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Journal Articles

Superconductivity in noncentrosymmetric iridium silicide Li$$_2$$IrSi$$_3$$

Pyon, S.*; Kudo, Kazutaka*; Matsumura, Junichi*; Ishii, Hiroyuki*; Matsuo, Genta*; Nohara, Minoru*; Hojo, Hajime*; Oka, Kengo*; Azuma, Masaki*; Garlea, V. O.*; et al.

Journal of the Physical Society of Japan, 83(9), p.093706_1 - 093706_5, 2014/09

 Times Cited Count:33 Percentile:82.71(Physics, Multidisciplinary)

Journal Articles

Near term test plan using HTTR (High Temperature engineering Test Reactor)

Takada, Shoji; Iigaki, Kazuhiko; Shinohara, Masanori; Tochio, Daisuke; Shimazaki, Yosuke; Ono, Masato; Yanagi, Shunki; Nishihara, Tetsuo; Fukaya, Yuji; Goto, Minoru; et al.

Nuclear Engineering and Design, 271, p.472 - 478, 2014/05

 Times Cited Count:8 Percentile:53.31(Nuclear Science & Technology)

JAEA has carried out research and development to establish the technical basis of HTGRs using HTTR. To connect hydrogen production system to HTTR, it is necessary to ensure the reactor dynamics when thermal-load of the system is lost. Thermal-load fluctuation test is planned to demonstrate the reactor dynamics stability and to validate plant dynamics codes. It will be confirmed that the reactor become stable state during losing a part of removed heat at heat-sink. A temperature coefficient of reactivity is one of the important parameters for core dynamics calculations, and changes with burnup because of variance of fuel compositions. Measurement of temperature coefficient of reactivity has been conducted to confirm the validity of calculated temperature coefficient of reactivity. A LOFC test using HTTR has been carried out to verify the inherent safety under the condition of LOFC while the reactor shut-down system disabled.

JAEA Reports

Temperature coefficient measurement test of HTTR; Burn-up characteristic of temperature coefficients at reactor power 30 kW and 9 MW

Ono, Masato; Goto, Minoru; Shinohara, Masanori; Nojiri, Naoki; Tochio, Daisuke; Shimazaki, Yosuke; Yanagi, Shunki

JAEA-Technology 2013-001, 35 Pages, 2013/03

JAEA-Technology-2013-001.pdf:6.04MB

The temperature coefficient measurements of the HTTR have been carried out. In the beginning of the operation, temperature coefficients at the reactor power of 30 kW and 9 MW were obtained through 1999 to 2000. The operation days of the HTTR fuel reached 375 Effective Full Power Days (EFPD), which is over a half of design operation days (660 EFPD). The temperature coefficient measurements were conducted at the same power levels of 30 kW and 9 MW to evaluate burnup effect. Also, to measure temperature coefficient in high accuracy, technique of core temperature control and technique of core temperature homogenization were established.

Journal Articles

Long-term high-temperature operation of the HTTR

Goto, Minoru; Shinohara, Masanori; Tochio, Daisuke; Shimazaki, Yosuke; Hamamoto, Shimpei; Tachibana, Yukio

Nuclear Engineering and Design, 251, p.181 - 190, 2012/10

 Times Cited Count:24 Percentile:84.89(Nuclear Science & Technology)

30-days operation in rated operation mode and 50-days operation in high-temperature operation mode were performed to obtain various characteristic data of HTGR. The main test results are as follows:(1) Coated fuel particle (CFP) of the HTTR has excellent confinement ability of fission product which is the highest performance in the world, (2) The measurement temperature of the core internals is good agreement with the design value so that their structural integrity is maintained, and (3) The intermediate heat exchanger keeps excellent heat transfer performance from beginning of operation. Additionally, the following two issues were validated using the HTTR burnup data. (1) The effectiveness of rod-type burnable poisons on reactivity control in the HTTR, and (2) The whole core burnup calculation method for nuclear characteristics of the HTTR.

Journal Articles

Test plan using HTTR (High Temperature engineering Test Reactor)

Takada, Shoji; Iigaki, Kazuhiko; Shinohara, Masanori; Tochio, Daisuke; Shimazaki, Yosuke; Ono, Masato; Nishihara, Tetsuo; Fukaya, Yuji; Goto, Minoru; Tachibana, Yukio; et al.

