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論文

Investigation of the phonon dispersion associated with superlattice reflections in the BiS$$_{2}$$-based superconductor LaBiS$$_{2}$$O$$_{0.5}$$F$$_{0.5}$$

玉造 博夢; 長谷川 巧*; 佐賀山 基*; 水牧 仁一朗*; 村上 洋一*; 梶谷 丈*; 東中 隆二*; 松田 達磨*; 青木 勇二*; 筒井 智嗣*

Physical Review B, 107(2), p.024303_1 - 024303_8, 2023/01

https://doi.org/10.1103/PhysRevB.107.024303
 被引用回数：0 パーセンタイル：0.01(Materials Science, Multidisciplinary)

The phonon dispersion of a BiS$$_{2}$$-based superconductor LaBiS$$_{2}$$O$$_{0.5}$$F$$_{0.5}$$ is investigated by first-principles calculations and inelastic X-ray scattering experiments. The origin of superlattice (SL) reflections arising from transverse-type lattice modulation, which were recently reported in [J. Kajitani $textit{et al}$., J. Phys. Soc. Jpn. ${bf 90}$, 103601 (2021)], is discussed in terms of lattice dynamics. Our first-principles calculations of phonon dispersion and the Fermi surfaces (FSs) demonstrate that the phonon mode corresponding to the transverse-type lattice modulation is unstable, and the propagation vector corresponding to the SL reflections is close to the FS nesting vector, which suggests that the phonon softening originates from the FS nesting. Against these calculated expectations, measured phonon dispersion in LaBiS$$_{2}$$O$$_{0.5}$$F$$_{0.5}$$ along the Z-A direction, where the SL point is located, shows no remarkable temperature dependence, and there are no steeply declining branches accompanied with a softening around the SL point. Based on these results, we discuss the two possibilities for the transverse lattice modulation in LaBiS$$_{2}$$O$$_{0.5}$$F$$_{0.5}$$: the order-disorder type structural transition and the displacive structural transition with an overdamped mode, for both of which the local structure distortion or the short range correlation within the BiS$$_{2}$$ plane would be essential.

論文

Weyl-Kondo semimetal behavior in the chiral structure phase of Ce$$_{3}$$Rh$$_{4}$$Sn$$_{13}$$

岩佐 和晃*; Suyama, Kazuya*; 河村 聖子; 中島 健次; Raymond, S.*; Steffens, P.*; Yamada, Akira*; 松田 達磨*; Aoki, Yuji*; 川崎 郁斗; et al.

Physical Review Materials (Internet), 7(1), p.014201_1 - 014201_11, 2023/01

https://doi.org/10.1103/PhysRevMaterials.7.014201
 被引用回数：0

The spin dynamics, crystalline-electric-field (CEF) level scheme, specific heat, and X-ray photoemission spectra (XPS) of Ce$$_{3}$$Rh$$_{4}$$Sn$$_{13}$$ were investigated, which exhibits anomalous semimetal transport in the chiral crystallographic phase. CEF excitations observed at approximately 7 and 39 meV are consistent with the two inequivalent Ce-ion cites in the chiral structure. Because of broader CEF excitations and a strong 4$$f^{1}$$ peak at the Fermi level in the Ce 4$$f$$ on-resonance spectrum, the hybridized Ce 4$$f$$ electrons contribute to the semimetal carriers. In addition, the spin fluctuation associated with the Kramers doublet ground state is characterized by the peak located at 0.15 meV. The electronic state involving the spin fluctuation causes the $$T^{3}$$ behavior of specific heat below 0.6 K, which is attributed to linear dispersion relations of electrons of the Weyl Kondo semimetal in the chiral-lattice symmetry.

論文

Sm valence determination of Sm-based intermetallics using $$^{149}$$Sm M$"{o}$ssbauer and Sm L$$_{rm III}$$-edge X-ray absorption spectroscopies

筒井 智嗣; 東中 隆二*; 中村 頼人*; 藤原 孝将*; 中村 仁*; 小林 義男*; 伊藤 孝; 依田 芳卓*; 加藤 和男*; 新田 清文*; et al.

