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論文

Mechanism of paramagnetic spin Seebeck effect

大柳 洸一*; 高橋 三郎*; 吉川 貴史*; 齊藤 英治

Physical Review B, 107(1), p.014423_1 - 014423_8, 2023/01

 被引用回数:7 パーセンタイル:94.87(Materials Science, Multidisciplinary)

We have theoretically investigated the spin Seebeck effect (SSE) in a normal metal (NM)/paramagnetic insulator (PI) bilayer system. Through a linear response approach, we calculated the thermal spin pumping from PI to NM and backflow spin current from NM to PI, where the spin-flip scattering via the interfacial exchange coupling between conduction-electron spin in NM and localized spin in PI is taken into account. We found a finite spin current appears at the interface under the difference in the effective temperatures between spins in NM and PI, and its intensity increases by increasing the density of the localized spin S. Our model well reproduces the magnetic-field-induced reduction of the paramagnetic SSE in Pt/Gd$$_3$$Ga$$_5$$O$$_{12}$$ experimentally observed when the Zeeman energy is comparable to the thermal energy, which can be interpreted as the suppression of the interfacial spin-flip scattering. The present finding provides an insight into the mechanism of paramagnetic SSEs and the thermally induced spin-current generation in magnetic materials.

論文

Paramagnetic spin Hall magnetoresistance

大柳 洸一*; Gomez-Perez, J. M.*; Zhang, X.-P.*; 吉川 貴史*; Chen, Y.*; Sagasta, E.*; Chuvilin, A.*; Hueso, L. E.*; Golovach, V. N.*; Sebastian Bergeret, F.*; et al.

Physical Review B, 104(13), p.134428_1 - 134428_14, 2021/10

 被引用回数:14 パーセンタイル:77.64(Materials Science, Multidisciplinary)

We report the observation of the spin Hall magnetoresistance (SMR) in a paramagnetic insulator. By measuring the transverse resistance in a Pt/Gd$$_3$$Ga$$_5$$O$$_{12}$$ (GGG) system at low temperatures, paramagnetic SMR is found to appear with an intensity that increases with the magnetic field aligning GGG's spins. The observed effect is well supported by a microscopic SMR theory, which provides the parameters governing the spin transport at the interface. Our findings clarify the mechanism of spin exchange at a Pt/GGG interface, and demonstrate tunable spin-transfer torque through the field-induced magnetization of GGG. In this regard, paramagnetic insulators offer a key property for future spintronic devices.

論文

Triplon current generation in solids

Chen, Y.*; 佐藤 正寛*; Tang, Y.*; 塩見 雄毅*; 大柳 洸一*; 益田 隆嗣*; 南部 雄亮*; 藤田 全基*; 齊藤 英治

Nature Communications (Internet), 12, p.5199_1 - 5199_7, 2021/08

 被引用回数:8 パーセンタイル:61.37(Multidisciplinary Sciences)

A triplon refers to a fictitious particle that carries angular momentum $$S=1$$ corresponding to the elementary excitation in a broad class of quantum dimerized spin systems. Such systems without magnetic order have long been studied as a testing ground for quantum properties of spins. Although triplons have been found to play a central role in thermal and magnetic properties in dimerized magnets with singlet correlation, a spin angular momentum flow carried by triplons, a triplon current, has not been detected yet. Here we report spin Seebeck effects induced by a triplon current: triplon spin Seebeck effect, using a spin-Peierls system CuGeO$$_3$$. The result shows that the heating-driven triplon transport induces spin current whose sign is positive, opposite to the spin-wave cases in magnets. The triplon spin Seebeck effect persists far below the spin-Peierls transition temperature, being consistent with a theoretical calculation for triplon spin Seebeck effects.

論文

Observation of nuclear-spin Seebeck effect

吉川 貴史*; Reitz, D.*; 伊藤 宏陽*; 巻内 崇彦*; 杉本 宜陽*; 恒川 翔*; 大門 俊介*; 大柳 洸一*; Ramos, R.*; 高橋 三郎*; et al.