Proceedings of 6th International Topical Meeting on High Temperature Reactor Technology (HTR 2012) (USB Flash Drive), 8 Pages, 2012/10

JAEA has carried out research and development to establish the technical basis of HTGRs using HTTR. LOFC test to verify the inherent safety of HTGR under the condition of loss of forced cooling while the reactor shut-down system disabled was initiated. A temperature coefficient of reactivity is one of the important parameters for core dynamics calculations for safety analysis, and changes with burnup because of variance of fuel compositions, which has been measured to confirm the validity of the calculated ones. In order to connect hydrogen production system to HTTR, it is necessary to ensure the reactor safety when thermal-load of the hydrogen production system is lost. Thermal load fluctuation test is planned to demonstrate the reactor safety and gain the test data for validation of the plant dynamics code. It will be confirmed that the reactor become stable state during a part of removed heat at HTTR heat-sink is lost.

Journal Articles

Feasible evaluation of neutron capture therapy for hepatocellular carcinoma using selective enhancement of boron accumulation in tumour with intra-arterial administration of boron-entrapped water-in-oil-in-water emulsion

Yanagie, Hironobu*; Kumada, Hiroaki*; Nakamura, Takemi; Higashi, Shushi*; Ikushima, Ichiro*; Morishita, Yasuyuki*; Shinohara, Atsuko*; Fujiwara, Mitsuteru*; Suzuki, Minoru*; Sakurai, Yoshinori*; et al.

Proceedings of 14th International Congress on Neutron Capture Therapy (ICNCT-14) (CD-ROM), p.157 - 160, 2010/10

Journal Articles

Anomalous metallic state in the vicinity of metal to valence-bond solid insulator transition in LiVS$$_{2}$$

Katayama, Naoyuki*; Uchida, Masaya*; Hashizume, Daisuke*; Niitaka, Seiji*; Matsuno, Jobu*; Matsumura, Daiju; Nishihata, Yasuo; Mizuki, Junichiro; Takeshita, Nao*; Gauzzi, A.*; et al.

Physical Review Letters, 103(14), p.146405_1 - 146405_4, 2009/10

 Times Cited Count:59 Percentile:88.48(Physics, Multidisciplinary)

We investigate LiVS$$_{2}$$ and LiVSe$$_{2}$$ with a triangular lattice as itinerant analogues of LiVO$$_{2}$$ known for the formation of a valence-bond solid (VBS) state out of an S = 1 frustrated magnet. LiVS$$_{2}$$, which is located at the border between a metal and a correlated insulator, shows a first order transition from a paramagnetic metal to a VBS insulator at T$$_{c}$$ $$sim$$ 305 K upon cooling. The presence of a VBS state in the close vicinity of insulator-metal transition may suggest the importance of itinerancy in the formation of a VBS state. We argue that the high temperature metallic phase of LiVS$$_{2}$$ has a pseudogap, likely originating from the VBS fluctuation. LiVSe$$_{2}$$ was found to be a paramagnetic metal down to 2 K.

Journal Articles

Contribution to improvement of HTGR technology by using HTTR operation data

Nakagawa, Shigeaki; Tochio, Daisuke; Shinohara, Masanori; Nojiri, Naoki; Nishihara, Tetsuo; Goto, Minoru; Takamatsu, Kuniyoshi

Proceedings of 2009 International Congress on Advances in Nuclear Power Plants (ICAPP '09) (CD-ROM), p.9476_1 - 9476_6, 2009/05

Journal Articles

Hexafluoro complex of rutherfordium in mixed HF/HNO$$_{3}$$ solutions

Toyoshima, Atsushi; Haba, Hiromitsu*; Tsukada, Kazuaki; Asai, Masato; Akiyama, Kazuhiko*; Goto, Shinichi*; Ishii, Yasuo; Nishinaka, Ichiro; Sato, Tetsuya; Nagame, Yuichiro; et al.

