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Kawakita, Yukinobu; Kikuchi, Tatsuya*; Tahara, Shuta*; Nakamura, Mitsutaka; Inamura, Yasuhiro; Maruyama, Kenji*; Yamauchi, Yasuhiro*; Kawamura, Seiko; Nakajima, Kenji
JPS Conference Proceedings (Internet), 33, p.011071_1 - 011071_6, 2021/03
CuI is a well-known superionic conductor in a high temperature solid phase where the mobile cations migrate between interstitial sites in the f.c.c. sublattice formed by iodine ions. Even in the molten state, it shows several features suggesting collective or cooperative ionic motion. MD results show that Cu diffuses much faster than I. The Cu-Cu partial structure factor have a FSDP which indicates a medium-range ordering of Cu ions. Moreover the Cu-Cu partial pair distribution deeply penetrates into the nearest neighboring Cu-I shell. To reveal origin such anomalous behaviors of molten CuI, we performed quaiselastic neutron scattering (QENS) by the disk-chopper spectrometer AMATERAS at MLF, J-PARC. To interpret the total dynamic structure factor obtained from coherent QENS, the mode distribution analysis was applied. It is found that the motion of iodine is a kind of fluctuating within an almost local area while Cu ions diffuse much faster than iodine ions.
Kawakita, Yukinobu; Kikuchi, Tatsuya*; Inamura, Yasuhiro; Tahara, Shuta*; Maruyama, Kenji*; Hanashima, Takayasu*; Nakamura, Mitsutaka; Kiyanagi, Ryoji; Yamauchi, Yasuhiro*; Chiba, Kaori*; et al.
Physica B; Condensed Matter, 551, p.291 - 296, 2018/12
Times Cited Count：11 Percentile：43.99(Physics, Condensed Matter)There are elemental liquid metals with complex structures far from the hard sphere (HS) packing model. Liquid Bi has an asymmetric first peak in the structure factors S(Q). The pair distribution function g(r) exhibits strange distance ratio of 1:2 between the first and the second peaks. Since a HS model with two kinds of radius produces asymmetry of the main peak in S(Q), existence of short-lived covalent bonds was discussed. Contrarily, modulation of the atomic distribution by the Friedel oscillations of shielding electrons around metallic ions was discussed. To examine its bonding nature from viewpoints of dynamic correlation functions, we have measured neutron quasielastic scattering of liquid Bi by using cold disk chopper spectrometer installed at MLF of J-PARC. The van Hove function revealed that the shoulder structure located at a longer side of the first peak in g(r) exhibits a longer relaxation time than the main structures such as the first and second peaks.
Sakasai, Kaoru; Sato, Setsuo*; Seya, Tomohiro*; Nakamura, Tatsuya; To, Kentaro; Yamagishi, Hideshi*; Soyama, Kazuhiko; Yamazaki, Dai; Maruyama, Ryuji; Oku, Takayuki; et al.
Quantum Beam Science (Internet), 1(2), p.10_1 - 10_35, 2017/09
Neutron devices such as neutron detectors, optical devices including supermirror devices and 
He neutron spin filters, and choppers are successfully developed and installed at the Materials Life Science Facility (MLF) of the Japan Proton Accelerator Research Complex (J-PARC), Tokai, Japan. Four software components of MLF computational environment, instrument control, data acquisition, data analysis, and a database, have been developed and equipped at MLF. MLF also provides a wide variety of sample environment options including high and low temperatures, high magnetic fields, and high pressures. This paper describes the current status of neutron devices, computational and sample environments at MLF.
Ogoshi, Yurie; Satoyama, Tomonori; Kishimoto, Katsumi; Nanri, Tomohiro; Suzuki, Takeshi; Tomioka, Osamu; Takaizumi, Hirohide*; Kanno, Tomoyuki*; Maruyama, Tatsuya*
JAEA-Technology 2017-017, 152 Pages, 2017/08
JAEA-Technology-2017-017.pdf:15.97MB
At Nuclear Science Research Institute, clearance works for about 4,000 tons of extremely low-level radioactive concrete debris, which were generated from the modification activities of JRR-3 from FY 1985 to FY 1989 and stored in the waste storage facility NL, carried out. First of this clearance works, method for measuring and evaluating radioactivity concentration was approved by Minister of MEXT on July 25, 2008. And then, clearance works were started from FY 2009. Measuring and evaluating radioactivity concentration was achieved by using the approved method, and was confirmed by government. And then, clearance works were completed in FY 2014. The clearance concrete was recycled as a material for restoration works of the 2011 off the Pacific coast of Tohoku Earthquake. This report summarizes the results of measuring and evaluating radioactivity concentration, achievement of confirmation by government, recycling of cleared concrete and cost for clearance works.
