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JAEA Reports

Research plan on geosphere stability for long-term isolation of radioactive waste (Scientific program for fiscal year 2023)

Niwa, Masakazu; Shimada, Koji; Sueoka, Shigeru; Fujita, Natsuko; Yokoyama, Tatsunori; Ogita, Yasuhiro; Fukuda, Shoma; Nakajima, Toru; Kagami, Saya; Ogata, Manabu; et al.

JAEA-Review 2023-017, 27 Pages, 2023/10

JAEA-Review-2023-017.pdf:0.94MB

This report is a plan of research and development (R&D) on geosphere stability for long-term isolation of high-level radioactive waste (HLW) in Japan Atomic Energy Agency (JAEA), in fiscal year 2023. The objectives and contents in fiscal year 2023 are described in detail based on the JAEA 4th Medium- and Long-term Plan (fiscal years 2022-2028). In addition, the background of this research is described from the necessity and the significance for site investigation and safety assessment, and the past progress. The plan framework is structured into the following categories: (1) Development and systematization of investigation techniques, (2) Development of models for long-term estimation and effective assessment, (3) Development of dating techniques.

JAEA Reports

Annual report for research on geosphere stability for long-term isolation of radioactive waste in fiscal year 2022

Niwa, Masakazu; Shimada, Koji; Sueoka, Shigeru; Ishihara, Takanori; Ogawa, Hiroki; Hakoiwa, Hiroaki; Watanabe, Tsuyoshi; Nishiyama, Nariaki; Yokoyama, Tatsunori; Ogata, Manabu; et al.

JAEA-Research 2023-005, 78 Pages, 2023/10

JAEA-Research-2023-005.pdf:6.51MB

This annual report documents the progress of research and development (R&D) in the 1st fiscal year of the Japan Atomic Energy Agency 4th Medium- and Long-term Plan (fiscal years 2022-2028) to provide the scientific base for assessing geosphere stability for long-term isolation of high-level radioactive waste. The plan framework is structured into the following categories: (1) Development and systematization of investigation techniques, (2) Development of models for long-term estimation and effective assessment, (3) Development of dating techniques. The current status of R&D activities with previous scientific and technological progress is summarized.

Journal Articles

A Terrestrial SER Estimation Methodology Based on Simulation Coupled With One-Time Neutron Irradiation Testing

Abe, Shinichiro; Hashimoto, Masanori*; Liao, W.*; Kato, Takashi*; Asai, Hiroaki*; Shimbo, Kenichi*; Matsuyama, Hideya*; Sato, Tatsuhiko; Kobayashi, Kazutoshi*; Watanabe, Yukinobu*

IEEE Transactions on Nuclear Science, 70(8, Part 1), p.1652 - 1657, 2023/08

 Times Cited Count:0 Percentile:0.01(Engineering, Electrical & Electronic)

Single event upsets (SEUs) caused by neutrons is a reliability problem for microelectronic devices in the terrestrial environment. Acceleration tests using white neutron beam provide realistic soft error rates (SERs), but only a few facilities can provide white neutron beam in the world. If single-source irradiation applicable to diverse neutron source can be utilized for the evaluation of the SER in the terrestrial environment, it contributes to solve the shortage of beam time. In this study, we investigated the feasibility of the SER estimation in the terrestrial environment by any one of these measured data with the SEU cross sections obtained by PHITS simulation. It was found that the SERs estimated by our proposed method are within a factor of 2.7 of that estimated by the Weibull function. We also investigated the effect of simplification which reduce the computational cost in simulation to the SER estimation.

Journal Articles

Laser-driven neutron generation realizing single-shot resonance spectroscopy

Yogo, Akifumi*; Lan, Z.*; Arikawa, Yasunobu*; Abe, Yuki*; Mirfayzi, S. R.*; Wei, T.*; Mori, Takato*; Golovin, D.*; Hayakawa, Takehito*; Iwata, Natsumi*; et al.

Physical Review X, 13(1), p.011011_1 - 011011_12, 2023/01

 Times Cited Count:3 Percentile:88.42(Physics, Multidisciplinary)

Journal Articles

Sodium-cooled Fast Reactors

Ohshima, Hiroyuki; Morishita, Masaki*; Aizawa, Kosuke; Ando, Masanori; Ashida, Takashi; Chikazawa, Yoshitaka; Doda, Norihiro; Enuma, Yasuhiro; Ezure, Toshiki; Fukano, Yoshitaka; et al.

