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Journal Articles

Production of $$^{266}$$Bh in the $$^{248}$$Cm($$^{23}$$Na,5$$n$$)$$^{266}$$Bh reaction and its decay properties

Haba, Hiromitsu*; Fan, F.*; Kaji, Daiya*; Kasamatsu, Yoshitaka*; Kikunaga, Hidetoshi*; Komori, Yukiko*; Kondo, Narumi*; Kudo, Hisaaki*; Morimoto, Koji*; Morita, Kosuke*; et al.

Physical Review C, 102(2), p.024625_1 - 024625_12, 2020/08

 Times Cited Count:0 Percentile:100(Physics, Nuclear)

Journal Articles

Extraction behavior of rutherfordium as a cationic fluoride complex with a TTA chelate extractant from HF/HNO $$_{3}$$ acidic solutions

Yokoyama, Akihiko*; Kitayama, Yuta*; Fukuda, Yoshiki*; Kikunaga, Hidetoshi*; Murakami, Masashi*; Komori, Yukiko*; Yano, Shinya*; Haba, Hiromitsu*; Tsukada, Kazuaki; Toyoshima, Atsushi*

Radiochimica Acta, 107(1), p.27 - 32, 2019/01

 Times Cited Count:1 Percentile:58.8(Chemistry, Inorganic & Nuclear)

Journal Articles

Online chemical adsorption studies of Hg, Tl, and Pb on SiO$$_{2}$$ and Au surfaces in preparation for chemical investigations on Cn, Nh, and Fl at TASCA

Lens, L.*; Yakushev, A.*; D$"u$llmann, Ch. E.*; Asai, Masato; Ballof, J.*; Block, M.*; David, H. M.*; Despotopulos, J.*; Di Nitto, A.*; Eberhardt, K.*; et al.

Radiochimica Acta, 106(12), p.949 - 962, 2018/12

 Times Cited Count:1 Percentile:75.54(Chemistry, Inorganic & Nuclear)

Online gas-solid adsorption studies with single atom quantities of Hg, Tl, and Pb on SiO$$_{2}$$ and Au surfaces were carried out using short-lived radioisotopes with half-lives in the range of 4-49 s. This is a model study to measure adsorption enthalpies of superheavy elements Cn, Nh, and Fl. The short-lived isotopes were produced and separated by the gas-filled recoil separator TASCA at GSI. The products were stopped in He gas, and flushed into gas chromatography columns made of Si detectors whose surfaces were covered by SiO$$_{2}$$ or Au. The short-lived Tl and Pb were successfully measured by the Si detectors with the SiO$$_{2}$$ surface at room temperature. On the other hand, the Hg did not adsorb on the SiO$$_{2}$$ surface, but adsorbed on the Au surface. The results demonstrated that the adsorption properties of short-lived Hg, Tl, and Pb could be studied with this setup, and that this method is applicable to the experiment for Cn, Nh, and Fl.

Journal Articles

Complex chemistry with complex compounds

Eichler, R.*; Asai, Masato; Brand, H.*; Chiera, N. M.*; Di Nitto, A.*; Dressler, R.*; D$"u$llmann, Ch. E.*; Even, J.*; Fangli, F.*; Goetz, M.*; et al.

EPJ Web of Conferences, 131, p.07005_1 - 07005_7, 2016/12

 Times Cited Count:1 Percentile:48.2

In recent years gas-phase chemical studies assisted by physical pre-separation allowed for the productions and investigations of fragile single molecular species of superheavy elements. The latest highlight is the formation of very volatile hexacarbonyl compound of element 106, Sg(CO)$$_{6}$$. Following this success, second-generation experiments were performed to measure the first bond dissociation energy between the central metal atom and the surrounding ligand. The method using a tubular decomposition reactor was developed and successfully applied to short-lived Mo(CO)$$_{6}$$, W(CO)$$_{6}$$, and Sg(CO)$$_{6}$$.

