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川崎 卓郎; 福田 竜生; 山中 暁*; 村山 一郎*; 加藤 孝典*; 馬場 将亮*; 橋本 英樹*; Harjo, S.; 相澤 一也; 田中 裕久*; et al.
Journal of Applied Physics, 137(9), p.094101_1 - 094101_7, 2025/03
被引用回数：0 パーセンタイル：0.00(Physics, Applied)Energy harvesting from waste heat can improve energy efficiency in society. This research investigated the structural behaviors of lead zirconate titanate-based ferroelectric ceramics using operando neutron diffraction measurements under the conditions of two energy-harvesting cycles that involve consideration of the temperature changes of automobile exhaust gas for achieving good harvesting efficiencies. Input and output electrical energies and neutron diffraction data were simultaneously collected. The obtained time-resolved neutron-diffraction intensity data indicate that the applied electric fields and temperature changes induced 90
domain rotation and lattice strain. These structural changes and their variations depending on cycle conditions, such as temperature changes, applied electric fields, and circuit switching, provide insight into the origins of the differences in the behaviors of electrical input/output energies in the cycles.
photoproduction on the proton at 
= 1.3-2.4 GeV橋本 敏和*; 土川 雄介; LEPS BGOegg Collaboration*; 他58名*
Physical Review C, 106(3), p.035201_1 - 035201_15, 2022/09
被引用回数：5 パーセンタイル：60.14(Physics, Nuclear)We report exclusive measurements for the photoproduction on a proton target. The differential cross sections and photon beam asymmetries of the 
reaction are measured in a center-of-mass energy (
) range of 1.82-2.32 GeV and a polar angle range of 
by using a large acceptance calorimeter (BGOegg) and forward-angle charged-particle detectors at the SPring-8 LEPS2 beamline. The reaction is identified with a kinematic fitting method to select a recoil proton and two photons produced in an meson decay. A bump structure at W = 2.0-2.3 GeV in the differential cross section is confirmed at extremely backward polar angles, where the existing data are inconsistent with each other. This bump structure is likely associated with high-spin resonances that couple with 
quarks. The photon beam asymmetries in a wide polar angle range for the photon beam energies above 2.1 GeV are reported for the first time, providing an additional constraint to nucleon resonance studies at high energies.
structure observation of pyroelectric ceramics during power generation cycle川崎 卓郎; 福田 竜生; 山中 暁*; 坂本 友和*; 村山 一郎*; 加藤 孝典*; 馬場 将亮*; 橋本 英樹*; Harjo, S.; 相澤 一也; et al.
Journal of Applied Physics, 131(13), p.134103_1 - 134103_7, 2022/04
被引用回数：2 パーセンタイル：15.59(Physics, Applied)The microscopic origin of the pyroelectric power generation using ferroelectric ceramics for energy harvesting from time-varying waste heat can be understood by conducting 
neutron diffraction measurements. The behavior of the domain orientation and lattice strain in the lead zirconate titanate (PZT)-based ceramics with a tetragonal structure during the novel power generation cycle combining electric field and temperature change were investigated. The [001] domains and the lattice strain of the (111) plane in the direction of parallel to the electric field increase in the process of simultaneous rise in the electric field and temperature, and rapidly decrease in the process of the field drop. The alignment of the domain orientation by the electric field and its randomization by the higher temperature during the cycle are critical features of the current power generation system.
-state of a 
hypernucleus, 
吉本 雅浩*; 藤田 真奈美; 橋本 直; 早川 修平; 市川 裕大; 市川 真也; 今井 憲一*; 七村 拓野; 成木 恵; 佐甲 博之; et al.
