Imai, Masaki; Chudo, Hiroyuki; Matsuo, Mamoru; Maekawa, Sadamichi; Saito, Eiji
Physical Review B, 102(1), p.014407_1 - 014407_5, 2020/07
Takahashi, Ryo*; Chudo, Hiroyuki; Matsuo, Mamoru; Harii, Kazuya*; Onuma, Yuichi*; Maekawa, Sadamichi; Saito, Eiji
Nature Communications (Internet), 11, p.3009_1 - 3009_6, 2020/06
Saito, Hiroyuki*; Machida, Akihiko*; Hattori, Takanori; Sano, Asami; Funakoshi, Kenichi*; Sato, Toyoto*; Orimo, Shinichi*; Aoki, Katsutoshi*
Physica B; Physics of Condensed Matter, 587, p.412153_1 - 412153_6, 2020/06
The site occupancy of deuterium (D) atoms in face-centered-cubic nickel (fcc Ni) was measured along a cooling path from 1073 to 300 K at an initial pressure of 3.36 GPa via in situ neutron powder diffraction. Deuterium atoms predominantly occupy the octahedral (O) sites and slightly occupy the tetrahedral (T) sites of the fcc metal lattice. The O-site occupancy increases from 0.4 to 0.85 as the temperature is lowered from 1073 to 300 K. Meanwhile, the T-site occupancy remains c.a. 0.02. The temperature-independent behavior of the T-site occupancy is unusual, and its process is not yet understood. From the linear relation between the expanded lattice volume and D content, a D-induced volume expansion of 2.09(13) atom was obtained. This value is in agreement with the values of 2.14-2.2 atom previously reported for Ni and Ni Fe alloy.
Saito, Hiroyuki*; Machida, Akihiko*; Iizuka, Riko*; Hattori, Takanori; Sano, Asami; Funakoshi, Kenichi*; Sato, Toyoto*; Orimo, Shinichi*; Aoki, Katsutoshi*
Scientific Reports (Internet), 10, p.9934_1 - 9934_8, 2020/06
Neutron powder diffraction profiles were collected for iron deuteride (FeDx) while the temperature decreased from 1023 to 300 K for a pressure range of 4-6 GPa. The ' deuteride with a double hexagonal close-packed (dhcp) structure, which coexisted with other stable or metastable deutrides at each temperature and pressure condition, formed solid solutions with a composition of FeD at 673 K and 6.1 GPa and FeD at 603 K and 4.8 GPa. Upon stepwise cooling to 300 K, the D-content x increased to a stoichiometric value of 1.0 to form monodeuteride FeD. In the dhcp FeD at 300 K and 4.2 GPa, dissolved D atoms fully occupied the octahedral interstitial sites, slightly displaced from the octahedral centers in the dhcp metal lattice, and the dhcp sequence of close-packed Fe planes contained hcp-stacking faults at 12%. Magnetic moments with 2.11 0.06 B/Fe-atom aligned ferromagnetically in parallel on the Fe planes.
Mikami, Satoshi; Tanaka, Hiroyuki*; Matsuda, Hideo*; Sato, Shoji*; Hoshide, Yoshifumi*; Okuda, Naotoshi*; Suzuki, Takeo*; Sakamoto, Ryuichi*; Ando, Masaki; Saito, Kimiaki
Journal of Environmental Radioactivity, 210, p.105941_1 - 105941_12, 2019/12
The deposition densities of radiocesium and the air dose rates were repeatedly measured in a large number of undisturbed fields within the 80km zone that surrounds the Fukushima Dai-ichi Nuclear Power Plant site between 2011 and 2016, and features of their temporal changes were clarified. The average air dose rate excluding background radiation in this zone decreased to about 20% of the initial value during the period from June 2011 to August 2016, which was essentially a result of the radioactive decay of Cs with a half-life of 2.06y. The air dose rate reduction was faster than that expected from the decay of radiocesium by a factor of about two, with most of this reduction being attributed to the penetration of radiocesium into the soil. The average deposition densities of Cs and Cs in fields that were not decontaminated were found to have decreased nearly according to their expected radioactive decay, which indicated that the movement of radiocesium in the horizontal direction was relatively small. The effect of decontamination was apparently observed in the measurements of air dose rates and deposition densities. Nominally, the average air dose rates in the measurement locations were reduced by about 20% by decontamination and other human activities, of which accurate quantitative analysis is and continue to be a challenge.
