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Am
O
at 1473, 1573, and 1673 KWatanabe, Masashi; Yokoyama, Keisuke; Vauchy, R.; Kato, Masato; Sugata, Hiromasa*; Seki, Takayuki*; Hino, Tetsushi*
Journal of Nuclear Materials, 599, p.155232_1 - 155232_5, 2024/10
Oxygen potential data of UAmO
were measured at 1473, 1573, and 1673 K by thermogravimetry. In U
An
O, where An stands for Pu or Am, and for a given value of y and Oxygen/Metal ratio, the oxygen potential of UAmO is higher than that of UPuO. The valence of cations in the hypostoichiometric region is similar to that of Nd-doped UO. At the stoichiometric composition, it is estimated to be Am
, U
, and U
(for charge compensation of Am). The experimental data were analyzed using a defect chemistry model, and a relationship connecting the oxygen-to-metal ratio, the temperature, and the equilibrium oxygen partial pressure was proposed.
Horii, Yuta; Hirooka, Shun; Uno, Hiroki*; Ogasawara, Masahiro*; Tamura, Tetsuya*; Yamada, Tadahisa*; Furusawa, Naoya*; Murakami, Tatsutoshi; Kato, Masato
Journal of Nuclear Materials, 588, p.154799_1 - 154799_20, 2024/01
Times Cited Count：1 Percentile：63.33(Materials Science, Multidisciplinary)The thermal conductivities of near-stoichiometric (U,Pu,Am)O doped with NdO
/SmO, which is major fission product (FP) generated by a uranium-plutonium mixed oxides (MOX) fuel irradiation, as simulated fission products are evaluated at 1073-1673 K. The thermal conductivities are calculated from the thermal diffusivities that are measured using the laser flash method. To evaluate the thermal conductivity from a homogeneity viewpoint of Nd/Sm cations in MOX, the specimens with different homogeneity of Nd/Sm are prepared using two kinds of powder made by ball-mill and fusion methods. A homogeneous Nd/Sm distribution decreases the thermal conductivity of MOX with increasing Nd/Sm content, whereas heterogeneous Nd/Sm has no influence. The effect of Nd/Sm on the thermal conductivity is studied using the classical phonon transport model (A+BT)
. The dependences of the coefficients A and B on the Nd/Sm content (C
and C
, respectively) are evaluated as: A(mK/W)=1.70 
10
+ 0.93C + 1.20C, B(m/W)=2.39 10
.
mixed oxidesVauchy, R.; Matsumoto, Taku; Hirooka, Shun; Uno, Hiroki*; Tamura, Tetsuya*; Arima, Tatsumi*; Inagaki, Yaohiro*; Idemitsu, Kazuya*; Nakamura, Hiroki; Machida, Masahiko; et al.
Journal of Nuclear Materials, 588, p.154786_1 - 154786_13, 2024/01
Times Cited Count：1 Percentile：63.33(Materials Science, Multidisciplinary)Sato, Tetsuya*; Kato, Takeo*; Oue, Daigo*; Matsuo, Mamoru
Physical Review B, 107(18), p.L180406_1 - L180406_6, 2023/05
Times Cited Count：1 Percentile：44.21(Materials Science, Multidisciplinary)
Pu
Am
)O (z = 0.05, 0.10, and 0.15)Yokoyama, Keisuke; Watanabe, Masashi; Tokoro, Daishiro*; Sugimoto, Masatoshi*; Morimoto, Kyoichi; Kato, Masato; Hino, Tetsushi*
Nuclear Materials and Energy (Internet), 31, p.101156_1 - 101156_7, 2022/06
Times Cited Count：3 Percentile：63.91(Nuclear Science & Technology)In current nuclear fuel cycle systems, to reduce the amount of high-level radioactive waste, minor actinides (MAs) bearing MOX fuel is one option for burning MAs using fast reactor. However, the effects of Am content in fuel on thermal conductivity are unclear because there are no experimental data on thermal conductivity of high Am bearing MOX fuel. In this study, The thermal conductivities of near stoichiometric (UPuAm)O solid solutions(z = 0.05, 0.10, and 0.15) have been measured between room temperature (RT) and 1473 K. The thermal conductivities decreased with increasing Am content and satisfied the classical phonon transport model ((A+BT)) up to about 1473 K. A values increased linearly with increasing Am content because the change in ionic radius affects the conduction of the phonon due to the solid solution in U and Am. B values were independent of Am content.
Kato, Atsushi; Kubo, Shigenobu; Chikazawa, Yoshitaka; Miyagawa, Takayuki*; Uchita, Masato*; Suzuno, Tetsuji*; Endo, Junji*; Kubo, Koji*; Murakami, Hisatomo*; Uzawa, Masayuki*; et al.
