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IrSi大貫 惇睦*; 金子 良夫*; 青木 大*; 仲村 愛*; 松田 達磨*; 中島 美帆*; 芳賀 芳範; 竹内 徹也*
Journal of the Physical Society of Japan, 91(6), p.065002_1 - 065002_2, 2022/06
被引用回数：0 パーセンタイル：0(Physics, Multidisciplinary)Single crystals of MnIrSi were grown using Bridgman method. MnIrSi shows a remarkable increase of the electrical resistivity below antiferromagnetic transition temperature accompanied by a large jump of specific heat.
P, NiP, and PdSi大貫 惇睦*; 仲村 愛*; 青木 大*; 松田 達磨*; 芳賀 芳範; 播磨 尚朝*; 竹内 徹也*; 金子 良夫*
Journal of the Physical Society of Japan, 91(6), p.064712_1 - 064712_10, 2022/06
被引用回数：0 パーセンタイル：0(Physics, Multidisciplinary)Fermi surface of noncentrocymmetric FeP, NiP and PdSi was studied by means of de Haas-van Alphen experiments. The splitting energy of Fermi surfaces due to antisymmetric spin-orbit coupling is estimated.
Al
小泉 尭嗣*; 本多 史憲*; 佐藤 芳樹*; Li, D.*; 青木 大*; 芳賀 芳範; 郷地 順*; 長崎 尚子*; 上床 美也*; 金子 良夫*; et al.
Journal of the Physical Society of Japan, 91(4), p.043704_1 - 043704_5, 2022/04
被引用回数：0 パーセンタイル：0(Physics, Multidisciplinary)A new ternary europium compound EuPtAl is reported. It orders antiferromagnetically at 12.4 K. Application of hydrostatic pressure varies the transition temperature and the compound becomes non-magnetic above the critical pressure 9 GPa. The pressure-temperature phase diagram is indicative of a possible valence crossover at the critical pressure.
徳永 陽; 酒井 宏典; 神戸 振作; 芳賀 芳範; 常盤 欣文; Opletal, P.; 藤林 裕己*; 金城 克樹*; 北川 俊作*; 石田 憲二*; et al.
Journal of the Physical Society of Japan, 91(2), p.023707_1 - 023707_5, 2022/02
被引用回数：6 パーセンタイル：95.24(Physics, Multidisciplinary)ウラン系の強磁性超伝導体で議論されてきた、「強磁性ゆらぎによるスピン三重項超伝導対の形成」および「強磁性ゆらぎを介した磁場による対形成引力の制御」というコンセプトがUTeにおいても成り立つことを期待させる。しかしその一方、では静的な強磁性秩序は存在せず、低温の磁気状態がこれまでのウラン系強磁性超伝導体にどこまで近いのかという点については疑問を持たれていた。実際、最近の中性子散乱実験では、比較的高温側から反強磁性に近いq=0.57という波数を持った磁気ゆらぎの発達が示されている。本研究では
Te-NMR実験により低温で非常に遅いゆっくりとした揺らぎが発達する様子を捉えることに成功した。このことはこの系の低温における強い相関の発達を示唆している。
Raymond, S.*; Knafo, W.*; Knebel, G.*; 金子 耕士; Brison, J.-P.*; Flouquet, J.*; 青木 大*; Lapertot, G.*
Journal of the Physical Society of Japan, 90(11), p.113706_1 - 113706_5, 2021/11
被引用回数：6 パーセンタイル：77.38(Physics, Multidisciplinary)We investigate the spin dynamics in the superconducting phase of UTe by triple-axis inelastic neutron scattering on a single crystal sample. At the wave-vector 
= (0, 0.57, 0), where the normal state antiferromagnetic correlations are peaked, a modification of the excitation spectrum is evidenced, on crossing the superconducting transition, with a reduction of the relaxation rate together with the development of an inelastic peak at 
1 meV. The low dimensional nature and the a-axis polarization of the fluctuations, that characterise the normal state, are essentially maintained below Tsc. The high ratio of 
7.2 contrasts with the most common behaviour in heavy fermion superconductors.