Hyperfine Interactions, 242(1), p.32_1 - 32_10, 2021/12

https://doi.org/10.1007/s10751-021-01759-x
 被引用回数：0 パーセンタイル：1.69

$$^{149}$$Sm synchrotron-radiation-based M$"{o}$ssbauer spectroscopy was performed in Sm-based intermetallics having a cubic crystal structure, Sm$$_{3}Tr_{4}$$Ge$$_{13}$$, SmB$$_{6}$$, SmBe$$_{13}$$, and Sm$$Tr_{2}$$Al$$_{20}$$ ($$Tr$$ = transition metals). In spite of the difference of the local structure around the Sm sites, the observed M$"{o}$ssbauer spectra consist of a single line at 300 K. On the other hand, Sm L$$_{rm III}$$-edge X-ray absorption spectra consist of two components, suggesting Sm$$^{2+}$$ and Sm$$^{3+}$$ states. Difference of the number of the spectral components between the M$"{o}$ssbauer spectroscopy and X-ray absorption spectroscopy is caused by the difference of the time window in the scattering process of these measurements. Correlation between the isomer shifts in the M$"{o}$ssbauer spectroscopy and average Sm valence states estimated from the X-ray absorption spectroscopy exhibits a linear correlation.

論文

The Analytical study of inventories and physicochemical configuration of spallation products produced in Lead-Bismuth Eutectic of Accelerator Driven System

宮原 信哉*; 大平 直也*; 有田 裕二*; 前川 藤夫; 松田 洋樹; 佐々 敏信; 明午 伸一郎

Nuclear Engineering and Design, 352, p.110192_1 - 110192_8, 2019/10

https://doi.org/10.1016/j.nucengdes.2019.110192
 被引用回数：4 パーセンタイル：47.64(Nuclear Science & Technology)

鉛ビスマス共晶(LBE)合金は加速器駆動システム(ADS)の核破砕中性子ターゲットや冷却材として用いられ、核破砕生成物として多くの元素が生成するため、その放出および輸送挙動を評価することが重要である。そこで、J-PARCのADSターゲット試験施設(TEF-T)のLBEループについて、LBE中に生成する核破砕生成物のインベントリおよび物理化学的組成について検討した。LBE内の核破砕生成物インベントリは、PHITSコードを使用して評価した。LBE中の核破砕生成物の物理化学的組成は、350$$^{circ}$$C$$sim$$500$$^{circ}$$CのLBE運転温度及びLBE中の酸素濃度10ppb$$sim$$1ppmの条件下、Thermo-Calcコードを用いて計算した。計算の結果、Rb, Tl, Tc, Os, Ir, Pt, Au, Hgの8元素がすべての条件下でLBEに可溶であり、化合物は形成されなかった。Ce, Sr, Zr及びYの酸化物はLBE中でCeO$$_{2}$$, SrO, ZrO$$_{2}$$およびY$$_{2}$$O$$_{3}$$として安定であることが示唆された。

論文

Magnetic, thermal, and neutron diffraction studies of a coordination polymer; bis(glycolato)cobalt(II)

中根 僚宏*; 米山 翔太*; 兒玉 健*; 菊地 耕一*; 中尾 朗子*; 大原 高志; 東中 隆二*; 松田 達磨*; 青木 勇二*; 藤田 渉*

Dalton Transactions (Internet), 48(1), p.333 - 338, 2019/01

https://doi.org/10.1039/C8DT04358B
 被引用回数：2 パーセンタイル：13.9(Chemistry, Inorganic & Nuclear)