Progress of Theoretical and Experimental Physics (Internet), 2021(7), p.073D02_1 - 073D02_19, 2021/07
被引用回数：21 パーセンタイル：81.08(Physics, Multidisciplinary)Bound-systems of 
-
are studied via capture at rest followed by emission of a twin single-
hypernucleus in the emulsion detectors. Two events forming extremely deep bound states were obtained by analysis of a hybrid method in the E07 experiment at J-PARC and reanalysis of the E373 experiment at KEK-PS. The decay mode of one event was assigned as 
+
+
+
. Since there are no excited states for daughter particles, the binding energy of the hyperon, 
, in nucleus was uniquely determined to be 6.27 
0.27 MeV. Another - system via the decay 
+ + brings a value, 8.00 0.77 MeV or 4.96 0.77 MeV, where the two possible values of correspond to the ground and the excited states of the daughter nucleus, respectively. Because the values are larger than those of the previously reported events (KISO and IBUKI), which are both interpreted as the nuclear 
state of the - system, these new events give the first indication of the nuclear 
state of the hypernucleus, .
吉田 純也; 赤石 貴也; 藤田 真奈美; 長谷川 勝一; 橋本 直; 細見 健二; 市川 真也; 市川 裕大; 今井 憲一*; Kim, S.; et al.
JPS Conference Proceedings (Internet), 33, p.011112_1 - 011112_8, 2021/03
J-PARC E07 is the most ambitious and complex emulsion experiment to date investigating double hypernuclei with Hybrid emulsion method. The physics run at the K1.8 beam line in the J-PARC hadron experimental facility have been completed in 2017. The emulsion sheets are presently being analyzed with dedicated optical microscopes. Current statistics are estimated to be more 3 times than that of previous experiments. Quantitative data on the 
and 
interaction are being accumulated successfully via analysis of double and hypernuclei. Multiple hypernucleus candidates suggests several features about hypernucleus that the identification efficiency of 
C is significantly higher than other mode, many daughters of C are identified as He or Be, and multiple bound states of exist in the 
N nucleus. An analysis of X-ray spectroscopy of hyperatoms are ongoing.
-N system早川 修平; 藤田 真奈美; 長谷川 勝一; 橋本 直; 細見 健二; 市川 裕大; 今井 憲一*; 七村 拓野; 成木 恵; 佐甲 博之; et al.
Physical Review Letters, 126(6), p.062501_1 - 062501_6, 2021/02
被引用回数：45 パーセンタイル：93.51(Physics, Multidisciplinary)In an emulsion-counter hybrid experiment performed at J-PARC, a absorption event was observed which decayed into twin single- hypernuclei. Kinematic calculations enabled a unique identification of the reaction process as 
N
Be + 
He. For the binding energy of the 
hyperon in the -N system a value of 
MeV was deduced. The energy level of is likely a nuclear state which indicates a weak 
-
coupling.
scattering length from 
photoproduction on the proton near the reaction threshold石川 貴嗣*; 藤村 寿子*; 深澤 宏司*; 橋本 亮*; He, Q.*; 本多 佑記*; 保坂 淳; 岩田 高広*; 甲斐田 俊*; 笠木 治郎太*; et al.
Physical Review C, 101(5), p.052201_1 - 052201_6, 2020/05
被引用回数：4 パーセンタイル：36.67(Physics, Nuclear)Photoproduction of the omega meson on the proton has been experimentally studied near the threshold. The total cross sections are determined at incident energies ranging from 1.09 to 1.15 GeV. The 1/2 and 3/2 spin-averaged scattering length 
and effective range 
between the CO meson and proton are estimated from the shape of the total cross section as a function of the incident photon energy: = (-0.97 
+ 
(0.07 
) fm and = (+2.78 
) + (-0.01 
) fm, resulting in a repulsive force. The real and imaginary parts for and are determined separately for the first time. A small 
-wave contribution does not affect the obtained values.
Kim, J.*; 山中 暁*; 村山 一郎*; 加藤 孝典*; 坂本 友和*; 川崎 卓郎; 福田 竜生; 関野 徹*; 中山 忠親*; 武田 雅敏*; et al.
