Initialising ...
Initialising ...
Initialising ...
Initialising ...
Initialising ...
Initialising ...
Initialising ...
Ru
As
( = Sm and Yb)廣瀬 雄介; 津久井 拓樹*; 加藤 佑汰*; 庄野 里菜*; 本多 史憲*; 青木 大*; 摂待 力生*
Physical Review Materials (Internet), 10(8), p.084407_1 - 084407_8, 2026/08
We investigated the electronic properties of RuAs ( = La, Ce, Sm, and Yb) using single-crystalline samples grown by the Bi-flux method. These compounds crystallize in the non-centrosymmetric hexagonal LaCoP -type structure, featuring both a chain and triangular arrangement of magnetic ions. From the electrical resistivity, magnetic susceptibility, and specific heat measurements, we have found that SmRuAs 
As order antiferromagnetically below the N
el temperature of 1.5 and 9.5~K, respectively. Despite the relatively high transition temperature of YbRuAs, its magnetic field-temperature phase diagram reveals that the antiferromagnetic state collapses at a low field of 
~=~1.7~T, accompanied by a non-linear magnetization anomaly. The magnetization curve is similar to that of chiral helical magnets. The small critical field and characteristic magnetization curve in YbRuAs likely originate from magnetic frustration.
SO(OH)Prokhnenko, O.*; 金子 耕士; 田端 千紘; 赤木 満*; Lee, C.*; 山中 隆義*; 酒井 宏典; 廣瀬 雄介; Gazizulina, A.*; 常盤 欣文; et al.
Physical Review B, 114(1), p.014414_1 - 014414_13, 2026/07
We report a comprehensive study of spin-
quantum magnet brochantite, CuSO(OH), combining high-field thermodynamic measurements, polarized neutron diffraction, inelastic neutron scattering, and nuclear magnetic resonance spectroscopy. Using bulk magnetization and specific heat measurements we construct the magnetic 
-
phase diagram for magnetic fields applied along main crystallographic directions. Polarized neutron diffraction reveals a noncollinear magnetic ground state confined to the ab plane. A field-induced transition is observed for magnetic fields in the ab plane whose critical field and character evolve continuously with field direction in the ab plane. The experimental results demonstrate that the ground-state and field-induced phases cannot be explained by a simple XXZ model with a single dominant exchange interaction and that weaker interchain and anisotropic interactions have to be taken into account. Our work establishes brochantite as a low-symmetry Cu-based quantum magnet with noncollinear order and complex field-induced behavior.
Cd
廣瀬 雄介; 土塔 寛*; 竹内 徹也*; 三宅 厚志*; 徳永 将史*; 仲村 愛*; 本間 佳哉*; 青木 大*; 本多 史憲*; 摂待 力生*
Journal of Physics; Condensed Matter, 38(24), p.245601_1 - 245601_11, 2026/06
被引用回数：0 パーセンタイル：0.00(Physics, Condensed Matter)The electronic state of UPdCd, which exhibits a magnetic transition at 
5 K, is investigated by means of transport, high-field magnetization up to 55 T, specific heat in magnetic fields, and de Haas-van Alphen (dHvA) measurements, and compared with the non-5f compound ThPdCd. A metamagnetic transition is observed at 
15-20 T, which continuously connects to in the H-T phase diagram. Although the magnetization reaches large values at high fields, the ordered magnetic moment is estimated to be small from small anomalies in specific heat at and in magnetization at 
. The observed dHvA frequencies reveal enhanced cyclotron effective masses of 30 
, which are much heavier than those in ThPdCd. These experimental results indicate that 5f-derived bands contribute to the large electronic specific heat coefficient of 670 mJ/mol K
, demonstrating the dual localized-itinerant character of 5f electrons in UPdCd.
