Nguyen, P. L.; Daido, Hiroyuki; Yamada, Tomonori; Nishimura, Akihiko; Hasegawa, Noboru*; Kawachi, Tetsuya*
Journal of Laser Applications, 29(4), p.041501_1 - 041501_11, 2017/11
no abstracts in English
Nishikino, Masaharu; Ishino, Masahiko; Ichimaru, Satoshi*; Hatayama, Masatoshi*; Hasegawa, Noboru; Kawachi, Tetsuya
Reza Gakkai Dai-483-Kai Kenkyukai Hokoku; Tanhacho Ryoshi Bimu Hassei To Sono Oyo, p.25 - 28, 2015/12
X-ray ablation has been recently achieved using plasma soft X-ray lasers (SXRLs), laser plasma soft X-rays, and X-ray free electron lasers. In order to study the interactions between picosecond SXRL beams and material and multi-layered structure surfaces were irradiated with SXRL pulse. Following irradiation, the substrate surface was observed using a scanning electron microscope and an atomic force microscope. The surface modifications caused by the SXRL beam were clearly seen. The multi-layered mirror is the important component for the EUV lithography. Then, we have started the damage test of multi-layered structure, and the surface modifications caused by the SXRL pulse irradiations were confirmed.
Nuryanthi, N.*; Yamaki, Tetsuya; Kitamura, Akane; Koshikawa, Hiroshi; Yoshimura, Kimio; Sawada, Shinichi; Hasegawa, Shin; Asano, Masaharu; Maekawa, Yasunari; Suzuki, Akihiro*; et al.
Transactions of the Materials Research Society of Japan, 40(4), p.359 - 362, 2015/12
The ion-track grafting of a vinylbenzyl chloride (VBC) into a poly(ethylene-co-tetrafluoroethylene) (ETFE) film is necessary for preparing nanostructured hydroxide-ion-conductive electrolyte membranes. A key for success here is to obtain as high graft levels as possible (for higher conductivity) in a smaller number of tracks (for improving the other membrane properties). To this end, therefore, the effect of the medium for the VBC grafting was investigated as part of our continuing effort to optimize the experimental conditions. A 25 m-thick ETFE film was irradiated in a vacuum chamber with 560 MeV Xe at different fluences, and then the grafting was performed by immersing the irradiated films in a 20vol% VBC monomer at 60C. A medium was a mixture of water (HO) and isopropyl alcohol (iPrOH) at different volume ratios. The degree of grafting increased as the HO content became higher, and reached a maximum in pure HO. These results can be explained by considering the well-known Trommsdorff effect, in which poor solubility of the grafted polymer in polar media leads to an increased polymerization rate probably due to a lower termination rate.
Namba, Shinichi*; Hasegawa, Noboru; Kishimoto, Maki; Nishikino, Masaharu; Ishino, Masahiko; Kawachi, Tetsuya
AIP Advances (Internet), 5(11), p.117101_1 - 117101_10, 2015/11
To characterize the temporal evolution of ultrashort X-ray pulses emitted by laser plasmas using a pump-probe method, a magnetic bottle time-of-flight electron spectrometer is constructed. The design is determined by numerical calculations of a mirror magnetic field and of the electron trajectory in a flight tube. The performance of the spectrometer is characterized by measuring the electron spectra of xenon atoms irradiated with a laser-driven plasma X-ray pulse. In addition, as a preliminary experiment, two-color above-threshold ionization (ATI) is conducted, in which xenon atoms are simultaneously irradiated with an X-ray laser pump and an IR laser probe. The correlation in the intensity of the Auger sideband spectra and in the time delay of the two laser pulses yields an X-ray pulse width of 5.7 ps, in good agreement with the value obtained using an X-ray streak camera.
Kim, C. M.*; Steil, H.*; Matou, B.*; Nishikino, Masaharu; Hasegawa, Noboru; Kawachi, Tetsuya; Tran, K. A.*; Janulewicz, K. A.*
Physical Review A, 92(4), p.043807_1 - 043807_7, 2015/10
We present polarization measurement of a Ni-like Ag X-ray laser working in the transient collisional excitation scheme. A calibrated membrane multilayer beam splitter was used to determine the energies of two mutually perpendicular polarization components (s and p components). As a result, we observed a high degree of polarization that fluctuated from shot to shot. The dominant polarization component switched from s to p when pumping was made stronger. The measurement results are discussed from the point of view of the general polarization theory and supported by a numerical simulation based on Maxwell-Bloch equations.