Sustainable Energy & Fuels (Internet), 4(3), p.1143 - 1149, 2020/03
被引用回数：22 パーセンタイル：63.45(Chemistry, Physical)Waste heat is a potentially exploitable energy source but remains a problem awaiting a solution. To explore solutions for automobile applications, we investigate pyroelectric power generation from the temperature variation of exhaust gas using a novel electro-thermodynamic cycle. Niobium-doped lead zirconate titanate stannate (PNZST) ceramics were applied as pyroelectric materials, and their structural characteristics were investigated. In the driving cycle assessments (JC-08) using real exhaust gas, the maximum power generated was identified as 143.9 mW cm
(777.3 J L
per 1 cycle) over a temperature range of 150-220 C and an electric field of 13 kV cm-1. The net mean generating power of the total driving cycle was 40.8 mW cm, which is the most enhanced result in our power generating systems to date and 314 times greater than our first report. Materials with sharp transition behaviors with the temperature and electric field are worthy of study with regard to pyroelectric energy harvesting materials, and their corresponding crystal and domain structures were investigated to optimize performance.
江川 弘行; 足利 沙希子; 長谷川 勝一; 橋本 直; 早川 修平; 細見 健二; 市川 裕大; 今井 憲一; 金原 慎二*; 七村 拓野; et al.
Progress of Theoretical and Experimental Physics (Internet), 2019(2), p.021D02_1 - 021D02_11, 2019/02
被引用回数：31 パーセンタイル：82.94(Physics, Multidisciplinary)A double- hypernucleus, 
, was observed by the J-PARC E07 collaborationin nuclear emulsions tagged by the 
reaction. This event was interpreted as a production and decay of 
,
, or 
via capture in 
.By assuming the capture in the atomic 3D state, the binding energy of two hyperons
(
)of these double- hypernuclei are obtained to be
, 
, and 
, respectively. Based on the kinematic fitting, is the most likely explanation for the observed event.
佐藤 聡*; 今野 力; 中島 宏; 塩永 亮介*; 野瀬 裕之*; 伊藤 祐二*; 橋本 博英*
Journal of Nuclear Science and Technology, 55(4), p.410 - 417, 2018/04
被引用回数：1 パーセンタイル：9.77(Nuclear Science & Technology)中性子遮蔽性能の向上を目的に、ホウ素を重量濃度で10%以上含有するボロンコンクリートを新たに開発した。原子力機構FNSのDT中性子源と新たに開発したボロン含有コンクリートを用いて中性子遮蔽実験を実施し、
Nb(n,2n)
Nb及び
Au(n,
)
Au反応の反応率を測定した。この実験の解析をMCNP及びFENDL-2.1を用いて行った。計算値は実験値とよく一致し、ボロン含有コンクリートの原子組成データとその核データの精度は非常に良いことを確認した。加えて、ボロン含有コンクリート及びその他のコンクリート中の実効線量率及び
Co(n,)
Co及び
Eu(n,)
Eu反応の反応率を計算した。今回開発したボロン含有コンクリートは、他のコンクリートと比べ、DT中性子に対し非常に良い遮蔽性能を有していることがわかった。
Tc-radiopharmaceuticals obtained from 
Mo produced by 
Mo(n,2n)Mo and fission of 
U橋本 和幸; 永井 泰樹; 川端 方子; 佐藤 望*; 初川 雄一; 佐伯 秀也; 本石 章司*; 太田 雅之; 今野 力; 落合 謙太郎; et al.
Journal of the Physical Society of Japan, 84(4), p.043202_1 - 043202_4, 2015/04
被引用回数：8 パーセンタイル：50.77(Physics, Multidisciplinary)The distribution of Tc-radiopharmaceutical in mouse was obtained with SPECT for the first time using Tc, which was separated by thermochromatography from Mo produced via the Mo(n,2n)Mo reaction with accelerator neutrons. The SPECT image was comparable with that obtained from a fission product Mo. Radionuclidic purity and radiochemical purity of the separated Tc and its aluminum concentration met the United States Pharmacopeia regulatory requirements for Tc from the fission product Mo. These results provide important evidence that Tc radiopharmaceutical formulated using the 
Mo can be a promising substitute for the fission product Mo. A current and forthcoming problem to ensure a reliable and constant supply of Mo in Japan can be partially mitigated.
Si利根川 翔*; 橋本 顕一郎*; 井加田 洸輔*; 鶴原 悠悟*; Lin, Y.-H.*; 宍戸 寛明*; 芳賀 芳範; 松田 達磨; 山本 悦嗣; 大貫 惇睦; et al.