Cd廣瀬 雄介; 本多 史憲*; 土塔 寛*; 河村 直己*; Kvashnina, K. O.*; Amidani, L.*; Uhl
ov
, K.*; Koloren
, J.*; Havela, L.*
Physical Review B, 113(24), p.L241103_1 - L241103_6, 2026/06
被引用回数：1 パーセンタイル：82.33(Materials Science, Multidisciplinary)The regime of valence fluctuations, known from anomalous rare-earth systems with slow fluctuations between two different fn states, has not yet been identified by microscopic techniques at any Uranium compound. The reason may be in the predominant band character of U intermetallic compounds. Here we present U-L3 and M4 X-ray absorption spectra taken on UPdCd, which is a heavy-Fermion antiferromagnet. Although it has only one type of U site, the spectra obtained in the High Energy Resolution Fluorescence Detection mode display two edges, each associated with different valence states, 5f2 and 5f3. This is strongly suggestive of slow f2 - f3 fluctuations on the timescale longer than the characteristic time of the spectroscopy technique. Unlike 4f systems in which such fluctuations lead to a destruction of magnetism due to involvement of one non-magnetic state, the f2 and f3 states in U are both possibly magnetic, allowing for the magnetic ordering in the fluctuating state. Such a new situation can bring more light into emergent phenomena observable in U systems at the verge of 5f localization.
In
( = Co, Rh, Ir)栗原 綾輔*; 廣瀬 雄介; 松井 一樹*; 三宅 厚志*; 角田 竜馬*; 近藤 雅起*; 摂待 力生*; 赤津 光洋*; 根本 祐一*; 矢口 宏*; et al.
JJAP Conference Proceedings (Internet), 12, p.011006_1 - 011006_6, 2026/02
強磁場における量子限界状態では、電子相関や電子格子相互作用に由来する新奇な電子状態が提案されている。本研究では、7Tという比較的低磁場で量子限界に達すると考えられているLaRhIn及び関連物質LaIn (T:遷移金属)を対象とし、強磁場での超音波測定を行った。音響ドハース振動から、先行研究と同様のLaRhInの小さなフェルミ面を観測し、T=CoおよびIrでも量子振動がみられこれまで観測されていなかった100T以下の小さなフェルミ面の存在を明らかにした。遷移金属の
電子が小さなフェルミ面への寄与を示唆する結果であった。
Ti
)
NiSe
土田 駿*; 廣瀬 雄介; 関川 卓也; 大野 義章*; 平原 卓也*; 佐野 純佳*; 河口 彰吾*; 小林 慎太郎*; 上床 美也*; 摂待 力生*
Journal of the Physical Society of Japan, 94(11), p.114703_1 - 114703_7, 2025/10
被引用回数：2 パーセンタイル：37.78(Physics, Multidisciplinary)本研究では、励起子絶縁体TaNiSeへのキャリアドープ効果を調べるために、(TaTi)NiSeの単結晶合成し、電気抵抗
ホール係数
およびバンド計算を行った。TaサイトのTi元素置換により、結晶構造は変化せず励起子絶縁体転移温度
は連続的に抑制され
=0.104で83Kまで抑制された。置換量を増やしていくと、半導体的なやの低温での増大が著しく抑制され、
では金属的な振る舞いに変わることを見出し、励起子相関のある金属状態が実現されている可能性がある。この金属化はバンド計算により、キャリアドーピング効果によって説明できる。このキャリアドープ物質を加圧していくと、2.6GPa以上で超伝導となることを明らかにした。この圧力は母物質TaNiSeの圧力誘起超伝導が現れる8GPaよりもはるかに小さく、Ti置換によるキャリアドープが超伝導に有利に働いたと考えられる。
OProkhnenko, O.*; Nikitin, S. E.*; 金子 耕士; 田端 千紘; 廣瀬 雄介; 常盤 欣文; 芳賀 芳範; 藤田 全基; 野尻 浩之*; Anovitz, L. M.*; et al.
Physical Review B, 112(9), p.094402_1 - 094402_7, 2025/09
被引用回数：0 パーセンタイル：0.00(Materials Science, Multidisciplinary)The spin dynamics in the natural mineral aegirine, NaFeSiO, a member of the pyroxene family, was studied using elastic and inelastic neutron scattering. Magnetization and specific heat measurements as well as single-crystal neutron diffraction maps confirm two successive magnetic transitions at 8.8 and 5.8~K, consistent with previous studies. The observed spin-wave excitations emerge from the incommensurate magnetic Bragg peaks corresponding to the propagation vector 
, and extend up to energies of about 1.5 meV. In the low-temperature helical phase, the spin dynamics of the Fe
ions is well described by a simple linear spin-wave model. The observed excitations can be modeled using a spin Hamiltonian that includes three primary exchange interactions. Our results show that no single exchange interaction dominates the spin dynamics. The similar strengths of the intrachain and interchain couplings point to the fact that the magnetic interactions in aegirine are three-dimensional, rather than being confined along one direction. As a result, the system cannot be considered quasi-one-dimensional, as previously suggested, and calls for further investigations.
