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Fujita, Natsuko; Miyake, Masayasu; Matsubara, Akihiro*; Ishii, Masahiro*; Jinno, Satoshi; Watanabe, Takahiro; Nishio, Tomohiro*; Ogawa, Yumi; Omae, Akiomi*; Kimura, Kenji; et al.
Dai-36-Kai Tandemu Kasokuki Oyobi Sono Shuhen Gijutsu No Kenkyukai Hokokushu, p.90 - 92, 2025/03
The JAEA-AMS-TONO facility at the Tono Geoscience Center, JAEA has three accelerator mass spectrometers. We report the present status of the JAEA-AMS-TONO.
Jinno, Satoshi; Matsubara, Akihiro*; Fujita, Natsuko; Kimura, Kenji
Nuclear Instruments and Methods in Physics Research B, 557, p.165545_1 - 165545_4, 2024/12
Times Cited Count：0 Percentile：0.00(Instruments & Instrumentation)This study introduces the development of a downsized Accelerator Mass Spectrometry (AMS) system aiming to enhance accessibility and cost-effectiveness in radiocarbon analysis. The "crystal surface stripper method" is introduced as a solution to challenges in AMS downsizing, demonstrating effective ion detection with a smaller angular spread compared to conventional gas stripper methods. The experimental results provide insights into charge conversion capabilities, scattering angle broadening, and energy loss associated with surface scattering.
Ishida, Reiya; Sonobe, Hiroshi; Kimura, Akihiro
JAEA-Review 2024-030, 75 Pages, 2024/08
JAEA-Review-2024-030.pdf:8.53MB
Department of JMTR Hot Laboratory (HL) had been construction since 1967 (concrete and lead cells have been in service since 1971 and steel cells since 1982). Because the HL is old, there is a high possibility that asbestos is used in heat insulation material wrapped around the piping installed in the HL. If asbestos is contained in that of such pipes, it may be dispersed into the air during repair, remodeling, or removal of such pipes, causing lung cancer, mesothelioma, or other health problems to workers. Therefore, it is also important to understand the status of asbestos use in the facility. The HL has been investigating the presence of asbestos in heat insulation material wrapped around piping in several systems installed in the facility. As a result, asbestos was detected in some of heat insulation material. This report describes the results of the asbestos survey conducted so far.
Fujita, Natsuko; Miyake, Masayasu; Matsubara, Akihiro*; Ishii, Masahiro*; Takahashi, Yuto*; Watanabe, Takahiro; Jinno, Satoshi; Nishio, Tomohiro*; Ogawa, Yumi; Kimura, Kenji; et al.
Dai-25-Kai AMS Shimpojiumu Hokokushu (Internet), 3 Pages, 2024/03
The JAEA-AMS-TONO facility at the Tono Geoscience Center, JAEA has three accelerator mass spectrometers. We report the present status of the JAEA-AMS-TONO.
Fujita, Natsuko; Miyake, Masayasu; Matsubara, Akihiro*; Ishii, Masahiro*; Watanabe, Takahiro; Jinno, Satoshi; Nishio, Tomohiro*; Ogawa, Yumi; Kimura, Kenji; Shimada, Akiomi; et al.
Dai-35-Kai Tandemu Kasokuki Oyobi Sono Shuhen Gijutsu No Kenkyukai Hokokushu, p.17 - 19, 2024/03
The JAEA-AMS-TONO facility at the Tono Geoscience Center, JAEA has three accelerator mass spectrometers. We report the present status of the JAEA-AMS-TONO.
Fujita, Natsuko; Matsubara, Akihiro*; Jinno, Satoshi; Kimura, Kenji
Hoshasen (Internet), 48(4), p.137 - 138, 2024/02
We have been developing a downsized AMS with a size of about 2 m 
2 m. This AMS is developed to demonstrate a new method of separating same-mass molecules, which are interfering nuclides during AMS measurement of carbon-14, using ion channeling.
