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論文

The Influence of structural dynamics in two-dimensional hybrid organic-inorganic perovskites on their photoluminescence efficiency; Neutron scattering analysis

Rajeev, H. S.*; Hu, X.*; Chen, W.-L.*; Zhang, D.*; Chen, T.*; 古府 麻衣子*; 梶本 亮一; 中村 充孝; Chen, A. Z.*; Johnson, G. C.*; et al.

Journal of the Physical Society of Japan, 94(3), p.034602_1 - 034602_14, 2025/03

https://doi.org/10.7566/JPSJ.94.034602
 被引用回数：0 パーセンタイル：0.00(Physics, Multidisciplinary)

Two-dimensional hybrid organic-inorganic perovskites (HOIPs) have emerged as promising materials for light-emitting diode applications. In this study, by using time-of-flight neutron spectroscopy we identified and quantitatively separated the lattice vibrational and molecular rotational dynamics of two perovskites, butylammonium lead iodide (BA)$$_{2}$$PbI$$_{4}$$ and phenethyl-ammonium lead iodide (PEA)$$_{2}$$PbI$$_{4}$$. By examining the corresponding temperature dependence, we found that the lattice vibrations, as evidenced by neutron spectra, are consistent with the lattice dynamics obtained from Raman scattering. We revealed that the rotational dynamics of organic molecules in these materials tend to suppress their photoluminescence quantum yield (PLQY) while the vibrational dynamics did not show predominant correlations with the same. Additionally, we observed photoluminescence emission peak splitting for both systems, which becomes prominent above certain critical temperatures where the suppression of PLQY begins. This study suggests that the rotational motions of polarized molecules may lead to a reduction in exciton binding energy or the breaking of degeneracy in exciton binding energy levels, enhancing non-radiative recombination rates, and consequently reducing photoluminescence yield. These findings offer a deeper understanding of fundamental interactions in 2D HOIPs and could guide the design of more efficient light-emitting materials for advanced technological applications.

論文

Unique magnetic transition process demonstrating the effectiveness of bond percolation theory in a quantum magnet

Zheng, X.-G.*; 山内 一宏*; 萩原 雅人; 西堀 英治*; 河江 達也*; 渡邊 功雄*; 内山 智貴*; Chen, Y.*; Xu, C.-N.*

Nature Communications (Internet), 15, p.9989_1 - 9989_12, 2024/11

https://doi.org/10.1038/s41467-024-54335-6
 被引用回数：0 パーセンタイル：0.00(Multidisciplinary Sciences)

Like the crystallization of water to ice, magnetic transition occurs at a critical temperature after the slowing down of dynamically fluctuating short-range correlated spins. Here, we report a unique type of magnetic transition characterized by a linear increase in the volume fraction of unconventional static short-range-ordered spin clusters, which triggered a transition into a long-range order at a threshold fraction perfectly matching the bond percolation theory in a new quantum antiferromagnet of pseudo-trigonal Cu$$_{4}$$(OH)$$_{6}$$Cl$$_{2}$$. Static short-range order appeared in its Kagome lattice plane below Ca. 20 K from a pool of coexisting spin liquid, linearly increasing its fraction to 0.492(8), then all Kagome spins transitioned into a stable two-dimensional spin order at $$T$$_${rm N}$$$ = 5.5 K. Inspection on the magnetic interactions and quantum magnetism revealed an intrinsic link to the spin liquid material Herbertsmithite, ZnCu$$_${3}$$$(OH)$$_${6}$$$Cl$$_${2}$$. The unconventional static nature of the short-range order was inferred to be due to a pinning effect by the strongly correlated coexisting spin liquids. This work presents a unique magnetic system to demonstrate a complete bond percolation process toward the critical transition. Meanwhile, the unconventionally developed magnetic order in this chemically clean system should shed new light on spin-liquid physics.

論文

Magnetic excitation in the hyperkagome antiferromagnet Mn$$_{3}$$RhSi

社本 真一; 山内 宏樹; 飯田 一樹*; 池内 和彦*; 金子 耕士; Chen, Y.-S.*; 矢野 真一郎*; Hsu, P.-T.*; Lee, M. K.*; Hall, A. E.*; et al.

