Annual report for research on geosphere stability for long-term isolation of radioactive waste in fiscal year 2023

Niwa, Masakazu; Shimada, Koji; Sueoka, Shigeru; Ishihara, Takanori; Hakoiwa, Hiroaki; Asamori, Koichi; Murakami, Osamu; Fukuda, Shoma; Ogita, Yasuhiro; Kagami, Saya; et al.

JAEA-Research 2024-013, 65 Pages, 2024/11

JAEA-Research-2024-013.pdf:4.22MB

This annual report documents the progress of research and development (R&D) in the 2nd fiscal year of the JAEA 4th Medium- and Long-term Plan (fiscal years 2022-2028) to provide the scientific base for assessing geosphere stability for long-term isolation of high-level radioactive waste. The plan framework is structured into the following categories: (1) Development and systematization of investigation techniques, (2) Development of models for long-term estimation and effective assessment, (3) Development of dating techniques. The current status of R&D activities with previous scientific and technological progress is summarized.

Analysis of the stress field around concealed active fault from minor faults-slip data collected by geological survey; An Example in the 1984 Western Nagano Earthquake region

Nishiyama, Nariaki; Nakajima, Toru; Goto, Akira*; Hakoiwa, Hiroaki; Nagata, Mitsuhiro; Shimada, Koji; Niwa, Masakazu

Earth and Space Science (Internet), 11(6), p.e2023EA003360_1 - e2023EA003360_15, 2024/06

https://doi.org/10.1029/2023EA003360

Earthquakes with magnitudes of 6-7 have been reported even in various active tectonic settings where fault deformation topography have not been detected. Therefore, delineating concealed active faults generating such earthquakes is necessary to reduce earthquake damage; however, few studies exist to provide its clues regarding such faults. The 1984 Western Nagano Earthquake in Japan was a main shock with a magnitude of Mj 6.8 and a depth of 2 km at the source. Solid bedrocks are well-exposed in the earthquake source region; however, no surface rupture have been identified, and the active fault is known to be concealed. In this study, we collected data on striations observed in fractures by geological survey around the source area of the 1984 Western Nagano Earthquake. Using the collected data, the multiple inverse method was used to estimate the stresses that affected the striation formation. Consequently, stresses similar to acting faults in this area were detected in minor faults around the known concealed active fault. This suggests that the minor faults might be part of the damage zone that has been developed around the concealed active fault. Some minor faults were recognized in Quaternary volcanic rocks, confirming that they experienced displacements recently. This study indicates the possibility of detecting concealed active faults in the bedrock by geological survey.

Stable hydrogen and oxygen isotope analyses of geological samples using a thermal conversion elemental analyzer-isotope ratio mass spectrometer at Tono Geoscience Center

Yamamoto, Yusuke*; Watanabe, Takahiro; Niwa, Masakazu; Shimada, Koji

JAEA-Testing 2023-003, 67 Pages, 2024/02

JAEA-Testing-2023-003.pdf:4.63MB

A long-term geosphere stability for geological disposal is evaluated by the past geological environmental changes and modern conditions. Stable hydrogen and oxygen isotope ratios (D, O) of geological samples are useful information to estimate the past environmental changes and modern conditions. Recently, the thermal conversion elemental analyzer and isotope ratio mass spectrometer (TC-EA/IRMS) were installed in the Tono Geoscience Center for D and O measurements of geological samples. In this study, we reported analytical methods of D and O using international standard reference materials. In addition, evaluation tests of uncertainty by repeated analyses of the standards were performed using the TC-EA/IRMS. Furthermore, the D and O analyses by the TC- EA/IRMS were also applied to fault rock samples.

Field-based description of near-surface crustal deformation in a high-strain shear zone; A Case study in southern Kyushu, Japan

Niwa, Masakazu; Shimada, Koji; Terusawa, Shuji*; Goto, Akira*; Nishiyama, Nariaki; Nakajima, Toru; Ishihara, Takanori; Hakoiwa, Hiroaki

Island Arc, 33(1), p.e12516_1 - e12516_16, 2024/02

https://doi.org/10.1111/iar.12516

To investigate the geological evidence of near-surface crustal deformations in a high-strain shear zone that has been geodetically identified but not associated with clear tectonic landforms, a fieldwork was conducted in E-W trending southern Kyushu high-strain shear zone, Japan. According to our study, an investigation based on the slip data from minor faults and the occurrences of fracture zones could help to identify a concealed fault that is small in terms of size to record tectonic landforms but can trigger large earthquakes.

