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JAEA Reports

Development of high temperature LBE corrosion test loop "OLLOCHI"

Saito, Shigeru; Wan, T.*; Okubo, Nariaki; Kita, Satoshi*; Obayashi, Hironari; Sasa, Toshinobu

JAEA-Technology 2021-034, 94 Pages, 2022/03

JAEA-Technology-2021-034.pdf:5.91MB

Lead-bismuth eutectic alloy (LBE) is a major candidate for a spallation target material and core coolant of an accelerator driven system (ADS) which has been developed in the Japan Atomic Energy Agency (JAEA) to transmute high-level radioactive wastes. A proton irradiation facility to build a material irradiation database for future ADS development is under considering in the J-PARC. To realize both the ADS and the above-mentioned facility, there are many issues on operational safety of LBE to be solved. Especially, corrosion data for the major materials such as T91 (Modified 9Cr-1Mo steel) and SS316L at the temperature range between 400 and 550 $$^{circ}$$C under the conditions of flowing LBE with a controlled oxygen are not sufficient to design the ADS and the facility. JAEA developed a new large-scale corrosion test loop named "OLLOCHI (Oxygen-controlled LBE LOop for Corrosion tests in HIgh-temperature)" aiming to perform the compatibility tests between the LBE and the steels, as well as to develop the LBE operation technology. OLLOCHI has a function to automatically control the oxygen concentration in LBE. The maximum temperature at the regions of high-temperature and low-temperature of the OLLOCHI are 550 $$^{circ}$$C and 450 $$^{circ}$$C respectively to cover the ADS designed condition. As a result of 2,000 hours operation, it was demonstrated that the OLLOCHI showed the designed performance. In this report, outline of the OLLOCHI, details of the components, results of characteristic tests, and the future experimental plan are described.

Journal Articles

Flow measurement in high temperature liquid metal by using electro-magnet probe

Ariyoshi, Gen; Obayashi, Hironari; Saito, Shigeru; Sasa, Toshinobu

Proceedings of 19th International Topical Meeting on Nuclear Reactor Thermal Hydraulics (NURETH-19) (Internet), 10 Pages, 2022/03

To clarify the flow characteristics of heavy liquid-metal (HLM) is important to achieve the construction of nuclear transmutation facility that utilizes HLM as a spallation target and coolant. At present, lead-bismuth eutectic (LBE) spallation target plans to be installed in Japan proton accelerator research complex (J-PARC). LBE is also selected as one of the candidate media of a spallation target and a coolant for innovative nuclear systems such as accelerator-driven system (ADS) and LBE-cooled fast reactor, due to its adequate physical/chemical properties. The characteristics of LBE flowing inside the target are usually clarified with computational fluid dynamics analysis since the measurement techniques for the HLM flow are not well established, especially for high temperature region over 450$$^{circ}$$C that is delivered from ADS's criteria. Therefore, the objective of this study is to develop measurement method for flow characteristics in the high temperature LBE. A miniature electro-magnet is introduced to electro-magnetic probe to overcome the limitation caused by a curie temperature of permanent magnet. To evaluate performance of the new probe, experimental apparatus equipping annular rotating vessel were also manufactured. The new probe was applied to high temperature LBE up to 480$$^{circ}$$C. As a result, proportional induced voltage to the rotation speed of LBE were clearly observed, where excitation currents of the miniature electro-magnet were 0.2 A or 1 A. In this paper, configuration and performance of the newly developed electro-magnet probe to the high temperature LBE will be presented.

Journal Articles

Status of LBE study and experimental plan at JAEA

Saito, Shigeru; Wan, T.*; Okubo, Nariaki; Obayashi, Hironari; Watanabe, Nao; Ohdaira, Naoya*; Kinoshita, Hidetaka; Yamaki, Kenichi*; Kita, Satoshi*; Yoshimoto, Hidemitsu*; et al.