Dinh, T.-H.*; Suzuki, Yuhei*; Arai, Goki*; Li, B.*; Dunne, P.*; O'Sullivan, G.*; Fujioka, Shinsuke*; Hasegawa, Noboru; Kawachi, Tetsuya; Nishikino, Masaharu; et al.
Applied Physics Letters, 107(12), p.121101_1 - 121101_5, 2015/09
Ishino, Masahiko; Hasegawa, Noboru; Nishikino, Masaharu; Pikuz, T.*; Skobelev, I. Y.*; Faenov, A.*; Inogamov, N.*; Kawachi, Tetsuya; Yamagiwa, Mitsuru
X-Ray Lasers and Coherent X-Ray Sources; Development and Applications XI (Proceedings of SPIE, Vol.9589), p.958904_1 - 958904_6, 2015/09
To study the ablation process induced by the soft X-ray laser pulse, we investigated the electron temperature of the ablating material. Focused soft X-ray laser pulses having a wavelength of 13.9 nm and duration of 7 ps were irradiated onto target surfaces, and we observed the optical emission from surfaces by use of an optical camera. On target surfaces, we could confirm damage structures, but no emission signal in the visible spectral range during ablation could be observed. Then, we estimated the electron temperature in the ablating matter, and we estimated the electron temperature to be lower than 1 eV and the process duration was shorter than 1000 ps. This result is in good accordance with the theoretical prediction. Our investigation implies that the spallative ablation occurs in the low electron temperature region of a non-equilibrium state of warm dense matter. We will present the current state of our eperimental results.
Nishikino, Masaharu; Kawachi, Tetsuya; Hasegawa, Noboru; Ishino, Masahiko; Minami, Yasuo*; Suemoto, Toru*; Onishi, Naofumi*; Ito, Atsushi*; Sato, Katsutoshi*; Faenov, A.*; et al.
X-Ray Lasers and Coherent X-Ray Sources; Development and Applications XI (Proceedings of SPIE, Vol.9589), p.958902_1 - 958902_7, 2015/09
Hasegawa, Noboru; Nishikino, Masaharu; Tomita, Takuro*; Onishi, Naofumi*; Ito, Atsushi*; Eyama, Tsuyoshi*; Kakimoto, Naoya*; Izutsu, Rui*; Minami, Yasuo*; Baba, Motoyoshi*; et al.
X-Ray Lasers and Coherent X-Ray Sources; Development and Applications XI (Proceedings of SPIE, Vol.9589), p.95890A_1 - 95890A_8, 2015/09
We have improved a soft X-ray laser (SXRL) interferometer synchronized with a Ti:Sapphire laser pulse to observe the single-shot imaging of the nano-scaled structure dynamics of the laser induced materials. By the precise imaging optics and double time fiducial system having been installed, the lateral resolution on the sample surface and the precision of the temporal synchronization between the SXRL and Ti:Sapphire laser pulses were improved to be 700 nm and 2 ps, respectively. By using this system, the initial stage (before 200 ps) of the ablation process of the Pt surface pumped by 80 fs Ti:Sapphire laser pulse was observed by the comparison between the soft X-ray reflective image and interferogram. We have succeeded in the direct observation of the unique ablation process around the ablation threshold such as the rapid increase of the surface roughness and surface vibration.
Janulewicz, K. A.*; Kim, C. M.*; Steil, H.*; Kawachi, Tetsuya; Nishikino, Masaharu; Hasegawa, Noboru
X-Ray Lasers and Coherent X-Ray Sources; Development and Applications XI (Proceedings of SPIE, Vol.9589), p.95890N_1 - 95890N_7, 2015/09
We describe measurement results on the polarization state of amplified spontaneous emission signal from a collisionally pumped Ni-like Ag soft X-ray laser with a transient inversion. The result obtained with a calibrated membrane beam splitter as a polarization state (P-state) selector shows that dominance one of the mutually perpendicular electric field components (p- or s-) in the output signal depends on the hydrodynamic state of the plasma medium. Two different hydrodynamic states were referred as a low gain and high gain regimes and the allocated P-states had dominant s- and p-component, respectively. It was also shown that due to correlations between p- and s-components in the process of coherent amplification of noise, correct description of the polarization state requires applying the generalized theory of polarization and formulated there the generalized degree of polarization.