Radiochimica Acta, 96(3), p.125 - 134, 2008/03

 Times Cited Count:28 Percentile:85.1(Chemistry, Inorganic & Nuclear)

Formation of an anionic fluoride-complex of element 104, rutherfordium (Rf) produced in the $$^{248}$$Cm($$^{18}$$O,5n)$$^{261}$$Rf reaction was studied by an anion-exchange method based on an atom-at-a-time scale. It was found that the hexafluoro complex of Rf, [RfF$$_{6}$$]$$^{2-}$$, was formed in the studied fluoride ion concentrations of 0.0005 - 0.013 M. Formation of [RfF$$_{6}$$]$$^{2-}$$ was significantly different from that of the homologues Zr and Hf, [ZrF$$_{6}$$]$$^{2-}$$ and [HfF$$_{6}$$]$$^{2-}$$; the evaluated formation constant of [RfF$$_{6}$$]$$^{2-}$$ is at least one-order of magnitude smaller than those of [ZrF$$_{6}$$]$$^{2-}$$ and [HfF$$_{6}$$]$$^{2-}$$.

JAEA Reports

Countermeasure to prevent residence nitrogen gas in Pressurized Water Cooling System

Furusawa, Takayuki; Saikusa, Akio; Hamamoto, Shimpei; Nemoto, Takahiro; Shinohara, Masanori; Isozaki, Minoru

JAEA-Technology 2007-066, 38 Pages, 2008/01

JAEA-Technology-2007-066.pdf:15.66MB

In the HTTR rise-to-power test which was performed from April in 2000 as phase 1 up to 10MW, nitrogen gas remained in the air cooler which release the heat to atmosphere. This residence nitrogen gas causes the reduction of the thermal performance of the air cooler. So, it was impossible that heat generated reactor core could not remove when reactor operated full power operation. A mockup test was carried out to investigate the occurrence mechanism of the residence nitrogen gas. From a result of the mockup test, we clarified that the marked wave rise in the water pressurizer and the melting velocity of the nitrogen gas into the pressurized water is thought to be higher than expected. Therefore, we installed a hollow type plate, multi-hole type plate and so on in the water pressurizer. As a result, it was confirmed that no residence nitrogen gas in the air cooler during rise-to-power test and normal operation. Consequently, the hollow type plate and multi-hole type plate were effective for prevention of the residence nitrogen gas in the air cooler. This paper describes the results of the mockup test and the improvement of the water pressurizer.

JAEA Reports

Evaluation of heat exchange performance for secondary pressurized water cooler in HTTR

Tochio, Daisuke; Watanabe, Shuji; Saikusa, Akio; Oyama, Sunao; Nemoto, Takahiro; Hamamoto, Shimpei; Shinohara, Masanori; Isozaki, Minoru; Nakagawa, Shigeaki

JAEA-Technology 2006-005, 83 Pages, 2006/02

JAEA-Technology-2006-005.pdf:6.09MB

In High Temperature Engineering Test Reactor (HTTR), the rated thermal power of 30MW, the generated heat at reactor core is finally dissipated at the air-cooler by way of the heat exchangers of the primary cooling system, such as the intermediate heat exchanger (IHX) and the secondary pressurized water cooler (SPWC). The heat exchangers in the main cooling system are required the heat exchange performance to remove the reactor-generated-heat of 30MW under the condition of reactor coolant outlet temperature of 850 $$^{circ}$$C/ 950 $$^{circ}$$C. Therefore, the heat exchanges are required to satisfy the design criteria of heat exchange performance. In this report, heat exchange performance of the SPWC in the main cooling system was evaluated with the rise-to-power-up test and the in-service operation data. Moreover, evaluated value is compared with designed one, it is confirmed that the SPWC has required heat exchange performance.

Journal Articles

Chemical studies on rutherfordium (Rf) at JAERI

Nagame, Yuichiro; Tsukada, Kazuaki; Asai, Masato; Toyoshima, Atsushi; Akiyama, Kazuhiko; Ishii, Yasuo; Sato, Tetsuya; Hirata, Masaru; Nishinaka, Ichiro; Ichikawa, Shinichi; et al.