Sodium-cooled Fast Reactors; JSME Series in Thermal and Nuclear Power Generation, Vol.3, 631 Pages, 2022/07

This book is a collection of the past experience of design, construction, and operation of two reactors, the latest knowledge and technology for SFR designs, and the future prospects of SFR development in Japan. It is intended to provide the perspective and the relevant knowledge to enable readers to become more familiar with SFR technology.

Journal Articles

Improving the safety of the high temperature gas-cooled reactor "HTTR" based on Japan's new regulatory requirements

Hamamoto, Shimpei; Shimizu, Atsushi; Inoi, Hiroyuki; Tochio, Daisuke; Homma, Fumitaka; Sawahata, Hiroaki; Sekita, Kenji; Watanabe, Shuji; Furusawa, Takayuki; Iigaki, Kazuhiko; et al.

Nuclear Engineering and Design, 388, p.111642_1 - 111642_11, 2022/03

 Times Cited Count:2 Percentile:53.91(Nuclear Science & Technology)

Following the Fukushima Daiichi Nuclear Power Plant accident in 2011, the Japan Atomic Energy Agency adapted High-Temperature engineering Test Reactor (HTTR) to meet the new regulatory requirements that began in December 2013. The safety and seismic classifications of the existing structures, systems, and components were discussed to reflect insights regarding High Temperature Gas-cooled Reactors (HTGRs) that were acquired through various HTTR safety tests. Structures, systems, and components that are subject to protection have been defined, and countermeasures to manage internal and external hazards that affect safety functions have been strengthened. Additionally, measures are in place to control accidents that may cause large amounts of radioactive material to be released, as a beyond design based accident. The Nuclear Regulatory Commission rigorously and appropriately reviewed this approach for compliance with the new regulatory requirements. After nine amendments, the application to modify the HTTR's installation license that was submitted in November 2014 was approved in June 2020. This response shows that facilities can reasonably be designed to meet the enhanced regulatory requirements, if they reflect the characteristics of HTGRs. We believe that we have established a reference for future development of HTGR.

JAEA Reports

Mizunami Underground Research Laboratory Project, Annual report for fiscal year 2019

Takeuchi, Ryuji; Onoe, Hironori; Murakami, Hiroaki; Watanabe, Yusuke; Mikake, Shinichiro; Ikeda, Koki; Iyatomi, Yosuke; Nishio, Kazuhisa*; Sasao, Eiji

JAEA-Review 2021-003, 63 Pages, 2021/06

JAEA-Review-2021-003.pdf:12.67MB

The Mizunami Underground Research Laboratory (MIU) Project is being pursued by the Japan Atomic Energy Agency (JAEA) to enhance the reliability of geological disposal technologies through investigations of the deep geological environment in the crystalline rock (granite) at Mizunami City, Gifu Prefecture, central Japan. On the occasion of JAEA reformation in FY2014, JAEA identified three remaining important issues on the geoscientific research program based on the synthesized latest results of research and development (R&D): "Development of countermeasure technologies for reducing groundwater inflow", "Development of modeling technologies for mass transport" and "Development of drift backfilling technologies". At the MIU, the R&D are being pursued with a focus on the remaining important issues from FY2015, and satisfactory results have been achieved. Based on this situation, the R&D on the MIU Project were completed at the end of FY2019. In this report, the results of R&D and construction activities of the MIU Project in FY2019 are summarized.

JAEA Reports

Hydrochemical investigation at the Mizunami Underground Research Laboratory; Compilation of groundwater chemistry data in the Mizunami Group and the Toki Granite (fiscal year 2019)

Fukuda, Kenji; Watanabe, Yusuke; Murakami, Hiroaki; Amano, Yuki; Aosai, Daisuke*; Hara, Naohiro*

JAEA-Data/Code 2020-012, 80 Pages, 2020/10

JAEA-Data-Code-2020-012.pdf:3.55MB

Japan Atomic Energy Agency has been investigating groundwater chemistry to understand the influence of excavation and maintenance of underground facilities as part of the Mizunami Underground Research Laboratory (MIU) Project in Mizunami, Gifu, Japan. In this report, we compiled data of groundwater chemistry and microbiology obtained at the MIU in the fiscal year 2019. In terms of ensuring traceability of data, basic information (e.g. sampling location, sampling time, sampling method and analytical method) and methodology for quality control are described.

