Multiple mechanisms in proton-induced nucleon removal at 100 MeV/nucleon

Pohl, T.*; Sun, Y. L.*; Obertelli, A.*; Lee, J.*; Gmez-Ramos, M.*; Ogata, Kazuyuki*; Yoshida, Kazuki; Cai, B. S.*; Yuan, C. X.*; Brown, B. A.*; et al.

Physical Review Letters, 130(17), p.172501_1 - 172501_8, 2023/04

https://doi.org/10.1103/PhysRevLett.130.172501

We report on the first proton-induced single proton- and neutron-removal reactions from the neutron deficient O nucleus with large Fermi-surface asymmetry at 100 MeV/nucleon. Our results provide the first quantitative contributions of multiple reaction mechanisms including the quasifree knockout, inelastic scattering, and nucleon transfer processes. It is shown that the inelastic scattering and nucleon transfer, usually neglected at such energy regime, contribute about 50% and 30% to the loosely bound proton and deeply bound neutron removal, respectively.

Status of the uncertainty quantification for severe accident sequences of different NPP-designs in the frame of the H-2020 project MUSA

Brumm, S.*; Gabrielli, F.*; Sanchez-Espinoza, V.*; Groudev, P.*; Ou, P.*; Zhang, W.*; Malkhasyan, A.*; Bocanegra, R.*; Herranz, L. E.*; Berda, M.*; et al.

Proceedings of 10th European Review Meeting on Severe Accident Research (ERMSAR 2022) (Internet), 13 Pages, 2022/05

Long decay length of magnon-polarons in BiFeO/LaSrMnO heterostructures

Zhang, J.*; Chen, M.*; Chen, J.*; Yamamoto, Kei; Wang, H.*; Hamdi, M.*; Sun, Y.*; Wagner, K.*; He, W.*; Zhang, Y.*; et al.

Nature Communications (Internet), 12, p.7258_1 - 7258_8, 2021/12

https://doi.org/10.1038/s41467-021-27405-2

Phase transition and chemical reactivity of 1H-tetrazole under high pressure up to 100 GPa

Gao, D.*; Tang, X.*; Wang, X.*; Yang, X.*; Zhang, P.*; Che, G.*; Han, J.*; Hattori, Takanori; Wang, Y.*; Dong, X.*; et al.

Physical Chemistry Chemical Physics, 23(35), p.19503 - 19510, 2021/09

https://doi.org/10.1039/D1CP02913D

Pressure-induced phase transition and polymerization of nitrogen-rich molecules are widely focused due to its extreme importance for the development of green high energy density materials. Here, we present a study of the phase transition and chemical reaction of 1H-tetrazole up to 100 GPa by using Raman, IR, X-ray diffraction, neutron diffraction techniques and theoretical calculation. A phase transition above 2.6 GPa was identified and the high-pressure structure was determined with one molecule in a unit cell. The 1H-tetrazole polymerizes reversibly below 100 GPa, probably through a carbon-nitrogen bonding instead of nitrogen-nitrogen bonding. Our studies updated the structure model of the high pressure phase of 1H-tetrazole, and presented the possible intermolecular bonding route for the first time, which gives new insights to understand the phase transition and chemical reaction of nitrogen-rich compounds, and benefit for designing new high energy density materials.

Distance-selected topochemical dehydro-diels-alder reaction of 1,4-Diphenylbutadiyne toward crystalline graphitic nanoribbons

Zhang, P.*; Tang, X.*; Wang, Y.*; Wang, X.*; Gao, D.*; Li, Y.*; Zheng, H.*; Wang, Y.*; Wang, X.*; Fu, R.*; et al.