山岸 茂直*; 林田 健志*; 三澤 龍介*; 木村 健太*; 萩原 雅人; 村田 智城*; 廣瀬 左京*; 木村 剛*
Chemistry of Materials, 35(2), p.747 - 754, 2023/01
被引用回数：22 パーセンタイル：76.73(Chemistry, Physical)The so-called "ferroaxial transition" characterized by a rotational structural distortion that breaks a mirror symmetry has gained growing interest in terms of a new class of ferroic state in crystalline materials. RbFe(MoO
) which belongs to glaserite-type compounds, X□;1 Y□;2 [M(TO
], is one of the most representative materials showing a ferroaxial transition, i.e., ferroaxial materials. Considering a variety of glaserite-type compounds, we expect that they provide a good arena for ferroaxial materials. In this work, we explored new ferroaxial materials by formula-based screening using regular expression search and symmetry detection algorithm. As a result, we found that a glaserite-type compound, KZr(PO), is one of the promising candidates for ferroaxial materials. Experimentally, we demonstrate that KZr(P O) shows a ferroaxial transition at about 700 K, which is well explained by ab initio phonon calculations. The ferroaxial nature of KZr(PO) is further confirmed by the observation of its domain structures using a linear electrogyration effect, that is, optical rotation in proportion to an applied electric field. Our work provides an effective approach to exploring ferroaxial materials.
吉田 雅幸*; 西端 樹*; 松田 朋己*; 伊藤 佑介*; 杉田 直彦*; 城 鮎美*; 菖蒲 敬久; 荒河 一渡*; 廣瀬 明夫*; 佐野 智一*
Journal of Applied Physics, 132(7), p.075101_1 - 075101_9, 2022/08
被引用回数：16 パーセンタイル：70.35(Physics, Applied)This study aims to investigate the influence of the pulse duration on the mechanical properties and dislocation density of a aluminum alloy treated using dry laser peening. The results of the micro-Vickers hardness test, residual stress measurement, and dislocation density measurement demonstrate that over a pulse duration range of 180 fs to 10 ps, the maximum peening effects are achieved with a pulse duration of 1 ps. Moreover, the most significant dry laser peening effects are obtained by choosing a pulse duration that achieves a laser intensity that simultaneously generates the strongest shock pressure, suppresses optical nonlinear effects, and realizes the least thermal effects, which weaken the shock effects.
北里 宏平*; Milliken, R. E.*; 岩田 隆浩*; 安部 正真*; 大竹 真紀子*; 松浦 周二*; 高木 靖彦*; 中村 智樹*; 廣井 孝弘*; 松岡 萌*; et al.
Nature Astronomy (Internet), 5(3), p.246 - 250, 2021/03
被引用回数：66 パーセンタイル：95.03(Astronomy & Astrophysics)2019年4月「はやぶさ2」ミッションは、地球に近い炭素質の小惑星(162173)リュウグウの人工衝撃実験を成功させた。これは露出した地下物質を調査し、放射加熱の潜在的な影響をテストする機会を提供した。はやぶさ2の近赤外線分光器(NIRS3)によるリュウグウの地下物質の観測結果を報告する。発掘された材料の反射スペクトルは、表面で観測されたものと比較して、わずかに強くピークがシフトした水酸基(OH)の吸収を示す。これは、宇宙風化や放射加熱が最上部の表面で微妙なスペクトル変化を引き起こしたことを示している。ただし、このOH吸収の強度と形状は、表面と同様に、地下物質が300
Cを超える加熱を経験したことを示している。一方、熱物理モデリングでは、軌道長半径が0.344AUに減少しても、推定される掘削深度1mでは放射加熱によって温度が200Cを超えて上昇しないことが示されている。これは、リュウグウ母天体が放射加熱と衝撃加熱のいずれか、もしくは両方により熱変化が発生したという仮説を裏付けている。
佐々木 宏和*; 西久保 英郎*; 西田 真輔*; 山崎 悟志*; 中崎 竜介*; 磯松 岳己*; 湊 龍一郎*; 衣川 耕平*; 今村 明博*; 大友 晋哉*; et al.