Radiochimica Acta, 93(9-10), p.519 - 526, 2005/00

 Times Cited Count:30 Percentile:87.1(Chemistry, Inorganic & Nuclear)

no abstracts in English

JAEA Reports

Annual Report on the Effluent Control of Tokai Works FY2003

Shinohara, Kunihiko; Takeishi, Minoru; Hitoshi, Watanabe,; Uezu, Yasuhiro; Mizutani, Tomoko; Hiyama, Yoshinori*; Fujii, Jun*

JNC TN8440 2004-015, 138 Pages, 2004/12

JNC-TN8440-2004-015.pdf:7.78MB

This report was written about the effluent control in JNC Tokai Works from 1st April 2003 to 31th March 2004. In this period, the quantities and concentrations of retroactivities in liquid waste from Tokai Works were under the discharge limits of "Safety Regulations for the Tokai Reprocessing Plant" and regulations of government.

Journal Articles

Fluoride complexation of element 104, rutherfordium

Haba, Hiromitsu*; Tsukada, Kazuaki; Asai, Masato; Toyoshima, Atsushi; Akiyama, Kazuhiko; Nishinaka, Ichiro; Hirata, Masaru; Yaita, Tsuyoshi; Ichikawa, Shinichi; Nagame, Yuichiro; et al.

Journal of the American Chemical Society, 126(16), p.5219 - 5224, 2004/04

 Times Cited Count:43 Percentile:72.51(Chemistry, Multidisciplinary)

Fluoride complexation of element 104, rutherfordium (Rf), produced in the $$^{248}$$Cm($$^{18}$$O,5n)$$^{261}$$Rf reaction has been studied by anion-exchange chromatography on an atom-at-a-time scale. The anion-exchangechromatographic behavior of Rf was investigated in 1.9-13.9 M hydrofluoric acid together with those of the group-4 elements Zr and Hf produced in the $$^{18}$$O-induced reactions on Ge and Gd targets, respectively. It was found that the adsorption behavior of Rf on anion-exchange resin is quite different from those of Zr and Hf, suggesting the influence of relativistic effect on the fluoride complexation of Rf.

JAEA Reports

Annual Report on the Effluent Control of Tokai Works FY2003

Mizutani, Tomoko; Uezu, Yasuhiro; Hitoshi, Watanabe,; Takeishi, Minoru; Shinohara, Kunihiko; Hiyama, Yoshinori*; Kikuchi, Masaaki*

JNC TN8440 2003-024, 144 Pages, 2003/11

JNC-TN8440-2003-024.pdf:7.72MB

This report was written about the effluent control in JNC Tokai Works from 1st April 2002 to 31th March 2003. In this period, the quantities and concentrations of retroactivities in liquid waste from Tokai Works were under the discharge limits of "Safety Regulations for the Tokai Reprocessing Plant" and regulations of government.

JAEA Reports

Annual Report on Activities of Radiation Protection Division at JNC Tokai Works in Fiscal Year of 2002

Shinohara, Kunihiko; Asano, Tomohiro; Momose, Takumaro; Takeishi, Minoru; Kobayashi, Hirohide; Oka, Tsutomu; Takasaki, Koji

JNC TN8440 2003-020, 125 Pages, 2003/09

JNC-TN8440-2003-020.pdf:11.14MB

This annual report summarizes the activities of the Radiation Protection Division at JNC Tokai Works in fiscal 2002.The Tokai Works undertakes various research and development for the reprocessing of spent fuel, plutonium fuel fabrication, fast reactor fuel recycling technology, and radioactive waste treatment and disposal, all of which are done under strict safety management.The major radiation facilities in the Tokai Works are the Tokai Reprocessing Plant (TRP), which has been in operation since 1977, three MOX fuel fabrication facilities, the first of which has been in operation since 1965, the Chemical Processing Facility (CPF) where fast reactor (FR) reprocessing technologies are being developed, and various other radioisotope and uranium research laboratories.The Radiation Protection Division is responsible for radiation control in and around these facilities, including personnel monitoring, workplace monitoring, consultation on radiological work planning and evaluation, monitoring of gas and liquid waste effluents, environmental monitoring, instrumentation, calibration, quality assurance, and safety research. The Division also provides technical support and cooperation to other international and domestic institutes in the radiation protection field.In fiscal 2002, the results of radiological monitoring showed the situation to be normal, and no radiological incident or accident occurred. The maximum annual effective dose to radiation workers was 6.5 mSv and the mean annual effective dose was 0.1 mSv. Individual doses were kept within the annual dose limit specified in the safety regulations. The estimated effective dose caused by gas and liquid effluents from the TRP to members of the public around the Tokai Works was 4.2 * 10$$^{-4}$$mSv. Environmental monitoring and effluent control were performed appropriately in compliance with safety regulation and standards.