Physical Review Research (Internet), 6(3), p.033303_1 - 033303_7, 2024/09

https://doi.org/10.1103/PhysRevResearch.6.033303

Mn$$_{3}$$RhSiの磁気励起は少なくとも0.3から140meVに広がる。200Kでの非弾性散乱強度を積分することで、Mnサイト当たり約5$$mu_{B}$$の磁気モーメントは、約5$$mu_{B}$$であることがわかった。一方で、長距離磁気秩序の磁気モーメントは4Kでわずか2.61$$mu_{B}$$であり、多くの部分が低温まで揺らいでいることがわかった。

論文

Gradient residual strain determination of surface impacted railway S38C axles by neutron Bragg-edge transmission imaging

Hu, F. F.*; Qin, T. Y.*; Ao, N.*; Su, Y. H.; Zhou, L.*; 徐 平光; Parker, J. D.*; 篠原 武尚; Chen, J.*; Wu, S. C.*

Engineering Fracture Mechanics, 306, p.110267_1 - 110267_18, 2024/08

https://doi.org/10.1016/j.engfracmech.2024.110267
 被引用回数：2 パーセンタイル：60.53(Mechanics)

Non-destructive and quantitative mapping of gradient residual strain distribution in surface-hardened railway S38C axles could provide a positive reference for determining service lifetime and maintenance strategy. To tackle this concern, time-of-flight neutron Bragg-edge transmission imaging was employed by real axle samples with and without impacted crater. A novel and simple procedure to formulate the residual strain field was also developed in this work, with the transmission batch code in Appendix A. By mapping the global two- dimensional residual strains, it can be verified that the residual strains into the axle are uniformly distributed in the hoop direction. Subsequently, it was revealed that the axial and hoop residual strains, respectively in the cylinder and the long strip samples prepared from a real S38C hollow axle, indicated a gradient evolution distribution with a depth of $$sim$$ 8 mm, covering a range of -5500 $$sim$$ 1000 $$mu$$$$varepsilon$$ for axial strains and -6500 $$sim$$ 1000 $$mu$$$$varepsilon$$ for hoop strains. More importantly, the maximum compressive lattice strain of the cylinder sample was increased by 15.61%, and 22.35% at the impacting speeds of 100, and 125 m/s, respectively; and that of the long strip sample increased by 29.17%, and 43.70%, respectively. It can thus be concluded that lattice strains have redistributed around the impact crater, demonstrating the local alteration of the residual strain field. These new findings suggest the localized variation in residual strains should be taken into account while evaluating the service damage evolution of railway axles, especially those affected by high-speed impacts during operation.

論文

Dual nanoprecipitation and nanoscale chemical heterogeneity in a secondary hardening steel for ultrahigh strength and large uniform elongation

Wang, S.*; Wang, J.*; Zhang, S.*; Wei, D.*; Chen, Y.*; Rong, X.*; Gong, W.; Harjo, S.; Liu, X.*; Jiao, Z.*; et al.

Journal of Materials Science & Technology, 185, p.245 - 258, 2024/06

https://doi.org/10.1016/j.jmst.2023.10.048
 被引用回数：15 パーセンタイル：97.90(Materials Science, Multidisciplinary)

Nanoprecipitates and nanoscale retained austenite (RA) with suitable stability play crucial roles in determining the yield strength (YS) and ductility of ultrahigh strength steels (UHSSs). However, owing to the kinetics incompatibility between nanoprecipitation and austenite reversion, it is highly challenging to simultaneously introduce high-density nanoprecipitates and optimized RA in UHSSs. In this work, through the combination of austenite reversion treatment (ART) and subsequent flash austenitizing (FA), nanoscale chemical heterogeneity was successfully introduced into a low-cost UHSS prior to the aging process. This chemical heterogeneity involved the enrichment of Mn and Ni in the austenite phase. The resulting UHSS exhibited dual-nanoprecipitation of Ni(Al,Mn) and (Mo,Cr)$$_{2}$$ C and nanoscale austenite stabilized via Mn and Ni enrichment. The hard martensitic matrix strengthened by high-density dual-nanoprecipitates constrains the plastic deformation of soft RA with a relatively low fraction, and the presence of relatively stable nanoscale RA with adequate Mn and Ni enrichment leads to a marginal loss in YS but keeps a persistent transformation-induced plasticity (TRIP) effect. As a result, the newly-developed UHSS exhibits an ultrahigh YS of 1.7 GPa, an ultimate tensile strength (UTS) of 1.8 GPa, a large uniform elongation (UE) of 8.5 percent, and a total elongation (TE) of 13 percent. The strategy of presetting chemical heterogeneity to introduce proper metastable phases before aging can be extended to other UHSSs and precipitation-hardened alloys.

