sparse-ir; Optimal compression and sparse sampling of many-body propagators

Wallerberger, M.*; Badr, S.*; Hoshino, Shintaro*; Huber, S.*; Kakizawa, Fumiya*; Koretsune, Takashi*; Nagai, Yuki; Nogaki, Kosuke*; Nomoto, Takuya*; Mori, Hitoshi*; et al.

Software X (Internet), 21, p.101266_1 - 101266_7, 2023/02

https://doi.org/10.1016/j.softx.2022.101266

no abstracts in English

Safe and rapid development of capillary electrophoresis for ultratrace uranyl ions in radioactive samples by way of fluorescent probe selection for actinide ions from a chemical library

Haraga, Tomoko; Ouchi, Kazuki; Sato, Yoshiyuki; Hoshino, Hitoshi*; Tanana, Rei*; Fujihara, Takashi*; Kurokawa, Hideki*; Shibukawa, Masami*; Ishimori, Kenichiro; Kameo, Yutaka; et al.

Analytica Chimica Acta, 1032, p.188 - 196, 2018/11

https://doi.org/10.1016/j.aca.2018.05.077

The development of safe, rapid and highly sensitive analytical methods for radioactive samples, especially actinide (An) ions, represents an important challenge. Here we propose a methodology for selecting appropriate emissive probes for An ions with very low consumption and emission of radioactivity by capillary electrophoresis-laser-induced fluorescence detection (CE-LIF), using a small chemical library of probes with eight different chelating moieties. It was found that the emissive probe, which possesses the tetradentate chelating moiety, was suitable for detecting uranyl ions. The detection limit for the uranyl-probe complex using CE-LIF combined with dynamic ternary complexation and on-capillary concentration techniques was determined to be 0.7 ppt. This method was successfully applied to real radioactive liquid samples collected from nuclear facilities.

Effect of topsoil removal and selective countermeasures on radiocesium accumulation in rice plants in Fukushima paddy field

Yang, B.*; Onda, Yuichi*; Omori, Yoshihiro*; Sekimoto, Hitoshi*; Fujiwara, Toru*; Wakiyama, Yoshifumi*; Yoshimura, Kazuya; Takahashi, Junko*; Sun, X.*

Science of the Total Environment, 603-604, p.49 - 56, 2017/12

https://doi.org/10.1016/j.scitotenv.2017.06.026

Application of capillary electrophoresis with laser-induced fluorescence detection for the determination of trace neodymium in spent nuclear fuel using complexation with an emissive macrocyclic polyaminocarboxylate probe

Haraga, Tomoko; Saito, Shingo*; Sato, Yoshiyuki; Asai, Shiho; Hanzawa, Yukiko; Hoshino, Hitoshi*; Shibukawa, Masami*; Ishimori, Kenichiro; Takahashi, Kuniaki

Analytical Sciences, 30(7), p.773 - 776, 2014/07

https://doi.org/10.2116/analsci.30.773

A simple and rapid method with low radiation exposure risk was developed for the determination of neodymium in spent nuclear fuel by CE with LIF detection using a fluorescent ligand having a macrocyclic hexadentate polyaminocarboxylate structure. The concentration of Nd(III) in a spent nuclear fuel sample was determined with no interference from various matrix elements, including lanthanides and uranium (at a 200-fold excess), with 92 3% recovery. This is due to method's high resolution based on establishing a ternary complex equilibrium during migration in which the hydroxyl ion plays an auxiliary role.

Electronic structure of heavy fermion uranium compounds studied by core-level photoelectron spectroscopy

Fujimori, Shinichi; Okochi, Takuo*; Kawasaki, Ikuto; Yasui, Akira; Takeda, Yukiharu; Okane, Tetsuo; Saito, Yuji; Fujimori, Atsushi; Yamagami, Hiroshi; Haga, Yoshinori; et al.

Journal of the Physical Society of Japan, 81(1), p.014703_1 - 014703_9, 2012/01

https://doi.org/10.1143/JPSJ.81.014703

High-energy-resolution core-level and valence-band photoelectron spectroscopic studies were performed for the heavy Fermion uranium compounds UGe, UCoGe, URhGe, URuSi, UNiAl, UPdAl, and UPt as well as typical localized and itinerant uranium compounds to understand the relationship between the uranium valence state and their core-level spectral line shapes. The core-level spectra of UGe, UCoGe, URhGe, URuSi, and UNiAl are rather similar to those of itinerant compounds, suggesting that U 5 electrons in these compounds are well hybridized with ligand states. On the other hand, the core-level spectra of UPdAl and UPt show considerably different spectral line shapes from those of the itinerant compounds, suggesting that U 5 electrons in UPdAl and UPt are less hybridized with ligand states, leading to the correlated nature of U 5 electrons in these compounds.