JPS Conference Proceedings (Internet), 33, p.011041_1 - 011041_6, 2021/03

An Accelerator Driven System (ADS) for waste transmutation investigated in JAEA employs lead-bismuth eutectic (LBE) as a neutron production target material and coolant. The neutrons are to be produced via the spallation with 1.5 GeV proton beam injection. As materials irradiation data are important for ADS development, JAEA plans to construct an irradiation facility with LBE neutron production target in J-PARC. There are many technical issues on LBE for practical use. In JAEA, various R&Ds are being carried out. Concerning corrosion study, conditioning operation and functional tests of OLLOCHI started. Oxygen concentration control technology has also developing. In the large scale LBE loop experiment, the operation for steady state and transient experiments was performed by using IMMORTAL. In the area of instrument, development of ultrasonic flow meter and freeze seal valve are progressing as a key technology for the LBE loop system. Investigation of behavior of impurities in LBE, which is important for design of the irradiation facility, started. In this paper, the status of the LBE studies and experimental plan will be presented.

Journal Articles

Remote handling technology for lead-bismuth spallation target system

Obayashi, Hironari; Yoshimoto, Hidemitsu*; Kita, Satoshi*; Yamaki, Kenichi*; Wan, T.*; Saito, Shigeru; Sasa, Toshinobu

JPS Conference Proceedings (Internet), 33, p.011048_1 - 011048_6, 2021/03

Journal Articles

250 kW LBE spallation target for ADS development in J-PARC

Sasa, Toshinobu; Saito, Shigeru; Obayashi, Hironari; Ariyoshi, Gen

JPS Conference Proceedings (Internet), 33, p.011051_1 - 011051_6, 2021/03

To realize Accelerator-driven system (ADS) for minor actinide transmutation, JAEA proposes to construct the Proton Irradiation Facility in J-PARC. The facility is planned to solve technical issues for safe application of Lead-bismuth Eutectic Alloy (LBE). The 250 kW LBE spallation target will be located in the facility to prepare material irradiation database by both proton and neutron irradiation in the temperature range for typical LBE-cooled ADS. Various studies for important technologies required to build the facilities are investigated such as oxygen concentration control, instruments development, remote handling techniques for target maintenance, and spallation target design. The large scale LBE loops for mock up the 250 kW LBE spallation target and material corrosion studies are also manufactured and applied to various experiments. The latest status of 250 kW LBE spallation target design works will be summarized.

JAEA Reports

Development of logging data processing tool for lead-bismuth experimental devices

Yamaki, Kenichi*; Kita, Satoshi*; Obayashi, Hironari; Ariyoshi, Gen; Saito, Shigeru; Sasa, Toshinobu

JAEA-Technology 2020-021, 26 Pages, 2021/02

JAEA-Technology-2020-021.pdf:2.34MB

As digitalization of measuring instruments, Programmable Logic Controller is mainly used for controlling large-scale devices, and many test devices are controlled in digital. Together with increase of the data storage capacity, it has become possible to record the measured values over the entire experimental period. By collecting the entire experimental data, it became easy to appropriately record the test environment during the corrosion test of materials and to analyze the changes and transients during continuous operation from various viewpoints. On the other hand, in a long-term test, the large number of measurement data were recorded, which requires long time for data processing and data extraction for analyses. In addition, it is necessary to pay attention to organize the data collected by different data formats. To solve these problems, a processing tool were produced to extract and process the data efficiently from the sequencer installed in the lead-bismuth test device.

Journal Articles

Experimental validation of tensile properties measured with thick samples taken from MEGAPIE target

Saito, Shigeru; Suzuki, Kazuhiro; Hatakeyama, Yuichi; Suzuki, Miho; Dai, Y.*

Journal of Nuclear Materials, 534, p.152146_1 - 152146_16, 2020/06

 Times Cited Count:1 Percentile:39.17(Materials Science, Multidisciplinary)

A post-irradiation examination (PIE) was performed on the tensile specimens prepared from the MEGAPIE (MEGAwatt Pilot Experiment) target which were irradiated in flowing lead-bismuth eutectic (LBE). Thicknesses of the specimens were over two times larger than that of the standard specimen. The PIE revealed that the T91 specimens showed a 1.5-2.0 times larger total elongation (TE) compared to the literature values for a specimen with standard t/w (ratio of thickness to width). It could be suggested that the t/w and TE were strongly correlated. Then, we tried to investigate the effects of the t/w on the TE by comparing unirradiated specimens. We found that there was no t/w dependence on the strength and uniform elongation. On the other hand, the TE increases with increasing t/w. Based on the experimental data, we correlated the TE with various specimens t/w to estimate appropriate TE values, including that for the standard specimen.

