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Tomiyasu, Keisuke*; Ito, Naoko*; Okazaki, Ryuji*; Takahashi, Yuki*; Onodera, Mitsugi*; Iwasa, Kazuaki*; Nojima, Tsutomu*; Aoyama, Takuya*; Ogushi, Kenya*; Ishikawa, Yoshihisa*; et al.
Advanced Quantum Technologies (Internet), 1(3), p.1800057_1 - 1800057_7, 2018/12
Spin-state transition, also known as spin crossover, plays a key role in diverse systems. In theory, the boundary range between the low- and high-spin states is expected to enrich the transition and give rise to unusual physical states. However, no compound that realizes a nearly degenerate critical range as the ground state without requiring special external conditions has yet been experimentally identified. This study reports that the Sc substitution in LaCoO3 destabilizes its nonmagnetic low-spin state and generates an anomalous paramagnetic state accompanied by the enhancement of transport gap and magneto-lattice-expansion as well as the contraction of Co-O distance with the increase of electron site transfer. These phenomena are not well described by the mixture of conventional low- and high-spin states, but by their quantum superposition occurring on the verge of a spin-state transition.
Sato, Takahiro*; Iwasaki, Atsushi*; Owada, Shigeki*; Yamanouchi, Kaoru*; Takahashi, Eiji*; Midorikawa, Katsumi*; Aoyama, Makoto; Yamakawa, Koichi; Togashi, Tadashi*; Fukami, Kenji*; et al.
Journal of Physics B; Atomic, Molecular and Optical Physics, 46(16), p.164006_1 - 164006_6, 2013/08
Times Cited Count:3 Percentile:18.32(Optics)By introducing 13th- (61.7 nm) and 15th-order harmonics (53.4 nm) of femtosecond laser pulses at 800 nm into an undulator of SCSS (SPring-8 Compact SASE Source) test accelerator at RIKEN, these harmonic pulses were amplified by a factor of more than 10 with a high contrast ratio through the interaction between accelerated electron bunches and the harmonic pulses. From numerical simulations of the amplification processes of high-order harmonic pulses in the undulator, optimum conditions of the electron bunch duration interacting with the high-order harmonic pulses were investigated for generating full-coherent and intense pulses in the extreme ultraviolet wavelength region.
Ogawa, Kanade*; Sato, Takahiro*; Matsubara, Shinichi*; Okayasu, Yuichi*; Togashi, Tadashi*; Watanabe, Takahiro*; Takahashi, Eiji*; Midorikawa, Katsumi*; Aoyama, Makoto; Yamakawa, Koichi; et al.
Proceedings of 10th Conference on Lasers and Electro-Optics Pacific Rim and 18th OptoElectronics and Communications Conference and Photonics in Switching 2013 (CLEO-PR & OECC/PS 2013) (USB Flash Drive), 2 Pages, 2013/06
no abstracts in English
Togashi, Tadashi*; Takahashi, Eiji*; Midorikawa, Katsumi*; Aoyama, Makoto; Yamakawa, Koichi; Sato, Takahiro*; Iwasaki, Atsushi*; Owada, Shigeki*; Yamanouchi, Kaoru*; Hara, Toru*; et al.
Proceedings of Ultrafast Optics IX (CD-ROM), 2 Pages, 2013/03
We have demonstrated free-electron laser radiation seeded by high-order harmonics in the extreme-ultraviolet region. Strong enhancement of the radiation intensity by a factor of 104 was observed with timing control of an electro-optical sampling technique.
Togashi, Tadashi*; Takahashi, Eiji*; Midorikawa, Katsumi*; Aoyama, Makoto; Yamakawa, Koichi; Sato, Takahiro*; Iwasaki, Atsushi*; Owada, Shigeki*; Yamanouchi, Kaoru*; Hara, Toru*; et al.
Proceedings of 11th International School and Symposium on Synchrotron Radiation in Natural Science (ISSRNS 2012), p.1 - 21, 2012/05
The 13th harmonic of a Ti:sapphire laser has been significantly amplified with the SCSS test accelerator. The temporal and spatial overlap of the electron beam and the high harmonic radiation were precisely tuned for achieving the seeded free electron laser operation. With numerical simulation the present HH-seeded FEL scheme could readily be applied to the wavelength region down to 10 nm.
Takahashi, Eiji*; Togashi, Tadashi*; Midorikawa, Katsumi*; Aoyama, Makoto; Yamakawa, Koichi; Sato, Takahiro*; Iwasaki, Atsushi*; Owada, Shigeki*; Yamanouchi, Kaoru*; Hara, Toru*; et al.