論文

Direct observations of dynamic and reverse transformation of Ti-6Al-4V alloy and pure titanium

Guo, B.*; Chen, H.*; Chong, Y.*; Mao, W.; Harjo, S.; Gong, W.; Zhang, Z.*; Jonas, J. J.*; 辻 伸泰*

Acta Materialia, 268, p.119780_1 - 119780_11, 2024/04

https://doi.org/10.1016/j.actamat.2024.119780
 被引用回数：9 パーセンタイル：92.77(Materials Science, Multidisciplinary)

This paper focused on the characterization and mechanism of the dynamic transformation from the alpha to beta phase during the hot deformation of Ti-6Al-4V alloy and pure titanium. The investigation employed in-situ neutron diffraction and atomistic simulations for a comprehensive understanding of the process. Dynamic transformations were observed during deformation of the Ti-6Al-4V alloy and pure titanium below the beta transus temperatures. During isothermal holding after unloading, the in-situ neutron diffraction results for Ti-6Al-4V and pure titanium indicated a sluggish reverse transformation from the beta to alpha phase. The mechanism of dynamic transformation was explored through in-situ neutron diffraction and atomistic simulations, which revealed twofold effects of deformation on dynamic transformation. Firstly, deformation led to a significant rise in the Gibbs energy of the alpha phase relative to the beta phase, expanding the beta phase region and diminishing the alpha phase region. Secondly, deformation lowered the energy barriers associated with dynamic transformation, facilitating the activation of dynamic transformation more readily than in the equilibrium state before deformation.

論文

Onset of collectivity for argon isotopes close to $$N=32$$

Linh, B. D.*; Corsi, A.*; Gillibert, A.*; Obertelli, A.*; Doornenbal, P.*; Barbieri, C.*; Duguet, T.*; G$'o$mez-Ramos, M.*; Holt, J. D.*; Hu, B. S.*; et al.

Physical Review C, 109(3), p.034312_1 - 034312_15, 2024/03

https://doi.org/10.1103/PhysRevC.109.034312
 被引用回数：2 パーセンタイル：58.81(Physics, Nuclear)

理化学研究所RIビームファクトリーにて中性子過剰核$$^{50}$$Arビームからの1中性子ノックアウト反応実験を行い、$$^{49}$$Arのエネルギー準位および分光学的因子を導出した。特に、第一励起状態の$$1/2^-$$への分光学的因子が大きいことから、始状態の$$^{50}$$Arの基底状態において中性子が$$p_{1/2}$$軌道を多く占めていることがわかった。これは、中性子数32がよい魔法数として知られる$$^{52}$$Caとは異なった性質であり、カルシウムからアルゴンへと陽子が2個減ることで閉殻構造が大きく崩れることが明らかになった。

論文

Quantum critical behavior of the hyperkagome magnet Mn$$_3$$CoSi

山内 宏樹; Sari, D. P.*; 安井 幸夫*; 坂倉 輝俊*; 木村 宏之*; 中尾 朗子*; 大原 高志; 本田 孝志*; 樹神 克明; 井川 直樹; et al.

Physical Review Research (Internet), 6(1), p.013144_1 - 013144_9, 2024/02

https://doi.org/10.1103/PhysRevResearch.6.013144

$$beta$$-Mn-type family alloys Mn$$_3$$$$TX$$ have three-dimensional antiferromagnetic (AFM) corner-shared triangular network. The antiferromagnet Mn$$_3$$RhSi shows magnetic short-range order (SRO) over a wide temperature range of approximately 500 K above the N$'{e}$el temperature $$T_{rm N}$$ = 190 K. Mn$$_3$$CoSi has the smallest lattice parameter and the lowest $$T_{rm N}$$ in the family compounds. The quantum critical point (QCP) from AFM to the quantum paramagnetic state is expected near a cubic lattice parameter of 6.15 $AA. Although $T_N$$ of Mn$$_3$$CoSi is only 140 K, quantum critical behavior is observed in Mn$$_3$$CoSi as the enhancement of the electronic specific heat coefficient $$gamma$$. We study how the magnetic SRO appears in Mn$$_3$$CoSi by using neutron scattering, $$mu$$SR, and physical property measurements. The experimental results show that the neutron scattering intensity of the magnetic SRO does not change much regardless of the suppressed magnetic moment in the long-range magnetic ordered state compared to those of Mn$$_3$$RhSi. The initial asymmetry drop ratio of $$mu$$SR above $$T_{rm N}$$ becomes small, and the magnetic SRO temperature $$T_{SRO}$$ is suppressed to 240 K. The results suggest that the Mn$$_3$$CoSi is close to the QCP in the Mn$$_3$$$$TX$$ system.

