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論文

Eustatic change modulates exhumation in the Japanese Alps

King, G. E.*; Ahadi, F.*; 末岡 茂; Herman, F.*; Anderson, L.*; Gautheron, C.*; 塚本 すみ子*; Stalder, N.*; Biswas, R.*; Fox, M.*; et al.

Geology, 51(2), p.131 - 135, 2023/02

The exhumation of bedrock is controlled by the interplay between tectonics, surface processes, and climate. The highest exhumation rates of centimeters per year are recorded in zones of highly active tectonic convergence such as the Southern Alps of New Zealand or the Himalayan syntaxes, where high rock uplift rates combine with very active surface processes. Using a combination of different thermochronometric systems including trapped-charge thermochronometry, we show that such rates also occur in the Hida Mountain Range, Japanese Alps. Our results imply that centimeter per year rates of exhumation are more common than previously thought. Our thermochronometry data allow the development of time series of exhumation rate changes at the time scale of glacial-interglacial cycles, which show a fourfold increase in baseline rates to rates of $$sim$$10 mm/yr within the past $$sim$$65 k.y. This increase in exhumation rate is likely explained by knickpoint propagation due to a combination of very high precipitation rates, climatic change, sea-level fall, range-front faulting, and moderate rock uplift. Our data resolve centimeter-scale sub-Quaternary exhumation rate changes, which show that in regions with horizontal convergence, coupling between climate, surface processes, and tectonics can exert a significant and rapid effect on rates of exhumation.

論文

Enhanced covalency and nanostructured-phonon scattering lead to high thermoelectric performance in $$n$$-type PbS

Rathore, E.*; Juneja, R.*; Sarkar, D.*; Roychowdhury, S.*; 古府 麻衣子; 中島 健次; Singh, A. K.*; Biswas, K.*

Materials Today Energy (Internet), 24, p.100953_1 - 100953_9, 2022/03

 被引用回数:12 パーセンタイル:87.17(Chemistry, Physical)

We demonstrate a high thermoelectric figure of merit (zT) of 1.45 at 900 K for Ge doped (4-10 mol%) $$n$$-type PbS, which is the one of the highest values among all $$n$$-type PbS-based thermoelectric materials. This high performance is achieved by simultaneous (a) enhancement of covalency in chemical bonding which increases the electrical conductivity, and (b) reduction of lattice thermal conductivity to an ultra-low value of 0.56 W m$$^{-1}$$K$$^{-1}$$ at 900 K by the introduction of nanometer-sized (5-10 nm) precipitates of Pb$$_{2}$$GeS$$_{4}$$ in PbS matrix which strongly scatter the heat-carrying phonons. The presence of low-lying transverse acoustic (TA) and longitudinal acoustic (LA) phonon modes at 48.24 cm$$^{-1}$$ and 91.83 cm$$^{-1}$$, respectively are experimentally revealed from inelastic neutron scattering (INS) experiments. The softening of low-frequency modes at a higher temperature and ultra-short phonon lifetime (1-4.5 ps) further explain the ultra-low thermal conductivity.

論文

Structure of the $$11/2^-$$ isomeric state in $$^{133}$$La

Laskar, Md. S. R.*; Palit, R.*; Mishra, S. N.*; 清水 則孝*; 宇都野 穣; 井手口 栄治*; Garg, U.*; Biswas, S.*; Babra, F. S.*; Gala, R.*; et al.

Physical Review C, 101(3), p.034315_1 - 034315_8, 2020/03

 被引用回数:4 パーセンタイル:46.04(Physics, Nuclear)

質量数130領域の中重核では、カイラルバンドなどの新規な集団運動が出現するメカニズムとして、$$h_{11/2}$$軌道が重要な役割を果たしていると考えられている。その一粒子状態と集団運動状態との相互作用を調べるため、$$^{133}$$Laの$$11/2^-$$アイソマー状態の$$g$$因子と四重極モーメントをタタ基礎科学研究所にて測定した。得られた$$g$$因子は$$g=1.16pm0.07$$、四重極モーメントの大きさは、$$|Q|=1.71pm 0.34$$ $$b$$だった。測定された四重極モーメントから四重極変形度$$beta=0.28pm 0.10$$を導き出した。これらの実験値を大規模殻模型計算と比較した結果、$$^{133}$$Laの$$11/2^-$$アイソマー状態は、中程度のプロレート変形したコアに$$h_{11/2}$$軌道の陽子が結合した状態であることがわかり、この領域の$$h_{11/2}$$準位を得る大きな手がかりを得た。