The two-dimensional quadratic lattice magnet, bis(glycolato)cobalt(II) ([Co(HOCH$$_{2}$$CO$$_{2}$$)$$_{2}$$]), showed anti-ferromagnetic ordering at 15.0 K and an abrupt increase in magnetisation at H = 22 600 Oe and 2 K, thereby acting as a metamagnet. Neutron diffraction studies suggested that the magnetic moment vectors of the Co(II) ions had an amplitude of 3.59 mB and were not aligned in a fully antiparallel fashion to those of their neighbours, which caused canting between the magnetic moment vectors in the sheet. The canting angle was determined to be 7.1deg. Canting induced net magnetisation in the sheet, but this magnetisation was cancelled between sheets. The magnetisations in the sheets were oriented parallel to the magnetic field at the critical magnetic field.

論文

Element-specific observation of the ferromagnetic ordering process in UCoAl via soft X-ray magnetic circular dichroism

竹田 幸治; 斎藤 祐児; 岡根 哲夫; 山上 浩志; 松田 達磨*; 山本 悦嗣; 芳賀 芳範; 大貫 惇睦*

Physical Review B, 97(18), p.184414_1 - 184414_7, 2018/05

AA2018-0316.pdf:0.62MB

https://doi.org/10.1103/PhysRevB.97.184414
 被引用回数：1 パーセンタイル：5.84(Materials Science, Multidisciplinary)

We have performed soft X-ray magnetic circular dichroism (XMCD) experiments on the itinerant-electron metamagnet UCoAl at the U 4$$d$$-5$$f$$ ($$N_mathrm{4, 5}$$) and Co 2$$p$$-3$$d$$ ($$L_mathrm{2, 3}$$) absorption edges in order to investigate the magnetic properties of the U 5$$f$$ and Co 3$$d$$ electrons separately. From the line shape of the XMCD spectrum, it is deduced that the orbital magnetic moment of the Co 3$$d$$ electrons is unusually large. Through the systematic temperature ($$T$$)- and magnetic field ($$H$$)-dependent XMCD measurements, we have obtained two types of the magnetization curve as a function of $$H$$ and $$T$$ (M-H curve and M-T curve, respectively). The metamagnetic transition from a paramagnetic state to a field-induced ferromagnetic state was observed clearly under 15 K at $$H_mathrm{M}$$. The value of the $$H_mathrm{M}$$ and its $$T$$-dependence agree well between the U and Co sites, and the bulk magnetization. Whereas, we have discovered the remarkable differences in the M-H and M-T curves between the U and Co sites. The present findings show clearly that the role of the Co 3$$d$$ electrons should be considered more carefully in order to understand the origin of the magnetic ordering in UCoAl.

論文

New precise measurement of muonium hyperfine structure interval at J-PARC

上野 恭裕*; 青木 正治*; 深尾 祥紀*; 東 芳隆*; 樋口 嵩*; 飯沼 裕美*; 池戸 豊*; 石田 勝彦*; 伊藤 孝; 岩崎 雅彦*; et al.

Hyperfine Interactions, 238(1), p.14_1 - 14_6, 2017/11

https://doi.org/10.1007/s10751-016-1381-7
 被引用回数：3 パーセンタイル：87.03

MuSEUM is an international collaboration aiming at a new precise measurement of the muonium hyperfine structure at J-PARC (Japan Proton Accelerator Research Complex). Utilizing its intense pulsed muon beam, we expect a ten-fold improvement for both measurements at high magnetic field and zero magnetic field. We have developed a sophisticated monitoring system, including a beam profile monitor to measure the 3D distribution of muonium atoms to suppress the systematic uncertainty.

論文

Maximizing $$T_c$$ by tuning nematicity and magnetism in FeSe$$_{1-x}$$S$$_x$$ superconductors

松浦 康平*; 水上 雄太*; 新井 佑基*; 杉村 優一*; 前島 尚行*; 町田 晃彦*; 綿貫 徹*; 福田 竜生; 矢島 健*; 廣井 善二*; et al.