Proceedings of European Conference on Lasers and Electro-Optics and the 12th European Quantum Electronics Conference (CLEO/Europe-EQEC 2011) (CD-ROM), 1 Pages, 2011/05
We succeeded in generating the seeded free electron laser (FEL) with wavelengths of 61 nm at the SCSS test accelerator. The 13th (61 nm) harmonics generated by focusing the high peak power Ti:Sapphire laser to the Xe gas cell was directed to the undulator. This is first realization of the seeded FEL in extreme ultraviolet region.
Takahashi, Eiji*; Togashi, Tadashi*; Aoyama, Makoto; Yamakawa, Koichi; Sato, Takahiro*; Iwasaki, Atsushi*; Owada, Shigeki*; Yamanouchi, Kaoru*; Hara, Toru*; Matsubara, Shinichi*; et al.
Proceedings of International Quantum Electronics Conference and the Pacific Rim Conference on Lasers and Electro-Optics (IQEC/CLEO Pacific Rim 2011) (CD-ROM), p.199 - 200, 2011/05
We succeeded in generating the seeded free electron laser (FEL) with wavelengths of 61 nm at the SCSS test accelerator. The 13th (61 nm) harmonics generated by focusing the high peak power Ti:Sapphire laser to the Xe gas cell was directed to the undulator. This is first realization of the seeded FEL in extreme ultraviolet region.
Togashi, Tadashi*; Takahashi, Eiji*; Midorikawa, Katsumi*; Aoyama, Makoto; Yamakawa, Koichi; Sato, Takahiro*; Iwasaki, Atsushi*; Owada, Shigeki*; Okino, Tomoya*; Yamanouchi, Kaoru*; et al.
Optics Express (Internet), 19(1), p.317 - 324, 2011/01
Times Cited Count:97 Percentile:96.13(Optics)The 13th harmonic of a Ti:sapphire (Ti:S) laser in the plateau region was injected as a seeding source to a 250-MeV free-electron-laser (FEL) amplifier. When the amplification conditions were fulfilled, strong enhancement of the radiation intensity by a factor of 650 was observed. The random and uncontrollable spikes, which appeared in the spectra of the Self-Amplified Spontaneous Emission (SASE) based FEL radiation without the seeding source, were found to be suppressed drastically to form to a narrow-band, single peak profile at 61.2 nm. The properties of the seeded FEL radiation were well reproduced by numerical simulations. We discuss the future precept of the seeded FEL scheme to the shorter wavelength region.
Sherrill, M. E.*; Abdallah, J.*; Csanak, G.*; Dodd, E. S.*; Fukuda, Yuji; Akahane, Yutaka; Aoyama, Makoto; Inoue, Norihiro*; Ueda, Hideki*; Yamakawa, Koichi; et al.
High-Power Laser Ablation VII (Proceedings of SPIE Vol.7005), p.70051R_1 - 70051R_11, 2008/06
Fukuda, Yuji; Akahane, Yutaka; Aoyama, Makoto; Hayashi, Yukio; Homma, Takayuki; Inoue, Norihiro*; Kando, Masaki; Kanazawa, Shuhei; Kiriyama, Hiromitsu; Kondo, Shuji; et al.
Physics Letters A, 363(2-3), p.130 - 135, 2007/02
Collimated relativistic electrons up to 58 MeV with an electron charge of 2.1 nC were generated by the interaction of intense laser pulses with the Ar cluster target at the laser intensity of 3.510
W/cm
. The resulting spectrum does not fit a Maxwellian distribution, but is well described by a two-temperature Maxwellian, which indicates two mechanisms of the electron acceleration. Two dimensional particle-in-cell simulations demonstrate an important role of clusters. The higher energy electrons are injected when they are expelled from the clusters by the laser pulse field. They then gain their energy during the direct acceleration by the laser pulse, whose phase velocity in the underdense plasma is larger than speed of light in vacuum. The lower energy electrons, which are injected during the plasma wave breaking, are accelerated by the wakefield.
Sherrill, M. E.*; Abdallah, J. Jr.*; Csanak, G.*; Dodd, E. S.*; Fukuda, Yuji; Akahane, Yutaka; Aoyama, Makoto; Inoue, Norihiro*; Ueda, Hideki*; Yamakawa, Koichi; et al.
Physical Review E, 73(6), p.066404_1 - 066404_6, 2006/06
Times Cited Count:29 Percentile:74.68(Physics, Fluids & Plasmas)A model that solves simultaneously both the electron and atomic kinetics was used to generate synthetic He X-ray spectra to characterize a high intensity ultrashort laser driven Ar cluster target experiment. In particular, level populations were obtained from a detailed collisional-radiative model where collisional rates were computed from a time varying electron distribution function obtained from the solution of the zero dimensional Boltzmann equation. In addition, aparticle-in-cell simulation was used to model the laser interaction with the cluster target and provided the initial electron energy distribution function (EEDF) for the Boltzmann solver. This study suggests that the high density plasma contribution to the time-integrated He
spectrum was in a highly non-equilibrium state in both the EEDF and the ion level populations and provides a prediction of 5.7 ps for the average cluster integrity time for this high density state.
