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Journal Articles

Polarized and unpolarized neutron scattering for magnetic materials at the triple-axis spectrometer PONTA in JRR-3

Nakajima, Taro*; Saito, Hiraku*; Kobayashi, Naoki*; Kawasaki, Takuro; Nakamura, Tatsuya; Furukawa, Hazuki*; Asai, Shinichiro*; Masuda, Takatsugu*

Journal of the Physical Society of Japan, 93(9), p.091002_1 - 091002_5, 2024/09

 Times Cited Count:0

Journal Articles

Lattice dynamics of CH(NH$$_{2}$$)$$_{2}$$PbI$$_{3}$$ and CH(NH$$_{2}$$)$$_{2}$$SnI$$_{3}$$ investigated by inelastic X-ray scattering and comparison of their elastic properties

Tamatsukuri, Hiromu; Murakami, Yoichi*; Saito, Noriko*; Ohashi, Naoki*; Tsutsui, Satoshi*

Physical Review B, 110(2), p.024301_1 - 024301_8, 2024/07

 Times Cited Count:0 Percentile:0.00(Materials Science, Multidisciplinary)

JAEA Reports

Differential pressure rise event for filters of HTTR primary helium gas circulators, 2; Investigation of filter deposits and recurrence prevention measures

Nemoto, Takahiro; Fujiwara, Yusuke; Arakawa, Ryoki; Choyama, Yuya; Nagasumi, Satoru; Hasegawa, Toshinari; Yokoyama, Keisuke; Watanabe, Masashi; Onishi, Takashi; Kawamoto, Taiki; et al.

JAEA-Technology 2024-003, 17 Pages, 2024/06

JAEA-Technology-2024-003.pdf:1.91MB

In order to investigate the cause of the increase in differential pressure in the primary helium circulator filter that occurred during the RS-14 cycle, a clogged filter was investigated. As a result of the investigation, deposits caused by silicone oil were confirmed on the surface of the filter element. These results revealed that the cause of filter clogging was silicone oil mixed into the primary system due to performance deterioration of the charcoal filter in the gas circulator of primary helium purification system. As a measure to prevent the recurrence of this event, in addition to the conventional management based on operating hours for replacing of charcoal filter in the gas circulator of primary helium purification system, we have established a new replacement plan for every three years.

Journal Articles

Adsorption behavior of platinum-group metals and Co-existing metal ions from simulated high-level liquid waste using HONTA and Crea impregnated adsorbent

Osawa, Naoki*; Kim, S.-Y.*; Kubota, Masahiko*; Wu, H.*; Watanabe, So; Ito, Tatsuya; Nagaishi, Ryuji

Nuclear Engineering and Technology, 56(3), p.812 - 818, 2024/03

 Times Cited Count:1 Percentile:82.00(Nuclear Science & Technology)

Journal Articles

Band gap formation in graphene by hybridization with Hex-Au(001) reconstructed surface

Terasawa, Tomoo; Matsunaga, Kazuya*; Hayashi, Naoki*; Ito, Takahiro*; Tanaka, Shinichiro*; Yasuda, Satoshi; Asaoka, Hidehito

Vacuum and Surface Science, 66(9), p.525 - 530, 2023/09

As Au (001) surfaces exhibit a quasi-one-dimensional corrugated structure, Hex-Au(001), its periodicity was predicted to change the electronic structure of graphene when graphene was grown on this surface. Furthermore, the hybridization between graphene and Au is known to introduce bandgap and spin polarization into graphene. Here, we report angle-resolved photoemission spectroscopy and density functional theory calculation of graphene on a Hex-Au(001) surface. A bandgap of 0.2 eV in the graphene Dirac cone was observed at the crossing point of the graphene Dirac cone and Au 6sp bands, indicating that the origin of the bandgap formation was the hybridization between the graphene Dirac cone and Au 6sp band. We discussed the hybridization mechanism and anticipated spin injection into the graphene Dirac cone.

JAEA Reports

Differential pressure rise event for filters of HTTR primary helium gas circulators, 1; Investigation of differential pressure rise event

Nemoto, Takahiro; Arakawa, Ryoki; Kawakami, Satoru; Nagasumi, Satoru; Yokoyama, Keisuke; Watanabe, Masashi; Onishi, Takashi; Kawamoto, Taiki; Furusawa, Takayuki; Inoi, Hiroyuki; et al.

