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Sugiura, Yuki; Ishidera, Takamitsu; Aoyagi, Noboru; Mei, H.; Saito, Takumi*; Tachi, Yukio
Applied Clay Science, 258, p.107476_1 - 107476_10, 2024/09
Tsuchida, Hidetsugu*; Tezuka, Tomoya*; Kai, Takeshi; Matsuya, Yusuke*; Majima, Takuya*; Saito, Manabu*
Journal of Chemical Physics, 161(10), p.104503_1 - 104503_8, 2024/09
Although fast ion beams can damage DNA by chemical products such as secondary electrons produced by their interaction with water in living cells, the process of formation of these chemical products in the Bragg peak region used in particle therapy is not fully understood. To investigate this process, we performed experiments to evaluate the yields of radiolytic products produced when a liquid water jet in vacuum is irradiated with a MeV-energy carbon beam. In addition, ionization processes in water due to incident ions and secondary electrons were simulated using a radiation transport Monte Carlo code. The results indicated that the primary source of ionization in water is secondary electrons. Finally, we show that these elementary processes contribute to the development of radiation biophysics and biochemistry to study the formation mechanism of DNA damage.
Nakajima, Taro*; Saito, Hiraku*; Kobayashi, Naoki*; Kawasaki, Takuro; Nakamura, Tatsuya; Furukawa, Hazuki*; Asai, Shinichiro*; Masuda, Takatsugu*
Journal of the Physical Society of Japan, 93(9), p.091002_1 - 091002_5, 2024/09
Namie, Masanari; Saito, Junichi; Ikeda, Asuka; Oka, Ryotaro*; Kim, J.-H.*
Surfaces (Internet), 7(3), p.550 - 559, 2024/09
-dioctylthiodiglycolamic acid; Effect of S donor on metal extractionShimojo, Kojiro; Fujiwara, Iori*; Saito, Takumi*; Oshima, Tatsuya*
Analytical Sciences, 40(8), p.1429 - 1436, 2024/08
Extraction ability of -dioctylthiodiglycolamic acid (T-DODGAA), a soft-base sulfur donor ligand with an amide group and a carboxylic acid connected by a thioether chain, for 56 metal ions have been comprehensively investigated and compared with that of N,N-dioctyldiglycolamic acid (DODGAA) with an etheric oxygen atom, a hard-base donor. The p
of the thiodiglycolamic acid framework was determined to be 3.71 
0.06 in water (0.1 M LiCl, 25
C ) by potentiometric titration, indicating that T-DODGAA is a slightly weaker acid than DODGAA (p = 3.54 0.03). T-DODGAA can quantitatively extract various metal ions from the 56 metal ions through a proton-exchange reaction. T-DODGAA provided higher extraction performance than DODGAA for Hf(IV), Cr(III), Fe(III), Ni(II), Cu(II), Pd(II), Ag(I), Au(III), Hg(II), Al(III), and Ga(III), especially for soft metal ions. Furthermore, to demonstrate the practical feasibility of T-DODGAA for hydrometallurgy and metal recycling, we performed selective separation tests of rare metal ions such as Sc(III), Ni(II), Co(II), Pd(II), Au(III), In(III), and Ga(II) in metal-mixed extraction systems.
Shibata, Hiroki; Saito, Hiroaki; Hayashi, Hirokazu; Takano, Masahide
Nihon Genshiryoku Gakkai Wabun Rombunshi (Internet), 23(3), p.74 - 80, 2024/08
Partitioning and transmutation of minor actinides techniques have been developed to reduce the radiotoxicity and volume in the high-level radioactive wastes. Minor actinide nitride fuel has been chosen as a candidate for transmutation of long-lived nuclides by accelerator-driven system. Understanding irradiation behavior of nitride fuel is important for its design and development, however, experimental data on irradiation tests of actinide nitrides and these solid solutions are scarce. Recently, in JAEA, nitride fuel performance analysis module based on light water reactor fuel performance code, FEMAXI-7, has been developed to simulate irradiation behavior of the nitride fuel. In this study, performance analysis was carried out focusing on the pellet-cladding mechanical interaction (PCMI), which was pointed out as the most effective factor for the fuel safety during irradiation. Simulation results show that PCMI does not cause the creep rupture of the cladding.