Journal Articles

Mechanical and thermal properties of Zr-B and Fe-B alloys

Sun, Y.*; Abe, Yuta; Muta, Hiroaki*; Oishi, Yuji*

Journal of Nuclear Science and Technology, 57(8), p.917 - 925, 2020/08

 Times Cited Count:5 Percentile:53.85(Nuclear Science & Technology)

Journal Articles

How different is the core of $$^{25}$$F from $$^{24}$$O$$_{g.s.}$$ ?

Tang, T. L.*; Uesaka, Tomohiro*; Kawase, Shoichiro; Beaumel, D.*; Dozono, Masanori*; Fujii, Toshihiko*; Fukuda, Naoki*; Fukunaga, Taku*; Galindo-Uribarri, A.*; Hwang, S. H.*; et al.

Physical Review Letters, 124(21), p.212502_1 - 212502_6, 2020/05

 Times Cited Count:14 Percentile:74.18(Physics, Multidisciplinary)

The structure of a neutron-rich $$^{25}$$F nucleus is investigated by a quasifree ($$p,2p$$) knockout reaction. The sum of spectroscopic factors of $$pi 0d_{5/2}$$ orbital is found to be 1.0 $$pm$$ 0.3. The result shows that the $$^{24}$$O core of $$^{25}$$F nucleus significantly differs from a free $$^{24}$$O nucleus, and the core consists of $$sim$$35% $$^{24}$$O$$_{rm g.s.}$$, and $$sim$$65% excited $$^{24}$$O. The result shows that the $$^{24}$$O core of $$^{25}$$F nucleus significantly differs from a free $$^{24}$$O nucleus. The result may infer that the addition of the $$0d_{5/2}$$ proton considerably changes the neutron structure in $$^{25}$$F from that in $$^{24}$$O, which could be a possible mechanism responsible for the oxygen dripline anomaly.

JAEA Reports

Hydrochemical investigation at the Mizunami Underground Research Laboratory; Compilation of groundwater chemistry data in the Mizunami group and the Toki granite (fiscal year 2018)

Fukuda, Kenji; Watanabe, Yusuke; Murakami, Hiroaki; Amano, Yuki; Aosai, Daisuke*; Kumamoto, Yoshiharu*; Iwatsuki, Teruki

JAEA-Data/Code 2019-019, 74 Pages, 2020/03

JAEA-Data-Code-2019-019.pdf:3.53MB

Japan Atomic Energy Agency has been investigating groundwater chemistry to understand the influence of excavation and maintenance of underground facilities as part of the Mizunami Underground Research Laboratory (MIU) Project in Mizunami, Gifu, Japan. In this report, we compiled data of groundwater chemistry and microbiology obtained at the MIU in the fiscal year 2018. In terms of ensuring traceability of data, basic information (e.g. sampling location, sampling time, sampling method and analytical method) and methodology for quality control are described.

Journal Articles

Intercomparison of numerical atmospheric dispersion prediction models for emergency response to emissions of radionuclides with limited source information in the Fukushima Dai-ichi Nuclear Power Plant accident

Iwasaki, Toshiki*; Sekiyama, Tsuyoshi*; Nakajima, Teruyuki*; Watanabe, Akira*; Suzuki, Yasushi*; Kondo, Hiroaki*; Morino, Yu*; Terada, Hiroaki; Nagai, Haruyasu; Takigawa, Masayuki*; et al.

Atmospheric Environment, 214, p.116830_1 - 116830_11, 2019/10

 Times Cited Count:6 Percentile:26.43(Environmental Sciences)

The utilization of numerical atmospheric dispersion prediction (NDP) models for accidental discharge of radioactive substances was recommended by a working group of the Meteorological Society of Japan. This paper is to validate the recommendation through NDP model intercomparison in the accidental release from the Fukushima Dai-ichi Nuclear Power Plant in 2011. Emission intensity is assumed to be constant during the whole forecast period for the worst-case scenario unless time sequence of emission is available. We expect to utilize forecasts of surface air contaminations for preventions of inhalations of radioactive substances, and column-integrated amounts for mitigation of radiation exposure associated with wet deposition. Although NDP forecasts have ensemble spread, they commonly figure out relative risk in space and time. They are of great benefit to disseminating effective warnings to public without failure. The multi-model ensemble technique may be effective to improve the reliability.