Proceedings of International Conference on Fast Reactors and Related Fuel Cycles; Sustainable Clean Energy for the Future (FR22) (Internet), 11 Pages, 2022/04
The authors are carrying out conceptual design studies for a pool-type sodium-cooled fast reactor. There are main challenges such as measures against severe earthquake in Japan, thermal hydraulic in a reactor vessel (RV), a decay heat removal system design. When the JP-pool SFR of 650 MWe is installed in Japan, it shall be designed against the severe seismic conditions. Additionally, a newly three-dimensional seismic isolation system is under development.
Sato, Tetsuya*; Tatsuno, Masahiro*; Matsuo, Mamoru; Kato, Takeo*
Journal of Magnetism and Magnetic Materials, 546, p.168814_1 - 168814_6, 2022/03
Times Cited Count：0 Percentile：0.00(Materials Science, Multidisciplinary)Wei, D.*; Wang, L.*; Zhang, Y.*; Gong, W.; Tsuru, Tomohito; Lobzenko, I.; Jiang, J.*; Harjo, S.; Kawasaki, Takuro; Bae, J. W.*; et al.
Acta Materialia, 225, p.117571_1 - 117571_16, 2022/02
Times Cited Count：61 Percentile：99.71(Materials Science, Multidisciplinary)Kato, Tetsu*; Kawamura, Yamato*; Tahara, Junichiro*; Baba, Shoichiro*; Sanada, Yukihisa; Fujii, Shun*
International Journal of Offshore and Polar Engineering, 31(3), p.316 - 324, 2021/09
Times Cited Count：2 Percentile：19.12(Engineering, Civil)The development of a side thruster system (vehicle (ASV)) that can maintain the direction of travel on the autonomous surface will be explained. Currently, we are working on a mud radioactivity survey in collaboration with Japan Agency for Marine-Earth Science and Technology, Japan Atomic Energy Agency, and Tokyo University of Marine Science and Technology. Deposited at the mouth of Fukushima Prefecture, Japan, the main purpose is to collect unmanned mud using ASV. The Mad Collection has developed a side thruster system and implemented it in ASV. We have confirmed the operation of the ASV with the joystick by using the thruster system for operating the ASV by one person using the joystick.
Fujii, Shun*; Kato, Tetsu*; Kawamura, Yamato*; Tahara, Junichiro*; Baba, Shoichiro*; Sanada, Yukihisa
Proceedings of 26th International Symposium on Artificial Life and Robotics (AROB 26th 2021), p.280 - 285, 2021/01
In recent years, autonomously navigating unmanned vessels have been actively studied, and many of these vessels are designed to perform unmanned operations such as observation and transportation. On the other hand, this study uses an unmanned ship with a moon pool that collects seabed mud, which is difficult for ordinary ships. Vessels used since the area are highly turbulent due to wind, so it is necessary to maintain a fixed point and orientation when removing mud. The ship is equipped with side thrusters to maintain a fixed point and bow direction. In this study, the control method was devised to maintain fixed point and orientation, and the control method is based on robust sliding mode control. The proposed control method was verified by simulation, and the desired behavior was confirmed.
Kato, Tetsu*; Kawamura, Yamato*; Tahara, Junichiro*; Baba, Shoichiro*; Sanada, Yukihisa
Proceedings of the 30th (2020) International Ocean and Polar Engineering Conference (ISOPE 2020) (USB Flash Drive), p.1255 - 1260, 2020/10
AlGaO
scintillators by gamma-ray-induced positron annihilation lifetime spectroscopyFujimori, Kosuke*; Kitaura, Mamoru*; Taira, Yoshitaka*; Fujimoto, Masaki*; Zen, H.*; Watanabe, Shinta*; Kamada, Kei*; Okano, Yasuaki*; Kato, Masahiro*; Hosaka, Masahito*; et al.
Applied Physics Express, 13(8), p.085505_1 - 085505_4, 2020/08
Times Cited Count：5 Percentile：31.64(Physics, Applied)To clarify the existence of cation vacancies in Ce-doped GdAlGaO (Ce:GAGG) scintillators, we performed gamma-ray-induced positron annihilation lifetime spectroscopy (GiPALS). GiPAL spectra of GAGG and Ce:GAGG comprised two exponential decay components, which were assigned to positron annihilation at bulk and defect states. By an analogy with Ce:YAl
O, the defect-related component was attributed to Al/Ga-O divacancy complexes. This component was weaker for Ce, Mg:GAGG, which correlated with the suppression of shallow electron traps responsible for phosphorescence. Oxygen vacancies were charge compensators for Al/Ga vacancies. The lifetime of the defect-related component was significantly changed by Mg co-doping. This was understood by considering aggregates of Mg
ions at Al/Ga sites with oxygen vacancies, which resulted in the formation of vacancy clusters.