Machida, Akihiko*; Saito, Hiroyuki*; Hattori, Takanori; Sano, Asami; Funakoshi, Kenichi*; Sato, Toyoto*; Orimo, Shinichi*; Aoki, Katsutoshi*
Scientific Reports (Internet), 9(1), p.12290_1 - 12290_9, 2019/08
Hexagonal close-packed iron hydride, hcp FeHx, is absent from the conventional phase diagram of the Fe-H system, although hcp metallic Fe exists stably over extensive temperature () and pressure () conditions, including those corresponding to the Earth's inner core. X-ray and neutron diffraction measurements at temperatures ranging from 298 to 1073 K and H pressures ranging from 4 to 7 GPa revealed that the hcp hydride was formed for FeH compositions when . Hydrogen atoms occupied the octahedral interstitial sites of the host metal lattice both partially and randomly. The hcp hydride exhibited a H-induced volume expansion of 2.48(5) /H-atom, which was larger than that of the face-centered cubic (fcc) hydride. The hcp hydride showed an increase in with , whereas the fcc hydride showed a corresponding decrease. The present study provides guidance for further investigations of the Fe-H system over an extensive -- region.
Kawaguchi, Munemichi; Saito, Junichi; Daido, Hiroyuki*; Suemoto, Toru*
UVSOR-46, P. 89, 2019/08
To elucidate theoretically the transparent metallic sodium in the vacuum ultraviolet spectral range, the aim of this research is to obtain the accurate spectrum using UVSOR. The sodium sample maintained metallic luster by designing the special cells to prevent from oxidizing. The results of UVSOR measurement showed the possibility to occur the intransparent layer for vacuum ultraviolet light on the MgF windows. In the near future, we will improve the sodium sample to solve the problems and conduct the measurement again
Wang, H.*; Otsu, Hideaki*; Chiga, Nobuyuki*; Kawase, Shoichiro*; Takeuchi, Satoshi*; Sumikama, Toshiyuki*; Koyama, Shumpei*; Sakurai, Hiroyoshi*; Watanabe, Yukinobu*; Nakayama, Shinsuke; et al.
Communications Physics (Internet), 2(1), p.78_1 - 78_6, 2019/07
Searching for effective pathways for the production of proton- and neutron-rich isotopes through an optimal combination of reaction mechanism and energy is one of the main driving forces behind experimental and theoretical nuclear reaction studies as well as for practical applications in nuclear transmutation of radioactive waste. We report on a study on incomplete fusion induced by deuteron, which contains one proton and one neutron with a weak binding energy and is easily broken up. This reaction study was achieved by measuring directly the cross sections for both proton and deuteron for Pd at 50 MeV/u via inverse kinematics technique. The results provide direct experimental evidence for the onset of a cross-section enhancement at high energy, indicating the potential of incomplete fusion induced by loosely-bound nuclei for creating proton-rich isotopes and nuclear transmutation of radioactive waste.
Harii, Kazuya; Seo, Y.-J.*; Tsutsumi, Yasumasa*; Chudo, Hiroyuki; Oyanagi, Koichi*; Matsuo, Mamoru; Shiomi, Yuki*; Ono, Takahito*; Maekawa, Sadamichi; Saito, Eiji
Nature Communications (Internet), 10(1), p.2616_1 - 2616_5, 2019/06
Imai, Masaki; Chudo, Hiroyuki; Ono, Masao; Harii, Kazuya; Matsuo, Mamoru; Onuma, Yuichi*; Maekawa, Sadamichi; Saito, Eiji
Applied Physics Letters, 114(16), p.162402_1 - 162402_4, 2019/04
Saeki, Morihisa*; Matsumura, Daiju; Yomogida, Takumi; Taguchi, Tomitsugu*; Tsuji, Takuya; Saito, Hiroyuki*; Oba, Hironori*
Journal of Physical Chemistry C, 123(1), p.817 - 824, 2019/01
Reaction kinetics of laser-induced particle formation in an aqueous solution of PdCl was investigated by transmission electron microscope (TEM) and dispersive X-ray absorption fine structure (DXAFS). The Pd particle was generated by irradiation of nanosecond pulsed 266-nm laser. The TEM observation showed dependence of the particle size on the laser fluence and promotion of the particle growth by irradiation of high-fluence laser. The DXAFS data give us the Pd concentration. Temporal changes of the Pd concentration analyzed based on Finke-Watzky two step mechanism. The analysis elucidates that the laser photon contributes to the reduction of the PdCl ion by the one-photon process and to the autocatalytic growth of the Pd particles by the multi-photon process.
Imai, Masaki; Ogata, Yudai*; Chudo, Hiroyuki; Ono, Masao; Harii, Kazuya; Matsuo, Mamoru*; Onuma, Yuichi*; Maekawa, Sadamichi; Saito, Eiji
Applied Physics Letters, 113(5), p.052402_1 - 052402_3, 2018/07
Sugimoto, Taro*; Saito, Shimpei*; Kaneko, Akiko*; Abe, Yutaka*; Uchibori, Akihiro; Ohshima, Hiroyuki
Proceedings of 26th International Conference on Nuclear Engineering (ICONE-26) (Internet), 7 Pages, 2018/07
A computational fluid dynamics code for a sodium-water reaction phenomenon in a steam generator of sodium-cooled fast reactors has been developed. In order to provide the data for validation of this code, the visualization experiment on liquid droplet entrainment in the high-pressure air jet submerged in the water pool was carried out. The experiment successfully elucidated the behavior, such as atomization of the relatively large diameter liquid droplet generated from the gas-liquid interface.