Nature Communications (Internet), 12, p.4356_1 - 4356_7, 2021/07

 被引用回数:19 パーセンタイル:88.38(Multidisciplinary Sciences)

Thermoelectric effects have been applied to power generators and temperature sensors that convert waste heat into electricity. The effects, however, have been limited to electrons to occur, and inevitably disappear at low temperatures due to electronic entropy quenching. Here, we report thermoelectric generation caused by nuclear spins in a solid: nuclear-spin Seebeck effect. The sample is a magnetically ordered material MnCO$$_3$$ having a large nuclear spin $$(I=5/2)$$ of $$^{55}$$Mn nuclei and strong hyperfine coupling, with a Pt contact. In the system, we observe low-temperature thermoelectric signals down to 100 mK due to nuclear-spin excitation. Our theoretical calculation in which interfacial Korringa process is taken into consideration quantitatively reproduces the results. The nuclear thermoelectric effect demonstrated here offers a way for exploring thermoelectric science and technologies at ultralow temperatures.

論文

Observation of quantum interference conductance fluctuations in metal rings with strong spin-orbit coupling

Ramos, R.*; 巻内 崇彦*; 吉川 貴史*; 大門 俊介*; 大柳 洸一*; 齊藤 英治

Applied Physics Letters, 117(24), p.242402_1 - 242402_5, 2020/12

 被引用回数:1 パーセンタイル:5.55(Physics, Applied)

We investigated the magnetotransport properties of mesoscopic platinum nanostructures (wires and rings) with sub-100 nm lateral dimensions at very low temperatures. Despite the strong spin-orbit interaction in platinum, oscillation of the conductance as a function of the external magnetic field due to quantum interference effects was found to appear. The oscillation was decomposed into Aharonov-Bohm periodic oscillations and aperiodic fluctuations of the conductance due to a magnetic flux piercing the loop of the ring and the metal wires forming the nanostructures, respectively. We also investigated the magnetotransport under different bias currents to explore the interplay between electron phase coherence and spin accumulation effects in strong spin-orbit conductors.

論文

Magnetic field dependence of the nonlocal spin Seebeck effect in Pt/YIG/Pt systems at low temperatures

大柳 洸一*; 吉川 貴史*; 齊藤 英治

AIP Advances (Internet), 10(1), p.015031_1 - 015031_5, 2020/01

 被引用回数:15 パーセンタイル:71.02(Nanoscience & Nanotechnology)

We report the nonlocal spin Seebeck effect (nlSSE) in a lateral configuration of Pt/Y$$_3$$Fe$$_5$$O$$_{12}$$(YIG)/Pt systems as a function of the magnetic field $$B$$ (up to 10 T) at various temperatures $$T$$ (3 K $$< T <$$ 300 K). The nlSSE voltage decreases with increasing B in a linear regime with respect to the input power (the applied charge-current squared $$I^2$$). The reduction of the nlSSE becomes substantial when the Zeeman energy exceeds thermal energy at low temperatures, which can be interpreted as freeze-out of magnons relevant for the nlSSE. Furthermore, we found the nonlinear power dependence of the nlSSE with increasing $$I$$ at low temperatures ($$T <$$ 20 K), at which the B-induced signal reduction became less visible. Our experimental results suggest that in the nonlinear regime, high-energy magnons are overpopulated compared to those expected from the thermal energy. We also estimate the magnon spin diffusion length as functions of $$B$$ and $$T$$.