JAEA Reports

Annual report on the environmental radiation monitoring around Tokai reprocessing plant; FY 2002

Shinohara, Kunihiko; Takeishi, Minoru; ; ; ; Takeyasu, Masanori;

JNC TN8440 2003-010, 148 Pages, 2003/06

JNC-TN8440-2003-010.PDF:4.22MB

Environmental radiation monitoring around the Tokai Reprocessing Plant has been performed since 1975, based on "Safety Regulations for the Tokai Reprocessing Plant, Chapter IV - Environmental Monitoring". This annual report presents the results of the environmental monitoring and the dose estimation to the hypothetical inhabitant due to the radioactivity discharged from the plant during April 2002 to March 2003. Appendices present comprehensive information, such as monitoring program, monitoring results, meteorological data and annual discharges from the plant.

JAEA Reports

Data book on the current of Tokai Reprocessing plant; January - December, 1998

Shinohara, Kunihiko; Takeishi, Minoru; ; ; Isozaki, Tokuju; Ao, Hidetoshi*; *

JNC TN8450 2003-004, 99 Pages, 2002/11

JNC-TN8450-2003-004.pdf:4.64MB

Current direction, velocity water temperature, salinity and etc. were observed by current meters which were set near the outlet (36$$^{circ}$$ 26' 51" N, 140$$^{circ}$$ 39' 02" E) of the discharge pipe of the reprocessing plant in JNC Tokai Works. Besides, the horizontal (26 points) and vertical (14 points) observation of water temperature and salinity were executed using the monitoring ship (Seikai). The observation region ranged from 36$$^{circ}$$ 22' N to 36$$^{circ}$$ 30' N and from 140$$^{circ}$$ 37' E to 140$$^{circ}$$ 42'. The data, which were observed in 1999, were described in this report.

JAEA Reports

Data book on the current of Tokai Reprocessing plant; January - December, 1998

Shinohara, Kunihiko; Takeishi, Minoru; ; ; Isozaki, Tokuju; Ao, Hidetoshi*; *

JNC TN8450 2003-003, 99 Pages, 2002/11

JNC-TN8450-2003-003.pdf:4.73MB

Current direction, velocity water temperature, salinity and etc. were observed by current meters which were set near the outlet (36$$^{circ}$$ 26' 51" N, 140$$^{circ}$$ 39' 02" E) of the discharge pipe of the reprocessing plant in JNC Tokai Works. Besides, the horizontal (26 points) and vertical (14 points) observation of water temperature and salinity were executed using the monitoring ship (Seikai). The observation region ranged from 36$$^{circ}$$ 22' N to 36$$^{circ}$$ 30' N and from 140$$^{circ}$$ 37' E to 140$$^{circ}$$ 42'. The data, which were observed in 1998, were described in this report.

JAEA Reports

Data book on the current of Tokai Reprocessing Plant; January - December, 1997

Shinohara, Kunihiko; Takeishi, Minoru; ; ; Isozaki, Tokuju; Ao, Hidetoshi*; *

JNC TN8450 2003-002, 99 Pages, 2002/11

JNC-TN8450-2003-002.pdf:4.59MB

Current direction, velocity, water temperature, salinity and etc. were observed by current meters which were set near the outlet (36$$^{circ}$$ 26' 51" N, 140$$^{circ}$$ 39' 02" E) of the discharge pipe of the reprocessing plant in JNC Tokai Works. Besides, the horizontal (26 points) and vertical (14 points) observation of water temperature and salinity were executed using the monitoring ship (Seikai). The observation region ranged from 36$$^{circ}$$C 22' N to 36$$^{circ}$$ 30' N and from 140$$^{circ}$$ 37' E to 140$$^{circ}$$ 42'. The data, which were observed in 1997, were described in this report.

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