Journal Articles

Study on loss-of-cooling and loss-of-coolant accidents in spent fuel pool, 1; Overview

Kaji, Yoshiyuki; Nemoto, Yoshiyuki; Nagatake, Taku; Yoshida, Hiroyuki; Tojo, Masayuki*; Goto, Daisuke*; Nishimura, Satoshi*; Suzuki, Hiroaki*; Yamato, Masaaki*; Watanabe, Satoshi*

Proceedings of 27th International Conference on Nuclear Engineering (ICONE-27) (Internet), 8 Pages, 2019/05

In this research program, cladding oxidation model in SFP accident condition, and numerical simulation method to evaluate capability of spray cooling system which was deployed for spent fuel cooling during SFP accident, have been developed. These were introduced into the severe accident codes such as MAAP and SAMPSON, and SFP accident analyses were conducted. Analyses using Computational Fluid Dynamics (CFD) code were conducted as well for the comparison with SA code analyses and investigation of detail in the SFP accident. In addition, three-dimensional criticality analysis method was developed as well, and safer loading pattern of spent fuels in pool was investigated.

JAEA Reports

Hydrochemical investigation at the Mizunami Underground Research Laboratory; Compilation of groundwater chemistry data in the Mizunami group and the Toki granite (fiscal year 2017)

Fukuda, Kenji; Watanabe, Yusuke; Murakami, Hiroaki; Amano, Yuki; Hayashida, Kazuki*; Aosai, Daisuke*; Kumamoto, Yoshiharu*; Iwatsuki, Teruki

JAEA-Data/Code 2018-021, 76 Pages, 2019/03

JAEA-Data-Code-2018-021.pdf:3.78MB

Japan Atomic Energy Agency has been investigating groundwater chemistry to understand the influence of excavation and maintenance of underground facilities as part of the Mizunami Underground Research Laboratory (MIU) Project in Mizunami, Gifu, Japan. In this report, we compiled data of groundwater chemistry and microbiology obtained at the MIU in the fiscal year 2017. In terms of ensuring traceability of data, basic information (e.g. sampling location, sampling time, sampling method and analytical method) and methodology for quality control are described.

Journal Articles

Hydrochemical influence of shotcrete used in underground facilities on groundwater chemistry; Proposal of the evaluation method by geochemical simulation code

Iwatsuki, Teruki; Shibata, Masahito*; Murakami, Hiroaki; Watanabe, Yusuke; Fukuda, Kenji

Doboku Gakkai Rombunshu, G (Kankyo) (Internet), 75(1), p.42 - 54, 2019/03

In order to clarify the influence of shotcrete in the underground facility on the groundwater chemistry, an in-situ closed test was conducted in the mock-up tunnel at the depth of 500 m. Brucite, Ettringite, Ca(OH) $$_{2}$$, Gibbsite, K$$_{2}$$CO$$_{3}$$, Na$$_{2}$$CO$$_{3}$$ $$cdot$$ 10H$$_{2}$$O, SiO$$_{2}$$ (a) and Calcite were identified as the dominant minerals affecting the water chemistry. Furthermore, the shotcrete constructed in the tunnel has a reaction capacity which can produce about 570 m$$^{3}$$ of alkaline groundwater (pH12.4) saturated with Ca(OH)$$_{2}$$. The estimation would improve the accuracy of prediction analysis of the long-term chemical influence of cement materials after the closure of the tunnel.

Journal Articles

Nanoscale ice-type structural fluctuation in spinel titanates

Torigoe, Shuhei*; Hattori, Takayuki*; Kodama, Katsuaki; Honda, Takashi*; Sagayama, Hajime*; Ikeda, Kazutaka*; Otomo, Toshiya*; Nitani, Hiroaki*; Abe, Hitoshi*; Murakawa, Hiroshi*; et al.