論文

Absence of evidence of spin transport through amorphous Y$$_3$$Fe$$_5$$O$$_{12}$$

Gomez-Perez, J. M.*; 大柳 洸一*; 八尋 黎明*; Ramos, R.*; Hueso, L. E.*; 齊藤 英治; Casanova, F.*

Applied Physics Letters, 116(3), p.032401_1 - 032401_5, 2020/01

 被引用回数:9 パーセンタイル:53.43(Physics, Applied)

We probe the current-induced magnetic switching of insulating antiferromagnet-heavy-metal systems, by electrical spin Hall magnetoresistance measurements and direct imaging, identifying a reversal occurring by domain wall (DW) motion. We observe switching of more than one-third of the antiferromagnetic domains by the application of current pulses. Our data reveal two different magnetic switching mechanisms leading together to an efficient switching, namely, the spin-current induced effective magnetic anisotropy variation and the action of the spin torque on the DWs.

論文

Magnon polarons in the spin Peltier effect

八尋 黎明*; 吉川 貴史*; Ramos, R.*; 大柳 洸一*; 日置 友智*; 大門 俊介*; 齊藤 英治

Physical Review B, 101(2), p.024407_1 - 024407_7, 2020/01

 被引用回数:19 パーセンタイル:77.9(Materials Science, Multidisciplinary)

We report the observation of anomalous peak structures induced by hybridized magnon-phonon excitation (magnon polarons) in the magnetic field dependence of the spin Peltier effect (SPE) in a Lu$$_2$$Bi$$_1$$Fe$$_4$$Ga$$_1$$O$$_{12}$$ (BiGa:LuIG) with Pt contact. The SPE peaks coincide with magnetic fields tuned to the threshold of magnonpolaron formation, consistent with the previous observation in the spin Seebeck effect. The enhancement of SPE is attributed to the lifetime increase in spin current caused by magnon-phonon hybridization in BiGa:LuIG.

論文

Spin transport in insulators without exchange stiffness

大柳 洸一*; 高橋 三郎*; Cornelissen, L. J.*; Shan, J.*; 大門 俊介*; 吉川 貴史*; Bauer, G. E. W.*; Van Wees, B. J.*; 齊藤 英治

Nature Communications (Internet), 10, p.4740_1 - 4740_6, 2019/10

 被引用回数:38 パーセンタイル:89.44(Multidisciplinary Sciences)

The discovery of new materials that efficiently transmit spin currents has been important for spintronics and material science. The electric insulator Gd$$_3$$Ga$$_5$$O$$_{12}$$ (GGG), a standard substrate for growing magnetic films, can be a spin current generator, but has never been considered as a superior conduit for spin currents. Here we report spin current propagation in paramagnetic GGG over several microns. Surprisingly, spin transport persists up to temperatures of 100 K $$gg$$ T$$_g$$=180 mK, the magnetic glass-like transition temperature of GGG. At 5 K and 3.5 T, we find a spin diffusion length $$lambda_mathrm{GGG}=1.8pm0.2$$ $$mu$$m and a spin conductivity $$sigma_mathrm{GGG}=(7.3 pm 0.3)times 10^4$$ Sm$$^{-1}$$ that is larger than that of the record quality magnet Y$$_3$$Fe$$_5$$O$$_{12}$$ (YIG). We conclude that exchange stiffness is not required for efficient spin transport, which challenges conventional models and provides new material-design strategies for spintronic devices.

論文

Spin Seebeck mechanical force

針井 一哉; Seo, Y.-J.*; 堤 康雅*; 中堂 博之; 大柳 洸一*; 松尾 衛; 塩見 雄毅*; 小野 崇人*; 前川 禎通; 齊藤 英治

Nature Communications (Internet), 10, p.2616_1 - 2616_5, 2019/06

 被引用回数:28 パーセンタイル:81.46(Multidisciplinary Sciences)

Electric current has been used to send electricity to far distant places. On the other hand, spin current, a flow of electron spin, can in principle also send angular momentum to distant places. In a magnet, there is a universal spin carrier called a spin wave, a wave-type excitation of magnetization. Since spin waves exhibit a long propagation length, it should be able to send angular momentum that can generate torque and force at a distant place: a new function of magnets. Here we observe mechanical angular momentum transmission and force generation due to spin waves injected into Y$$_3$$Fe$$_5$$O$$_{12}$$ by the spin-Seebeck effect. The spin-wave current, transmitted through a Y$$_3$$Fe$$_5$$O$$_{12}$$ micro cantilever, was found to create a mechanical force on the cantilever as a non-local reaction of the spin-Seebeck effect. Spin-wave current can be generated remotely even in open circuits, and it can be used to drive micro mechanical devices.

