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木村 尚次郎*; 大西 弘明; 奥西 巧一*; 赤木 暢*; 鳴海 康雄*; 萩原 政幸*; 金道 浩一*; 菊池 彦光*
Journal of the Physical Society of Japan, 92(9), p.094701_1 - 094701_9, 2023/09
被引用回数:0 パーセンタイル:0(Physics, Multidisciplinary)High-field electron spin resonance (ESR) measurements were performed on the =1/2 Ising-like antiferromagnetic chain CsCoCl in the frequency range up to 4.4THz and magnetic fields for up to 53T. We observed softening of the spinon excitation, which drives the spin chain into the quantum critical state at the critical field =33.0T. Above , we observed the string excitation at the wave number =, which is characteristic of the =1/2 spin chain in the quantum critical state in the magnetic fields. We also observed a crossover of the string excitation to the magnon bound state above the saturation fields =43.9T upon increasing the magnetic fields. Finally, we discuss how the string excitation and magnon bound state can be excited by the electric dipole transition due to spin quadrupolar resonance.
木村 尚次郎*; 大西 弘明; 奥谷 顕*; 赤木 暢*; 鳴海 康雄*; 萩原 政幸*; 奥西 巧一*; 金道 浩一*; He, Z.*; 谷山 智康*; et al.
Physical Review B, 105(1), p.014417_1 - 014417_9, 2022/01
被引用回数:3 パーセンタイル:34.67(Materials Science, Multidisciplinary)In this study, we clarify the selection rules of optical transitions from the ground state to the magnetic excited states in the quasi-one-dimensional quantum Ising-like antiferromagnet BaCoVO with spin = using the high-field electron spin resonance measurement with illuminating polarized electromagnetic waves. We demonstrate that the unconventional magnetic excitation via the pair creation of quasipaticles at wave numbers and in the field-induced quantum critical state can couple with both oscillating magnetic and electric fields. Our density matrix renormalization group calculations indicate that the observed selection rules can be explained by two- and four-fold periodical spin interactions, originating from the screw chain structure in BaCoVO, in addition to the magnetoelectric coupling between spins and electric dipoles.
安井 幸夫*; 宮本 拓馬*; 郡 俊輔*; 寺崎 一郎*; 吉澤 大智*; 赤木 暢*; 萩原 政幸*; 松川 健*; 吉田 幸彦*; 星川 晃範*; et al.
no journal, ,
RCrTiO多結晶試料について、50Tまでの磁場中における比熱および磁化を測定し、また、NdCrTiOおよびNdPrCrTiOの粉末中性子回折測定を行った。50Tまでの比熱データと磁化曲線から、Cr-Cr間およびCr-R間の磁気モーメントの磁気相互作用を評価した。また、NdCrTiOの中性子磁気反射強度の温度依存性から、CrモーメントとNdモーメントがで同時にオーダーすることが明らかとなった。本発表では、実験で得られた磁気挙動を基に、RCrTiOの磁気電気効果機構について議論する。