論文

Strongly coupled spin waves and surface acoustic waves at room temperature

Hwang, Y.*; Puebla, J.*; 近藤 浩太*; Gonzalez-Ballestero, C.*; 一色 弘成*; S$'a$nchez Mu$~n$oz, C.*; Liao, L.*; Chen, F.*; Luo, W.*; 前川 禎通*; et al.

Physical Review Letters, 132(5), p.056704_1 - 056704_7, 2024/01

https://doi.org/10.1103/PhysRevLett.132.056704
 被引用回数：16 パーセンタイル：97.43(Physics, Multidisciplinary)

Here, we report the observation of strong coupling between magnons and surface acoustic wave (SAW) phonons in a thin CoFeB film constructed in an on-chip SAW resonator by analyzing SAW phonon dispersion anticrossings. We employ a nanostructured SAW resonator design that, in contrast to conventional SAW resonators, allows us to enhance shear-horizontal strain. Crucially, this type of strain couples strongly to magnons. Our device design provides the tunability of the film thickness with a fixed phonon wavelength, which is a departure from the conventional approach in strong magnon-phonon coupling research. We detect a monotonic increase in the coupling strength by expanding the film thickness, which agrees with our theoretical model. Our work offers a significant way to advance fundamental research and the development of devices based on magnon-phonon hybrid quasiparticles.

論文

Fully strange tetraquark states with the exotic quantum numbers $$J^{PC}=0^{+-}$$ and $$2^{+1-}$$

Xi, H.-Z.*; Jiang, Y.-W.*; Chen, H.-X.*; 保坂 淳; Su, N.*

Physical Review D, 108(9), p.094019_1 - 094019_13, 2023/11

https://doi.org/10.1103/PhysRevD.108.094019
 被引用回数：4 パーセンタイル：51.67(Astronomy & Astrophysics)

$$J^{PC}=0^{+-}$$と$$2^{+1-}$$の量子数をもつ、ストレンジクォークのみからなるテトラクォークを理論的に調べた結果を報告する。前者および後者の質量はそれぞれ2.47GeV、3.07GeVであるなど、いくつかの予言値を得た。

論文

Validation of the $$^{10}$$Be ground-state molecular structure using $$^{10}$$Be($$p,palpha$$)$$^{6}$$He triple differential reaction cross-section measurements

Li, P. J.*; Beaumel, D.*; Lee, J.*; Assi$'e$, M.*; Chen, S.*; Franchoo, S.*; Gibelin, J.*; Hammache, F.*; Harada, T.*; 延与 佳子*; et al.

Physical Review Letters, 131(21), p.212501_1 - 212501_7, 2023/11

https://doi.org/10.1103/PhysRevLett.131.212501
 被引用回数：21 パーセンタイル：93.59(Physics, Multidisciplinary)

$$^{10}$$Beのクラスター構造を($$p,palpha$$)反応を用いて調査した。三重微分断面積が実験的に測定され、Tohsaki-Horiuchi-Schuck-R$"o$pke波動関数の方法や反対称化分子動力学を用いた歪曲波インパルス近似計算と比較した。実験データと理論計算の顕著な一致が確認され、$$^{10}$$Beの比較的コンパクトな分子状態を確認した。

論文

Spiral spin cluster in the hyperkagome antiferromagnet Mn$$_{3}$$RhSi

社本 真一; 山内 宏樹; 飯田 一樹*; 池内 和彦*; Hall, A. E.*; Chen, Y.-S.*; Lee, M. K.*; Balakrishnan, G.*; Chang, L.-J.*

Communications Physics (Internet), 6, p.248_1 - 248_6, 2023/09

https://doi.org/10.1038/s42005-023-01363-1
 被引用回数：2 パーセンタイル：40.37(Physics, Multidisciplinary)