Journal of the American Chemical Society, 142(41), p.17662 - 17669, 2020/10

https://doi.org/10.1021/jacs.0c08274

Solid-state topochemical polymerization (SSTP) is a promising method to construct functional crystalline polymeric materials, but in contrast to various reactions that happen in solution, only very limited types of SSTP reactions are reported. Diels-Alder (DA) and dehydro-DA (DDA) reactions are textbook reactions for preparing six-membered rings in solution but are scarcely seen in solid-state synthesis. Here, using multiple cutting-edge techniques, we demonstrate that the solid 1,4-diphenylbutadiyne (DPB) undergoes a DDA reaction under 10-20 GPa with the phenyl as the dienophile. The crystal structure at the critical pressure shows that this reaction is "distance-selected". The distance of 3.2 between the phenyl and the phenylethynyl facilitates the DDA reaction, while the distances for other DDA and 1,4-addition reactions are too large to allow the bonding. The obtained products are crystalline armchair graphitic nanoribbons, and hence our studies open a new route to construct the crystalline carbon materials with atomic-scale control.

Status of study of long-term assessment of transport of radioactive contaminants in the environment of Fukushima (FY2018)

Nagao, Fumiya; Niizato, Tadafumi; Sasaki, Yoshito; Ito, Satomi; Watanabe, Takayoshi; Dohi, Terumi; Nakanishi, Takahiro; Sakuma, Kazuyuki; Hagiwara, Hiroki; Funaki, Hironori; et al.

JAEA-Research 2019-002, 235 Pages, 2019/08

JAEA-Research-2019-002.pdf:21.04MB

The accident of the Fukushima Daiichi Nuclear Power Station (hereinafter referred to 1F), Tokyo Electric Power Company Holdings, Inc. occurred due to the Great East Japan Earthquake, Sanriku offshore earthquake, of 9.0 magnitude and the accompanying tsunami. As a result, large amount of radioactive materials was released into the environment. Under these circumstances, JAEA has been conducting Long-term Environmental Dynamics Research concerning radioactive materials released in environment, especially migration behavior of radioactive cesium since November 2012. This report is a summary of the research results that have been obtained in environmental dynamics research conducted by JAEA in Fukushima Prefecture.

Formation of advanced tokamak plasmas without the use of an ohmic-heating solenoid

Shiraiwa, Shunichi*; Ide, Shunsuke; Ito, Satoshi*; Mitarai, Osamu*; Naito, Osamu; Ozeki, Takahisa; Sakamoto, Yoshiteru; Suzuki, Takahiro; Takase, Yuichi*; Tanaka, Shigetoshi*; et al.

Physical Review Letters, 92(3), p.035001_1 - 035001_4, 2004/01

https://doi.org/10.1103/PhysRevLett.92.035001

no abstracts in English

Results of ITER test blanket module mock-up experiments on DIII-D

Snipes, J. A.*; Schaffer, M. J.*; Gohil, P.*; de Vries, P.*; Fenstermacher, M. E.*; Evans, T. E.*; Gao, X. M.*; Garofalo, A.*; Gates, D. A.*; Greenfield, C. M.*; et al.

no journal, , 

A series of experiments was performed on DIII-D to mock-up the field that will be induced in a pair of ferromagnetic Test Blanket Modules (TBMs) in ITER to determine the effects of such error fields on plasma operation and performance. A set of coils producing both poloidal and toroidal fields was placed inside a re-entrant horizontal port close to the plasma. The coils produce a localized ripple due to the toroidal field (TF) + TBM up to 5.7%, which is more than four times that expected from a pair of representative 1.3 ton TBMs in ITER. The experiments show that the reduction in the toroidal rotation is sensitive to the ripple. On the other hand, the confinement is reduced by up to 15-18% for local ripple 3% but is hardly affected at 1.7% local ripple.

Investigation of in-reactor cesium chemical behavior in TEPCO's Fukushima Daiichi Nuclear Power Station accident, 8; Behavior of Si in oxide layer on stainless steel

Zheng, L.*; Hosoi, Kazuya*; Ueda, Shigeru*; Gao, X.*; Kitamura, Shinya*; Kobayashi, Yoshinao*; Osaka, Masahiko

no journal, , 

Si source for Cs-bearing particle formed by Fukushima-Daiichi NPS accident has yet to be revealed. Stainless steel is possible Si source since it is used as structure material in the reactor and includes Si. In this study, Si vaporization behavior was evaluated by investigation of Si behavior in oxide layer formed in steam atmosphere at 1473 K.