Journal Articles

Rare earth elements (REE) in deep groundwater from granite and fracture-filling calcite in the Tono area, central Japan; Prediction of REE fractionation in paleo- to present-day groundwater

Munemoto, Takashi; Omori, Kazuaki*; Iwatsuki, Teruki

Chemical Geology, 417, p.58 - 67, 2015/12

 Times Cited Count:17 Percentile:30.31(Geochemistry & Geophysics)

Rare earth elements (REEs) combined with yttrium (YREE) in deep groundwater from granite and fracture-filling calcite are being studied at the Mizunami Underground Research Laboratory (MIU, Tono area, central Japan).

Journal Articles

Hydrochemical disturbances measured in groundwater during the construction and operation of a large-scale underground facility in deep crystalline rock in Japan

Iwatsuki, Teruki; Hagiwara, Hiroki; Omori, Kazuaki; Munemoto, Takashi; Onoe, Hironori

Environmental Earth Sciences, 74(4), p.3041 - 3057, 2015/08

 Times Cited Count:13 Percentile:33.95(Environmental Sciences)

Changes of hydrochemical condition resulting from large-scale underground facility construction to 500 m depth in sedimentary and granitic rock were evaluated at the Mizunami Underground Research Laboratory (MIU), Japan. The investigation of hydrochemical impact around the facility suggests that an understanding of hydrogeological structures, including hydrogeological compartments prior to facility construction and the locating of shafts/galleries in low permeability rock area is essential to minimize hydrochemical disturbances.

JAEA Reports

Results of borehole investigation in -500m access/research gallery-north (13MI38$$sim$$13MI44 Boreholes)

Hasegawa, Takashi; Kawamoto, Koji; Yamada, Nobuto; Onuki, Kenji; Omori, Kazuaki; Takeuchi, Ryuji; Iwatsuki, Teruki; Sato, Toshinori

JAEA-Technology 2015-011, 135 Pages, 2015/07

JAEA-Technology-2015-011.pdf:28.63MB
JAEA-Technology-2015-011-appendix(CD-ROM).zip:566.32MB

The geological, hydraulic and geochemical data such as rock mass classification, groundwater inflow points and the volume, water pressure, and hydraulic conductivity were obtained from boreholes (13MI38$$sim$$13MI44) in the -500m Access/Research Gallery-North of Mizunami Underground Research laboratory (MIU). In addition to data acquisition, monitoring systems were installed to observe hydrochemical changes in the groundwater, and rock strain during and after the groundwater recovery experiment.

Journal Articles

Production of $$^{88}$$Nb and $$^{170}$$Ta for chemical studies of element 105, Db, using the GARIS gas-jet system

Huang, M.*; Haba, Hiromitsu*; Murakami, Masashi*; Asai, Masato; Kaji, Daiya*; Kanaya, Jumpei*; Kasamatsu, Yoshitaka*; Kikunaga, Hidetoshi*; Kikutani, Yuki*; Komori, Yukiko*; et al.

Journal of Radioanalytical and Nuclear Chemistry, 304(2), p.845 - 849, 2015/05

 Times Cited Count:3 Percentile:63.46(Chemistry, Analytical)

A technique to utilize radioisotopes of Nb and Ta was developed for chemical studies of element 105, Db, by coupling a gas-jet transport system to the RIKEN gas-filled recoil ion separator (GARIS). The short-lived $$^{88}$$Nb and $$^{170}$$Ta were produced with nuclear reactions using a $$^{19}$$F beam whose energy was the same as that to produce $$^{262}$$Db. Then, they were separated with GARIS and extracted to a chemistry laboratory with the gas-jet transport system. By changing only magnetic field of GARIS and inserting an energy degrader and a shutter for recoil ions, we could deliver the $$^{88}$$Nb and $$^{170}$$Ta to a chemistry device for $$^{262}$$Db without changing other experimental conditions.

JAEA Reports

Mizunami Underground Research Laboratory Project, Annual report for fiscal year 2013

Hama, Katsuhiro; Mikake, Shinichiro; Nishio, Kazuhisa; Kawamoto, Koji; Yamada, Nobuto; Ishibashi, Masayuki; Murakami, Hiroaki; Matsuoka, Toshiyuki; Sasao, Eiji; Sanada, Hiroyuki; et al.