Study on potential impacts of natural phenomena on a HLW geological disposal system

Kawamura, Makoto; Makino, Hitoshi; Sasao, Eiji; Niizato, Tadafumi; Yasue, Kenichi; Asamori, Koichi; Umeda, Koji; Ishimaru, Tsuneari; Osawa, Hideaki; Ebashi, Takeshi; et al.

JAEA-Research 2010-027, 85 Pages, 2010/09

JAEA-Research-2010-027.pdf:9.37MB

Japan Atomic Energy Agency (JAEA) have developed a formal evaluation method to assess the potential impacts of natural phenomena (earthquakes and faulting; volcanism; uplift, subsidence, denudation and sedimentation; climatic and sea-level changes) on a high level radioactive waste (HLW) disposal system for the purpose of maintenance of evaluation method for potential impacts of natural phenomena within more realistic view. In this report, we developed a framework as a part of the total system performance assessment for two purposes: the first one is quantification of relationship of characteristic of natural phenomena between geological environmental conditions (T-H-M-C-G), and the other one is quantification of relationship of T-H-M-C-G condition between parameters of performance assessment. We tried to apply the framework to all natural phenomena to confirm the effectiveness of the framework. On the other hand, we applied an argument-diagram that was developed one of the methods of the knowledge management to elicit future tasks. As a result, to apply the framework, we could show that information integration could carry out efficiently, and information integration was attained by the common framework by combining information on geohistory and existing information of natural phenomena and geological environmental conditions as modern-analogue. We could show that suitable scenarios might be chosen by information integration. Furthermore, we were able to elicit future tasks to this study by applying the argument-diagram.

Experimental observation of bulk band dispersions in the oxide semiconductor ZnO using soft X-ray angle-resolved photoemission spectroscopy

Kobayashi, Masaki*; Song, G.-S.*; Kataoka, Takashi*; Sakamoto, Yuta*; Fujimori, Atsushi; Okochi, Takuo*; Takeda, Yukiharu; Okane, Tetsuo; Saito, Yuji; Yamagami, Hiroshi; et al.

Journal of Applied Physics, 105(12), p.122403_1 - 122403_4, 2009/06

BB2009-1947.pdf:0.84MB

https://doi.org/10.1063/1.3116223

Study on evaluation method of potential impact of natural phenomena on a HLW disposal system

Kawamura, Makoto; Oi, Takao; Niizato, Tadafumi; Yasue, Kenichi; Tokiwa, Tetsuya; Niwa, Masakazu; Shimada, Koji; Kurosawa, Hideki; Asamori, Koichi; Kawachi, Susumu; et al.

JAEA-Research 2008-018, 47 Pages, 2008/03

JAEA-Research-2008-018.pdf:24.18MB

In this report, we sophisticated the framework as a part of the total system performance assessment for two purposes: the first one is quantification of relationship of characteristic of natural phenomena between geological environmental conditions (THMCG), and the other one is quantification of relationship of THMCG condition between parameters of performance assessment. On the other hand, we applied the sophisticated framework to all natural phenomena. As a result, to apply the sophisticated framework, we could show that information integration could carry out efficiently. Moreover, we have checked that the framework was applicable to all phenomena. Furthermore, we could show that suitable scenarios might be chosen by information integration.

Construction of the vertical test system for the superconducting cavity in KEK-STF

Yamamoto, Yasuchika*; Hayano, Hitoshi*; Kako, Eiji*; Noguchi, Shuichi*; Sato, Masato*; Shishido, Toshio*; Umemori, Kensei*; Watanabe, Ken*; Sakai, Hiroshi*; Shinoe, Kenji*; et al.

Proceedings of 5th Annual Meeting of Particle Accelerator Society of Japan and 33rd Linear Accelerator Meeting in Japan (CD-ROM), p.888 - 891, 2008/00

In KEK, the new Superconducting RF Test Facility(STF) is being constructed, including the electro-polish system (EP), the high pressure rinsing system (HPR), the clean-room, the refrigerator system, the high power RF source system, and the vertical test system. The cavity is generally measured in the vertical cryostat for the performance test. The new vertical test facility was constructed since the last year, and completed at the beginning of March. The first test was done for the total system check at the beginning of July.

Characterization of magnetic components in the diluted magnetic semiconductor ZnCoO by X-ray magnetic circular dichroism

Kobayashi, Masaki*; Ishida, Yukiaki*; Hwang, J. I.*; Mizokawa, Takashi*; Fujimori, Atsushi*; Mamiya, Kazutoshi*; Okamoto, Jun*; Takeda, Yukiharu; Okane, Tetsuo; Saito, Yuji; et al.

Physical Review B, 72(20), p.201201_1 - 201201_4, 2005/11

https://doi.org/10.1103/PhysRevB.72.201201

no abstracts in English