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Bayesian sparse modeling of extended X-ray absorption fine structure to determine interstitial oxygen positions in yttrium oxyhydride epitaxial thin film

熊添 博之*; 五十嵐 康彦*; Iesari, F.*; 清水 亮太*; 小松 遊矢*; 一杉 太郎*; 松村 大樹; 齋藤 寛之*; 岩満 一功*; 岡島 敏浩*; et al.

AIP Advances (Internet), 11(12), p.125013_1 - 125013_5, 2021/12

This letter presents a Bayesian sparse modeling method to analyze extended X-ray absorption fine structure (EXAFS) data with basis functions built on two-body signals. This method allows us to evaluate regression coefficients proportional to the radial distribution functions of the respective elements and their errors and is very effective for analysis of EXAFS with weak absorption intensity and severe signal-to-noise ratio. As an application example, we used it to analyze EXAFS of an yttrium oxyhydride (YO$$_{x}$$H$$_{y}$$) epitaxial thin film. This EXAFS data shows weak absorption intensity due to the small amount of X-ray absorption in the thin film sample. However, this approach revealed that the radial distance ratio of the second neighbor yttrium to the first neighbor oxygen coincides with that of a tetrahedral configuration. This result demonstrates that the interstitial oxygen position is tetrahedral in the YO$$_{x}$$H$$_{y}$$ thin film.


$$q$$=0 long-range magnetic order in centennialite CaCu$$_{3}$$(OD)$$_{6}$$Cl$$_{2}$$ $$cdot$$ 0.6D$$_{2}$$O; A Spin-$$frac{1}{2}$$ perfect kagome antiferromagnet with $$J_{1}$$-$$J_{2}$$-$$J_{d}$$

飯田 一樹*; 吉田 紘行*; 中尾 朗子*; Jeschke, H. O.*; Iqbal, Y.*; 中島 健次; 河村 聖子; 宗像 孝司*; 稲村 泰弘; 村井 直樹; et al.

Physical Review B, 101(22), p.220408_1 - 220408_6, 2020/06

 被引用回数:6 パーセンタイル:75.71(Materials Science, Multidisciplinary)

鉱物センテニアライトCaCu$$_{3}$$(OD)$$_{6}$$Cl$$_{2}$$ $$cdot$$ 0.6D$$_{2}$$Oの結晶構造と磁気構造をシンクロトロンX線回折と中性子回折測定に密度汎関数理論(DFT)と疑似フェルミオン汎関数繰り込み群(PFFRG)の計算を組み合わせることで調べた。CaCu$$_{3}$$(OD)$$_{6}$$Cl$$_{2}$$ $$cdot$$ 0.6D$$_{2}$$OではCu$$^{2+}$$イオンは反強磁性$$J_{1}$$と幾何学的に完全なカゴメネットワークを形成する。Cu$$^{2+}$$とCa$$^{2+}$$イオン間のサイト間無秩序は見つからなかった。CaCu$$_{3}$$(OD)$$_{6}$$Cl$$_{2}$$ $$cdot$$ 0.6D$$_{2}$$Oは$$T$$$$_{rm N}$$=7.2K以下で磁気秩序を示し、負のベクトルスピンキラリティーを持つ$$q$$=0の磁気構造が現れる。0.3Kでの秩序モーメントは0.58(2)$$mu$$Bに抑えられている。我々のDFT計算では、この系が量子臨界点の近くにあり、$$J_{1}$$-$$J_{2}$$-$$J_{d}$$カゴメ反強磁性体の優れた実現であることを示唆している。


First direct mass measurements of nuclides around $$Z$$ = 100 with a multireflection time-of-flight mass spectrograph

伊藤 由太*; Schury, P.*; 和田 道治*; 新井 郁也*; 羽場 宏光*; 平山 賀一*; 石澤 倫*; 加治 大哉*; 木村 創大*; 小浦 寛之; et al.