Knafo, W.*; Knebel, G.*; Steffens, P.*; 金子 耕士; Rosuel, A.*; Brison, J.-P.*; Flouquet, J.*; 青木 大*; Lapertot, G.*; Raymond, S.*
Physical Review B, 104(10), p.L100409_1 - L100409_6, 2021/09
被引用回数：22 パーセンタイル：96.77(Materials Science, Multidisciplinary)Inelastic-neutron-scattering measurements were performed on a single crystal of the heavy-fermion paramagnet UTe above its superconducting temperature. We confirm the presence of antiferromagnetic fluctuations with the incommensurate wave-vector 
= (0, 0.57, 0). A quasielastic signal is found, whose momentum-transfer dependence is compatible with fluctuations of magnetic moments 
, with a sine-wave modulation of wave-vector and in-phase moments on the nearest U atoms. Low dimensionality of the magnetic fluctuations, consequence of the ladder structure, is indicated by weak correlations along the direction 
. These results constitute constraints for models of magnetically-mediated superconductivity in UTe.
丸山 龍治; 山崎 大; 青木 裕之; 阿久津 和宏*; 花島 隆泰*; 宮田 登*; 曽山 和彦; Bigault, T.*; Saerbeck, T.*; Courtois, P.*
Journal of Applied Physics, 130(8), p.083904_1 - 083904_10, 2021/08
被引用回数：2 パーセンタイル：42.69(Physics, Applied)Ferromagnetic (FM) interlayer exchange coupling of ion-beam sputtered Fe/Ge multilayers was investigated by off-specular polarized neutron scattering measurements. We observed a monotonously growing correlation of magnetic moments in the out-of-plane direction with decreasing Ge thickness. The results of the Fe/Ge multilayers were used to invoke FM interlayer exchange coupling in a neutron polarizing supermirror in order to extend its bandwidth. Typically, the bandwidth is limited due to a Curie temperature close to room temperature of the thinnest Fe layers with less than 3 nm. We propose a modified layer sequence of the neutron polarizing supermirror, where the minimum Fe thickness was set to 3.5 nm whereas the Ge thickness was reduced. A performance test of the neutron polarizing supermirror showed that the FM interlayer exchange coupling contributed to the presence of the magnetization comparable to the bulk and resulted in a marked extension in the bandwidth.
野間 雄一郎*; 小手川 恒*; 久保 徹郎*; 藤 秀樹*; 播磨 尚朝*; 芳賀 芳範; 山本 悦嗣; 大貫 惇睦*; 伊藤 公平*; 仲村 愛*; et al.
Journal of the Physical Society of Japan, 90(7), p.073707_1 - 073707_5, 2021/07
被引用回数：0 パーセンタイル：0(Physics, Multidisciplinary)Ferromagnetic fluctuation relevant to the pressure-induced superconductivity in UGe is investigated by means of NMR spectroscopy. Longitudinal magnetic fluctuations were observed in the spin-echo decay rate near the ferromagnetic critical point where superconductivity takes place. This result strongly suggests that superconductivity in ferromagnets is universally mediated by anisotropic magnetic fluctuations.
SR and NMR studies比嘉 野乃花*; 伊藤 孝; 與儀 護*; 服部 泰佑; 酒井 宏典; 神戸 振作; Guguchia, Z.*; 髭本 亘; 中島 美帆*; 本間 佳哉*; et al.