Fuyushima, Takumi; Takabe, Yugo; Sayato, Natsuki; Kimura, Akihiro; Takemoto, Noriyuki
The IV International Scientific Forum "Nuclear Science and Technologies"; AIP Conference Proceedings 3020, p.040007_1 - 040007_6, 2024/01
We studied irradiation tests of structural materials simulating fast reactor conditions in JMTR. We fabricated capsules that can simulate fast reactor irradiation in JMTR by using He/dpa ratio as index. To simulate fast reactor, cadmium, which shield thermal neutrons, was placed inside the capsule to adjust the neutron spectrum. According to the result of irradiation tests by neutron spectrum adjusting capsule, we confirmed that it can simulate the He/dpa ratio of fast reactor. Currently, since it is impossible to conduct irradiation tests in Japan, a plan is underway to partly replace the irradiation function of JMTR with overseas reactors. The alternative irradiation will be carried out by succeeding and developing the irradiation technology accumulated in the JMTR, and as a part of this, a trial of such irradiation in which the neutron spectrum is adjusted is under consideration.
Shibanuma, Tomohiro; Hirano, Hiroshi*; Kimura, Yasuhisa; Aita, Takahiro; Yoshida, Masato; Nagai, Yuya; Kitamura, Akihiro
Hoken Butsuri (Internet), 58(2), p.91 - 98, 2023/08
We developed new containment tents that are more easily assembled and effectively functioned, by improving and refurbishing the shortcomings of the conventional tents. The new tents have been already tested in the real airborne contamination situation occurred at the plutonium fuel fabricating facility. The tents appropriately functioned for intended use but other shortcomings emerged and therefore we had modified the structure of the tents further.
Kokubu, Yoko; Fujita, Natsuko; Watanabe, Takahiro; Matsubara, Akihiro; Ishizaka, Chika; Miyake, Masayasu*; Nishio, Tomohiro*; Kato, Motohisa*; Ogawa, Yumi*; Ishii, Masahiro*; et al.
Nuclear Instruments and Methods in Physics Research B, 539, p.68 - 72, 2023/06
Times Cited Count：2 Percentile：43.92(Instruments & Instrumentation)The JAEA-AMS-TONO facility at the Tono Geoscience Center, JAEA has an accelerator mass spectrometer (JAEA-AMS-TONO-5MV). The spectrometer enabled us to use a multi-nuclide AMS of carbon-14 (
C), beryllium-10, aluminium-26 and iodine-129, and we have recently been proceeding test measurement of chlorine-36. In response to an increase of samples, we installed a state-of-the-art multi-nuclide AMS with a 300 kV Tandetron accelerator in 2020. Recently, we are driving the development of techniques of isobar separation in AMS and of sample preparation. Ion channeling is applied to remove isobaric interference and we are building a prototype AMS based on this technique for downsizing of AMS. The small sample graphitization for C has been attempted using an automated graphitization equipment equipped with an elemental analyzer.
Matsubara, Akihiro*; Fujita, Natsuko; Miyake, Masayasu; Ishii, Masahiro*; Watanabe, Takahiro; Kokubu, Yoko; Nishio, Tomohiro*; Ogawa, Yumi; Jinno, Satoshi; Kimura, Kenji; et al.
JAEA-Conf 2022-002, p.55 - 62, 2023/03
We report the present status of the JAEA-AMS-TONO. Particularly, the destructions of varistors used in the beamline equipment will be presented. The cause of the destruction as well as implementation of the safety measures are mentioned.
Fujita, Natsuko; Miyake, Masayasu; Matsubara, Akihiro*; Ishii, Masahiro*; Watanabe, Takahiro; Jinno, Satoshi; Nishio, Tomohiro*; Ogawa, Yumi; Yamamoto, Yusuke; Kimura, Kenji; et al.
Dai-23-Kai AMS Shimpojiumu Hokokushu, p.1 - 4, 2022/12
The JAEA-AMS-TONO facility at the Tono Geoscience Center, JAEA has three accelerator mass spectrometers. We report the present status of the JAEA-AMS-TONO.