Ninomiya, Kazuhiko*; Kubo, Kenya*; Inagaki, Makoto*; Yoshida, Go*; Takeshita, Soshi*; Tampo, Motonobu*; Shimomura, Koichiro*; Kawamura, Naritoshi*; Strasser, P.*; Miyake, Yasuhiro*; et al.
Journal of Radioanalytical and Nuclear Chemistry, 333(7), p.3445 - 3450, 2024/07
Sanada, Yukihisa; Urabe, Yoshimi*; Saito, Madoka*; Shiribiki, Takehiko*; Misono, Toshiharu; Funaki, Hironori
Kankyo Gijutsu, 53(4), p.188 - 193, 2024/07
no abstracts in English
Terada, Noriki*; Khalyavin, D. D.*; Manuel, P.*; Asai, Shinichiro*; Masuda, Takatsugu*; Saito, Hiraku*; Nakajima, Taro*; Osakabe, Toyotaka
Physical Review B, 110(2), p.024406_1 - 024406_9, 2024/07
The frustrated antiferromagnet CuFeO exhibits pressure-induced complex magnetic phase transitions from the commensurate collinear (CM1) phase to several incommensurate noncollinear phases. To study the effect of high pressure on magnetic interactions, we performed neutron diffraction and inelastic neutron scattering experiments under high-pressure conditions. With increasing pressure, the CM1 ground state becomes less stable against application of a magnetic field even below the critical pressure (
3 GPa), as proved by the significant reduction in the critical magnetic field from 
=7.5 T to 4.5 T at 2.1 GPa. Additionally, the energy gap in the spin-wave dispersion relation is reduced from 1.0 to 0.88 meV by the application of a pressure of = 2.1 GPa. Comparing the experimental results with spin-wave calculations revealed that the change in the spin-wave excitation can be explained by the reduction in either the uniaxial anisotropy term or the degree of separation in the nearest-neighbor exchange interactions.
)PbI
and CH(NH)SnI investigated by inelastic X-ray scattering and comparison of their elastic propertiesTamatsukuri, Hiromu; Murakami, Yoichi*; Saito, Noriko*; Ohashi, Naoki*; Tsutsui, Satoshi*
Physical Review B, 110(2), p.024301_1 - 024301_8, 2024/07
Nemoto, Takahiro; Fujiwara, Yusuke; Arakawa, Ryoki; Choyama, Yuya; Nagasumi, Satoru; Hasegawa, Toshinari; Yokoyama, Keisuke; Watanabe, Masashi; Onishi, Takashi; Kawamoto, Taiki; et al.
JAEA-Technology 2024-003, 17 Pages, 2024/06
JAEA-Technology-2024-003.pdf:1.91MB
In order to investigate the cause of the increase in differential pressure in the primary helium circulator filter that occurred during the RS-14 cycle, a clogged filter was investigated. As a result of the investigation, deposits caused by silicone oil were confirmed on the surface of the filter element. These results revealed that the cause of filter clogging was silicone oil mixed into the primary system due to performance deterioration of the charcoal filter in the gas circulator of primary helium purification system. As a measure to prevent the recurrence of this event, in addition to the conventional management based on operating hours for replacing of charcoal filter in the gas circulator of primary helium purification system, we have established a new replacement plan for every three years.
Aoyagi, Noboru; Motokawa, Ryuhei; Okumura, Masahiko; Ueda, Yuki; Saito, Takumi*; Nishitsuji, Shotaro*; Taguchi, Tomitsugu*; Yomogida, Takumi; Sazaki, Gen*; Ikeda, Atsushi
Communications Chemistry (Internet), 7, p.128_1 - 128_13, 2024/06
Yoshida, Hidekazu*; Yamamoto, Koshi*; Asahara, Yoshihiro*; Maruyama, Ippei*; Karukaya, Koichi*; Saito, Akane*; Matsui, Hiroya; Mochizuki, Akihito; Jo, Mayumi*; Katsuta, Nagayoshi*; et al.