JAEA-Technology 2023-005, 33 Pages, 2023/05

JAEA-Technology-2023-005.pdf:5.25MB

During shut down of the HTTR (High Temperature engineering Test Reactor) RS-14 cycle, an increasing trend of filter differential pressure for the helium gas circulator was observed. In order to investigate this phenomenon, the blower of the primary helium purification system was disassembled and inspected. As a result, it is clear that the silicon oil mist entered into the primary coolant due to the deterioration of the charcoal filter performance. The replacement and further investigation of the filter are planning to prevent the reoccurrence of the same phenomenon in the future.

Journal Articles

Band gap opening in graphene by hybridization with Au (001) reconstructed surfaces

Terasawa, Tomoo; Matsunaga, Kazuya*; Hayashi, Naoki*; Ito, Takahiro*; Tanaka, Shinichiro*; Yasuda, Satoshi; Asaoka, Hidehito

Physical Review Materials (Internet), 7(1), p.014002_1 - 014002_10, 2023/01

 Times Cited Count:7 Percentile:79.50(Materials Science, Multidisciplinary)

Au(001) surfaces exhibit a complex reconstructed structure [Hex-Au(001)] comprising a hexagonal surface and square bulk lattices, yielding a quasi-one-dimensional corrugated surface. When graphene was grown on this surface, the periodicity of the corrugated surface was predicted to change the electronic structure of graphene, forming bandgaps and new Dirac points. Furthermore, the graphene-Au interface is promising for bandgap generation and spin injection due to band hybridization. Here, we report the angle-resolved photoemission spectroscopy and density functional calculation of graphene on a Hex-Au(001) surface. The crossing point of the original and replica graphene $$pi$$ bands showed no bandgap, suggesting that the one-dimensional potential was too small to modify the electronic structure. A bandgap of 0.2 eV was observed at the crossing point of the graphene $$pi$$ and Au $$6sp$$ bands, indicating that the bandgap is generated using hybridization of the graphene $$pi$$ and Au $$6sp$$ bands. We discussed the hybridization mechanism and concluded that the R30 configuration between graphene and Au and an isolated electronic structure of Au are essential for effective hybridization between graphene and Au. We anticipate that hybridization between graphene $$pi$$ and Au $$6sp$$ would result in spin injection into graphene.

Journal Articles

Design and actual performance of J-PARC 3 GeV rapid cycling synchrotron for high-intensity operation

Yamamoto, Kazami; Kinsho, Michikazu; Hayashi, Naoki; Saha, P. K.; Tamura, Fumihiko; Yamamoto, Masanobu; Tani, Norio; Takayanagi, Tomohiro; Kamiya, Junichiro; Shobuda, Yoshihiro; et al.

Journal of Nuclear Science and Technology, 59(9), p.1174 - 1205, 2022/09

 Times Cited Count:7 Percentile:72.25(Nuclear Science & Technology)

In the Japan Proton Accelerator Research Complex, the purpose of the 3 GeV rapid cycling synchrotron (RCS) is to accelerate a 1 MW, high-intensity proton beam. To achieve beam operation at a repetition rate of 25 Hz at high intensities, the RCS was elaborately designed. After starting the RCS operation, we carefully verified the validity of its design and made certain improvements to establish a reliable operation at higher power as possible. Consequently, we demonstrated beam operation at a high power, namely, 1 MW. We then summarized the design, actual performance, and improvements of the RCS to achieve a 1 MW beam.

Journal Articles

Improving the safety of the high temperature gas-cooled reactor "HTTR" based on Japan's new regulatory requirements

Hamamoto, Shimpei; Shimizu, Atsushi; Inoi, Hiroyuki; Tochio, Daisuke; Homma, Fumitaka; Sawahata, Hiroaki; Sekita, Kenji; Watanabe, Shuji; Furusawa, Takayuki; Iigaki, Kazuhiko; et al.

Nuclear Engineering and Design, 388, p.111642_1 - 111642_11, 2022/03

 Times Cited Count:3 Percentile:52.93(Nuclear Science & Technology)

Following the Fukushima Daiichi Nuclear Power Plant accident in 2011, the Japan Atomic Energy Agency adapted High-Temperature engineering Test Reactor (HTTR) to meet the new regulatory requirements that began in December 2013. The safety and seismic classifications of the existing structures, systems, and components were discussed to reflect insights regarding High Temperature Gas-cooled Reactors (HTGRs) that were acquired through various HTTR safety tests. Structures, systems, and components that are subject to protection have been defined, and countermeasures to manage internal and external hazards that affect safety functions have been strengthened. Additionally, measures are in place to control accidents that may cause large amounts of radioactive material to be released, as a beyond design based accident. The Nuclear Regulatory Commission rigorously and appropriately reviewed this approach for compliance with the new regulatory requirements. After nine amendments, the application to modify the HTTR's installation license that was submitted in November 2014 was approved in June 2020. This response shows that facilities can reasonably be designed to meet the enhanced regulatory requirements, if they reflect the characteristics of HTGRs. We believe that we have established a reference for future development of HTGR.