Yoshimoto, Tatsuya*; Ishikawa, Jun; Okamoto, Koji*; Maruyama, Yu
Proceedings of 9th Korea-Japan Symposium on Nuclear Thermal Hydraulics and Safety (NTHAS-9) (CD-ROM), 5 Pages, 2014/11
Takeda, Masayasu; Yamazaki, Dai; Soyama, Kazuhiko; Maruyama, Ryuji; Hayashida, Hirotoshi; Asaoka, Hidehito; Yamazaki, Tatsuya; Kubota, Masato; Aizawa, Kazuya; Arai, Masatoshi; et al.
Chinese Journal of Physics, 50(2), p.161 - 170, 2012/04
Yamazaki, Tatsuya; Asaoka, Hidehito; Taguchi, Tomitsugu; Yamamoto, Shunya; Yamazaki, Dai; Maruyama, Ryuji; Takeda, Masayasu; Shamoto, Shinichi
Thin Solid Films, 520(8), p.3300 - 3303, 2012/02
Times Cited Count：2 Percentile：9.23(Materials Science, Multidisciplinary)We succeeded in realizing the epitaxial growth of a Sr layer on Si(111) with an atomically abrupt heterointerface - in spite of its large lattice mismatch (12%) with Si - by introducing a monoatomic layer of H on Si. In order to identify the buried H, we carried out a combination analysis involving neutron reflectometry and resonant nuclear reaction of 
H(
N,
)
C analysis. We found different neutron reflectivity profiles resulting from a contrast variation between the H and D atoms at the buried heterointerface. Furthermore, the depth -ray intensity profiles revealed that the H at the heterointerface acts as an effective buffer layer that enables it to manage the highly mismatched epitaxy on Si.
Nakajima, Kenji; Kawamura, Seiko; Kikuchi, Tatsuya; Nakamura, Mitsutaka; Kajimoto, Ryoichi; Inamura, Yasuhiro; Takahashi, Nobuaki; Aizawa, Kazuya; Suzuya, Kentaro; Shibata, Kaoru; et al.
Journal of the Physical Society of Japan, 80(Suppl.B), p.SB028_1 - SB028_6, 2011/05
Times Cited Count：140 Percentile：95.93(Physics, Multidisciplinary)AMATERAS is a cold-neutron disk-chopper spectrometer in MLF, J-PARC. The construction of main part of the spectrometer has been completed in spring of 2009. Soon after that, we have started the commissioning work on AMATERAS. The performance of AMATERAS has been examined by test experiments in the course of commissioning. In parallel to these works, we have started the user program on AMATERAS from December 2009 and we are getting scientific results from our spectrometer. In this presentation, we will report the current status of AMATERAS including the results of performance tests and some of examples of scientific outputs.
Nakajima, Hideo; Hamada, Kazuya; Okuno, Kiyoshi; Abe, Kanako*; Shimizu, Tatsuya; Kakui, Hideo*; Yamaoka, Hiroto*; Maruyama, Naoyuki*; Takayanagi, Tadatoshi*
Fusion Engineering and Design, 82(5-14), p.1473 - 1480, 2007/10
Times Cited Count：7 Percentile：46.20(Nuclear Science & Technology)no abstracts in English
activity distribution in concrete wastes generated from JRR-3 renewal for clearanceTsutsumi, Masahiro; Kogure, Hiroto; Satoyama, Tomonori; Maruyama, Tatsuya; Kishimoto, Katsumi
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Kubota, Masato; Takeda, Masayasu; Yamazaki, Dai; Hayashida, Hirotoshi; Maruyama, Ryuji; Soyama, Kazuhiko; Asaoka, Hidehito; Yamazaki, Tatsuya; Sakasai, Kaoru; To, Kentaro; et al.
no journal, ,
no abstracts in English
Takeda, Masayasu; Yamazaki, Dai; Hayashida, Hirotoshi; Maruyama, Ryuji; Soyama, Kazuhiko; Kubota, Masato; Asaoka, Hidehito; Yamazaki, Tatsuya; Sakasai, Kaoru; To, Kentaro; et al.