Physical Review B, 88(24), p.245131_1 - 245131_13, 2013/12
被引用回数：12 パーセンタイル：46.74(Materials Science, Multidisciplinary)Detailed analyses of the cyclotron resonance lines in a uranium compound URuSi are reported. The analyses of the resonance profiles reveals that the heavier branch of the split line has a larger scattering rate, providing evidence for the existence of hot-spot along the [110] direction. The result is consistent with the broken fourfold symmetry in the hidden-order phase.
Si利根川 翔*; 橋本 顕一郎*; 井加田 洸輔*; Lin, Y.-H.*; 宍戸 寛明*; 芳賀 芳範; 松田 達磨; 山本 悦嗣; 大貫 惇睦; 池田 浩章*; et al.
Physical Review Letters, 109(3), p.036401_1 - 036401_5, 2012/07
被引用回数：53 パーセンタイル：86.50(Physics, Multidisciplinary)First observation of cyclotron resonance in the hidden-order phase of ultra clean URuSi is reported. An anomalous splitting of the sharpest resonance line under in-plane magnetic field rotation was found. This is most naturally explained by the domain formation, which breaks the fourfold rotational symmetry of the underlying tetragonal lattice. The result is consistent with the "nematic" Fermi liquid state, in which itinerant electrons have unidirectional correlations.
平山 賀一*; 三原 基嗣*; 渡辺 裕*; Jeong, S. C.*; 宮武 宇也*; 百田 佐多夫*; 橋本 尚志*; 今井 伸明*; 松多 健策*; 石山 博恒*; et al.
European Physical Journal A, 48(5), p.54_1 - 54_10, 2012/05
被引用回数：2 パーセンタイル：16.19(Physics, Nuclear)The tilted-foil method for producing spin-polarized radioactive isotope beams has been studied for the application to nuclear physics and materials science, using the radioactive nucleus 
Li produced at the Tokai Radioactive Ion Accelerator Complex (TRIAC). We successfully produced polarization in a Li beam using 15 thin polystyrene foils fabricated especially for this purpose. A systematic study of the nuclear polarization as a function of the number of foils, beam energy, tilt angles and foil material has been performed, confirming the features of the tilted-foil technique experimentally. The contributions made to the nuclear polarization of Li nuclei by the atomic states was investigated.
初川 雄一; 永井 泰樹; 金 政浩; 瀬川 麻里子; 原田 秀郎; 岩本 修; 岩本 信之; 落合 謙太郎; 高倉 耕祐; 今野 力; et al.
Proceedings in Radiochemistry, 1(1), p.327 - 329, 2011/09
核医学において最もよく用いられているTcの供給は危機に面しており、新たな製造プロセスの開発は喫緊の問題である。本研究は
TcをFNSより発生される14MeV高速中性子を用いて効率よく製造することを提案するものであり、試験的に作成したチタン酸ゲルを用いたTc/Moジェネレータについても併せて発表を行う。
Tc-MDP using Tc separated from Mo produced by Mo(
,2)Mo永井 泰樹; 初川 雄一; 金 政浩; 橋本 和幸; 本石 章司; 今野 力; 落合 謙太郎; 高倉 耕祐; 佐藤 裕一*; 河内 幸正*; et al.
Journal of the Physical Society of Japan, 80(8), p.083201_1 - 083201_4, 2011/08
被引用回数：15 パーセンタイル：64.17(Physics, Multidisciplinary)加速器で生成される中性子を酸化モリブデン100に照射して、Mo(,2)Mo反応で生成したMoから放射性の不純物を除去してTcを分離抽出すること、そして、Tc-MDP標識化合物を合成することに、世界で初めて成功した。親核のMoは、原子力機構の核融合中性子源施設で、トリチウムに重陽子を照射して得られる14MeVの中性子を用いて、Mo(,2)Mo反応で生成した。そして、Tcは、昇華法でMoから分離抽出し、その放射核純度は、99.99%以上であることを、分光で確認した。また、Tc-MDP標識率は、99%以上であることを、薄膜クロマト法で確かめた。これらの値は、米国薬局方が高濃縮ウランの核分裂反応で生成されるMoに対する要請値を超えるものである。そのため、本方法で生成するMoは、核分裂法の代替えとして有効であり、我が国の安定かつ信頼性の高いMo供給に寄与するであろう。
Li, T.*; Garg, U.*; Liu, Y.*; Marks, R.*; Nayak, B. K.*; Madhusudhana Rao, P. V.*; 藤原 守*; 橋本 尚信*; 中西 康介*; 奥村 瞬*; et al.