Sherrill, M. E.*; Abdallah, J. Jr.*; Csanak, G.*; Kilcrease, D. P.*; Dodd, E. S.*; Fukuda, Yuji; Akahane, Yutaka; Aoyama, Makoto; Inoue, Norihiro*; Ueda, Hideki; et al.
Journal of Quantitative Spectroscopy & Radiative Transfer, 99(1-3), p.584 - 594, 2006/05
Times Cited Count:3 Percentile:18.03(Optics)In this work, we present a model that solves self-consistently the electron and atomic kinetics to characterize highly non-equilibrium plasmas, in particular for those systems where both the electron distribution function is far from Maxwellian and the evolution of the ion level populations are dominated by time dependent atomic kinetics. In this model, level populations are obtained from a detailed collisional-radiative model where collision rates are computed from a time varying electron distribution function obtained from the solution of the zero-dimensional Boltzmann equation. The Boltzmann collision term includes the effects of electron-electron collisions, electron collisional ionization, excitation and de-excitation. An application for He spectra from a short pulse laser irradiated argon cluster target will be shown to illustrate the results of our model.
Akahane, Yutaka; Ma, J.-L.; Fukuda, Yuji; Aoyama, Makoto; Kiriyama, Hiromitsu; Sheldakova, J. V.*; Kudryashov, A. V.*; Yamakawa, Koichi
Review of Scientific Instruments, 77(2), p.023102_1 - 023102_7, 2006/02
Times Cited Count:47 Percentile:85.72(Instruments & Instrumentation)An improvement of laser-focused peak intensity has been achieved in a JAERI 100-TW Ti:sapphire chirped-pulse amplifier chain with a feedback controlled adaptive optics system operating at a 10 Hz repetition rate. The Strehl ratio was enhanced to 0.8 by means of a Bimorph deformable mirror with a Shack-Hartmann wavefront sensor. Measurements of optical parameters of the laser pulse and an experimental tunneling ionization yield of helium have practically confirmed focusing to ultra-relativistic intensities of over 10 W/cm
within 16 % accuracy.
Akahane, Yutaka; Ma, J.; Fukuda, Yuji; Aoyama, Makoto; Kiriyama, Hiromitsu; Inoue, Norihiro*; Tsuji, Koichi*; Nakai, Yoshiki*; Yamamoto, Yoichi*; Sheldakova, J. V.*; et al.
Japanese Journal of Applied Physics, Part 1, 44(8), p.6087 - 6089, 2005/08
Times Cited Count:1 Percentile:4.61(Physics, Applied)An improvement of laser-focused peak intensity has been achieved in a JAERI 100 TW Ti:sapphire chirped-pulse amplifier chain with a feedback-controlled adaptive optics system. Measurements of optical parameters of the laser pulse and an experimental tunneling ionization ratio of a rare gas atom with laser energy scaling have practically confirmed an ultrarelativistic intensity of over 10 W/cm
operating at a 10 Hz repetition rate.
Okutsu, Kazuo*; Morikawa, Seiji*; Shimbo, Hiroshi*; Kuroyanagi, Mikio*; Sahara, Fumihiro*; Murakami, Takeshi*; Aoyama, Yuji*
JNC TJ8400 2005-013, 117 Pages, 2005/02
To integrate the system for evaluation of long-term hydraulic condition in near field of TRU waste disposal, the engineered barrier, which consists of bentonite buffer and cementitious materials, was employed in the series of laboratory tests. On the bentonite buffer, with the aim of investigating of the effect of (i) interlayer cation in bentonite, (ii) content of siliceous sand and (iii) the ionic strength of ground water on its mechanical and hydraulic properties, series of laboratory tests were conducted. The same lot of bentonite was used in the series of tests to obtain consistent data. In addition, the swelling test of the laminated bentonite with caliumization front was conducted for verification of the proposed constitutive model. On cementitious materials, the altered specimen that produced immersing was investigated the water permeation and also characteristics. The hardened cement paste specimens with W/C=40 to 105% were immersed into deionized water and alteration behavior under diffusion condition was investigated.
Okutsu, Kazuo*; Morikawa, Seiji*; Shimbo, Hiroshi*; Kuroyanagi, Mikio*; Sahara, Fumihiro*; Murakami, Takeshi*; Aoyama, Yuji*
JNC TJ8400 2005-012, 272 Pages, 2005/02
To integrate the system for evaluation of long-term hydraulic condition in near field of TRU waste disposal, the engineered barrier, which consists of bentonite buffer and cementitious materials, was employed in the series of laboratory tests.On the bentonite buffer, with the aim of investigating of the effect of (i)interlayer cation in bentonite, (ii)content of siliceous sand and (iii)the ionic strength of ground water on its mechanical and hydraulic properties, series of laboratory tests were conducted. The same lot of bentonite was used in the series of tests to obtain consistent data. In addition, the swelling test of the laminated bentonite with caliumization front was conducted for verification of the proposed constitutive model.On cementitious materials, the altered specimen that produced immersing was investigated the water permeation and also characteristics. The hardened cement paste specimens with W/C=40 to 105% were immersed into deionized water and alteration behavior under diffusion condition was investigated.