Physical Review B, 104(4), p.045145_1 - 045145_7, 2021/07
被引用回数：0 パーセンタイル：0(Materials Science, Multidisciplinary)We report the results of SR and 
Si NMR measurements carried out on the cubic chiral magnet EuPtSi. Our zero-field SR experiments revealed the development of critical slowing down of Eu spin fluctuations over a relatively wide critical region above 
. We also found from Si NMR that the spin fluctuations are strongly suppressed by magnetic field in the paramagnetic state above 20K. These characteristic spin dynamics observed over a wide region of temperature and magnetic field suggest the presence of magnetic frustration in the spin system. Such frustration would underlie the mechanism stabilizing the short-period skyrmion lattice observed in this compound.
Te NMR on UTe仲嶺 元輝*; 金城 克樹*; 北川 俊作*; 石田 憲二*; 徳永 陽; 酒井 宏典; 神戸 振作; 仲村 愛*; 清水 悠晴*; 本間 佳哉*; et al.
Journal of the Physical Society of Japan, 90(6), p.064709_1 - 064709_7, 2021/06
被引用回数：8 パーセンタイル：87.04(Physics, Multidisciplinary)UTe is a recently discovered promising candidate for a spin-triplet superconductor. In contrast to conventional spin-singlet superconductivity, spin-triplet superconductivity possesses spin and angular momentum degrees of freedom. We previously reported that the shoulder signal appears in NMR spectra below the superconducting (SC) transition temperature 
in 
, and a slight decrease in the Knight shift along the 
and 
axes (
and 
, respectively) below at a low magnetic field 
. Although the decrease in vanished above 5.5 T, the decrease in was independent of up to 6.5 T. To clarify the origin of the shoulder signal and the trace of the decrease in , we compared the Te-NMR spectra obtained when and 
and measured the Te-NMR spectra for up to 14.5 T.
丸山 龍治; 山崎 大; 阿久津 和宏*; 花島 隆泰*; 宮田 登*; 青木 裕之; 曽山 和彦
JPS Conference Proceedings (Internet), 33, p.011092_1 - 011092_6, 2021/03
中性子偏極スーパーミラーは、熱及び冷中性子ビームを偏極するための光学素子であり、実機への応用には高偏極率であるとともに必要な外部磁場を小さく抑えること、即ち偏極スーパーミラーを構成する磁気多層膜が磁気的にソフトであることが重要である。本発表では、J-PARC MLFの共用ビームラインBL17等を用いて得られた偏極スーパーミラーの高偏極率化、及び磁気多層膜の軟磁性化を目指しこれを構成する多層膜特有の磁気特性の解明に関する成果について議論する。
probed with Te-NMR measurement仲嶺 元輝*; 金城 克樹*; 北川 俊作*; 石田 憲二*; 徳永 陽; 酒井 宏典; 神戸 振作; 仲村 愛*; 清水 悠晴*; 本間 佳哉*; et al.
Physical Review B, 103(10), p.L100503_1 - L100503_5, 2021/03
被引用回数：15 パーセンタイル：94.76(Materials Science, Multidisciplinary)To investigate spin susceptibility in a superconducting (SC) state, we measured the Te-NMR Knight shifts at magnetic fields () up to 6.5 T along the and axes of single-crystal UTe, a promising candidate for a spin-triplet superconductor. In the SC state, the Knight shifts along the and axes ( and , respectively) decreased slightly, and the decrease in was almost constant up to 6.5 T. The reduction in decreased with increasing , and was unchanged through the SC transition temperature at 5.5 T, excluding the possibility of spin-singlet pairing. Our results indicate that spin susceptibilities along the and axes slightly decrease in the SC state in low , and the response of SC spin susceptibility is anisotropic on the 
plane.
B佐藤 芳樹*; 本多 史憲*; Maurya, A.*; 清水 悠晴*; 仲村 愛*; 本間 佳哉*; Li, D.*; 芳賀 芳範; 青木 大*
Physical Review Materials (Internet), 5(3), p.034411_1 - 034411_9, 2021/03
被引用回数：1 パーセンタイル：0(Materials Science, Multidisciplinary)Single-crystal growth and magnetic properties of NdPtB are reported on a enantiopure crystal. We observed multiple phase transitions at 9.5 and 11 K under zero magnetic field. Nontrivial magnetic phase diagram demonstrates the competitive interactions in this system.