Communications Engineering (Internet), 3, p.67_1 - 67_10, 2024/05
A capability to permanently seal fluid flow-paths through bedrock, like boreholes or underground tunnels, is needed to ensure the long-term safety and effectiveness of many underground activities e.g. CO storage, hydrocarbon field abandonment, and nuclear waste disposal. Commonly used cementitious seals may not be sufficiently durable due to chemical and physical degradation. Learning from natural calcite (CaCO) concretion formation, a more durable sealing method was developed using a "concretion-forming solvent". The method was tested by sealing flow-paths next to a tunnel in an underground research laboratory at 350 meters depth. The flow-paths initially sealed rapidly, then resealed after disturbance by earthquakes (M5.4). The treated rock recovered its very low natural permeability, demonstrating permanent sealing that is robust.
Miyazaki, Kanako*; Takehara, Masato*; Minomo, Kenta*; Horie, Kenji*; Takehara, Mami*; Yamasaki, Shinya*; Saito, Takumi*; Onuki, Toshihiko*; Takano, Masahide; Shiotsu, Hiroyuki; et al.
Journal of Hazardous Materials, 470(15), p.134104_1 - 134104_11, 2024/05
Makiuchi, Takahiko*; Hioki, Tomosato*; Shimizu, Hiroki*; Hoshi, Kojiro*; Elyasi, M.*; Yamamoto, Kei; Yokoi, Naoto*; Serga, A. A.*; Hillebrands, B.*; Bauer, G. E. W.*; et al.
Nature Materials, 23(5), p.627 - 632, 2024/05
Baccou, J.*; Glantz, T.*; Ghione, A.*; Sargentini, L.*; Fillion, P.*; Damblin, G.*; Sueur, R.*; Iooss, B.*; Fang, J.*; Liu, J.*; et al.
Nuclear Engineering and Design, 421, p.113035_1 - 113035_16, 2024/05
Times Cited Count：0 Percentile：0.05Elyasi, M.*; Yamamoto, Kei; Hioki, Tomosato*; Makiuchi, Takahiko*; Shimizu, Hiroki*; Saito, Eiji*; Bauer, G. E. W.*
Physical Review B, 109(18), p.L180402_1 - L180402_7, 2024/05
Sr in highly radioactive aqueous samples via conversion to a kinetically stable 1,4,7,10-tetraazacyclododecane-1,4,7,10-tetraacetic acid complex followed by concentration-separation-fractionation based on capillary electrophoresis-liquid scintillationOuchi, Kazuki; Haraga, Tomoko; Hirose, Kazuki*; Kurosawa, Yuika*; Sato, Yoshiyuki; Shibukawa, Masami*; Saito, Shingo*
Analytica Chimica Acta, 1298, p.342399_1 - 342399_7, 2024/04
Times Cited Count：0 Percentile：0.01Given that conventional methods of high-dose sample analysis pose substantial exposure risks and generate large amounts of secondary radioactive waste, faster procedures allowing for decreased radiation emission are highly desirable. To address this need, we developed a Sr
quantitation technique that is based on liquid scintillation counting-coupled capillary transient isotachophoresis (ctITP) with two-point detection and relies on the rapid concentration, separation, and fractionation of 1,4,7,10-tetraazacyclododecane-1,4,7,10-tetraacetic acid (DOTA)-complexed Sr in a single run. This method, which allows for the handling of high-dose radioactive specimens at the microliter level and is substantially faster than conventional ion-exchange protocols, was used to selectively quantify Sr in real high-dose waste. The successful concentration-separation in ctITP was ascribed to the inertness of the Sr-DOTA complex to dissociation.
Warashina, Tomoro*; Sato, Asako*; Hinai, Hiroshi; Shaikhutdinov, N.*; Shagimardanova, E.*; Mori, Hiroshi*; Tamaki, Satoshi*; Saito, Motofumi*; Sanada, Yukihisa; Sasaki, Yoshito; et al.
Applied and Environmental Microbiology, 90(4), p.e02113-23_1 - e02113-23_23, 2024/04
Namie, Masanari; Saito, Junichi
Computational Materials Science, 239, p.112963_1 - 112963_7, 2024/04
