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Ikeuchi, Hirotomo; Koyama, Shinichi; Osaka, Masahiko; Takano, Masahide; Nakamura, Satoshi; Onozawa, Atsushi; Sasaki, Shinji; Onishi, Takashi; Maeda, Koji; Kirishima, Akira*; et al.
JAEA-Technology 2022-021, 224 Pages, 2022/10
A set of technology, including acid dissolving, has to be established for the analysis of content of elements/nuclides in the fuel debris samples. In this project, a blind test was performed for the purpose of clarifying the current level of analytical accuracy and establishing the alternative methods in case that the insoluble residue remains. Overall composition of the simulated fuel debris (homogenized powder having a specific composition) were quantitatively determined in the four analytical institutions in Japan by using their own dissolving and analytical techniques. The merit and drawback for each technique were then evaluated, based on which a tentative flow of the analyses of fuel debris was constructed.
Koyama, Shinichi; Nakagiri, Toshio; Osaka, Masahiko; Yoshida, Hiroyuki; Kurata, Masaki; Ikeuchi, Hirotomo; Maeda, Koji; Sasaki, Shinji; Onishi, Takashi; Takano, Masahide; et al.
Hairo, Osensui Taisaku jigyo jimukyoku Homu Peji (Internet), 144 Pages, 2021/08
JAEA performed the subsidy program for the "Project of Decommissioning and Contaminated Water Management (Development of Analysis and Estimation Technology for Characterization of Fuel Debris (Development of Technologies for Enhanced Analysis Accuracy and Thermal Behavior Estimation of Fuel Debris))" in 2020JFY. This presentation summarized briefly the results of the project, which will be available shortly on the website of Management Office for the Project of Decommissioning and Contaminated Water Management.
Toyokawa, Takuya; Usami, Koji; Shiina, Hidenori; Onozawa, Atsushi
Proceedings of 49th Conference on Hot Laboratories and Remote Handling (HOTLAB 2012) (Internet), 6 Pages, 2012/09
Matsui, Yoshinori; Takahashi, Hiroyuki; Yamamoto, Masaya; Nakata, Masahito; Yoshitake, Tsunemitsu; Abe, Kazuyuki; Yoshikawa, Katsunori; Iwamatsu, Shigemi; Ishikawa, Kazuyoshi; Kikuchi, Taiji; et al.
JAEA-Technology 2009-072, 144 Pages, 2010/03
"R&D Project on Irradiation Damage Management Technology for Structural Materials of Long-life Nuclear Plant" was carried out from FY2006 in a fund of a trust enterprise of the Ministry of Education, Culture, Sports, Science and Technology. The coupled irradiations or single irradiation by JOYO fast reactor and JRR-3 thermal reactor were performed for about two years. The irradiation specimens are very important materials to establish of "Evaluation of Irradiation Damage Indicator" in this research. For the acquisition of the examination specimens irradiated by the JOYO and JRR-3, we summarized about the overall plan, the work process and the results for the study to utilize these reactors and some facilities of hot laboratory (WASTEF, JMTR-HL, MMF and FMF) of the Oarai Research-and-Development Center and the Nuclear Science Research Institute in the Japan Atomic Energy Agency.
Onozawa, Atsushi; Harada, Akio; Honda, Junichi; Nakata, Masahito; Kanazawa, Hiroyuki; Sagawa, Tamio
JAEA-Conf 2008-010, p.325 - 332, 2008/12
The measurement technique for hydrogen concentration using Backscattered Electron Image analysis (BEI method) had been developed by Studsvik Nuclear AB. The hydride in claddings is identified using BEIs with SEM and the hydrogen concentration is calculated from the area fractions of the hydride in those BEIs. In the RFEF, the sample polishing techniques and image processing procedure for BEI method were improved to measure the hydrogen concentration in the irradiated fuel claddings more precisely. In the previous tests using the un-irradiated fuel claddings, it is confirmed improved BEI method has high reliability. The radial and axial hydrogen concentration profiles of the irradiated fuel claddings were measured with improved BEI method. As the results of these measurements, the local hydrogen concentration could be indicated more precisely with the improved BEI method compared to the other methods for the hydrogen concentration measurement and observation.