古河電工時報, (138), p.2 - 10, 2019/02
電子顕微鏡や放射光等の先端解析技術は、試料の構造や化学状態について多くの有用な情報をもたらし、材料研究に欠かせないツールとなっている。本稿では、これらの先端解析技術の中から、電子線ホログラフィや放射光を用いたX線小角散乱法(SAXS)等の手法を中心に、材料研究への応用事例を紹介する。これらの手法を活用することにより、未知であった材料の本質を明らかにすることができ、新製品開発の指針を定める上で重要な知見を得ることができる。
Zn and UCoZn広瀬 雄介*; 竹内 徹也*; 本多 史憲*; 吉内 伸吾*; 萩原 政幸*; 山本 悦嗣; 芳賀 芳範; 摂待 力生*; 大貫 惇睦
Journal of the Physical Society of Japan, 84(7), p.074704_1 - 074704_10, 2015/07
被引用回数：8 パーセンタイル：49.22(Physics, Multidisciplinary)Magnetic phase diagram of two heavy fermion metamagnets UIrZn and UCoZn is investigated. UIrZn shows a reconstruction of the electronic states across the metamagnetic crossover. However, UCoZn shows a rather continuous evolution. The remarkable difference in both compounds can be accounted for by different degree of hybridization between 5
and ligand electrons.
Zn (T: Rh and Ir)本多 史憲*; 広瀬 雄介*; 三宅 厚志*; 水牧 仁一朗*; 河村 直己*; 筒井 智嗣*; 綿貫 徹; 渡辺 真仁*; 竹内 徹也*; 摂待 力生*; et al.
Journal of Physics; Conference Series, 592(1), p.012021_1 - 012021_5, 2015/03
被引用回数：3 パーセンタイル：68.71(Physics, Atomic, Molecular & Chemical)重い電子系化合物YbTZn(T: Rh and Ir)について、X線吸収分光法によりYb価数観察を行った。いずれの化合物でもYb価数は温度依存性を示し、約100K以下で冷却とともにYb価数が減少する変化が見られた。これは、同型化合物であるYbCoZnにおいて温度依存性が見られないこととは対照的な結果である。
Zn金子 耕士; Raymond, S.*; Ressouche, E.*; Lapertot, G.*; 竹内 徹也*; 広瀬 雄介*; 本多 史憲*; 大貫 惇睦
JPS Conference Proceedings (Internet), 3, p.011061_1 - 011061_5, 2014/06
YbCoZn has a heavy-fermion ground state with an enormously large Sommerfeld coefficient of 8 J/molK
, and that is sensitive to external fields. Whereas pressure induces antiferromagnetic order, magnetic field induces metamagnetic transitions around 0.5 T, and new ordered state appears above 6 T for 
. In order to get insights into electronic states and its magnetic field response, neutron scattering experiments on single crystalline samples were carried. In a field-induced phase, magnetic reflections were successfully observed, which has a different propagation vector to that of pressure induced phase. Inelastic neutron scattering probes a crystal-field excitation at a low excitation energy which overlaps to quasielastic response. The results suggest degenerated energy scale, and that leads to variety of external response in YbCoZn.
Zn (T: Co, Ir)広瀬 雄介*; 竹内 徹也*; 吉内 伸吾*; 山本 悦嗣; 芳賀 芳範; 摂待 力生*; 大貫 惇睦
JPS Conference Proceedings (Internet), 3, p.011056_1 - 011056_6, 2014/06
Transport properties of UTZn (T: Co, Ir) have been investigated by measuring Hall effect. Overall behavior is explained by the skew scattering on the impurity model at high temperatures and the periodic Anderson model at low temperatures. Rather complicated behavior was observed in UIrZn with ferromagnetic instability, implying the electronic modification under magnetic field.
and EuAl仲村 愛*; 平仲 裕一*; 辺土 正人*; 仲間 隆男*; 三浦 泰直*; 堤 泰樹*; 森 晶宣*; 石田 一裕*; 三田村 勝哉*; 広瀬 雄介*; et al.