Journal Articles

"Live-autoradiography" technique reveals genetic variation in the rate of Fe uptake by barley cultivars

Higuchi, Kyoko*; Kurita, Keisuke; Sakai, Takuro; Suzui, Nobuo*; Sasaki, Minori*; Katori, Maya*; Wakabayashi, Yuna*; Majima, Yuta*; Saito, Akihiro*; Oyama, Takuji*; et al.

Plants (Internet), 11(6), p.817_1 - 817_11, 2022/03

 Times Cited Count:2 Percentile:24.37(Plant Sciences)

Genetic diversity in the rate of Fe uptake by plants has not been broadly surveyed among plant species or genotypes, although plants have developed various Fe acquisition mechanisms. We adopted the "Live-autoradiography" technique with radioactive $$^{59}$$Fe to directly evaluate the uptake rate of Fe by barley cultivars from a nutrient solution containing a very low concentration of Fe. Our observations revealed that the ability to acquire Fe from the low Fe solution was not always the sole determinant of tolerance to Fe deficiency among the barley genotypes.

Journal Articles

Extraction behavior of a novel functionalized ionic liquid for separation of platinum group metals from aqueous nitric acid solution

Ito, Tatsuya; Osugi, Haruka*; Osawa, Naoki*; Takahashi, Tadayuki*; Kim, S.-Y.*; Nagaishi, Ryuji

Analytical Sciences, 38(1), p.91 - 97, 2022/01

 Times Cited Count:3 Percentile:19.70(Chemistry, Analytical)

A novel ionic liquid (IL) functionalized with thiodiglycol amic acid containing a soft S donor was synthesized for the effective and efficient extraction of platinum group metals (Ru, Rh, and Pd) from aqueous nitric acid solutions, such as high-level radioactive liquid waste (HLLW). The IL allowed a rapid extraction of Pd(II) with an extraction ratio of approximately 100%. The extractions of Ru(III) and Rh(III) by the IL were slower than that of Pd(II), but the rates were accelerated by temperature elevation. The extractions of Ru(III) and Rh(III) at 50$$^{circ}$$C reached equilibrium within 4 and 8 h, respectively, with the extraction ratios of over 90% without assisting agents or other methods for the extraction system. Furthermore, the IL could extract more than 90% of Ru(III), Rh(III), and Pd(II) from the simulated HLLW within 2 h at 50$$^{circ}$$C.

Journal Articles

Review of engagement activities to promote awareness of radiation and its associated risk amongst the Japanese public before and after the Fukushima Daiichi Nuclear Power Plant accident

Sakoda, Akihiro; Nomura, Naoki*; Kuroda, Yujiro*; Kono, Takahiko; Naito, Wataru*; Yoshida, Hiroko*

Journal of Radiological Protection, 41(4), p.1258 - 1287, 2021/12

 Times Cited Count:1 Percentile:8.38(Environmental Sciences)

Following the Fukushima Daiichi Nuclear Power Plant accident, many radiation experts directly experienced a vast gap between ideal and real public understanding (PU) of radiation in risk communication. Therefore, this study collated and reviewed information about PU activities for radiation and its risk that six Japanese academic societies - which seemed to be socially neutral expert communities - related to radiation and radiation risk conducted before and after the accident. Activities these radiation-related societies provided to general public were discussed from the following perspectives: (1) difficulties in two-way communication due to resources, motivation, public interest and concerns; (2) balance between academic research and PU activities; (3) academic societies' building trust with the public whilst ensuring member experts' neutrality and independence; (4) discussions among academic societies to prepare for public engagement. We hope that this paper encourages experts and academic societies in radiation protection to hold more national and international discussions about their roles in public communication and outreach.

Journal Articles

Development of next-generation timing system for the Japan Proton Accelerator Research Complex

Tamura, Fumihiko; Takahashi, Hiroki; Kamikubota, Norihiko*; Ito, Yuichi*; Hayashi, Naoki

IEEE Transactions on Nuclear Science, 68(8), p.2043 - 2050, 2021/08

 Times Cited Count:0 Percentile:0.00(Engineering, Electrical & Electronic)

A precise and stable timing system is necessary for high intensity proton accelerators such as the J-PARC. The existing timing system, which was developed during the construction period of the-PARC, has been working without major issues since 2006. After a decade of operation, the optical modules, which are key components for signal transfer, were discontinued already. Thus, the next-generation timing system for the J-PARC is under development. The new system is designed to be compatible with the existing system in terms of the operating principle. The new system utilizes modern high speed signal communication for the transfer of the clock, trigger, and type code. We present the system configuration of the next-generation timing system and current status.