Thermochronology of hydrothermal alteration zones in the Kii Peninsula, southwest Japan; An Attempt for detecting the thermal anomalies and implications to the regional exhumation history

Sueoka, Shigeru; Iwano, Hideki*; Danhara, Toru*; Niwa, Masakazu; Kanno, Mizuho; Kohn, B. P.*; Kawamura, Makoto; Yokoyama, Tatsunori; Kagami, Saya; Ogita, Yasuhiro; et al.

Earth, Planets and Space (Internet), 75(1), p.177_1 - 177_24, 2023/12

https://doi.org/10.1186/s40623-023-01921-5

Fluid-inclusion and thermochronometric analyses have been applied to hydrothermal alteration zones and their host rocks outcropping in the Hongu area of the Kii Peninsula, southwestern Japan in an attempt to detect thermal anomalies related to hydrothermal events and quantify the thermal effects on the host rocks. Hydrothermal events at ca 150 deg. C and ca 200 deg. C were identified by fluid-inclusion microthermometry of quartz veins in the alteration zones. For the host rocks and alteration zones, in the youngest population zircon yielded U-Pb dates ranging between ca 74.7-59.2 Ma, fission-track dates of ca 27.2-16.6 Ma, and (U-Th)/He single-grain dates of ca 23.6-8.7 Ma. Apatite yielded pooled fission-track ages of ca 14.9-9.0 Ma. The zircon U-Pb dates constrain the maximum depositional ages of the sedimentary samples. However, the fission-track and (U-Th)/He dates show no clear trend as a function of distance from the alteration zones. Hence, no thermal anomaly was detected in the surrounding host rocks based on the thermochronometric data patterns. The fission-track and (U-Th)/He dates are rather thought to record regional thermal and exhumation histories rather than a direct thermal imprint of fluid flow, probably because the duration of such activity was too short or because fluid flow occurred before regional cooling events and were later thermally overprinted. Apatite fission-track ages of ca 10 Ma may reflect regional mountain uplift and exhumation related to the obduction of the SW Japan lithospheric sliver onto the Shikoku Basin, or the rapid subduction of the Philippine Sea slab associated with the clockwise rotation of the Southwest Japan Arc.

Research plan on geosphere stability for long-term isolation of radioactive waste (Scientific program for fiscal year 2023)

Niwa, Masakazu; Shimada, Koji; Sueoka, Shigeru; Fujita, Natsuko; Yokoyama, Tatsunori; Ogita, Yasuhiro; Fukuda, Shoma; Nakajima, Toru; Kagami, Saya; Ogata, Manabu; et al.

JAEA-Review 2023-017, 27 Pages, 2023/10

JAEA-Review-2023-017.pdf:0.94MB

This report is a plan of research and development (R&D) on geosphere stability for long-term isolation of high-level radioactive waste (HLW) in Japan Atomic Energy Agency (JAEA), in fiscal year 2023. The objectives and contents in fiscal year 2023 are described in detail based on the JAEA 4th Medium- and Long-term Plan (fiscal years 2022-2028). In addition, the background of this research is described from the necessity and the significance for site investigation and safety assessment, and the past progress. The plan framework is structured into the following categories: (1) Development and systematization of investigation techniques, (2) Development of models for long-term estimation and effective assessment, (3) Development of dating techniques.

LA-ICPMS U-Pb dating of zircon in paleotsunami deposits from Miyazaki plain, southwest Japan

Watanabe, Takahiro; Kagami, Saya; Yokoyama, Tatsunori; Niwa, Masakazu

Chigaku Zasshi, 132(4), p.353 - 361, 2023/08

https://doi.org/10.5026/jgeography.132.353

U-Pb dating of detrital zircons in paleotsunami deposits from the 1662 CE Kanbun-Hyuganada sea earthquake, Miyazaki plain on the Pacific coast of southwest Japan, was performed by a laser ablation multi-collector inductively coupled plasma mass spectrometry (LA-ICPMS) system at Tono Geoscience Center, Japan Atomic Energy Agency. Twenty-five zircon grains were separated from the paleotsunami deposits by chemical abrasion and analyzed by the LA-ICPMS. U-Pb ages of the detrital zircons showed from ca. 14 Ma to 2405 Ma, and the age spectrum revealed high relative probability values around ca. 100 Ma and 2000 Ma. Detrital zircons with the age of ca. 100 Ma in the 1662 CE paleotsunami deposits could be partly originated from the Shimanto supergroup in southwest Japan. Moreover, the age spectrum of detrital zircons with Precambrian grains from the paleotsunami deposits was similar with those of fore-arc sandstones from central Kyushu Island.