Nature Communications (Internet), 8, p.1143_1 - 1143_6, 2017/10

https://doi.org/10.1038/s41467-017-01277-x
 被引用回数：72 パーセンタイル：91.82(Multidisciplinary Sciences)

A fundamental issue concerning iron-based superconductivity is the roles of electronic nematicity and magnetism in realising high transition temperature ($$T_c$$). To address this issue, FeSe is a key material, as it exhibits a unique pressure phase diagram involving nonmagnetic nematic and pressure-induced antiferromagnetic ordered phases. However, as these two phases in FeSe have considerable overlap, how each order affects superconductivity remains perplexing. Here we construct the three-dimensional electronic phase diagram, temperature ($$T$$) against pressure ($$P$$) and iso-valent S-substitution ($$x$$), for FeSe$$_{1-x}$$S$$_x$$. By simultaneously tuning chemical and physical pressures, against which the chalcogen height shows a contrasting variation, we achieve a complete separation of nematic and antiferromagnetic phases. In between, an extended nonmagnetic tetragonal phase emerges, where $$T_c$$ shows a striking enhancement. The completed phase diagram uncovers that high-$$T_c$$ superconductivity lies near both ends of the dome-shaped antiferromagnetic phase, whereas $$T_c$$ remainslow near the nematic critical point.

論文

Benchmark study of the recent version of the PHITS code

岩元 洋介; 佐藤 達彦; 橋本 慎太郎; 小川 達彦; 古田 琢哉; 安部 晋一郎; 甲斐 健師; 松田 規宏; 細山田 龍二*; 仁井田 浩二*

Journal of Nuclear Science and Technology, 54(5), p.617 - 635, 2017/05

https://doi.org/10.1080/00223131.2017.1297742
 被引用回数：75 パーセンタイル：99.7(Nuclear Science & Technology)

粒子・重イオン輸送計算コードPHITSは、加速器遮蔽設計、医学物理計算など様々な目的で利用されている。本研究では、最新のPHITSバージョン2.88を用いて、核反応による粒子生成断面積、中性子輸送計算、電磁カスケード等に対する58ケースのベンチマーク計算を実施した。本稿では、このうち特徴的な結果を示した22のケースについて詳細に報告する。ベンチマーク計算の結果、100MeV以上の陽子、中性子、重イオン等の入射反応や電磁カスケードについては、PHITSによる計算結果は実験値を概ね再現した。一方、100MeV未満の粒子入射反応は、PHITSが設定を推奨している核内カスケードモデルINCL4の適用範囲外のエネルギー領域であるため、再現性が悪いことが確認された。また、100MeV以上の陽子入射反応のうち、核分裂成分の収率に対して、蒸発モデルGEMの高エネルギー核分裂過程の取り扱いの問題から実験値を再現しない場合があった。これらの課題は、評価済み核データJENDL4.0/HEをPHITSに組み込むこと等で改善していく予定である。以上のように、本研究でPHITSの様々な適用分野における計算精度を検証するとともに、今後の効率的な改善に重要な指針を得ることができた。

論文

New muonium HFS measurements at J-PARC/MUSE

Strasser, P.*; 青木 正治*; 深尾 祥紀*; 東 芳隆*; 樋口 嵩*; 飯沼 裕美*; 池戸 豊*; 石田 勝彦*; 伊藤 孝; 岩崎 雅彦*; et al.

Hyperfine Interactions, 237(1), p.124_1 - 124_9, 2016/12

https://doi.org/10.1007/s10751-016-1331-4
 被引用回数：7 パーセンタイル：92.26

At the Muon Science Facility (MUSE) of J-PARC (Japan Proton Accelerator Research Complex), the MuSEUM collaboration is planning new measurements of the ground state hyperfine structure (HFS) of muonium both at zero field and at high magnetic field. The previous measurements were performed both at LAMPF (Los Alamos Meson Physics Facility) with experimental uncertainties mostly dominated by statistical errors. The new high intensity muon beam that will soon be available at MUSE H-Line will provide an opportunity to improve the precision of these measurements by one order of magnitude. An overview of the different aspects of these new muonium HFS measurements, the current status of the preparation, and the results of a first commissioning test experiment at zero field are presented.