論文

Electron Spin Resonance (ESR) thermochronometry of the Hida range of the Japanese Alps; Validation and future potential

King, G. E.*; 塚本 すみ子*; Herman, F.*; Biswas, R. H.*; 末岡 茂; 田上 高広*

Geochronology (Internet), 2(1), p.1 - 15, 2020/01

石英の電子スピン共鳴(ESR)法は、岩石の冷却史の推定に有効な可能性が示唆されていたが検証が不十分だった。本研究では飛騨山脈の試料を用いてESR熱年代法の検証を行った。Al中心とTi中心の熱安定性は従来の予想より低く、長石のルミネッセンスと同程度と推定された。ESRデータから推定された熱史は、同じ試料のルミネッセンスデータから推定された熱史と同様のパターンを示した。一方、ESRの方がより長期間の熱史を復元することができ、石英のESR熱年代法が第四紀後期の地形発達史の解明に広く有用である可能性が示された。

論文

$$g$$-factor measurement of the 2738 keV isomer in $$^{135}$$La

Laskar, Md. S. R.*; Saha, S.*; Palit, R.*; Mishra, S. N.*; 清水 則孝*; 宇都野 穣; 井手口 栄治*; Naik, Z.*; Babra, F. S.*; Biswas, S.*; et al.

Physical Review C, 99(1), p.014308_1 - 014308_6, 2019/01

 被引用回数:6 パーセンタイル:60.34(Physics, Nuclear)

タタ基礎物理学研究所の重イオン加速器にて、$$^{11}$$B($$^{128}$$Te, 4n)$$^{135}$$La反応によって$$^{135}$$Laの励起状態を生成し、2738keVにあるアイソマーの$$g$$因子を時間微分型摂動角分布(TDPAD)法によって測定した。得られた$$g$$因子の値は$$-0.049(3)$$であった。このアイソマーの核構造を理解するため、$$^{135}$$Laに対し、大規模殻模型計算を行った。殻模型計算は低励起状態のバンド構造を非常によく再現し、2738keVのアイソマーのスピンパリティは$$23/2^+$$であることを強く示唆する結果が得られた。このアイソマーは、$$^{134}$$Baの$$10^+_1$$$$d_{5/2}$$軌道にいる陽子が結合してできる配位が主であると解釈された。

論文

EXILL; A High-efficiency, high-resolution setup for $$gamma$$-spectroscopy at an intense cold neutron beam facility

Jentschel, M.*; Blanc, A.*; de France, G.*; K$"o$ster, U.*; Leoni, S.*; Mutti, P.*; Simpson, G.*; Soldner, T.*; Ur, C.*; Urban, W.*; et al.

Journal of Instrumentation (Internet), 12(11), p.P11003_1 - P11003_33, 2017/11

 被引用回数:34 パーセンタイル:84.59(Instruments & Instrumentation)

A highly efficient array of high-purity germanium (HPGe) detectors was developed and operated at the cold neutron beam facility PF1B of the Institut Laue-Langevin (ILL) to carry out nuclear structure studies, via measurements of $$gamma$$-rays following neutron-induced capture and fission reactions. The setup consisted of a collimation system producing a pencil beam with a thermal capture equivalent flux of about 10$$^8$$ns$$^{-1}$$cm$$^{-2}$$ at the target position and negligible neutron halo. The target was surrounded by an array of eight to ten anti-Compton shielded EXOGAM Clover detectors, four to six anti-Compton shielded large coaxial GASP detectors and two standard Clover detectors. For a part of the campaign the array was combined with 16 LaBr$$_{3}$$:(Ce) detectors from the FATIMA collaboration.