Fujita, Natsuko; Matsubara, Akihiro; Kimura, Kenji; Jinno, Satoshi; Kokubu, Yoko
Nuclear Instruments and Methods in Physics Research B, 532, p.13 - 18, 2022/12
Times Cited Count：2 Percentile：31.55(Instruments & Instrumentation)Over the last decade, significant technological advances were made to downsize the AMS systems. Japan Atomic Energy Agency has started a project for developing a prototype downsized AMS system (with the footprint of the system is 1.9 m 1.9 m) based on the surface stripper technique. Although the system configuration using an ion source, magnets, and detectors is similar to that in conventional systems, there is no tandem accelerator as well as a gas stripper. The ion acceleration is provided in the ion source (maximum ion energy 40 keV). For proof-of-principle experiments, we have planned two steps: (1) Observation of the specular reflection and the dissociation by using a compact electrostatic analyzer located just behind the stripper, and (2) Demonstration of C measurement, along with the experimental confirmation of the isobar suppression capability of the surface stripper.
Nishimura, Arashi; Okada, Yuji; Sugaya, Naoto; Sonobe, Hiroshi; Kimura, Nobuaki; Kimura, Akihiro; Hanawa, Yoshio; Nemoto, Hiroyoshi
JAEA-Technology 2021-003, 51 Pages, 2021/05
JAEA-Technology-2021-003.pdf:5.55MB
In the Japan Materials Testing Reactor (JMTR), the leakage accidents of radioactive waste liquid were occurred from the tanks and pipes of the liquid waste disposal facility in the JMTR tank-yard building in JFY2014. In order to respond to the accident, obtain the approval of the JAEA to the design and construction method from JFY2016, the tanks and pipes were replaced from JFY2016 to 2019. In the replaced, the production of the tanks and pipes of the liquid waste disposal facility applied Japanese technical standards correspondingly. On the other hand, the valve did not fall under the category of Japanese technical standards. The manufacturing specifications when replacing the valve were decided based on the including the selecting the standards of production and inspection for valves, Fluid properties, experience in JMTR. The production proceeded while carrying out the decided inspection. The valves that passed all the inspections were installed together with the tanks and pipes of the liquid waste, and the finished inspection was performed as a systems. The construction was completed with those inspection passed. This report is summarized valve Design, production and installation.
Sugaya, Naoto; Okada, Yuji; Nishimura, Arashi; Sonobe, Hiroshi; Kimura, Nobuaki; Kimura, Akihiro; Hanawa, Yoshio; Nemoto, Hiroyoshi
JAEA-Testing 2020-004, 67 Pages, 2020/08
JAEA-Testing-2020-004.pdf:8.17MB
In the Japan Materials Testing Reactor (JMTR), the leakage accidents of radioactive waste liquid were occurred from the tanks and pipes of the liquid waste disposal facility in the JMTR tank-yard building in JFY2014. In order to respond to the accident, the tanks and pipes were replaced from JFY2016 to 2019. On the other hand, a lot of cracks were occurred on the concreate wall of the tank-yard building when the frame structure supports were fixed to the concrete wall in the replacement work. Thus, it is necessary to repair the concreate wall of the tank-yard building. Especially, some cracks with swelling (cone-shaped fracture) were raised around some anchor bolts (the post-installed chemical anchor bolts) fixed the frame structure supports. The repairing method for the cone-shaped fracture of the concrete wall is standardized, but there was no reference value of tensile strength for the validation of the post-installed chemical anchor bolts after the repairing method. In this report, the repairing method was selected for the cone-shaped fracture on the concreate wall and the reference value of tensile strength for the validation of the post-installed chemical anchor bolts by this repairing method. The mock-ups for repairing cone-shaped fracture were fabricated by the selected repairing method and the tensile tests of the post-installed chemical anchor bolts were performed. From the results, the validation of the repairing method was obtained in this test and it was obvious the repairing of cone-shaped fracture is preferable method for the concreate wall of the JMTR tank-yard building.