JAEA-Review 2014-038, 137 Pages, 2014/12

JAEA-Review-2014-038.pdf:162.61MB

Japan Atomic Energy Agency (JAEA) at Tono Geoscience Center (TGC) is pursuing a geoscientific research and development project namely the Mizunami Underground Research Laboratory (MIU) Project in crystalline rock environment in order to construct scientific and technological basis for geological disposal of High-level Radioactive Waste (HLW). The MIU Project has three overlapping phases: Surface-based Investigation phase (Phase I), Construction phase (Phase II), and Operation phase (Phase III). The MIU Project has been ongoing the Phase II and the Phase III in fiscal year 2013. This report presents the results of the investigations, construction and collaboration studies in fiscal year 2013, as a part of the Phase II and Phase III based on the MIU Master Plan updated in 2010.

JAEA Reports

Hydrochemical investigation at the Mizunami Underground Research Laboratory; Compilation of groundwater chemistry data in the Mizunami group and the Toki granite (fiscal year 2013)

Omori, Kazuaki; Hasegawa, Takashi; Munemoto, Takashi; Masuda, Kaoru*; Aosai, Daisuke*; Inui, Michiharu*; Iwatsuki, Teruki

JAEA-Data/Code 2014-019, 121 Pages, 2014/12

JAEA-Data-Code-2014-019.pdf:56.12MB

Japan Atomic Energy Agency has been investigating the groundwater chemistry on excavating the underground facilities as part of the Mizunami Underground research Laboratory (MIU) Project at Mizunami City, Gifu Prefecture, Japan. In this report, we compiled data obtained by geochemical research for groundwater at the MIU in the fiscal year 2013.

JAEA Reports

Methodology development for colloid investigation in groundwater

Omori, Kazuaki; Munemoto, Takashi; Hasegawa, Takashi; Shingu, Shinya*; Hagiwara, Hiroki; Iwatsuki, Teruki

JAEA-Research 2014-013, 29 Pages, 2014/08

JAEA-Research-2014-013.pdf:48.04MB

We summarized investigation method of colloid in groundwater. We examined the ultrafiltration of groundwater by using in-situ water monitoring system and batch type airtight container. Additionally, we examined the cross flow filtration method replaced by ultrafiltration. The knowledge of investigating methods is obtained.

JAEA Reports

Results of pilot borehole investigation in -500m access/research gallery-south (12MI32 borehole)

Kawamoto, Koji; Kuroiwa, Hiroshi; Yamada, Nobuto; Onuki, Kenji; Omori, Kazuaki; Takeuchi, Ryuji; Ogata, Nobuhisa; Omori, Masaki; Watanabe, Kazuhiko

JAEA-Technology 2014-011, 92 Pages, 2014/07

JAEA-Technology-2014-011.pdf:24.65MB
JAEA-Technology-2014-011-appendix(DVD).zip:331.54MB

This document summarizes the data of pilot boreholes (12MI32) in the -500m Access/Research Gallery-South. The geological, hydraulic and geochemical data were obtained. In addition, groundwater monitoring system was installed to observe the groundwater pressure in initial condition and change during the excavation of gallery. The results of investigation, biotite granite with medium to coarse-grained equigranular texture are characterized. Rock mass classification is B from CM class. Minor fault with fault breccia are observed around 48.90mabh. However, S200_13 fault and IF_SB3_13_3 fault (that were presumed by an original model) were not observed. Density of fracture is large in the section of 40.00 to 80.00mabh. Water inflow was a maximum of 600 L/min in 78.83mabh. Permeability ranges from 2.0E-9 to 1.5E-08m/sec at the zone with low inflow, from 1.1E-05 to 1.6E-05m/sec at the zone with high inflow, respectively. Groundwater chemistry is rich in Na and Cl ion.