口頭

Constraining the Quaternary evolution of the Hida range of the Japanese Alps

King, G.*; 末岡 茂; 塚本 すみ子*; Biswas, R.*; Herman, F.*; Ahadi, F.*; Gautheron, C.*; Delpech, G.*; 田上 高広*

no journal, , 

閉鎖温度が極めて低い熱年代手法(光ルミネッセンス法, 電子スピン共鳴法)を用いて、第四紀における飛騨山脈の削剥史の復元を試みた。いずれの測定結果からも、第四紀における急激な冷却・削剥が推定された。60$$^{circ}$$C/kmの地温勾配を仮定すると、削剥速度は、MIS4では約10mm/yrだったのが、最近2万年間では約1-3mm/yrに減少した可能性がある。

口頭

Using a 3-D heat transport model (PeCUBE) to invert OSL- and ESR-derived rock cooling histories into erosion rate changes in the Hida Range of Japan

Anderson, L.*; Bartz, M.*; King, G.*; Fox, M.*; Herman, F.*; Stalder, N.*; Biswas, R.*; 末岡 茂; 塚本 すみ子*; Ahadi, F.*; et al.

no journal, , 

Optically stimulated luminescence (OSL) and electron spin resonance (ESR) thermochronometry have the potential to resolve continuous erosion histories from rapidly eroding settings. These thermochronometers are viable over the past few hundred thousand to a million years. These time periods are defined by persistent oscillations between warm and cold states. During the Quaternary, fundamental questions about the relationship between climate and erosion remain unanswered. With further development, the OSL and ESR thermochronometers could answer these questions. To realize this potential new strategies are required to invert low-temperature thermal histories for erosion rates. Here, we explore the use of PeCUBE (Braun, 2003), a three-dimensional finite-element model that simulates heat conduction and advection in the upper crust. As a training dataset we use cooling histories derived from eight samples from the Tateyama region in the Hida Mountains of Japan. The flexibility of PeCUBE allows us to quantify the role of time varying surface temperatures between glacial and interglacial periods. In high-relief settings the three-dimensionality of the topography, for example between valleys and ridges, can substantially perturb rock temperatures. PeCUBE allows us to quantify and remove these confounding topographic effects. We additionally explore the role of changing topographic relief on time varying thermal fields and erosion rates. Lastly, we explore a generous range of model parameters to quantify the sensitivity and robustness of our inversions.

口頭

Eustatic change modulates exhumation in the Japanese Alps

King, G. E.*; Ahadi, F.*; 末岡 茂; Herman, F.*; Anderson, L.*; Gautheron, C.*; 塚本 すみ子*; Stalder, N.*; Biswas, R.*; Fox, M.*; et al.

no journal, , 

The exhumation of bedrock is controlled by the interplay between tectonics, surface processes and climate. The highest exhumation rates of cm/yr are recorded in zones of highly active tectonic convergence. Here, we use a combination of different thermochronometric systems, and notably trapped-charge thermochronometery, to show that such rates also occur in the Hida Range, Japanese Alps. Our results imply that cm/yr rates of exhumation may be more common than previously thought. The Hida Range is the most northern and most extensive of the Japanese Alps, and reaches elevations of up to 3000 m a.s.l. The Hida Range is thought to have uplifted in the last 3 Myr in response to E-W compression and magmatism. Our study focuses on samples from the Kurobe gorge, which is one of the steepest gorges in Japan. Previous work has shown that exhumation rates in this region are exceptionally high, as documented by the exposure of the ~0.8 Ma Kurobe granite in the gorge. We combined 12 new zircon (U-Th/He) ages and 11 new OSL-thermochronometry ages together with existing thermochronometric data to investigate the late Pleistocene exhumation of this region. We found that exhumation rates increased to ~10 mm/yr within the past 300 kyr, likely in response to river base-level fall that increased channel steepness due to climatically controlled eustatic changes. Our data allow the development of time-series of exhumation rate changes at the timescale of glacial-interglacial cycles and show a four-fold increase in baseline rates over the past ~65 kyr. This increase in exhumation rate is likely explained by knickpoint propagation due to a combination of very high precipitation rates, climatic change, sea-level fall, range-front faulting and moderate rock uplift. Our data show that in regions with horizontal convergence, coupling between climate, surface processes and tectonics can exert a significant effect on rates of exhumation.

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