論文

Fermi surface of ThRu$$_{2}$$Si$$_{2}$$ as a reference to the strongly correlated isostructural metals investigated by quantum oscillations

松本 裕司*; 芳賀 芳範; 立岩 尚之; 青木 晴善*; 木村 憲彰*; 山村 朝雄*; 山本 悦嗣; 松田 達磨*; Fisk, Z.*; 山上 浩志*

Journal of the Physical Society of Japan, 85(10), p.104709_1 - 104709_7, 2016/10

https://doi.org/10.7566/JPSJ.85.104709
 被引用回数：2 パーセンタイル：21.32(Physics, Multidisciplinary)

dHvA oscillations were detected on an actinide compound ThRu$$_2$$Si$$_2$$ which is regarded as a reference to strongly correlated electron systems URu$$_2$$Si$$_2$$ and CeRu$$_2$$Si$$_2$$. Observed Fermi surfaces well coincides with the band structure calculations, as well as experimentally obtained ones for a heavy fermion compound CeRu$$_2$$Si$$_2$$. On the other hand, Fermi surfaces of URu$$_2$$Si$$_2$$ have significantly different characteristics, suggesting an itinerant ground state of 5f electrons.

論文

Colossal thermomagnetic response in the exotic superconductor URu$$_2$$Si$$_2$$

山下 卓也*; 下山 祐介*; 芳賀 芳範; 松田 達磨*; 山本 悦嗣; 大貫 惇睦; 住吉 浩明*; 藤本 聡*; Levchenko, A.*; 芝内 孝禎*; et al.

Nature Physics, 11(1), p.17 - 20, 2015/01

https://doi.org/10.1038/nphys3170
 被引用回数：47 パーセンタイル：89.34(Physics, Multidisciplinary)

Observation of a colossal Nernst signal is reported. URu$$_2$$Si$$_2$$ is known as a heavy fermion superconductor. The superconductivity coexists with the so-called hidden-order phase. The Nernst coefficient is enhanced by as large as million times over the theoretically expected value within the standard framework of superconducting fluctuations. Moreover, contrary to the conventional wisdom, the enhancement is more significant with the reduction of the impurity scattering rate. This anomalous Nernst effect intimately reflects the highly unusual superconducting state in URu$$_2$$Si$$_2$$.

論文

Single-crystal growth and de Haas-van Alphen effect study of ThRu$$_2$$Si$$_2$$

松本 裕司*; 芳賀 芳範; 立岩 尚之; 青木 晴善*; 木村 憲彰*; 松田 達磨*; 山本 悦嗣; Fisk, Z.; 山上 浩志*

JPS Conference Proceedings (Internet), 3, p.011096_1 - 011096_5, 2014/06

https://doi.org/10.7566/JPSCP.3.011096

Electronic differences between heavy Fermion CeRu$$_2$$Si$$_2$$ and isoelectronic nonmagnetic ThRu$$_2$$Si$$_2$$ have been investigated. We succeeded in observing the de Haas-van Alphen oscillation in a high quality single crystal of ThRu$$_2$$Si$$_2$$. The mean free path of conduction carriers has been estimated as 6400 ${AA}$, indicating the high quality of the present sample.

論文

Direct observation of lattice symmetry breaking at the hidden-order transition in URu$$_2$$Si$$_2$$

利根川 翔*; 笠原 成*; 福田 竜生; 杉本 邦久*; 安田 伸広*; 鶴原 悠悟*; 渡邊 大樹*; 水上 雄太*; 芳賀 芳範; 松田 達磨*; et al.