Hansen, S. B.*; Fournier, K. B.*; Faenov, A. Y.*; Magunov, A. I.*; Pikuz, T. A.*; Skobelev, I. Y.*; Fukuda, Yuji; Akahane, Yutaka; Aoyama, Makoto; Inoue, Norihiro*; et al.
Physical Review E, 71(1), p.016408_1 - 016408_9, 2005/01
Times Cited Count:16 Percentile:56.87(Physics, Fluids & Plasmas)X-ray line emission from ' transitions in Ne-like Kr and nearby ions has been observed from
1
m Kr clusters irradiated by fs-scale laser pulses at the JAERI facility in Kyoto, Japan. The dependence of X-ray spectral features and intensity on the incident laser intensity is rather weak, indicating that the 1-2 ps cluster lifetimes limit the number of ions beyond Ne-like Kr that can be produced by collisional ionization. A collisional-radiative model based on the relativistic multiconfigured FAC code has been constructed and used to determine that the cluster plasma has electron densities near 10
cm
, temperature of a few hundred eV and hot electron fraction of a few percent.
Fukuda, Yuji; Akahane, Yutaka; Aoyama, Makoto; Inoue, Norihiro*; Ueda, Hideki; Nakai, Yoshiki*; Tsuji, Koichi*; Yamakawa, Koichi; Hironaka, Yoichiro*; Kishimura, Hiroaki*; et al.
Applied Physics Letters, 85(21), p.5099 - 5101, 2004/11
Times Cited Count:11 Percentile:42.19(Physics, Applied)We have demonstrated diffraction from Si(111) crystal using X-rays from highly ionized Ar ions produced by laser irradiation with an intensity of 610
W/cm
and a pulse duration of 30 fs acting upon micron-sized Ar clusters. The measured total photon flux and line width in the He
line (3.14 keV) were 4
10
photons/shot/4
sr and 3.7 eV (FWHM), respectively, which is sufficient to utilize as a debris-free light source for time-resolved X-ray diffraction studies.
Fukuda, Yuji; Akahane, Yutaka; Aoyama, Makoto; Inoue, Norihiro*; Ueda, Hideki; Kishimoto, Yasuaki; Yamakawa, Koichi; Faenov, A. Y.*; Magunov, A. I.*; Pikuz, T. A.*; et al.
Laser and Particle Beams, 22(3), p.215 - 220, 2004/07
Times Cited Count:42 Percentile:78.93(Physics, Applied)High resolution K-shell spectra of a plasma created by superintense laser irradiation of micron-sized Ar clusters have been measured with an intensity above 10 W/cm
and a pulse duration of 30 fs. The total photon flux of 2
10
photons/pulse was achieved for He
resonant line of Ar (
=3.9491 AA , 3.14 keV). In parallel with X-ray measurements, energy distributions of emitted ions have been measured. The multiply-charged ions with kinetic energies up to 800 keV were observed. It is found that hot electrons produced by high contrast laser pulses allow the isochoric heating of clusters and shift the ion balance towards the higher charge states, which enhances both the X-ray line yield of the He-like argon ion and the ion kinetic energy.
Smirnov, M. B.*; Skobelev, I. Y.*; Magunov, A. I.*; Faenov, A. Y.*; Pikuz, T. A.*; Fukuda, Yuji; Yamakawa, Koichi; Akahane, Yutaka; Aoyama, Makoto; Inoue, Norihiro*; et al.
Journal of Experimental and Theoretical Physics, 98(6), p.1123 - 1132, 2004/06
Interaction between high-power ultrashort laser pulse and giant clusters (microdroplets) consisting of 10 to 10
atoms is considered. The microdroplet size is comparable to the laser wavelength. A model of the evolution of a microdroplet plasma induced by a high-power laser pulse is developed, and the processes taking place after interaction with the pulse are analyzed. It is shown theoretically that the plasma is superheated: its temperature is approximately equal to the ionization potential of an ion having a typical charge. The microdroplet plasma parameters are independent of the pulse shape and duration. The theoretical conclusions are supported by experimental studies of X-ray spectra conducted at JAERI, where a 100-terawatt Ti-sapphire lasersystem was used to irradiate krypton and xenon microdroplets by laser pulses with pulse widths of 30 to 500 fs and intensities of 6
10
to 2
10
W/cm
.