論文

Magnetomechanical sensing based on delta-E effect in Y$$_3$$Fe$$_5$$O$$_{12}$$ micro bridge

有沢 洋希*; 大門 俊介*; 追川 康之*; Seo, Y.-J.*; 針井 一哉; 大柳 洸一*; 齊藤 英治

Applied Physics Letters, 114(12), p.122402_1 - 122402_5, 2019/03

 被引用回数:5 パーセンタイル:27.67(Physics, Applied)

We have investigated magnetic field effects on mechanical vibration of a magnetic microbridge made of ferrimagnetic insulator Y$$_3$$Fe$$_5$$O$$_{12}$$ at room temperature. The mechanical resonance frequency of the bridge exhibits a steep change at the saturation magnetic field of the microbridge. The steep change was shown to originate from magnetoelastic coupling combined with shape magnetic anisotropy. The competition between shape magnetic anisotropy and the external magnetic field can drive a delta-E effect, the modulation of Young modulus via the magnetoelastic coupling, in a narrow field range, which results in the observed steep change in the mechanical property.

論文

Fabrication and magnetic control of Y$$_3$$Fe$$_5$$O$$_{12}$$ cantilevers

Seo, Y.-J.*; 針井 一哉; 高橋 遼*; 中堂 博之; 大柳 洸一*; Qiu, Z.*; 小野 崇人*; 塩見 雄毅*; 齊藤 英治

Applied Physics Letters, 110(13), p.132409_1 - 132409_4, 2017/03

 被引用回数:12 パーセンタイル:50.89(Physics, Applied)

フェリ磁性体であるY$$_3$$Fe$$_5$$O$$_{12}$$を用いたサブミクロンカンチレバーを収束イオンビーム法によって作成し、その振動特性を磁場によって制御した。カンチレバーは縦横2つの振動モードを示し、それぞれのモードは外部磁場の印加によって共鳴周波数が減少、増大した。この結果は磁気力の磁場変化を取り扱った数値シミュレーションでよく再現された。周波数変化は数%に及ぶことから、磁場による高効率な振動制御が行われたと結論できる。

口頭

磁性絶縁体カンチレバーによるスピン波スピン流の検出

針井 一哉; Seo, Y.-J.*; 堤 康雅*; 中堂 博之; 大柳 洸一*; 松尾 衛*; 塩見 雄毅*; 小野 崇人*; 前川 禎通; 齊藤 英治

no journal, , 

スピントロニクス分野において、スピン角運動量と他の角運動量の間の変換は重要な役割を担ってきた。その中で、Einstein-de Haas効果に代表されるスピンから力学的な角運動量への変換は、角運動量保存則によって高効率に行われることが知られている。本研究では、スピン-力学的角運動量変換に、近年多くの注目を集めている磁性絶縁体中のスピン波スピン流を組み合わせることで、力学的角運動量の空間伝送を試みた。サンプルには、イットリウム鉄ガーネットを集束イオンビーム法で加工して作成したマイクロカンチレバー構造を用いた。カンチレバーの根元にパターニングしたヒーター線からの加熱によるスピンSeebeck効果を用いることでカンチレバーにスピン流を注入し、その際生じる振動をレーザーDoppler干渉計によって計測した。熱応力による振動を排除するため、交流熱流と交流磁場によるヘテロダイン信号を測定した結果、交流磁場とカンチレバーが直交する際のみ有意な振動が観測された。この振る舞いはスピン流-力学的角運動量変換の対称性によく対応している。講演では、スピン流を遮断した実験等、結果の詳細を報告する。

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