Nature Communications (Internet), 5, p.4188_1 - 4188_7, 2014/06

https://doi.org/10.1038/ncomms5188
 被引用回数：51 パーセンタイル：89.64(Multidisciplinary Sciences)

We report on the observation of lattice symmetry breaking from the fourfold to twofold structure by high-resolution synchrotron X-ray diffraction measurements at zero field. Small orthorhombic symmetry-breaking distortion sets in at the transition temperature with a jump, uncovering the weakly first-order nature of the hidden-order transition. This distortion is observed only in ultra pure samples, implying a highly unusual coupling nature between the electronic pneumaticity and underlying lattice.

論文

Magnetic-field-induced charge order in the filled skutterudite SmRu$$_{4}$$P$$_{12}$$; Evidence from resonant and nonresonant X-ray diffraction

松村 武*; 道村 真司*; 稲見 俊哉; 林 佑弥*; 伏屋 健吾*; 松田 達磨*; 東中 隆二*; 青木 勇二*; 菅原 仁*

Physical Review B, 89(16), p.161116_1 - 161116_5, 2014/04

https://doi.org/10.1103/PhysRevB.89.161116
 被引用回数：15 パーセンタイル：56.32(Materials Science, Multidisciplinary)

SmRu$$_4$$P$$_{12}$$の$$T_{rm MI}=16.5$$K以下の反強磁性相と$$T_{rm MI}$$と$$T^*$$(=14K)間の中間相を共鳴と非共鳴のX線回折法で研究した。中間相では非共鳴の$$q$$=(1,0,0)のThomson散乱が磁場によって誘起される。この現象は理論的に予言されている$$p$$バンドの電荷秩序を反映した原子変位によって引き起こされている。同時にSmの磁場方向の反強磁性モーメントが強調され、これは$$Gamma_7-Gamma_8$$結晶場状態の交互配列を反映していると考えられる。この結果は、軌道に依存した$$p$$-$$f$$混成とpバンドのネスティング不安定性がPrRu$$_4$$P$$_{12}$$やPrFe$$_4$$P$$_{12}$$と同様な非従来型電荷秩序を引き起こしていることを示している。

論文

Cyclotron resonance study of quasiparticle mass and scattering rate in the hidden-order and superconducting phases of URu$$_2$$Si$$_2$$

利根川 翔*; 橋本 顕一郎*; 井加田 洸輔*; 鶴原 悠悟*; Lin, Y.-H.*; 宍戸 寛明*; 芳賀 芳範; 松田 達磨; 山本 悦嗣; 大貫 惇睦; et al.

Physical Review B, 88(24), p.245131_1 - 245131_13, 2013/12

https://doi.org/10.1103/PhysRevB.88.245131
 被引用回数：12 パーセンタイル：50.24(Materials Science, Multidisciplinary)

Detailed analyses of the cyclotron resonance lines in a uranium compound URu$$_2$$Si$$_2$$ are reported. The analyses of the resonance profiles reveals that the heavier branch of the split line has a larger scattering rate, providing evidence for the existence of hot-spot along the [110] direction. The result is consistent with the broken fourfold symmetry in the hidden-order phase.

論文

$$^{29}$$Si-NMR study of antiferromagnet CeRh$$_2$$Si$$_2$$ using single crystals

酒井 宏典; 徳永 陽; 神戸 振作; 松本 裕司; 松田 達磨; 芳賀 芳範

Journal of the Korean Physical Society, 63(3), p.352 - 355, 2013/08

https://doi.org/10.3938/jkps.63.352
 被引用回数：3 パーセンタイル：28.07(Physics, Multidisciplinary)

正方晶ThCr$$_2$$Si$$_2$$型結晶構造を持つ反強磁性体CeRh$$_2$$Si$$_2$$のNMR研究を単結晶を用いて行った。磁化率と同じく、ナイトシフトは$$c$$軸方向にイジング型磁気異方性を示した。$$^{29}$$Si核の超微細結合定数を$$a$$軸方向、$$c$$軸方向に対して、ナイトシフトと磁化率のプロットから決定した。

論文

Single crystal growth and physical properties of UT$$_2$$Al$$_{20}$$ (T = transition metal)

松本 裕司; 松田 達磨; 立岩 尚之; 山本 悦嗣; 芳賀 芳範; Fisk, Z.