Journal Articles

Characterization of mechanical strain induced by lead-bismuth eutectic (LBE) freezing in stainless steel cup

Ohdaira, Naoya*; Saito, Shigeru

Heliyon (Internet), 6(2), p.e03429_1 - e03429_8, 2020/02

 Times Cited Count:2 Percentile:57.94(Multidisciplinary Sciences)

Lead-bismuth eutectic (LBE) is a candidate liquid metal coolant for a fast reactor, especially accelerator driven system (ADS). Freeze sealed valve is a candidate design to be possible to add passive safety to the reactor. On the other hand, since LBE is known that it causes expansion after its solidification, quantitative evaluation of the stress to the pipe produced by the LBE expansion should be considered. Many researchers produced related data for the expansion, however, evaluations of the strain by LBE expansion was barely reported. Therefore, the strain measurement using a stainless steel cup and the stress evaluation was performed together with visual observation using an optical microscopy. The results indicated keeping above room temperature (RT) was a significantly effective way to reduce the strain to the pipe.

Journal Articles

Current Status of R&D and PIE Program for ADS Material Development in JAEA

Saito, Shigeru; Okubo, Nariaki; Obayashi, Hironari; Wan, T.; Sugawara, Takanori; Sasa, Toshinobu; Maekawa, Fujio

JPS Conference Proceedings (Internet), 28, p.071003_1 - 071003_6, 2020/02

Japan Atomic Energy Agency (JAEA) proposes transmutation of minor actinides (MA) by accelerator-driven systems (ADS). The ADS designed by JAEA is a system composed by LBE (Lead-Bismuth Eutectic) spallation target and a subcritical core. In the ADS, a beam window (BW) is exposed in complex field of heavy irradiation by proton/neutron and corrosion by flowing LBE. To develop ADS structural materials, it is of critical importance to investigate materials used in such environment. Thus, JAEA plans to construct a proton irradiation facility at the J-PARC to prepare an irradiation database for candidate ADS structural materials and to investigate irradiation effects in flowing LBE environment. In this paper, giving a whole scope of the JAEA ADS development, some results of experimental measurements and the specific program for planed R&D will be presented.

Journal Articles

Steady-state and transient experiments in mock-up of J-PARC LBE spallation target system using mock-up loop "IMMORTAL"

Obayashi, Hironari; Yamaki, Kenichi; Kita, Satoshi; Yoshimoto, Hidemitsu; Wan, T.; Saito, Shigeru; Sasa, Toshinobu

Proceedings of 18th International Topical Meeting on Nuclear Reactor Thermal Hydraulics (NURETH-18) (USB Flash Drive), p.262 - 274, 2019/08

Construction of an experimental facility using LBE spallation target is under planning in the framework of J-PARC project to understand the compatibility of candidate ADS structural materials under flowing high temperature LBE environment with proton / neutron irradiation. We constructed a mock-up test loop, IMMORTAL to verify the feasibility of a primary cooling system in the target system. Including the layout considering remote maintainability, the same design as the actual JAEA's LBE target is reflected in most devices of IMMORTAL such as an electromagnetic pump (EMP), a heat exchanger and instrumentations. During the integrated tests, the individually developed devices of LBE loop system worked without significant malfunction. Several experimental data to verify the safety analysis model for LBE loop system using RELAP5-3D was acquired by simulation experiment of transient events such as beam over power and decrease of forced cooling.

JAEA Reports

Development of prototype for TEF-T integral control system of J-PARC

Sakai, Kenji; Obayashi, Hironari; Saito, Shigeru; Sasa, Toshinobu; Sugawara, Takanori; Watanabe, Akihiko*

JAEA-Technology 2019-009, 18 Pages, 2019/07

JAEA-Technology-2019-009.pdf:2.34MB

Construction of Transmutation Experimental Facility (TEF) is under planning in the Japan Proton Accelerator Research Complex (J-PARC) program to promote R&D on the transmutation technology with using accelerator driven systems (ADS). ADS Target Test Facility (TEF-T) in TEF will develop spallation target technology and study on target materials with irradiating high intensity proton beams on a lead-bismuth eutectic (LBE) target. For safe and efficient beam operation, a general control system (GCS) will be constructed in TEF-T. GCS comprises several subsystems, such as a network system (LAN), an integral control system (ICS), an interlock system (ILS), and a timing distribution system (TDS) according to their roles. Especially, the ICS plays the important role that executes integral operations in the entire facility, acquires, stores and distributes operation data. We planned to develop a prototype of the ICS, to evaluate its concrete performances such as data transmission speeds, data storage capability, control functions, long-term stability of the system, and to utilize them for design of the actual ICS. This report mentions to product the prototype of ICS and to apply it to remote operations of instruments for developing LBE target technology.