Endo, Shinya; Usami, Koji; Nakata, Masahito; Fukuda, Takuji*; Onozawa, Atsushi; Harada, Akio; Kizaki, Minoru; Kikuchi, Hiroyuki
HPR-366, Vol.1 (CD-ROM), 10 Pages, 2007/03
no abstracts in English
Onozawa, Atsushi; Harada, Akio; Honda, Junichi; Yasuda, Ryo; Nakata, Masahito; Kanazawa, Hiroyuki; Nishino, Yasuharu
JAEA-Conf 2006-003, p.212 - 221, 2006/05
In the Reactor Fuel Examination Facility (RFEF), a measuring method of hydrogen concentration by backscattered electron image analysis was improved to obtain more local hydrogen concentration data in fuel claddings. The sample preparation and image analysis procedures of this were able to measure hydrogen concentration efficiently and precisely.
Onozawa, Atsushi; Harada, Akio; Honda, Junichi; Yasuda, Ryo; Nakata, Masahito; Kanazawa, Hiroyuki; Nishino, Yasuharu
JAEA-Technology 2006-010, 19 Pages, 2006/03
A measurement technique for hydrogen concentration using Backscattered Electron Image analysis (BEI method) had been developed by Studsvik Nuclear AB, Sweden. The hydrides in claddings are identified using BEIs which are imaged with Scanning Electron Microscope, and the hydrogen concentrations are calculated from the area fractions of the hydrides in the matrix. The BEI method is very useful for the measurement in local hydrogen concentrations of fuel claddings. In the Reactor Fuel Examination Facility, a sample preparation, imaging conditions of SEM and image analysis procedures for the BEI method were improved. In addition, the hydrogen concentrations obtained by the improved BEI method and Hot Vacuum Extraction (HVE) method were compared to confirm the reliability of the improved BEI method. The results showed, the improved BEI method has the same reliability as that of HVE method and can be applied for the Post-Irradiation Examination.
Onozawa, Atsushi; Kushida, Teruo; Kanazawa, Hiroyuki
JAERI-Tech 2004-061, 39 Pages, 2004/11
The swelling observed on irradiated fuels is caused by the accumulation of fission products and irradiation defects. The swelling ratio is changed along with radius region in the pellet due to burn up difference caused by that of neutron flux. To investigate the swelling behavior at the small area of the pellet, it is needed to measure the density of fuel fragments picked from an irradiated pellet. In this circumstance, once-through type densitometer was developed to measure the density of the small irradiated specimen precisely and to handle the samples easily with remote control systems. Several kinds of metallic and ceramic standard specimens are prepared to investigate the dependence of the sample weight, density and porosity on the accuracy. The results of characteristic examination using these specimens indicate that this densitometer has enough accuracy. In addition, some parts of this apparatus are controlled by motor drive units, which made it possible to measure the density full-automatically.
Yanagisawa, Kazuaki; Omichi, Toshihiko*; Shirasu, Noriko; Yamashita, Toshiyuki; ; Onozawa, Atsushi; ; Kanazawa, Hiroyuki; Kanaitsuka, Fumio; Amano, Hidetoshi
JAERI-Tech 99-044, 46 Pages, 1999/05
no abstracts in English
Takano, Masahide; Onozawa, Atsushi; Sudo, Ayako
no journal, ,
To understand the characteristics of MCCI products in Fukushima Daiichi Nuclear Power Station, the simulated MCCI products in laboratory scale were prepared by arc melting of compacted powder mixtures of core materials and concrete. Stainless steel, boron carbide, metallic zirconium, (U,Zr)O, GdO
, and platinum group elements were selected as the core materials. Phases, morphology, and micro hardness were analyzed on cross-section of the solidified specimens. The specimens consisted of oxide part (MO
corium and silicate glass or Al-Ca-O) and metallic part (alloys and borides). The phase relationships in the MCCI products were found to be dominated by the initial concrete/Zr mixing ratio, because the dehydration of concrete is the main oxidation factor and the metallic zirconium acts as a strong reductant. Micro hardness of main phases are 7 GPa for silicate glass, 13-15 GPa for (U,Zr,Gd,Ca)O
corium, and 25 GPa for ZrB
and ferrous borides, respectively.