Journal of the Korean Physical Society, 63(3), p.363 - 366, 2013/08

https://doi.org/10.3938/jkps.63.363
 被引用回数：6 パーセンタイル：44.56(Physics, Multidisciplinary)

We have studied single crystal growth and physical properties of the UT$$_2$$Al$$_{20}$$ system. We have successfully grown UT$$_2$$Al$$_{20}$$ (T = Cr, Ti, W and Mo) using Al self flux and characterized the crystals using electron probe microanalyzer (EPAM) and X-ray diffraction, and measured their magnetic and electric properties. The ground states of UT$$_2$$Al$$_{20}$$ (T = Cr, Mo and W) are Pauli paramagnetic as is likely also in UTi$$_2$$Al$$_{20}$$. The effective masses of UCr$$_2$$Al$$_{20}$$ and UTi$$_2$$Al$$_{20}$$ are only weakly enhanced.

論文

Separation of magnetic properties at uranium and cobalt sites in UCoAl using soft X-ray magnetic circular dichroism

竹田 幸治; 斎藤 祐児; 岡根 哲夫; 山上 浩志; 松田 達磨*; 山本 悦嗣; 芳賀 芳範; 大貫 惇睦; Fisk, Z.

Physical Review B, 88(7), p.075108_1 - 075108_6, 2013/08

https://doi.org/10.1103/PhysRevB.88.075108
 被引用回数：9 パーセンタイル：41.68(Materials Science, Multidisciplinary)

UCoAlは温度T=10K以下で、磁場H=1T以上で磁化の急激な増大を示し、常磁性状態から磁場誘起強磁性状態へのメタ磁性転移を示し、さらに磁場増大に伴い磁化も飽和することなく増大する。磁気コンプトン散乱(MCS)実験からは、メタ磁性転移に伴いスピン磁気モーメント(MS)も観測される。一方で、磁化測定では磁化は磁場印加とともに単調増大するのに対し、MCSの磁場依存性測定からはMSはH=3Tで消失する様子が観測されている。この原因は未解決であり、元素ごとの磁気構造及びその磁場依存性の研究が望まれていた。そこで本研究ではこの磁場誘起強磁性状態について、1Hz円偏光スイッチングを活用し、UとCo元素に対して元素選択磁化測定を行った。その結果、UとCoのMSは互いに逆の方向を向き、かつUとCoの磁場に対する磁気モーメントの増加率が異なることがわかった。これにより、MCSでのMSの消失に対して定性的な説明を与えることができた。さらに、磁場誘起強磁性状態でのUとCoの磁気モーメントの磁場依存性について、食い違いのある二つの偏極中性子散乱実験の先行研究があったが、この研究により決定的な情報を与えることができた。

論文

Single-crystal growth and physical properties of URhIn$$_5$$

松本 裕司*; 芳賀 芳範; 立岩 尚之; 酒井 宏典; 松田 達磨; 山本 悦嗣; Fisk, Z.

Physical Review B, 88(4), p.045120_1 - 045120_6, 2013/07

https://doi.org/10.1103/PhysRevB.88.045120
 被引用回数：7 パーセンタイル：34.48(Materials Science, Multidisciplinary)

We have grown the new uranium compound URhIn$$_5$$ with the tetragonal HoCoGa$$_5$$-type by the In self flux method. In contrast to the nonmagnetic ground state of the isoelectronic analogue URhGa$$_5$$, URhIn$$_5$$ is an antiferromagnet with antiferromagnetic transition temperature $$T_{rm N}$$ = 98 K. The moderately large electronic specific heat coefficient $$gamma$$ = 50 mJ/K$$^2$$mol demonstrates the contribution of 5f electrons to the conduction band.

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