JAEA Reports

Ocean current data obtained by Acoustic Doppler Current Profiler across the Tsugaru Strait (Joint research)

Kawamura, Hideyuki; Hirose, Naoki*; Nakayama, Tomoharu*; Ito, Toshimichi

JAEA-Data/Code 2021-004, 34 Pages, 2021/05

JAEA-Data-Code-2021-004.pdf:3.72MB

The Japan Atomic Energy Agency measured the ocean current across the Tsugaru Strait using an Acoustic Doppler Current Profiler attached on a ferryboat from October 1999 to January 2008. The characteristics of the ocean current in the Tsugaru Strait must be understood for predicting oceanic dispersion of radioactive materials released from nuclear facilities around the strait. Furthermore, it is critical to elucidate the mechanism of the Tsugaru Warm Current from an oceanography viewpoint. The dataset obtained in this investigation consists of daily ocean current data files that record the components of the current speed in the east-west and north-south directions from the surface layer to the bottom layer. The dataset stores 2,211 daily ocean current data files, despite some data periods missing from October 1999 to January 2008. In this study, information on the dataset is described for users to analyze the dataset properly for their purposes. Section 1 provides the background and purpose of the ocean current measurement, Section 2 explains the methodology of measurement using an Acoustic Doppler Current Profiler, and Section 3 explains the record format of the daily ocean current data files and data acquisition rate and presents analysis results. Finally, Section 4 concludes this study.

Journal Articles

Reliability of J-PARC accelerator system over the past decade

Yamamoto, Kazami; Hasegawa, Kazuo; Kinsho, Michikazu; Oguri, Hidetomo; Hayashi, Naoki; Yamazaki, Yoshio; Naito, Fujio*; Yoshii, Masahito*; Toyama, Takeshi*

JPS Conference Proceedings (Internet), 33, p.011016_1 - 011016_7, 2021/03

The Japan Proton Accelerator Research Complex (J-PARC) is a multipurpose facility for scientific experiments. The accelerator complex consists of a 400-MeV Linac, a 3-GeV Rapid-Cycling Synchrotron (RCS) and a 30-GeV Main Ring synchrotron (MR). The RCS delivers a proton beam to the neutron target and MR, and the MR delivers the beams to the neutrino target and the Hadron Experimental Facility. The first operation of the neutron experiments began in December 2008. Following this, the user operation has been continued with some accidental suspensions. These suspensions include the recovery work due to the Great East Japan Earthquake in March 2011 and the radiation leak incident at the Hadron Experimental Facility. In this report, we summarize the major causes of suspension, and the statistics of the reliability of J-PARC accelerator system is analyzed. Owing to our efforts to achieve higher reliability, the Mean Time Between Failure (MTBF) has been improved.

Journal Articles

Enhancement of element production by incomplete fusion reaction with weakly bound deuteron

Wang, H.*; Otsu, Hideaki*; Chiga, Nobuyuki*; Kawase, Shoichiro*; Takeuchi, Satoshi*; Sumikama, Toshiyuki*; Koyama, Shumpei*; Sakurai, Hiroyoshi*; Watanabe, Yukinobu*; Nakayama, Shinsuke; et al.

Communications Physics (Internet), 2(1), p.78_1 - 78_6, 2019/07

 Times Cited Count:9 Percentile:56.49(Physics, Multidisciplinary)

Searching for effective pathways for the production of proton- and neutron-rich isotopes through an optimal combination of reaction mechanism and energy is one of the main driving forces behind experimental and theoretical nuclear reaction studies as well as for practical applications in nuclear transmutation of radioactive waste. We report on a study on incomplete fusion induced by deuteron, which contains one proton and one neutron with a weak binding energy and is easily broken up. This reaction study was achieved by measuring directly the cross sections for both proton and deuteron for $$^{107}$$Pd at 50 MeV/u via inverse kinematics technique. The results provide direct experimental evidence for the onset of a cross-section enhancement at high energy, indicating the potential of incomplete fusion induced by loosely-bound nuclei for creating proton-rich isotopes and nuclear transmutation of radioactive waste.