Mn$$_{3}$$RhSi単結晶の中性子散乱測定により、局所スピン相関秩序がらせん構造を持つことがわかった。磁気クラスター形成の起源の可能性を、リフシッツ不変量とグリフィス相の観点から議論し、Co$$_{7}$$Zn$$_{7}$$Mn$$_{6}$$の室温スキルミオン相とMnの非フェルミ液体挙動と比較した。

論文

3D-printed epidermal sweat microfluidic systems with integrated microcuvettes for precise spectroscopic and fluorometric biochemical assays

Yang, D. S.*; Wu, Y.*; Kanatzidis, E. E.*; Avila, R.*; Zhou, M.*; Bai, Y.*; Chen, S.*; 関根 由莉奈; Kim, J.*; Deng, Y.*; et al.

Materials Horizons, 10(11), p.4992 - 5003, 2023/09

https://doi.org/10.1039/D3MH00876B
 被引用回数：12 パーセンタイル：79.80(Chemistry, Multidisciplinary)

本論文では、ハード及びソフトハイブリッド材料システムでの3Dプリントによって形成されたマイクロ流体ネットワーク、統合バルブ、およびマイクロスケール光学キュベットにより、汗成分に対してその場で分光および蛍光分析した成果を紹介する。一連の試験により、これらのマイクロキュベットシステムが汗中の銅、塩化物、グルコースの濃度と汗のpHを実験室レベルの精度と感度で評価できることが実証された。

論文

Extreme phonon anharmonicity underpins superionic diffusion and ultralow thermal conductivity in argyrodite Ag$$_{8}$$SnSe$$_{6}$$

Ren, Q.*; Gupta, M. K.*; Jin, M.*; Ding, J.*; Wu, J.*; Chen, Z.*; Lin, S.*; Fabelo, O.*; Rodriguez-Velamazan, J. A.*; 古府 麻衣子; et al.

Nature Materials, 22(8), p.999 - 1006, 2023/08

https://doi.org/10.1038/s41563-023-01560-x
 被引用回数：76 パーセンタイル：99.20(Chemistry, Physical)

Ultralow thermal conductivity and fast ionic diffusion endow superionic materials with excellent performance both as thermoelectric converters and as solid-state electrolytes. Yet the correlation and interdependence between these two features remain unclear owing to a limited understanding of their complex atomic dynamics. Here we investigate ionic diffusion and lattice dynamics in argyrodite Ag$$_{8}$$SnSe$$_{6}$$ using synchrotron X-ray and neutron scattering techniques along with machine-learned molecular dynamics. We identify a critical interplay of the vibrational dynamics of mobile Ag and a host framework that controls the overdamping of low-energy Ag-dominated phonons into a quasi-elastic response, enabling superionicity. Concomitantly, the persistence of long-wavelength transverse acoustic phonons across the superionic transition challenges a proposed 'liquid-like thermal conduction' picture. Rather, a striking thermal broadening of low-energy phonons, starting even below 50 K, reveals extreme phonon anharmonicity and weak bonding as underlying features of the potential energy surface responsible for the ultralow thermal conductivity ($$<$$ 0.5 Wm$$^{-1}$$K$$^{-1}$$) and fast diffusion. Our results provide fundamental insights into the complex atomic dynamics in superionic materials for energy conversion and storage.

論文

Level structures of $$^{56,58}$$Ca cast doubt on a doubly magic $$^{60}$$Ca

Chen, S.*; Browne, F.*; Doornenbal, P.*; Lee, J.*; Obertelli, A.*; 角田 佑介*; 大塚 孝治*; 茶園 亮樹*; Hagen, G.*; Holt, J. D.*; et al.

Physics Letters B, 843, p.138025_1 - 138025_7, 2023/08

https://doi.org/10.1016/j.physletb.2023.138025
 被引用回数：9 パーセンタイル：85.35(Astronomy & Astrophysics)

$$^{57,59}$$Scからの1陽子ノックアウト反応を用いて、$$^{56}$$Caと$$^{58}$$Caのガンマ崩壊を観測した。$$^{56}$$Caでは1456(12)keVの$$gamma$$線遷移が、$$^{58}$$Caでは1115(34)keVの遷移が観測された。どちらの遷移も暫定的に$$2^{+}_{1} rightarrow 0^{+}_{gs}$$と割り当てられた。有効核子間相互作用をわずかに修正した広い模型空間での殻模型計算では、$$2^{+}_{1}$$準位エネルギー、2中性子分離エネルギー、反応断面積が実験とよく一致し、N=34閉殻の上に新しい殻が形成されていることを裏付けた。その構成要素である$$0_{f5/2}$$と$$0_{g9/2}$$軌道はほぼ縮退しており、これは$$^{60}$$Caが二重魔法核である可能性を排除し、Ca同位体のドリップラインを$$^{70}$$Caあるいはそれ以上にまで広げる可能性がある。