武田 哲明*; 稲垣 嘉之; 相原 純; 青木 健; 藤原 佑輔; 深谷 裕司; 後藤 実; Ho, H. Q.; 飯垣 和彦; 今井 良行; et al.
High Temperature Gas-Cooled Reactors; JSME Series in Thermal and Nuclear Power Generation, Vol.5, 464 Pages, 2021/02
本書は、原子力機構における今までの高温ガス炉の研究開発の総括として、HTTRの設計、燃料、炉内構造物や中間熱交換器などの要素技術の開発、出力上昇試験、950
Cの高温運転、安全性実証試験などの運転経験及び成果についてまとめたものである。また、HTTRでの知見をもとに、商用炉の設計、高性能燃料、ヘリウムガスタービン、ISプロセスによる水素製造などの要素技術開発の現状について記述しており、今後の高温ガス炉の開発に非常に有用である。本書は、日本機械学会の動力エネルギーシステム部門による化石燃料及び原子力によるエネルギーシステムの技術書のシリーズの一冊として刊行されるものである。
藤森 伸一; 川崎 郁斗; 竹田 幸治; 山上 浩志; 仲村 愛*; 本間 佳哉*; 青木 大*
Journal of the Physical Society of Japan, 90(1), p.015002_1 - 015002_2, 2021/01
被引用回数：8 パーセンタイル：87.04(Physics, Multidisciplinary)The valence state of 
was studied by core-level photoelectron spectroscopy. The main peak position of the 
core-level spectrum of coincides with that of 
, which is anitinerant compound with a nearly 
configuration. However, the main peak of is broader than that of, and satellite structures are observed in the higher binding energy side of the main peak, which are characteristics of mixed-valence uranium compounds. These results suggest that the 
state in isin a mixed valence state with a dominant contribution from the itinerant configuration.
阿久津 和宏*; 吉良 弘*; 宮田 登*; 花島 隆泰*; 宮崎 司*; 笠井 聡*; 山崎 大; 曽山 和彦; 青木 裕之
Polymers (Internet), 12(10), p.2180_1 - 2180_10, 2020/10
被引用回数：2 パーセンタイル：13.7(Polymer Science)A large background scattering originating from the sample matrix is a major obstacle for fine-structure analysis of a nanometric layer buried in a bulk material. As polarization analysis can decrease undesired scattering in a neutron reflectivity (NR) profile, we performed NR experiments with polarization analysis on a polypropylene (PP)/perhydropolysilazane-derived SiO (PDS)/Si substrate sample, having a deep-buried layer of SiO to elucidate the fine structure of the nano-PDS layer. This method offers unique possibilities for increasing the amplitude of the Kiessig fringes in the higher scattering vector (Qz) region of the NR profiles in the sample by decreasing the undesired background scattering. Fitting and Fourier transform analysis results of the NR data indicated that the synthesized PDS layer remained between the PP plate and Si substrate with a thickness of approximately 109 
;. Furthermore, the scattering length density of the PDS layer, obtained from the background subtracted data appeared to be more accurate than that obtained from the raw data. Although the density of the PDS layer was lower than that of natural SiO, the PDS thin layer had adequate mechanical strength to maintain a uniform PDS layer in the depth-direction under the deep-buried condition.
宮崎 司*; 宮田 登*; 吉田 鉄生*; 有馬 寛*; 津村 佳弘*; 鳥飼 直也*; 青木 裕之; 山本 勝宏*; 金谷 利治*; 川口 大輔*; et al.