Sakamoto, Hiroyuki*; Akagi, Yosuke*; Yamada, Kazuo*; Tachi, Yukio; Fukuda, Daisuke*; Ishimatsu, Koichi*; Matsuda, Mikiya*; Saito, Nozomi*; Uemura, Jitsuya*; Namihira, Takao*; et al.
Nippon Genshiryoku Gakkai Wabun Rombunshi, 17(2), p.57 - 66, 2018/05
Concrete debris contaminated with radioactive cesium and other nuclides have been generated from the accident in the Fukushima Dai-ichi Nuclear Power Plant and there will be generated due to the decommissioning of nuclear power plants in the future. Although conventional decontamination techniques are effective for flat concrete surfaces such as floors and walls, it is not clear what techniques to apply for decontaminating radioactive concrete debris. In this study, focusing on a pulsed power discharge technique, fundamental experimental works were carried out. Decontamination of concrete by applying the aggregate recycling technique using the pulsed power discharge technique was evaluated by measuring radioactivity of aggregate and sludge separated from the contaminated concrete. The results suggest that the separation into aggregate and sludge of the contaminated concrete debris could achieve decontamination and volume reduction of the radioactive concrete debris.
Ueno, Yasuhiro*; Aoki, Masaharu*; Fukao, Yoshinori*; Higashi, Yoshitaka*; Higuchi, Takashi*; Iinuma, Hiromi*; Ikedo, Yutaka*; Ishida, Keiichi*; Ito, Takashi; Iwasaki, Masahiko*; et al.
Hyperfine Interactions, 238(1), p.14_1 - 14_6, 2017/11
Ogata, Yudai; Chudo, Hiroyuki; Gu, B.; Kobayashi, Nobukiyo*; Ono, Masao; Harii, Kazuya; Matsuo, Mamoru; Saito, Eiji; Maekawa, Sadamichi
Journal of Magnetism and Magnetic Materials, 442, p.329 - 331, 2017/11
Saito, Hiroyuki*; Yamada, Yumi*; Oyama, Kazuhiro*; Matsunaga, Shoko*; Yamano, Hidemasa; Kubo, Shigenobu
Proceedings of 2017 International Congress on Advances in Nuclear Power Plants (ICAPP 2017) (CD-ROM), 10 Pages, 2017/04
A self-actuated shutdown system (SASS) is a passive device, which can detach a control rod for reactor shutdown in response to excessive increase in coolant temperature. Since a detachment temperature, which triggers release of a control rod, and a response time are identified as important parameters for validity analyses, this study focused on investigation of the response time and the detachment temperature, and safety analysis to see feasibility of the SASS in low power. For this purpose, design modifications were made to shorten the response time and three-dimensional thermal-hydraulic analysis in a low power operation was carried out in order to confirm the response time. The resulting detachment temperature level is lower than previous studies, leading to improved safety parameters. Based on improved parameters, a safety analysis to see feasibility of the SASS in low power was carried out. From this safety evaluation, it was confirmed that core damage can be prevented by the SASS with flow collector in the case of LOF type ATWS event.
Seo, Y.-J.*; Harii, Kazuya; Takahashi, Ryo*; Chudo, Hiroyuki; Oyanagi, Koichi*; Qiu, Z.*; Ono, Takahito*; Shiomi, Yuki*; Saito, Eiji
Applied Physics Letters, 110(13), p.132409_1 - 132409_4, 2017/03
We have fabricated ferrite cantilevers in which their vibrational properties can be controlled by external magnetic fields. Submicron-scale cantilever structures were made from YFeO films by physical etching combined with the use of a focused ion beam milling technique. We found that the cantilevers exhibit two resonance modes which correspond to horizontal and vertical vibrations. Under external magnetic fields, the resonance frequency of the horizontal mode increases, while that of the vertical mode decreases, quantitatively consistent with our numerical simulation for magnetic forces. The changes in resonance frequencies with magnetic fields reach a few percent, showing that an efficient magnetic control of resonance frequencies was achieved.
Tada, Hiroyuki*; Kumasaka, Hiroo*; Saito, Akira*; Nakaya, Atsushi*; Ishii, Takashi*; Fujita, Tomoo; Sugita, Yutaka; Nakama, Shigeo; Sanada, Masanori*
Doboku Gakkai Rombunshu, F2 (Chika Kukan Kenkyu) (Internet), 73(1), p.11 - 28, 2017/03
This study examined the mechanical characteristics of rock segments and backfill materials and analyzed the stability of the drift that is supported by the rock segments and gravel backfill. The results confirmed the technical aspects of the formation of the rock segments and the effectiveness of the planned efforts to further reduce the amount of cement used.