論文

Cu $$K$$-edge X-ray absorption fine structure study of $$T'$$-type $$RE$$$$_{2}$$CuO$$_{4+alpha-delta}$$ ($$RE$$ = Rare Earth); Toward unified understanding of electronic state of $$T'$$-type cuprate

Chen, Y.*; 浅野 駿*; Wang, T.*; Xie, P.*; 北山 慎之介*; 石井 賢司*; 松村 大樹; 辻 卓也; 谷口 貴紀*; 藤田 全基*

JPS Conference Proceedings (Internet), 38, p.011050_1 - 011050_6, 2023/05

https://doi.org/10.7566/JPSCP.38.011050

To investigate the variation of the electronic state of $$T'$$-type cuprate due to annealing, we performed Cu $$K$$-edge X-ray absorption fine structure measurements on Pr$$_{2}$$CuO$$_{4+alpha-delta}$$ (PCO) and Pr$$_{1.3}$$La$$_{0.7}$$CuO$$_{4+alpha-delta}$$ (PLCO). The induced electrons due to annealing ($$n_{AN}$$) in PCO and PLCO were approximately 2$$delta$$, consistent with a model of electron doping to Mott insulator. Here, $$alpha$$ and $$delta$$ represent the amount of excess oxygen from the stoichiometric composition in the as-sintered compound and that of oxygen loss due to annealing, respectively. Furthermore, the energy of the Einstein oscillator ($$hbaromega_{E}$$) for the Cu-O$$_{p}$$ bond was evaluated by extended X-ray absorption fine structure analysis. (O$$_{p}$$ denotes the in-plane oxygen.) We found a small annealing effect on $$hbaromega_{E}$$ for both PCO and PLCO.

論文

Hybridized propagation of spin waves and surface acoustic waves in a multiferroic-ferromagnetic heterostructure

Chen, J.*; 山本 慧; Zhang, J.*; Ma, J.*; Wang, H.*; Sun, Y.*; Chen, M.*; Liu, S.*; Gao, P.*; Yu, D.*; et al.

Physical Review Applied (Internet), 19(2), p.024046_1 - 024046_9, 2023/02

https://doi.org/10.1103/PhysRevApplied.19.024046
 被引用回数：6 パーセンタイル：64.95(Physics, Applied)

Coherent coupling in magnon based hybrid system has many potential applications in quantum information processing. Magnons can propagate in magnetically ordered materials without any motion of electrons, offering a unique method to build low-power-consumption devices and information channels free of heat dissipation. In this article, we demonstrate the coherent propagation of hybridized modes between spin waves and Love surface acoustic waves in a multiferroic BiFeO$$_{3}$$ and ferromagnetic La$$_{0.67}$$Sr$$_{0.33}$$MnO$$_{3}$$ based heterostructure. The magneto-elastic coupling enables a giant enhancement of strength of the hybridized mode by a factor of 26 compared to that of the pure spin waves. A short wavelength down to 250 nm is demonstrated for the hybridized mode, which is desirable for nanoscale acousto-magnonic applications. Our combined experimental and theoretical analyses represent an important step towards the coherent control in hybrid magnonics, which may inspire the study of magnon-phonon hybrid systems for coherent information processing and manipulation.