A GIS-based approach for geomorphological analysis of volcanic edifices to estimate latent magma plumbing system (Contract research)

Nishiyama, Nariaki; Goto, Akira*; Tsukahara, Yuzuko; Kawamura, Makoto; Umeda, Koji*; Niwa, Masakazu

JAEA-Testing 2022-003, 51 Pages, 2022/09

JAEA-Testing-2022-003.pdf:5.24MB
JAEA-Testing-2022-003-appendix(CD-ROM).zip:1.12MB

Advancement of the evaluation technology of the magma activity range is essential as one of the technical issues related to volcanic and igneous activities in the evaluation of the long-term stability of the geological environment in the geological disposal of high-level radioactive waste. As an effective method, topographical analysis of volcanic edifices is expected to be used to determine the distribution area of dikes. In recent years, the development of computer-based topographic analysis technology has made it possible to simply perform a large volume of work that would otherwise be difficult due to the manual handling. This report describes an analysis method for the shape of contour lines that forms volcanic edifices using GIS software.

Efficient detection of methane seepage using a vehicle-mounted cavity ring-down spectroscopy analyzer

Niwa, Masakazu; Shimo, Michito*; Shimada, Koji; Goto, Akira

JAEA-Research 2022-004, 38 Pages, 2022/06

JAEA-Research-2022-004.pdf:2.86MB
JAEA-Research-2022-004-appendix(CD-ROM).zip:0.41MB

Methane (CH) seepage to the surface in the early stage of hydrocarbon exploration has attracted increasing attention. Also, detection of CH-rich fluid emission can be applied to reconnaissance surveys for safety management in geological disposal of radioactive waste because high-temperature fluids that come from slab dehydration along a subduction zone are often rich in CH. These fluids likely migrate along faults and fractures. In this study, we employed a portable analyzer that used a wavelength-scanned cavity ring-down spectroscopy (CRDS) with high accuracy (in ppb levels) and short measurement intervals (1 s). An on-vehicle measurement that employed the CRDS system was performed in the Hongu area in southeast Kii Peninsula, Japan, which included CH-bearing hot springs (Kawayu and Yunomine). The measurement near the hot springs detected a clear CH anomaly (2 ppm) that exceeded the background concentration. The estimation of CH diffusion in air based on the Gaussian plume model corresponded to the result of the on-vehicle measurement. This study confirmed that the method using the vehicle-mounted CRDS analyzer can help in quickly and easily identifying CH-bearing fluid emissions at the surface. Additionally, directions for use of the analyzer were summarized in this report.

Quantitative analyses of major and trace elements in geological samples using a portable energy dispersive X-ray fluorescence spectrometer at Tono Geoscience Center; An Analytical method of whole-rock geochemical composition by 3-mm diameter small spot measurements

Yamamoto, Yusuke; Watanabe, Takahiro; Niwa, Masakazu; Shimada, Koji

JAEA-Testing 2021-003, 58 Pages, 2022/01

JAEA-Testing-2021-003.pdf:6.82MB

A long term geosphere stability for geological disposal is evaluated by the past geological environmental changes and modern conditions. Whole-rock geochemical compositions in rocks and sediments are useful information to estimate the past environmental changes and modern conditions. Recently, the portable X-ray fluorescence (XRF) were installed in the Tono Geoscience Center for rapid and simple whole-rock geochemical analyses (original specification; 8 mm-diameter analysis). In particular, the 3 mm-diameter small spot analysis using the portable XRF was performed for quantitative analyses of small-weight geological samples. In this study, we reported a quantitative method for major and trace elements using calibration curves by standard reference materials, as well as evaluation tests of uncertainty by repeated analyses of the standards measured by the portable XRF (3 mm-diameter small spot analysis). Furthermore, the small spot quantitative analyses by the portable XRF were also applied to fault rock samples that have been analyzed in previous studies.