Saito, Kimiaki; Mikami, Satoshi; Ando, Masaki; Matsuda, Norihiro; Kinase, Sakae; Tsuda, Shuichi; Sato, Tetsuro*; Seki, Akiyuki; Sanada, Yukihisa; Wainwright-Murakami, Haruko*; et al.
Journal of Radiation Protection and Research, 44(4), p.128 - 148, 2019/12
Sakamoto, Tetsuo*; Morita, Masato*; Kanenari, Keita*; Tomita, Hideki*; Sonnenschein, V.*; Saito, Kosuke*; Ohashi, Masaya*; Kato, Kotaro*; Iguchi, Tetsuo*; Kawai, Toshihide*; et al.
Analytical Sciences, 34(11), p.1265 - 1270, 2018/11
Times Cited Count：8 Percentile：31.22(Chemistry, Analytical)Sato, Junya; Kikuchi, Hiroshi*; Kato, Jun; Sakakibara, Tetsuro; Matsushima, Ryotatsu; Sato, Fuminori; Kojima, Junji; Nakazawa, Osamu
QST-M-8; QST Takasaki Annual Report 2016, P. 62, 2018/03
no abstracts in English
Kato, Jun; Nakagawa, Akinori; Taniguchi, Takumi; Sakakibara, Tetsuro; Nakazawa, Osamu; Meguro, Yoshihiro
JAEA-Review 2017-015, 173 Pages, 2017/07
JAEA-Review-2017-015.pdf:6.67MB
Various radioactive wastes have been generated at the Fukushima Daiichi Nuclear Power Station (1F). To dispose of the wastes underground, it is necessary to make a suitable waste package by the volume reduction and solidification of the wastes. To plan the future decommissioning of 1F, it is also necessary to estimate feasibility of existing treatment technology for those wastes. Therefore the document survey has been performed about volume reduction and solidification technologies that have domestic or foreign experiences of practical treatment for radioactive wastes to assist selection of suitable treatment of the wastes. This report shows the arranged results. The 1F wastes are classified into two groups, homogeneous particulate and liquid wastes and heterogeneous solid wastes. The needful items for the feasibility study such as a technology name, a fundamental principle, treatment efficiency, and characteristic of solidified waste are summarized in each group.
Sato, Junya; Suzuki, Shinji*; Kato, Jun; Sakakibara, Tetsuro; Meguro, Yoshihiro; Nakazawa, Osamu
QST-M-2; QST Takasaki Annual Report 2015, P. 87, 2017/03
no abstracts in English
Sato, Junya; Suzuki, Shinji*; Kato, Jun; Sakakibara, Tetsuro; Meguro, Yoshihiro; Nakazawa, Osamu
QST-M-2; QST Takasaki Annual Report 2015, P. 88, 2017/03
no abstracts in English
Kimata, Tetsuya*; Kato, Sho*; Yamaki, Tetsuya; Yamamoto, Shunya; Kobayashi, Tomohiro*; Terai, Takayuki*
Surface & Coatings Technology, 306(Part A), p.123 - 126, 2016/11
Times Cited Count：13 Percentile：51.96(Materials Science, Coatings & Films)Platinum (Pt) nanoparticle catalysts with oxygen reduction reaction (ORR) activity are required for practical applications of polymer electrolyte fuel cells. We prepared Pt nanoparticles on an Ar
-irradiated glassy carbon (GC) surface by a radio-frequency magnetron sputtering method to investigate the influence of the ion-induced lattice defects in GC on the ORR activity of the deposited Pt nanoparticles. Interestingly, the Pt nanoparticles on the irradiated surface exhibited ca. 2.5 times higher specific activity than those on the non-irradiated one. X-ray photoelectron spectroscopy suggested the interfacial Pt-C interaction occurring between the irradiated GC and Pt nanoparticles, which should be a reason for improvement of the ORR activity.
Sakai, Kenji; Oi, Motoki; Watanabe, Akihiko; Kai, Tetsuya; Kato, Yuko; Meigo, Shinichiro; Takada, Hiroshi
JAEA-Conf 2015-002, p.593 - 598, 2016/02
For safe and stable beam operation, a MLF general control system (GCS) consists of several subsystems such as an integral control, interlock, server, network, and timing distribution systems. Since the first beam injection in 2008, the GCS has operated stably without any serious troubles in comparison with upgrade of target devices for ramping up beam power and increment of user apparatuses year by year. In recent years, however, it has been improved significantly in view of sustainable long-term operation and maintenance. The monitor and operation system of the GCS has been upgraded by changing its framework software to improve potential flexibility in its maintenance. Its interlock system was also modified in accordance with the re-examination of the risk management system of J-PARC. This paper reports recent progress of the MLF-GCS.