Physical Review Letters, 120(15), p.152501_1 - 152501_6, 2018/04

 被引用回数:47 パーセンタイル:95.52(Physics, Multidisciplinary)

冷たい核融合反応および熱い融合反応によって生成した変形閉殻中性子数152の近傍に位置する原子核$$^{246}$$Es, $$^{251}$$Fm、および超フェルミウム原子核$$^{249-252}$$Md, $$^{254}$$Noの質量の直接測定を、多反射時間飛行質量分析装置(MR-TOF)を用いて実施した。$$^{246}$$Esおよび$$^{249,250,252}$$Mdの質量測定は世界で初めての成果である。さらに$$^{249,250}$$Mdの質量を$$alpha$$崩壊連鎖のアンカーポイントとして用いて$$^{261}$$Bhおよび$$^{266}$$Mtまでの重い原子核の質量を決定した。これらの新測定された質量を理論質量計算と比較し、巨視的・微視的模型の予測値と良い一致が見られることを示した。近接する3つの質量値から求められる経験的殻ギャップエネルギー$$delta_{2n}$$を今回の質量値から求め、MdおよびLrに対する変形閉殻中性子数$$N=152$$の存在を裏付ける結果を得た。


High order harmonics from relativistic electron spikes

Pirozhkov, A. S.; 神門 正城; Esirkepov, T. Z.; Faenov, A. Y.*; Pikuz, T. A.*; 河内 哲哉; 匂坂 明人; Koga, J. K.; 森 道昭; 川瀬 啓悟*; et al.

RAL-TR-2015-025, P. 22, 2015/00

We provide a description of experiments performed with the J-KAREN and Astra Gemini lasers where we discovered a new regime of relativistic high-order harmonic generation by multi-terawatt femtosecond lasers in gas targets. The results were explained using particle-in-cell simulations and catastrophe theory. Our work paves the way towards a bright coherent X-ray source based on compact lasers and accessible, repetitive, and debris-free gas jet targets. Such a source will be crucial for fundamental research and numerous applications requiring pumping, probing, imaging of microscopic objects and for attosecond science.


High order harmonics from relativistic electron spikes

Pirozhkov, A. S.; 神門 正城; Esirkepov, T. Z.; Gallegos, P.*; Ahmed, H.*; Ragozin, E. N.*; Faenov, A. Ya.*; Pikuz, T. A.*; 河内 哲哉; 匂坂 明人; et al.

New Journal of Physics (Internet), 16(9), p.093003_1 - 093003_30, 2014/09

 被引用回数:25 パーセンタイル:81.51(Physics, Multidisciplinary)

We present a detailed description of our discovery of a new regime of high-order harmonic generation, including experimental data, simulations, and description of new harmonic generation mechanism. The harmonics are generated by multi-terawatt relativistic-irradiance ($$>$$ 10$$^{18}$$ W/cm$$^2$$) femtosecond ($$approx$$ 30-50 fs) lasers focused to gas jet targets. According to our model, the harmonics are produced by sharp, structurally stable, oscillating electron spikes at the joint of boundaries of wake and bow waves excited by the laser pulse.


Observation of preformed plasma generated from a thin-foil target for laser-driven proton acceleration

匂坂 明人; Pirozhkov, A. S.; 西内 満美子; 小倉 浩一; 榊 泰直; 余語 覚文; 森 道昭; 桐山 博光; 岡田 大; 金沢 修平; et al.

レーザー研究, 42(2), p.160 - 162, 2014/02



A Multi-reflection time-of-flight mass spectrograph for short-lived and super-heavy nuclei

Schury, P. H.*; 和田 道治*; 伊藤 由太*; Naimi, S.*; 園田 哲*; 三田 浩希*; 高峰 愛子*; 岡田 邦宏*; Wollnik, H.*; Chon, S.*; et al.

Nuclear Instruments and Methods in Physics Research B, 317(Part B), p.537 - 543, 2013/12

 被引用回数:26 パーセンタイル:92.04(Instruments & Instrumentation)



Relativistic high harmonic generation in gas jet targets

Pirozhkov, A. S.; 神門 正城; Esirkepov, T. Z.; Gallegos, P.*; Ahmed, H.*; Ragozin, E. N.*; Faenov, A. Ya.*; Pikuz, T.; 河内 哲哉; 匂坂 明人; et al.