Journal Articles

Status of J-PARC accelerators

Hasegawa, Kazuo; Kinsho, Michikazu; Oguri, Hidetomo; Yamamoto, Kazami; Hayashi, Naoki; Yamazaki, Yoshio; Naito, Fujio*; Yoshii, Masahito*; Toyama, Takeshi*; Yamamoto, Noboru*; et al.

Proceedings of 16th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.1235 - 1239, 2019/07

After the summer shutdown in 2018, the J-PARC restarted user operation in late October. While beam power to the Materials and Life Science Experimental Facility (MLF) was 500 kW as before the summer shutdown, linac beam current was increased from 40 to 50 mA. Operation of the Main Ring (MR) was suspended due to the modification and/or maintenance of the Superkamiokande (neutrino detector) and Hadron experimental facility. The user operation was resumed in the middle of February for the Hadron experimental facility at 51 kW. But on March 18, one of the bending magnets in the beam transport line to the MR had a failure. It was temporary recovered and restored beam operation on April 5, but the failure occurred again on April 24 and the beam operation of the MR was suspended. In the fiscal year of 2018, the availabilities for the MLF, neutrino and hadron facilities are 94%, 86%, and 74%, respectively.

Journal Articles

Next generation timing system for J-PARC

Tamura, Fumihiko; Takahashi, Hiroki; Kamikubota, Norihiko*; Ito, Yuichi; Hayashi, Naoki

Proceedings of 16th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.149 - 152, 2019/07

Precise timing pulses from the timing system are necessary for acceleration of high intensity proton beams in the J-PARC accelerators. The existing timing system was developed during the construction period of the J-PARC. The system has been working well for more than ten years, however, the optical modules for the signal transfer from the central control building to the accelerators are discontinued already. Although we have spares of the optical devices, maintenance of the system will be difficult. Therefore, we are developing the next generation timing system for the J-PARC. We present the design of the system, preliminary test results, and future plans.

Journal Articles

Status of J-PARC accelerators

Hasegawa, Kazuo; Kinsho, Michikazu; Oguri, Hidetomo; Yamamoto, Kazami; Hayashi, Naoki; Yamazaki, Yoshio; Naito, Fujio*; Yoshii, Masahito*; Yamamoto, Noboru*; Koseki, Tadashi*

Proceedings of 15th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.1317 - 1321, 2018/08

After the summer shutdown in 2017, the J-PARC restarted user operation in late October. The Materials and Life Science Experimental Facility (MLF) used a spare target and the beam power was limited to 150-200kW. The target was replaced with a new one in the summer shutdown. The beam power was for user operation gradually increased from 300 kW to 500 kW. We have successfully demonstrated 1MW 1hour operation in July 2018. The beam power for the neutrino experimental facility (NU) was 440 kW to 470 kW. The beam was delivered to the hadron experimental facility (HD) from January to February in 2018. The repetition rate of the main ring was shortened from 5.52 to 5.20 seconds, the beam power was increased from 44 to 50 kW. From March 2018, we delivered to the NU at 490 kW stably. In the fiscal year of 2017, the availabilities for the MLF, NU and HD are 93%, 89% and 66%, respectively.

Journal Articles

Estimation of mitigation effects of sodium nanofluid for SGTR accidents in SFR

Ichikawa, Kenta*; Kanda, Hironori; Yoshioka, Naoki*; Ara, Kuniaki; Saito, Junichi; Nagai, Keiichi

Proceedings of 26th International Conference on Nuclear Engineering (ICONE-26) (Internet), 6 Pages, 2018/07

Studies on the suppression of the reactivity of sodium itself have been performed on the basis of the concept of suspended nanoparticles in liquid sodium (sodium nanofluid). According to the experimental and theoretical results of studies for sodium nanofluid, velocity and heat of sodium nanofluid-water reaction are lower than those of the pure sodium-water reaction. The analytical model for the peak temperature of a sodium nanofluid-water reaction jet has been developed in consideration of these suppression effects by the authors. In this paper, the prediction method for mitigation effects for a damage of adjacent tubes in a steam generator tube rupture (SGTR) accidents is arranged by applying this analytical model for the peak temperature of the reaction jet. On the assumption that the sodium nanofluid is used for the secondary coolant of sodium-cooled fast reactor (SFR), mitigation effects under the design-base accident (DBA) condition and the design-extension condition (DEC) of SGTR are estimated by using this method. As a result, there is a possibility to reduce the number of damaged tubes and to suppress the pressure generated by SGTR accidents by using sodium nanofluid in the secondary coolant.

258 (Records 1-20 displayed on this page)