Langmuir, 36(13), p.3415 - 3424, 2020/04
被引用回数：11 パーセンタイル：69.79(Chemistry, Multidisciplinary)We investigated in detail the structures in the poly(vinyl alcohol) (PVA) adsorption layers on a Si substrate, which remained on the substrate after immersing the relatively thick 30 - 50 nm films in hot water, by neutron reflectometry under humid conditions. For the PVA with a degree of saponification exceeding 98 mol %, the adsorption layer exhibits a three-layered structure in the thickness direction. The bottom layer is considered to be the so-called inner adsorption layer that is not fully swollen with water vapor. This may be because the polymer chains in the inner adsorption layer are strongly constrained onto the substrate, which inhibits water vapor penetration. The polymer chains in this layer have many contact points to the substrate via the hydrogen bonding between the hydroxyl groups in the polymer chain and the silanol groups on the surface of the Si substrate and consequently exhibit extremely slow dynamics. Therefore, it is inferred that the bottom layer is fully amorphous. Furthermore, we consider the middle layer to be somewhat amorphous because parts of the molecular chains are pinned below the interface between the middle and bottom layers. The molecular chains in the top layer become more mobile and ordered, owing to the large distance from the strongly constrained bottom layer; therefore, they exhibit a much lower degree of swelling compared to the middle amorphous layer. Meanwhile, for the PVA with a much lower degree of saponification, the adsorption layer structure consists of the two-layers. The bottom layer forms the inner adsorption layer that moderately swells with water vapor because the polymer chains have few contact points to the substrate. The molecular chains in the middle layer, therefore, are somewhat crystallizable because of this weak constraint.
and EuAu with the characteristic hexagonal structure松田 進弥*; 太田 譲二*; 仲井間 憲李*; 伊覇 航*; 郷地 順*; 上床 美也*; 中島 美帆*; 天児 寧*; 本多 史憲*; 青木 大*; et al.
Philosophical Magazine, 100(10), p.1244 - 1257, 2020/04
被引用回数：3 パーセンタイル：31.67(Materials Science, Multidisciplinary)Single crystal samples of EuCu and EuAu have been successfully prepared. Using those samples, magnetic and electronic anisotropy has been clarified. Magnetic moment in the ferromagnetic state points to the hexagonal -axis for both compounds. Electronic anisotropy was found in both electrical resistivity and Fermi surface topology. These anisotropic characteristics are accounted for by the unique hexagonal structure.
-electron state of the heavy fermion superconductor NpPdAl and the isostructural family目時 直人; Aczel, A. A.*; 青木 大*; Chi, S.*; Fernandez-Baca, J. A.*; Griveau, J.-C.*; 萩原 雅人*; Hong, T.*; 芳賀 芳範; 池内 和彦*; et al.
JPS Conference Proceedings (Internet), 30, p.011123_1 - 011123_6, 2020/03
希土類(4)やアクチノイド(5)は、電子数の増加とともに複雑さを増し、様々な相互作用が競合して多様な状態が出現する。多体電子系の結晶場分裂はバンド幅より狭いため、(1)高分解能の実験が必要で、(2)遍歴的なCeやU化合物は本質的に明瞭なスペクトルを示さない。また、(3)国際規制物質NpやPuなど超アクチノイド元素の取り扱いは厳しく規制されている。そこで比較的局在性の強い物質や希土類関連物質の、中性子散乱実験による磁気励起の研究が有益である。本稿では重い電子系化合物NpPdAlと関連物質の電子状態について述べる。
大貫 惇睦*; 垣花 将司*; 伊覇 航*; 仲井間 憲李*; 青木 大*; 仲村 愛*; 本多 史憲*; 中島 美帆*; 天児 寧*; 郷地 順*; et al.
JPS Conference Proceedings (Internet), 29, p.012001_1 - 012001_9, 2020/02
EuPtSi with the cubic chiral structure exhibits a skyrmion phase under magnetic field. We succeeded in growing high-quality single crystals by the Bridgman method. Fermi surface splitting reflecting the noncentrosymmetric structure was successfully observed experimentally.