Journal Articles

Enhancement of element production by incomplete fusion reaction with weakly bound deuteron

Wang, H.*; Otsu, Hideaki*; Chiga, Nobuyuki*; Kawase, Shoichiro*; Takeuchi, Satoshi*; Sumikama, Toshiyuki*; Koyama, Shumpei*; Sakurai, Hiroyoshi*; Watanabe, Yukinobu*; Nakayama, Shinsuke; et al.

Communications Physics (Internet), 2(1), p.78_1 - 78_6, 2019/07

 Times Cited Count:5 Percentile:62.37(Physics, Multidisciplinary)

Searching for effective pathways for the production of proton- and neutron-rich isotopes through an optimal combination of reaction mechanism and energy is one of the main driving forces behind experimental and theoretical nuclear reaction studies as well as for practical applications in nuclear transmutation of radioactive waste. We report on a study on incomplete fusion induced by deuteron, which contains one proton and one neutron with a weak binding energy and is easily broken up. This reaction study was achieved by measuring directly the cross sections for both proton and deuteron for $$^{107}$$Pd at 50 MeV/u via inverse kinematics technique. The results provide direct experimental evidence for the onset of a cross-section enhancement at high energy, indicating the potential of incomplete fusion induced by loosely-bound nuclei for creating proton-rich isotopes and nuclear transmutation of radioactive waste.

Journal Articles

Flow-accelerated corrosion of type 316L stainless steel caused by turbulent lead-bismuth eutectic flow

Wan, T.; Saito, Shigeru

Metals, 8(8), p.627_1 - 627_22, 2018/08

 Times Cited Count:5 Percentile:43.06(Materials Science, Multidisciplinary)

Journal Articles

Design of LBE spallation target for ADS Target Test Facility (TEF-T) in J-PARC

Saito, Shigeru; Obayashi, Hironari; Wan, T.; Okubo, Nariaki; Sugawara, Takanori; Endo, Shinya; Sasa, Toshinobu

Proceedings of 13th International Topical Meeting on Nuclear Applications of Accelerators (AccApp '17) (Internet), p.448 - 457, 2018/05

JAEA proposes transmutation of minor actinides by accelerator-driven systems (ADS). To obtain the data for ADS design, JAEA plans to construct the ADS Target Test Facility (TEF-T) within the framework of the J-PARC project. In TEF-T, a 250 kW proton-beam-driven LBE (Lead-Bismuth Eutectic) spallation target will be installed to prepare an irradiation database for candidate ADS structural materials. Design activities of the LBE target and target trolley have been progressed. Conceptual design of hot-cells for LBE target loop maintenance and PIE (Post Irradiation Examination) of irradiated samples have been finished. Two LBE loops were manufactured. One is a loop for TEF-T target mock-up and the other is that for collection of material corrosion characteristics in flowing LBE. Oxygen potential control systems for LBE flow have been also developed. Remote handling tests for the target exchange are underway. In this paper, current activities and studies to realize TEF-T will be presented.

Journal Articles

${it In-situ}$ observation of dislocation evolution in ferritic and austenitic stainless steels under tensile deformation by using neutron diffraction

Sato, Shigeo*; Kuroda, Asumi*; Sato, Kozue*; Kumagai, Masayoshi*; Harjo, S.; Tomota, Yo*; Saito, Yoichi*; Todoroki, Hidekazu*; Onuki, Yusuke*; Suzuki, Shigeru*

Tetsu To Hagane, 104(4), p.201 - 207, 2018/00

 Times Cited Count:5 Percentile:43.06(Metallurgy & Metallurgical Engineering)

Journal Articles

Design of 250kW LBE spallation target for the Japan Proton Accelerator Research Complex (J-PARC)