Nishikino, Masaharu; Hasegawa, Noboru; Ishino, Masahiko; Ochi, Yoshihiro; Kawachi, Tetsuya; Yamagiwa, Mitsuru; Kato, Yoshiaki*
Chinese Optics Letters, 13(7), p.070002_1 - 070002_3, 2015/07
Hasegawa, Noboru; Tomita, Takuro*; Nishikino, Masaharu; Eyama, Tsuyoshi*; Kakimoto, Naoya*; Minami, Yasuo*; Baba, Motoyoshi*; Onishi, Naofumi*; Ito, Atsushi*; Kawachi, Tetsuya; et al.
JAEA-Conf 2015-001, p.17 - 20, 2015/07
We have succeeded in simultaneous observation of the ablation front and the expansion front with thin filmy structure in the femto-second laser ablation process of a gold target by using the 13.9 nm soft X-ray probe (incident angle to the sample 70 deg) with soft X-ray interferometer. The dependence on the laser local fluence and materials was obtained by the comparison between gold and tungsten.
Inogamov, N. A.*; Zhakhovsky, V. V.*; Hasegawa, Noboru; Nishikino, Masaharu; Yamagiwa, Mitsuru; Ishino, Masahiko; Agranat, M. B.*; Ashitkov, S. I.*; Faenov, A. Y.*; Khokhlov, V. A.*; et al.
Applied Physics B, 119(3), p.413 - 419, 2015/06
Nishikino, Masaharu; Hasegawa, Noboru; Tomita, Takuro*; Eyama, Tsuyoshi*; Kakimoto, Naoya*; Onishi, Naofumi*; Ito, Atsushi*; Baba, Motoyoshi*; Minami, Yasuo*; Kawachi, Tetsuya; et al.
Reza Gakkai Dai-471-Kai Kenkyukai Hokoku; Tanhacho Ryoshi Bimu Hassei To Sono Oyo, p.9 - 12, 2014/12
no abstracts in English
Ishino, Masahiko; Hasegawa, Noboru; Nishikino, Masaharu; Pikuz, T. A.*; Skobelev, I. Y.*; Faenov, A.*; Inogamov, N. A.*; Kawachi, Tetsuya; Yamagiwa, Mitsuru
Journal of Applied Physics, 116(18), p.183302_1 - 183302_6, 2014/11
We investigated the optical emission from the ablating surfaces induced by the irradiations of soft X-ray laser (SXRL) pulses with the aim of estimation of the maximum electron temperature. No emission signal in the spectral range of 400-800 nm could be observed despite the formation of damage structures on the target surfaces. Hence, we estimated an upper limit for the electron temperature of 0.4-0.7 eV for the process duration of 100-1000 ps. Our results imply that the ablation and/or surface modification by the SXRL is not accompanied by plasma formation but is induced by thermo-mechanical pressure, which is so called a spallative ablation. This spallative ablation process occurs in the low electron temperature region of a non-equilibrium state of warm dense matter.
Kawachi, Tetsuya; Hasegawa, Noboru; Iwamae, Atsushi*; Yoneda, Hitoki*
Journal of Physics; Conference Series, 548(1), p.012038_1 - 012038_7, 2014/11
Polarization is a fundamental property of light, and the effective use provides us powerful tools for probing materials and for plasma diagnostics. In plasmas, alignment of emission shows the plasma anisotropy, and Zeeman splitting informs us the magnetic field strength. We took the plasma-based soft X-ray laser as an example and observed the Zeeman splitting under the external magnetic field. A grazing incidence spectrograph, HIREFS, with the resolution of 15000 was used to observe the X-ray laser line. A magnetic coil driven by an electrical pulsed power supply provided the external magnetic field of 1035 T along the direction of the plasma column, and the left-handed and right-handed circular polarization components were obtained separately. The experimental result indicated that the magnetic field was larger by a factor of 4 than that of the applied field, which implied that the magnetic field compression occurred in the dynamics of the intense laser-plasma interaction.