論文

Unexpected dynamic transformation from $$alpha$$ phase to $$beta$$ phase in zirconium alloy revealed by in-situ neutron diffraction during high temperature deformation

Guo, B.*; Mao, W.; Chong, Y.*; 柴田 曉伸*; Harjo, S.; Gong, W.; Chen, H.*; Jonas, J. J.*; 辻 伸泰*

Acta Materialia, 242, p.118427_1 - 118427_11, 2023/01

https://doi.org/10.1016/j.actamat.2022.118427
 被引用回数：12 パーセンタイル：70.10(Materials Science, Multidisciplinary)

Dynamic transformation from alpha (HCP) to beta (BCC) phase in a zirconium alloy was revealed by the use of in-situ neutron diffraction during hot compression. The dynamic transformation was unexpectedly detected during isothermal compression at temperatures of 900$$^{circ}$$C and 950$$^{circ}$$C (alpha + beta two-phase region) and strain rates of 0.01 s$$^{-1}$$ and 0.001 s$$^{-1}$$, even though equilibrium two-phase states were achieved prior to the hot compression. Dynamic transformation was accompanied by diffusion of Sn from beta to alpha phase, which resulted in changes of lattice parameters and a characteristic microstructure of alpha grains. The details of dynamic transformation are discussed using the evolution of lattice constants.

論文

Study of the $$N=32$$ and $$N=34$$ shell gap for Ti and V by the first high-precision multireflection time-of-flight mass measurements at BigRIPS-SLOWRI

飯村 俊*; Rosenbusch, M.*; 高峰 愛子*; 角田 佑介*; 和田 道治*; Chen, S.*; Hou, D. S.*; Xian, W.*; 石山 博恒*; Yan, S.*; et al.

Physical Review Letters, 130(1), p.012501_1 - 012501_6, 2023/01

https://doi.org/10.1103/PhysRevLett.130.012501
 被引用回数：13 パーセンタイル：88.25(Physics, Multidisciplinary)

The atomic masses of $$^{55}$$Sc, $$^{56,58}$$Ti, and $$^{56-59}$$V have been determined using the high-precision multireflection time-of-flight technique. The radioisotopes have been produced at RIKEN's Radioactive Isotope Beam Factory (RIBF) and delivered to the novel designed gas cell and multireflection system, which has been recently commissioned downstream of the ZeroDegree spectrometer following the BigRIPS separator. For $$^{56,58}$$Ti and $$^{56-59}$$V, the mass uncertainties have been reduced down to the order of 10 keV, shedding new light on the $$N=34$$ shell effect in Ti and V isotopes by the first high-precision mass measurements of the critical species $$^{58}$$Ti and $$^{59}$$V. With the new precision achieved, we reveal the nonexistence of the $$N=34$$ empirical two-neutron shell gaps for Ti and V, and the enhanced energy gap above the occupied $$nu$$p$$_{3/2}$$ orbit is identified as a feature unique to Ca. We perform new Monte Carlo shell model calculations including the $$nu$$d$$_{5/2}$$ and $$nu$$g$$_{9/2}$$ orbits and compare the results with conventional shell model calculations, which exclude the $$nu$$g$$_{9/2}$$ and the $$nu$$d$$_{5/2}$$ orbits. The comparison indicates that the shell gap reduction in Ti is related to a partial occupation of the higher orbitals for the outer two valence neutrons at $$N = 34$$.

論文

"Southwestern" boundary of the $$N = 40$$ island of inversion; First study of low-lying bound excited states in $$^{59}$$V and $$^{61}$$V

Elekes, Z.*; Juh$'a$sz, M. M.*; Sohler, D.*; Sieja, K.*; 吉田 数貴; 緒方 一介*; Doornenbal, P.*; Obertelli, A.*; Achouri, N. L.*; 馬場 秀忠*; et al.

Physical Review C, 106(6), p.064321_1 - 064321_10, 2022/12

https://doi.org/10.1103/PhysRevC.106.064321
 被引用回数：3 パーセンタイル：32.42(Physics, Nuclear)

$$^{59}$$Vと$$^{61}$$Vの低励起準位構造を初めて探索した。$$^{61}$$Vについては中性子ノックアウト反応と陽子非弾性散乱が、$$^{59}$$Vについては中性子ノックアウト反応データが得られた。$$^{59}$$Vについては4つ、$$^{61}$$Vについては5つの新たな遷移が確認された。Lenzi-Nowacki-Poves-Sieja (LNPS)相互作用に基づく殻模型計算との比較によって、それぞれの同位体について確認されたガンマ線のうち3つが、first 11/2$$^{-}$$状態とfirst 9/2$$^{-}$$状態からの崩壊と決定された。$$^{61}$$Vについては、($$p$$,$$p'$$)非弾性散乱断面積は四重極変形と十六重極変形を想定したチャネル結合法により解析されたが、十六重極変形の影響により、明確に反転の島に属するとは決定できなかった。

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