性質であり、カルシウムからアルゴンへと陽子が2個減ることで閉殻構造が大きく崩れることが明らかになった。

論文

ALTEMIS: Using integrated hydrology and reactive transport modeling to support resilience at the Savannah River Site

Xu, Z.*; Litzinger, A.*; 佐久間 一幸; Arora, B.*; Hazenberg, P.*; Wang, L.*; Gonzalez Raymat, H.*; Fabricatore, E.*; Wainwright, Haruko*; Eddy-Dilek, C.*

Proceedings of Waste Management Symposia 2024 (WM2024) (Internet), 14 Pages, 2024/03

We leverage the Advanced Terrestrial Simulator (ATS), a comprehensive model encompassing overland flow, groundwater processes, canopy and ground evapotranspiration effects. ATS is integrated with reactive transport models, including PFLOTRAN and CrunchFlow, to capture the intricate dynamics of key nuclear-related geochemical species. The Advanced Long-term Environmental Monitoring Systems (ALTEMIS) project extends its efforts across multiple scales: 1) Watershed Scale ATS Model: At the Savannah River Site, we employ a watershed-scale ATS model to quantify the water budget and estimate evapotranspiration fluxes.; 2) Integrated Hydrology Model for Floodplains: Our integrated hydrology model zooms in on the floodplain of Fourmiles Creek, enabling quantification of upwelling groundwater fluxes into wetlands and surface ponds. It also used to assess contaminant migration into Fourmiles Creek; 3) Fully Integrated Reactive Transport Model: Focused on the F-Area seepage basin, one of the largest nuclear waste processing facilities, we develop both 2D transect and 3D basin models. These models estimate the behavior of radioactive elements such as uranium and tritium, as well as non-reactive geochemical species.; 4) Sr-90 Sorption Model: Informed by extensive Sr-90 sorption experiments on minerals and core samples, we parameterize both electrostatic and non-electrostatic sorption models for Sr-90. These models are integrated into multiple reactive transport frameworks, significantly enhancing our ability to accurately predict Sr-90 migration under varying pH conditions.

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