Baba, Motoyoshi*; Nishikino, Masaharu; Hasegawa, Noboru; Tomita, Takuro*; Minami, Yasuo*; Takei, Ryota*; Yamagiwa, Mitsuru; Kawachi, Tetsuya; Suemoto, Toru
Japanese Journal of Applied Physics, 53(8), p.080302_1 - 080302_4, 2014/08
A grazing incidence reflection-type soft X-ay microscope, using a Fresnel zone plate and a soft X-ray laser with wavelength 13.9 nm and pulse width 7 ps, was developed. Submicron size groove structures made on a Pt film were clearly captured at a single shot exposure, with spatial resolution of about 360 nm. A wide field view of 100 m square was secured under the Kohler illumination. This microscope also had a large depth of focus of more than 100 m and was proven to have a sufficient performance for observing surface morphological changes.
Takahashi, Hideyuki*; Handa, Nobuo*; Murano, Takanori*; Terauchi, Masami*; Koike, Masato; Kawachi, Tetsuya; Imazono, Takashi; Hasegawa, Noboru; Koeda, Masaru*; Nagano, Tetsuya*; et al.
Microscopy and Microanalysis, 20(Suppl.3), p.684 - 685, 2014/08
A novel wavelength dispersive soft X-ray emission spectrometer (SXES) having a X-ray energy range of 50-210 eV has been developed. One feature is that the SXES is parallel detection of the signals so that it can be used like a conventional energy dispersive spectrometer. The other is a high energy resolution, which is about 0.2 eV at Al-L comparable to those revealed by XPS and EELS. These features enable us to obtain meaningful information about chemical bonding in various bulk samples. The SXES can detect Li-K emission spectrum. In the case of an anode electrode of a lithium ion battery (LIB), two types of lithium peaks are observed: one lower energy peak at 50 eV and the other higher energy peak at 54 eV. It was found that the former peak corresponds to the amount of charging, whereas the latter corresponds to the metallic state of lithium.
Tomita, Takuro*; Nishikino, Masaharu; Hasegawa, Noboru; Minami, Yasuo*; Takei, Ryota*; Baba, Motoyoshi*; Eyama, Tsuyoshi*; Takayoshi, Shodai*; Kaihori, Takeshi*; Morita, Toshimasa; et al.
Journal of Laser Micro/Nanoengineering, 9(2), p.137 - 142, 2014/06
Femtosecond laser ablation processes on platinum, gold, and tungsten were observed by the single shot pump and probe reflective imaging using a soft X-ray laser probe. To avoid the timing error due to the jitter, we adopted a posteriori correction technique by simultaneous measurement of timing between the pump and probe pulses for every single shot, using a soft X-ray streak camera. A clear difference was found in the temporal behavior of the dynamical response of the soft X-ray reflectivity depending on the irradiated laser fluence in these three materials. On the other hand, the narrow dark rings were found in Pt and W, while an additional bright ring was found outside the dark disk in Au. Our result gives the experimental data comparable with various numerical simulations.
Inogamov, N. A.*; Zhakhovsky, V. V.*; Ashitkov, S. I.*; Emirov, Y. N.*; Faenov, A. Y.*; Pikuz, T. A.*; Ishino, Masahiko; Kando, Masaki; Hasegawa, Noboru; Nishikino, Masaharu; et al.
Journal of Physics; Conference Series, 500(11), p.112070_1 - 112070_6, 2014/05
The mechanism of formation and geometry of surface structures are discussed for the case of single pulse acting on a well-polished metal surface. We demonstrate that the complex surface nano-structures are formed after laser irradiation due to the thermomechanical spallation of ultrathin surface layer of melt. Spallation is accompanied by a strong foaming of melt followed by breaking of the foam. After several nanoseconds the foam remnants freeze up with formation of complex nano-structures on a target surface.