Physical Review C, 81(3), p.034309_1 - 034309_11, 2010/03
被引用回数：118 パーセンタイル：97.60(Physics, Nuclear)We have investigated the isoscalar giant resonances in the Sn isotopes using inelastic scattering of 386-MeV 
particles at extremely forward angles, including 0. The strength distributions for various multipoles were extracted by a multipole decomposition analysis based on the expected angular distributions of the respective multipoles. We find that the centroid energies of the isoscalar giant monopole resonance (ISGMR) in the Sn isotopes are significantly lower than the theoretical predictions. In addition, the asymmetry term, 
, in the expression for the nuclear incompressibility has been determined from the ISGMR data in Sn isotopes and is found to be consistent with a number of indirectly extracted values for this parameter.
Li(d,t)
Li reaction橋本 尚志; 石山 博恒*; 渡辺 裕*; 平山 賀一*; 今井 伸明*; 宮武 宇也; Jeong, S.-C.*; 田中 雅彦*; 吉川 宣治*; 野村 亨*; et al.
Physics Letters B, 674(4-5), p.276 - 280, 2009/04
被引用回数：7 パーセンタイル：46.18(Astronomy & Astrophysics)Li(d,t)Li反応の反応断面積を重心系で1.2から0.3MeVのエネルギーで7点直接測定した。これらのエネルギーは1
3
10
Kのガモフピーク領域をカバーする。重心系で0.8MeVのエネルギーで断面積の増大が観測され、これは複合核である
Beの22.4MeVの励起状態の寄与によると考えられる。また、この寄与によって天体核反応率は110Kで従来用いられていた値よりも1桁大きいことが明らかとなった。
塚田 和明; 羽場 宏光*; 浅井 雅人; 豊嶋 厚史; 秋山 和彦*; 笠松 良崇; 西中 一朗; 市川 進一; 安田 健一郎; 宮本 ユタカ; et al.
Radiochimica Acta, 97(2), p.83 - 89, 2009/02
被引用回数：22 パーセンタイル：78.82(Chemistry, Inorganic & Nuclear)105番元素ドブニウム(Db)及び周期表上同族の5族元素ニオブ(Nb),タンタル(Ta),擬5族のプロトアクチニウム(Pa)のフッ化水素酸水溶液中における陰イオン交換挙動を観測した。実験にはタンデム加速器施設に設置したオンライン自動迅速イオン交換分離装置を利用し、
Cm+
F反応で生成する
Db(半減期34秒)を対象に13.9Mフッ化水素酸水溶液におけるイオン交換樹脂への分配係数を測定した。上記元素とDbの溶離挙動を比較すると、Dbの分配係数は5族元素Nb及びTaに比べて小さく、その傾向はむしろ擬5族のPaに近いという結果を得た。この結果は超アクチノイド元素であるDbのフッ化物陰イオン錯体が同族元素と異なるという興味深いものである。
LiJeong, S.-C.*; 片山 一郎*; 川上 宏金*; 渡辺 裕*; 石山 博恒*; 今井 伸明*; 平山 賀一*; 宮武 宇也; 左高 正雄; 須貝 宏行; et al.
Japanese Journal of Applied Physics, 47(8), p.6413 - 6415, 2008/08
被引用回数：5 パーセンタイル：22.08(Physics, Applied)非破壊的方法によるリチウムイオン伝導体中でのオンライン拡散計測法を確立した。トレーサーとして、短寿命核Liのパルスビームを用い、LiGa中に注入した。インプラントされたLiからの粒子放出強度の時間依存性を調べることで精度の高いリチウムイオンの拡散測定が行える。今回の測定によりLiGaのリチウム欠乏
相中でのリチウム空孔の秩序化を、拡散係数の変化から初めて見いだすことができた。