AIP Conference Proceedings 1465, p.167 - 171, 2012/07

 被引用回数:1 パーセンタイル:49.39

We experimentally demonstrate new regime of high-order harmonic generation by relativistic-irradiance lasers in gas jet targets. Bright harmonics with both the odd and even orders are emitted in the forward direction, while the base harmonic frequency is downshifted. The harmonics are generated by linearly as well as circularly polarized pulses. With the 9 TW laser, the harmonics reach 360 eV, within the "water window" spectral region. Using 120 TW laser producing 40 uJ/sr per harmonic at 120 eV, we demonstrate the photon number scalability. The experimentally demonstrated harmonics cannot be explained by previously known mechanisms. We introduce a novel high-order harmonics generation mechanism, which explains our experimental findings.


High-order harmonics from bow wave caustics driven by a high-intensity laser

Esirkepov, T. Z.; Pirozhkov, A. S.; 神門 正城; Gallegos, P.*; Ahmed, H.*; Ragozin, E. N.*; Faenov, A.*; Pikuz, T.; 河内 哲哉; 匂坂 明人; et al.

AIP Conference Proceedings 1465, p.172 - 180, 2012/07

 被引用回数:0 パーセンタイル:0.13



X-ray emission from relativistically moving electron density cusps

神門 正城; Pirozhkov, A. S.; 中村 龍史; 林 由紀雄; 小瀧 秀行; 川瀬 啓悟*; Esirkepov, T. Z.; 福田 祐仁; 桐山 博光; 岡田 大; et al.

AIP Conference Proceedings 1465, p.159 - 166, 2012/07

 被引用回数:0 パーセンタイル:0.13

We report on novel method to generate ultra-short coherent X-rays using a laser-plasma interaction. Nonlinear interaction of intense laser pulses with plasma creates stable, specific structures such as electron cusps. For example wake waves excited in an underdense plasma by the laser become dense and propagate along with the laser pulse (Flying Mirror). The flying mirror can reflect a counter-propagating laser pulse and directly convert it into high-frequency radiation and compress the pulse. We have conducted experimental results using 9 TW laser with a He gas target. We observed 10$$^{10}$$ photons in the extreme ultra-violet region (12.8-22.0 nm).


Complementary characterization of radioactivity produced by repetitive laser-driven proton beam using shot-to-shot proton spectral measurement and direct activation measurement

小倉 浩一; 静間 俊行; 早川 岳人; 余語 覚文; 西内 満美子; 織茂 聡; 匂坂 明人; Pirozhkov, A. S.; 森 道昭; 桐山 博光; et al.

Japanese Journal of Applied Physics, 51(4), p.048003_1 - 048003_2, 2012/04

 被引用回数:2 パーセンタイル:10.01(Physics, Applied)



Soft-X-ray harmonic comb from relativistic electron spikes

Pirozhkov, A. S.; 神門 正城; Esirkepov, T. Z.; Gallegos, P.*; Ahmed, H.*; Ragozin, E. N.*; Faenov, A. Ya.*; Pikuz, T.; 河内 哲哉; 匂坂 明人; et al.

Physical Review Letters, 108(13), p.135004_1 - 135004_5, 2012/03

 被引用回数:64 パーセンタイル:91.71(Physics, Multidisciplinary)



Low-background prebunching system for heavy-ion beams at the Tokai radioactive ion accelerator complex

岡田 雅之*; 仁木 和昭*; 平山 賀一*; 今井 伸明*; 石山 博恒*; Jeong, S. C.*; 片山 一郎*; 宮武 宇也*; 小柳津 充広*; 渡辺 裕*; et al.

Physical Review Special Topics; Accelerators and Beams, 15(3), p.030101_1 - 030101_10, 2012/03

 被引用回数:1 パーセンタイル:10.62(Physics, Nuclear)

A novel beam-bunching technique has been implemented at a heavy-ion linear accelerator facility by installing a compact two-gap prebuncher and a multi-layer beam chopper. A pulsed beam of 2 to 4 MHz, having kinetic energy up to 1.1 MeV/u, is realized by bunching 2 keV/u continuous beams just upstream of the linac. Around 40% of the continuous beam particles are successively gathered in a single micro-bunch with a time width of around 15 ns in units of full-width at one-tenth maximum. The number of background beam particles over 250 ns just before the bunched beam is well suppressed to less than 10$$^{-4}$$ of the number of bunched particles. This technique has been adopted to generate intense $$alpha$$-particle beams for nuclear astrophysics experiments.