JPS Conference Proceedings (Internet), 3, p.011012_1 - 011012_6, 2014/06
Two europium compounds with the same structure EuGa and EuAl have been investigated. The Fermi surfaces revealed experimentally show a peculiar feature: flat Fermi surface sheets appear parallel to the tetragonal [110] planes. Reflecting this, a charge density wave transition due to the nesting of Fermi surface sheets has been observed in EuAl.
仲村 愛*; 平仲 裕一*; 辺土 正人*; 仲間 隆男*; 立津 慶幸*; 眞榮平 孝裕*; 三浦 泰直*; 森 晶宣*; 堤 泰樹*; 広瀬 雄介*; et al.
Journal of the Physical Society of Japan, 82(12), p.124708_1 - 124708_6, 2013/12
被引用回数：23 パーセンタイル：71.15(Physics, Multidisciplinary)Fermi surfaces and magnetic properties of an antiferromagnet EuBi were investigated on a flux-grown single crystal. A critical magnetic field of 225 kOe where the magnetic moments are forced to align ferromagnetically was well explained by the magnetic exchange interaction based on a two-sublattice model. The Fermi surface characteristics are in agreement with the theoretical prediction indicating a fully magnetic divalent state in Eu atoms.
仲村 愛*; 平仲 裕一*; 辺土 正人*; 仲間 隆男*; 三浦 泰直*; 堤 泰樹*; 森 晶宣*; 石田 一裕*; 三田村 勝哉*; 広瀬 雄介*; et al.
Journal of the Physical Society of Japan, 82(10), p.104703_1 - 104703_10, 2013/10
被引用回数：46 パーセンタイル：84.31(Physics, Multidisciplinary)High quality single crystals of EuGa have been grown from Ga flux. Electrical resistivity, magnetic susceptibility, high-field magnetization, specific heat, thermoelectric power and de Haas-van Alphen effect were investigated. Antiferromagnetic transition due to divalent Eu atoms were observed at 16.5 K. A charge density wave transition was also found under high pressure accompanied by a Fermi surface reconstruction. These observations were fully accounted for by the Fermi surface topology and corresponding band calculations.
広瀬 雄介*; 吉内 伸吾*; 西村 尚人*; 阪口 準也*; 榎 健太郎*; 岩川 健*; 三浦 泰直*; 杉山 清寛*; 大貫 惇睦; 摂待 力生*; et al.
Journal of the Korean Physical Society, 62(12), p.1858 - 1861, 2013/06
被引用回数：0 パーセンタイル：0.00(Physics, Multidisciplinary)We succeeded in growing single crystals of YbTIn (T: Co, Rh, Ir), YbGa, YbTZn (T: Co, Rh, Ir), etc. The electronic and magnetic properties are clarified by measuring the electrical resistivity, magnetic susceptibility, magnetization, specific heat and de Haas-van Alphen effect.
and reference compound ThCd; Studied by the de Haas-van Alphen effect広瀬 雄介*; 三浦 泰直*; 堤 泰樹*; 吉内 伸吾*; 大家 政洋*; 杉山 清寛*; 竹内 徹也*; 山上 浩志*; 山本 悦嗣; 芳賀 芳範; et al.
Physica Status Solidi (B), 250(3), p.642 - 645, 2013/03
被引用回数：5 パーセンタイル：22.76(Physics, Condensed Matter)Electronic states of an antiferromagnet UCd and its reference compound ThCd were investigated by means of de Haas-van Alphen (dHvA) effect. From the cyclotron effective mass determined from the dHvA oscillation, the electronic specific heat of UCd was estimated as 100 mJ/Kmol, much smaller than 840 in the previous report. The result suggests that magnetic excitation contributes significantly to the specific heat.