CsShibahara, Yuji*; Nakamura, Shoji; Uehara, Akihiro*; Fujii, Toshiyuki*; Fukutani, Satoshi*; Kimura, Atsushi; Iwamoto, Osamu
Journal of Radioanalytical and Nuclear Chemistry, 325(1), p.155 - 165, 2020/07
Times Cited Count：12 Percentile：74.60(Chemistry, Analytical)The measurements of isotopic ratios of Cs samples by thermal ionization mass spectrometry were performed for the analysis of their samples used to evaluate nuclear data obtained for Cs. To obtain a high intensity and stable ion beam, the effects of additive agents on the ionization of Cs were examined. The effect of silicotungstic acid on the ionization of Cs was the largest among the additive agents studied in the present study, while the silicotungstic acid also showed the largest isobaric interference of polyatomic ions. It was demonstrated that as small as 210
g of a Cs sample was sufficient to achieve the analytical precision required to measure the Cs/
Cs ratio in the case where an additive agent of TaO/glucose was employed. After examining of the analytical conditions, such as the interference effect due to Ba, the measurements of the isotopic ratios of two Cs samples used in our study using TIMS were conducted, and it was discussed how much the ratios contributed to evaluation of the neutron capture cross-section of Cs.
Matsubara, Akihiro*; Fujita, Natsuko; Ishii, Kunikazu*; Kimura, Kenji*
Hoshasen (Internet), 45(3), p.134 - 138, 2020/04
no abstracts in English
Nakamura, Shoji; Shibahara, Yuji*; Kimura, Atsushi; Iwamoto, Osamu; Uehara, Akihiro*; Fujii, Toshiyuki*
Journal of Nuclear Science and Technology, 57(4), p.388 - 400, 2020/04
Times Cited Count：3 Percentile：25.69(Nuclear Science & Technology)The thermal-neutron capture cross-section (
) and resonance integral(I
) were measured for the Cs(n,
)
Cs reaction by an activation method and mass spectrometry. We used Cs contained as an impurity in a normally available Cs standard solution. An isotope ratio of Cs and Cs in a standard Cs solution was measured by mass spectrometry to quantify Cs. The analyzed Cs samples were irradiated at the hydraulic conveyer of the research reactor in Institute for Integral Radiation and Nuclear Science, Kyoto University. Wires of Co/Al and Au/Al alloys were used as neutron monitors to measure thermal-neutron fluxes and epi-thermal Westcott's indices at an irradiation position. A gadolinium filter was used to measure the , and a value of 0.133 eV was taken as the cut-off energy. Gamma-ray spectroscopy was used to measure induced activities of Cs, Cs and monitor wires. On the basis of Westcott's convention, the and I values were derived as 8.57
0.25 barn, and 45.33.2 barn, respectively. The obtained in the present study agreed within the limits of uncertainties with the past reported value of 8.30.3 barn.
2 mMatsubara, Akihiro; Fujita, Natsuko; Kimura, Kenji
Proceedings of the 8th East Asia Accelerator Mass Spectrometry Symposium and the 22nd Japan Accelerator Mass Spectrometry symposium (EA-AMS 8 & JAMS-22), p.57 - 59, 2020/00
no abstracts in English
Mo/
Tc generator by (n,) methodFujita, Yoshitaka; Seki, Misaki; Namekawa, Yoji*; Nishikata, Kaori; Kimura, Akihiro; Shibata, Akira; Sayato, Natsuki; Tsuchiya, Kunihiko; Sano, Tadafumi*; Fujihara, Yasuyuki*; et al.
KURNS Progress Report 2018, P. 155, 2019/08
no abstracts in English
Nakamura, Shoji; Kimura, Atsushi; Iwamoto, Osamu; Shibahara, Yuji*; Uehara, Akihiro*; Fujii, Toshiyuki*
KURNS Progress Report 2018, P. 106, 2019/08
Under the ImPACT project, the neutron capture cross-section measurements of Cesium-135 (Cs) among the long-lived fission products have been performed at Kyoto University. This paper reports measurements of the thermal-neutron capture cross-section of Cs at the Kyoto University Research Reactor (KUR).