Development of a compact high-spatiotemporal-quality Yb:YAG thin-disk laser system using an optical parametric preamplifier

桐山 博光; 鈴木 将之*; 大東 出; 岡田 大; 越智 義浩; 佐藤 方俊*; 玉置 善紀*; 吉井 健裕*; 前田 純也*; 松岡 伸一*; et al.

レーザー研究, 40(2), p.143 - 145, 2012/02



Laser-driven proton generation with a thin-foil target

匂坂 明人; Pirozhkov, A. S.; 森 道昭; 余語 覚文; 小倉 浩一; 織茂 聡; 西内 満美子; Ma, J.*; 桐山 博光; 金沢 修平; et al.

NIFS-PROC-85, p.30 - 33, 2011/02



Laser ceramic materials for subpicosecond solid-state lasers using Nd$$^{3+}$$ -doped mixed scandium garnets

岡田 大; 田中 桃子; 桐山 博光; 中井 善基*; 越智 義浩; 杉山 僚; 大道 博行; 木村 豊秋*; 柳谷 高公*; 八木 秀喜*; et al.

Optics Letters, 35(18), p.3048 - 3050, 2010/09

 被引用回数:12 パーセンタイル:54.33(Optics)

We have successfully developed and demonstrated broadband emission Nd-doped mixed scandium garnets based on laser ceramic technology. The inhomogeneous broadening of Nd$$^{3+}$$ fluorescence lines results in a bandwidth above 5 nm that is significantly broader than that for Nd:YAG and enables subpicosecond mode-locked pulse durations. We have also found the emission cross-section of 7.8$$times$$10$$^{-20}$$ cm$$^{2}$$ to be adequate for efficient energy extraction and thermal conductivity of 4.7 W/mK from these new Nd-doped laser ceramics. The new laser ceramics are good candidates for laser host material in diode-pumped subpicosecond laser system with high efficiency and high repetition rate.



桐山 博光; 森 道昭; 中井 善基*; 下村 拓也; 笹尾 一*; 田中 桃子; 越智 義浩; 田上 学*; 近藤 修司; 金沢 修平; et al.

レーザー研究, 38(9), p.669 - 675, 2010/09



Proton generation and terahertz radiation from a thin-foil target with a high-intensity laser

匂坂 明人; Pirozhkov, A. S.; 森 道昭; 余語 覚文; 小倉 浩一; 織茂 聡; 西内 満美子; Ma, J.*; 桐山 博光; 金沢 修平; et al.

レーザー研究, 38(9), p.702 - 705, 2010/09



Measured and simulated transport of 1.9 MeV laser-accelerated proton bunches through an integrated test beam line at 1 Hz

西内 満美子; 榊 泰直; 堀 利彦; Bolton, P.; 小倉 浩一; 匂坂 明人; 余語 覚文; 森 道昭; 織茂 聡; Pirozhkov, A. S.; et al.

Physical Review Special Topics; Accelerators and Beams, 13(7), p.071304_1 - 071304_7, 2010/07

 被引用回数:25 パーセンタイル:81.88(Physics, Nuclear)

1.9MeVレーザー駆動陽子線のビームライン中に伝送した。ビームラインは、PMQ, RF cavity,monochrometerからなり、伝送の様子をPARMILAのシミュレーションによって再現した。このような試みは世界初のことである。ビームラインの最終端において、6nsのバンチ幅を道、5%のエネルギースプレッドを持つビームが10%の効率で検出された。この様子はPARMILAにより再現でき、PARMILAコードがレーザー駆動陽子線のビームラインの構築に使用できることを証明した。


Quantitative analysis of cisplatin sensitivity of human esophageal squamous cancer cell lines using in-air micro-PIXE

田中 成岳*; 木村 仁*; Faried, A.*; 酒井 真*; 佐野 孝昭*; 猪瀬 崇徳*; 宗田 真*; 岡田 幸士*; 中島 政信*; 宮崎 達也*; et al.

Cancer Science, 101(6), p.1487 - 1492, 2010/06

 被引用回数:12 パーセンタイル:34.46(Oncology)


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