JAEA Reports

Hydrochemical investigation at the Mizunami Underground Research Laboratory; Compilation of groundwater chemistry data in Mizunami group and Toki granite (fiscal year 2012)

Omori, Kazuaki; Shingu, Shinya*; Masuda, Kaoru*; Aosai, Daisuke*; Inui, Michiharu*; Iwatsuki, Teruki

JAEA-Data/Code 2013-024, 284 Pages, 2014/03

JAEA-Data-Code-2013-024.pdf:34.27MB

Japan Atomic Energy Agency has been investigating the groundwater chemistry on excavating the underground facilities as part of the Mizunami Underground research Laboratory (MIU) Project at Mizunami City, Gifu Prefecture, Japan. In this report, we compiled data of groundwater chemistry obtained at the MIU in the fiscal year 2012.

JAEA Reports

Mizunami Underground Research Laboratory Project, Annual report for fiscal year 2012

Hama, Katsuhiro; Mikake, Shinichiro; Nishio, Kazuhisa; Matsuoka, Toshiyuki; Ishibashi, Masayuki; Sasao, Eiji; Hikima, Ryoichi*; Tanno, Takeo*; Sanada, Hiroyuki; Onoe, Hironori; et al.

JAEA-Review 2013-050, 114 Pages, 2014/02

JAEA-Review-2013-050.pdf:19.95MB

Japan Atomic Energy Agency (JAEA) at Tono Geoscience Center (TGC) is pursuing a geoscientific research and development project namely the Mizunami Underground Research Laboratory (MIU) Project in crystalline rock environment in order to construct scientific and technological basis for geological disposal of High-level Radioactive Waste (HLW). The MIU Project has three overlapping phases: Surface-based Investigation phase (Phase I), Construction phase (Phase II), and Operation phase (Phase III). The MIU Project has been ongoing the Phase II and the Phase III in fiscal year 2012. This report presents the results of the investigations, construction and collaboration studies in fiscal year 2012, as a part of the Phase II and Phase III based on the MIU Master Plan updated in 2010.

Journal Articles

Production of $$^{262}$$Db in the $$^{248}$$Cm($$^{19}$$F,5$$n$$)$$^{262}$$Db reaction and decay properties of $$^{262}$$Db and $$^{258}$$Lr

Haba, Hiromitsu*; Huang, M.*; Kaji, Daiya*; Kanaya, Jumpei*; Kudo, Yuki*; Morimoto, Koji*; Morita, Kosuke*; Murakami, Masashi*; Ozeki, Kazutaka*; Sakai, Ryutaro*; et al.

Physical Review C, 89(2), p.024618_1 - 024618_11, 2014/02

 Times Cited Count:18 Percentile:18.34(Physics, Nuclear)

JAEA Reports

Hydrogeochemical research and development at Mizunami Underground Research Laboratory up to 500m depth

Iwatsuki, Teruki; Yuguchi, Takashi; Omori, Kazuaki; Hasegawa, Takashi; Munemoto, Takashi

JAEA-Research 2013-021, 63 Pages, 2013/12

JAEA-Research-2013-021.pdf:13.42MB

We evaluated the Phase I - hydrogeochemical model constructed by Surface-based investigation phase (Phase I), and observed hydrogeochemical change resulting from facility construction in Phase II research. Additionally we developed investigation technique on redox condition, colloid/organics, etc. at gallery in Phase III research. Hydrogeochemical changes in sedimentary rocks and granite resulting from facility construction have been caused by the change of mixing ratio among salinity-distinct groundwaters. Multivariate numerical analysis shows that the groundwater chemistry around drifts would change to that of shallow groundwater in the future. The know-hows on hydrochemical monitoring at the hydrogeological structures and numerical analysis were summarized to infer the hydrochemical changing processes during the facility construction.

JAEA Reports

Mizunami Underground Research Laboratory Project, Annual report for fiscal year 2011

Kunimaru, Takanori; Mikake, Shinichiro; Nishio, Kazuhisa; Tsuruta, Tadahiko; Matsuoka, Toshiyuki; Ishibashi, Masayuki; Sasao, Eiji; Hikima, Ryoichi; Tanno, Takeo; Sanada, Hiroyuki; et al.