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no abstracts in English
Takeda, Masayasu; Yamazaki, Dai; Soyama, Kazuhiko; Maruyama, Ryuji; Hayashida, Hirotoshi; Asaoka, Hidehito; Yamazaki, Tatsuya; Kubota, Masato; Aizawa, Kazuya; Arai, Masatoshi; et al.
no journal, ,
Takeda, Masayasu; Yamazaki, Dai; Hayashida, Hirotoshi; Kubota, Masato; Maruyama, Ryuji; Soyama, Kazuhiko; Asaoka, Hidehito; Yamazaki, Tatsuya; Yoshida, Noboru*; Sakaguchi, Yoshifumi*; et al.
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no abstracts in English
Kubota, Masato; Takeda, Masayasu; Yamazaki, Dai; Soyama, Kazuhiko; Maruyama, Ryuji; Hayashida, Hirotoshi; Asaoka, Hidehito; Oikawa, Kenichi; Yamazaki, Tatsuya*; Aizawa, Kazuya; et al.
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Nanri, Tomohiro; Kishimoto, Katsumi; Satoyama, Tomonori; Takaizumi, Hirohide; Kanno, Tomoyuki; Maruyama, Tatsuya; Yoshimori, Michiro
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no abstracts in English
Kishimoto, Katsumi; Satoyama, Tomonori; Takaizumi, Hirohide; Kanno, Tomoyuki; Maruyama, Tatsuya; Yoshimori, Michiro
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We have been storing about 4000 tons of very low-level radioactive concrete debris as radioactive wastes generated from the modification of JRR-3 between 1985 and 1990. At that time, the clearance system was not a part of our regulatory law. We conducted a preliminary survey of contamination levels, and then established procedures for measuring and evaluating the radioactivity concentration. In 2008, the government authorized our procedures for clearance. Since FY 2009, we have measured the radioactivity concentration of concrete debris, using the government-authorized procedures. By the end of FY 2012, the government had confirmed the correctness of our measurements and evaluation results on about 1900 tons of concrete debris. We processed the concrete debris that was approved by the government for recycling. By the end of FY 2012, we had reused about 600 tons of concrete debris as backfilling material in depressed areas around buildings in the Nuclear Science Research Institute.
Kawakita, Yukinobu; Kikuchi, Tatsuya*; Inamura, Yasuhiro; Tahara, Shuta*; Maruyama, Kenji*; Hanashima, Takayasu*; Nakamura, Mitsutaka; Kiyanagi, Ryoji; Yamauchi, Yasuhiro*; Chiba, Kaori*; et al.
no journal, ,
There are many polyvalent liquid metals with complex structure which cannot be reproduced by random packing model. To explain such complexity, coexistence of metallic and covalent bonds, dynamic model of short-lived covalent bonds, and quasi-crystal model where Peierls distortion still remains even in liquid phase have been proposed from structure analyses and theoretical calculations. To obtain concrete picture experimentally for complex structure, it is indispensable to measure dynamic structure with precise statistical accuracy. We performed inelastic neutron scattering of liquid bismuth by using AMATERAS installed at MLF in J-PARC and deduced its time-space correlation function. We got evidence that structure of Peierls distortion remains even in liquid by evaluating difference in relaxation time at specific atomic distances characterized by double layered structure.
Takeda, Masayasu; Yamazaki, Dai; Maruyama, Ryuji; Hayashida, Hirotoshi; Soyama, Kazuhiko; Yamazaki, Tatsuya; Hirano, Tatsumi*; Oikawa, Kenichi; Tamura, Itaru; Sakasai, Kaoru; et al.
no journal, ,
no abstracts in English
Takeda, Masayasu; Yamazaki, Dai; Soyama, Kazuhiko; Maruyama, Ryuji; Hayashida, Hirotoshi; Asaoka, Hidehito; Yamazaki, Tatsuya; Kubota, Masato; Aizawa, Kazuya; Inamura, Yasuhiro; et al.
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