Takano, Masahide; Onozawa, Atsushi
no journal, ,
(U,Zr)O solid solution is considered as the main component of oxide corium generated in the core-meltdown accident at Fukushima Daiichi NPS. The actual oxide corium is expected to contain some minor solutes such as lanthanides from burnable poison (Gd) and fission products, Fe from stainless steel, and Ca from see water and concrete. In this paper, influences of these minor elements on the phases, morphology, and oxidation behavior of (U,Zr)O
is investigated. As results of sample characterization, (1) the Fe inclusion tends to form a complicated microstructure of U-rich and Zr-rich phases tangled in
m-scale; (2) the influence of Ca inclusion is the stabilization of Zr-rich tetragonal phase into cubic phase when the O/M ratio is within hypostoichiometric range; (3) the impact of lanthanide inclusion is that the cubic (U,Zr)O
domain expands to lower temperatures region where UO
and (U,Zr)O
is oxidized to U
O
and orthorhombic U(V)-Zr-O.
Takano, Masahide; Onozawa, Atsushi; Suzuki, Miho; Obata, Hiroki
no journal, ,
For the decommissioning of damaged cores of Fukushima Daiichi NPS, the retrieval operation of solidified core melt (corium) and its safe management are essential tasks. To understand characteristics of corium specific to the 1F cores, we have prepared and analyzed various types of simulated corium specimens in laboratory scale. To verify the effect of cooling condition found on the simulated corium, we revisit the actual corium specimens collected from the TMI-2 accident core, which have been stored at the Reactor Fuel Examination Facility (RFEF) in JAEA Tokai since 1991. Comparing the phases and microstructure, rapid-cooled specimens have dense microstructure and consist of single phase of cubic structure. On the other hand, the slow-cooled specimens consist of U-rich cubic and Zr-rich tetragonal phases distributed minutely. From these observations we have confirmed the similar dependence of microstructure and mechanical property on the cooling condition.
Onozawa, Atsushi; Endo, Shinya; Nakata, Masahito; Yanagisawa, Hiroshi
no journal, ,
Onozawa, Atsushi
no journal, ,
On one of the sessions in HOTLAB2023 conference as "PIE technician Workshop - "Challenges associated with Sample Preparation for PIE", The discussion regarding "Moving from macro to micro scale - handling/tooling challenges" will be held. In a facility designed to handle large scale fuel such as assemblies and rods is not benefit to handle macro/micro size sample. In this session, the panelists and conference participants will be discuss about the PIE technique for micro size sample handling and treating. The discussion will be obtain how to handle it reliably, how to prepare the sample and how to prevent sample contamination.
Takano, Masahide; Onozawa, Atsushi; Sudo, Ayako
no journal, ,
no abstracts in English
Sudo, Ayako; Onozawa, Atsushi; Takano, Masahide
no journal, ,
To characterize the layer structure and respective temperatures of MCCI products, MCCI experiments using a light-concentrating furnace were performed. As the core-melt constituents, a powder mixture of (UZr
)O
(No.1) and (U
Zr
)O
/Zr/SUS316L/B
C (No.2) were compacted into tablets (10 mm in diameter) respectively. The tablet was placed on a cylindrical piece of basaltic concrete (25 mm in diameter). The light was concentrated on the tablet under argon gas flow and samples were heated. After heating, the vertical cross-section of the solidified sample piece was subjected to phase identification and elemental analysis by XRD and SEM/EDX. No.1 sample seemed to maintain original shape, but EDX analysis showed the inner region melted. This melt was identified as-melted (U,Zr)O
particle and silicate glass containing U and Zr. Ca, Fe and Mg oxide were dissolved in the particle. UO
and ZrO
were dissolved in the silicate glass. No.2 sample had same phases, but Fe-Cr oxide deposits from SS was identified.
Matsumura, Tatsuro; Iijima, Takahiko; Ishii, Sho; Takano, Masahide; Onozawa, Atsushi
no journal, ,
no abstracts in English
Takano, Masahide; Onozawa, Atsushi; Sudo, Ayako
no journal, ,
no abstracts in English
Shiina, Hidenori; Usami, Koji; Sakuraba, Naotoshi; Harada, Akio; Onozawa, Atsushi; Nakata, Masahito
no journal, ,