JAEA-Review 2013-018, 169 Pages, 2013/09

JAEA-Review-2013-018.pdf:15.71MB

Japan Atomic Energy Agency (JAEA) at Tono Geoscience Center (TGC) is pursuing a geoscientific research and development project namely the Mizunami Underground Research Laboratory (MIU) Project in crystalline rock environment in order to construct scientific and technological basis for geological disposal of High-level Radioactive Waste (HLW). The MIU Project has three overlapping phases: Surface-based Investigation phase (Phase I), Construction phase (Phase II), and Operation phase (Phase III). The MIU Project has been ongoing the Phase II and the Phase III in 2011 fiscal year. This report shows the results of the investigation, construction and collaboration studies in fiscal year 2011, as a part of the Phase II and Phase III based on the MIU Master Plan updated in 2010.

JAEA Reports

Hydrochemical investigation at the Mizunami Underground Research Laboratory; Compilation of groundwater chemistry data in Mizunami group and Toki granite (fiscal year 2011)

Omori, Kazuaki; Shingu, Shinya; Hagiwara, Hiroki; Masuda, Kaoru*; Iizuka, Masatoshi*; Inui, Michiharu*; Iwatsuki, Teruki

JAEA-Data/Code 2013-001, 330 Pages, 2013/05

JAEA-Data-Code-2013-001.pdf:23.85MB

Japan Atomic Energy Agency has been investigated the groundwater chemistry on excavating the underground facilities as part of the Mizunami Underground Research Laboratory (MIU) Project at Mizunami, Gifu, Japan. This report compiles data of the groundwater chemistry obtained at MIU in the fiscal year 2011. In terms of ensuring traceability of data, basic information (e.g. sampling location, sampling date, sampling method, analytical method) and methodology for quality control is described.

Journal Articles

Sulfate complexation of element 104, Rf, in H$$_{2}$$SO$$_{4}$$/HNO$$_{3}$$ mixed solution

Li, Z.*; Toyoshima, Atsushi; Asai, Masato; Tsukada, Kazuaki; Sato, Tetsuya; Sato, Nozomi; Kikuchi, Takahiro; Nagame, Yuichiro; Sch$"a$del, M.; Pershina, V.*; et al.

Radiochimica Acta, 100(3), p.157 - 164, 2012/03

 Times Cited Count:9 Percentile:34.7(Chemistry, Inorganic & Nuclear)

Journal Articles

Production of $$^{265}$$Sg in the $$^{248}$$Cm($$^{22}$$Ne,5$$n$$)$$^{265}$$Sg reaction and decay properties of two isomeric states in $$^{265}$$Sg

Haba, Hiromitsu*; Kaji, Daiya*; Kudo, Yuki*; Morimoto, Koji*; Morita, Kosuke*; Ozeki, Kazutaka*; Sakai, Ryutaro*; Sumita, Takayuki*; Yoneda, Akira*; Kasamatsu, Yoshitaka*; et al.

Physical Review C, 85(2), p.024611_1 - 024611_11, 2012/02

 Times Cited Count:39 Percentile:9.33(Physics, Nuclear)

Two isomeric states in $$^{265}$$Sg, i.e, $$^{265}$$Sg$$^{a}$$ and $$^{265}$$Sg$$^{b}$$ were produced in the $$^{248}$$Cm($$^{22}$$Ne,5$$n$$) reaction. Decay properties of $$^{265}$$Sg$$^{a,b}$$ were investigated with a rotating-wheel apparatus for $$alpha$$ and spontaneous fission (SF) spectrometry under low background condition attained by a gas-jet transport system coupled to the RIKEN gas-filled recoil ion separator. Based on genetically correlated $$alpha$$-$$alpha$$ (-$$alpha$$) and $$alpha$$-SF decay chains, 18 and 24 events were assigned to $$^{265}$$Sg$$^{a}$$ and $$^{265}$$Sg$$^{b}$$, respectively. The half-life and $$alpha$$-particle energy of $$^{265}$$Sg$$^{a}$$ were measured to be $$8.5^{+2.6}_{-1.6}$$ s and $$8.84 pm 0.05$$ MeV, respectively, and those of $$^{265}$$Sg$$^{b}$$ were $$14.4^{+3.7}_{-2.5}$$ s and $$8.69 pm 0.05$$ MeV.

62 (Records 1-20 displayed on this page)