Physical Review B, 98(13), p.134443_1 - 134443_7, 2018/10

 Times Cited Count:11 Percentile:52.03(Materials Science, Multidisciplinary)

Journal Articles

Onsite chelate resin solid-phase extraction of rare earth elements in natural water samples; Its implication for studying past redox changes by inorganic geochemistry

Watanabe, Takahiro; Kokubu, Yoko; Murakami, Hiroaki; Iwatsuki, Teruki

Limnology, 19(1), p.21 - 30, 2018/01

 Times Cited Count:11 Percentile:53.29(Limnology)

Rare earth element (REE) patterns in natural water and geological samples provides information on changes in past environmental conditions, such as redox changes and material cycles; however, quantitative analysis of REEs in these samples is complicated because of relative low content and mass interference from barium oxide in the inductively coupled plasma mass spectrometry (ICP-MS) analyses. In this study, we adopted onsite solid-phase extraction and preconcentration methods for REEs using an iminobisacetic acid-ethylenediaminetriacetic acid chelate resin for the analyses. Standard reference materials, natural ground water, and spring water samples were used for the evaluation of these methods. The REE patterns in the natural water samples were in good agreement with those obtained using previous methods. Therefore, it was deduced that onsite solid-phase extraction using chelate resin is a rapid and simple preparation technique for REE analyses.

Journal Articles

Magnetic Bragg dip and Bragg edge in neutron transmission spectra of typical spin superstructures

Mamiya, Hiroaki*; Oba, Yojiro; Terada, Noriki*; Watanabe, Norimichi*; Hiroi, Kosuke; Shinohara, Takenao; Oikawa, Kenichi

Scientific Reports (Internet), 7(1), p.15516_1 - 15516_8, 2017/11

 Times Cited Count:3 Percentile:17.1(Multidisciplinary Sciences)

no abstracts in English

Journal Articles

The Applicability of SiC-SiC fuel cladding to conventional PWR power plant

Furumoto, Kenichiro*; Watanabe, Seiichi*; Yamamoto, Teruhisa*; Teshima, Hideyuki*; Yamashita, Shinichiro; Saito, Hiroaki; Shirasu, Noriko

Proceedings of 2017 Water Reactor Fuel Performance Meeting (WRFPM 2017) (USB Flash Drive), 10 Pages, 2017/09

Since 2015, Mitsubishi Nuclear Fuel (MNF) has joined in a Japanese R&D project of ATF founded by the Ministry of Economy, Trade and Industry (METI) as a subcontractor to Japan Atomic Energy Agency (JAEA) which is the prime contractor to METI. In this program, MNF plans to evaluate an influence of Silicon Carbide (SiC) composite cladding upon fuel rod behavior in current pressurized water reactors (PWR). This paper reports the evaluation result of the applicability of fuel rod with SiC composite cladding for a conventional PWR. For the applicability evaluations of SiC composite to conventional PWR, both of analytical evaluations and out-of-pile tests for SiC composite were conducted. Analytical evaluations were performed by Mitsubishi's own fuel rod design code and the fuel rod behavior evaluation code developed by JAEA. These codes were modified to evaluate the behavior of the fuel rod with SiC composite cladding. As out-of-pile tests, thermal diffusivity measurement and autoclave corrosion test for SiC composite samples were performed. Test apparatus were developed for evaluation of performance of SiC composite under the condition simulated design basis accident (DBA).

Journal Articles

Study on the deterioration mechanism of layered rock-salt electrodes using epitaxial thin films; Li(Ni, Co, Mn)O$$_{2}$$ and their Zr-O surface modified electrodes

Abe, Machiko*; Iba, Hideki*; Suzuki, Kota*; Minamishima, Hiroaki*; Hirayama, Masaaki*; Tamura, Kazuhisa; Mizuki, Junichiro*; Saito, Tomohiro*; Ikuhara, Yuichi*; Kanno, Ryoji*

Journal of Power Sources, 345, p.108 - 119, 2017/03

 Times Cited Count:11 Percentile:38.74(Chemistry, Physical)

The surface structure of the Li(Ni, Co, Mn)O$$_{2}$$ electrode was studied during charge/discharge process using electrochemical methods and X-ray/Neutron scattering techniques. It was found that during charge/discharge process the coverage of spinel structure increased. The spinel structure has low electrochemical activity and is not involved in Li insertion/extraction. After the surface modification, it was found that the coverage of the spinel structure did not increase. Further, it was also found out that the Li concentration at the electrode/electrolyte interface increased.

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