Sasa, Toshinobu; Saito, Shigeru; Obayashi, Hironari; Sugawara, Takanori; Wan, T.; Yamaguchi, Kazushi*; Yoshimoto, Hidemitsu

NEA/CSNI/R(2017)2 (Internet), p.111 - 116, 2017/06

Japan Atomic Energy Agency (JAEA) proposes to reduce the environmental impact caused from high-level radioactive waste by using Accelerator-driven system (ADS). To realize ADS, JAEA plans to build the Transmutation Experimental Facility (TEF) within the framework of J-PARC project. For the JAEA-proposed ADS, lead-bismuth eutectic alloy (LBE) is adopted as a coolant for subcritical core and spallation target. By using TEF in J-PARC, we are planning to solve technical difficulties for LBE utilization by completion of the data for the design of ADS. The 250kW LBE spallation target will be located in TEF facility to prepare material irradiation database. Various R&Ds for important technologies required to build the facilities are investigated such as oxygen content control, instruments development, remote handling techniques for target maintenance, and spallation target design. The large scale LBE loops for 250kW target mock up and material corrosion studies are also manufactured and ready for various experiments. The latest status of 250kW LBE spallation target optimization will be described in the presentation.

Journal Articles

Status of LBE corrosion test loop "OLLOCHI" and experiments at JAEA

Saito, Shigeru; Okubo, Nariaki; Obayashi, Hironari; Sasa, Toshinobu

NEA/CSNI/R(2017)2 (Internet), p.195 - 200, 2017/06

An ADS (Accelerator Driven System) for waste transmutation investigated in JAEA employs LBE (Lead-Bismuth Eutectic) as spallation target material and core coolant. To realize future ADS and an ADS target experimental facility (TEF-T) planned for construction in J-PARC, there are many technical issues on LBE. In particular, corrosion data of relevant materials like T91 (Mod. 9Cr-1Mo) and SS316L steels at 400-550$$^{circ}$$C under oxygen concentration controlled and flowing condition are indispensable. JAEA has designed and built new LBE corrosion test loop named OLLOCHI (Oxygen-controlled LBE LOop Corrosion tests in HIgh-temperature), to obtain the corrosion data at the higher temperature. The piping of high temperature sections was made by T91 and 2.25Cr-1Mo steel. The maximum temperature of these parts is 550$$^{circ}$$C. At low temperature sections, piping and components were made by SS316L and the maximum temperature is limited to 450$$^{circ}$$C. The status for the OLLOCHI as of March 2016 is that the some modification and the conditioning operation without LBE have already finished. The oxygen sensors and the oxygen control system will be installed soon. After that, the conditioning operation with LBE and oxygen control test will be started. And more, additional flow meters will be installed in each test section until next March. In parallel with these tests, thermal hydraulic analysis of the two test sections will be performed to identify the flow pattern in the specimen holders.

JAEA Reports

Environmental remediation for the upstream of Yotsugi Mill Tailings Pond, Ningyo-toge Uranium Mine

Saito, Hiroshi; Sato, Yasushi*; Sakamoto, Atsushi*; Torikai, Kazuyoshi; Fukushima, Shigeru; Sakao, Ryota; Taki, Tomihiro

JAEA-Technology 2015-063, 119 Pages, 2016/03

JAEA-Technology-2015-063.pdf:86.2MB

Ningyo-toge Environmental Engineering Center has been conducting environmental remediation of the Ningyo-toge Uranium Mine, after decades of mine-related activities were terminated. Its purposes are to take measures to ensure safety and radiation protection from the exposure pathways to humans in future, and to prevent the occurrence of mining pollution. As part of the remediation, upstream part of the Yotsugi Mill Tailings Pond, the highest prioritized facility, has been remediated to fiscal year 2012. Multi-layered capping has been constructed using natural material, after specifications and whole procedure being examined in terms of long-term stability, radiation protection, economics, etc. Monitoring has been carried out to confirm the effectiveness of the capping, in terms of settlement, dose and radon exhalation rates, etc. Monitoring of drainage volume of penetrated rainwater is planned. Accumulated data will be examined and used for remediation of downstream part of the Pond.

Journal Articles

Flexible heat-flow sensing sheets based on the longitudinal spin Seebeck effect using one-dimensional spin-current conducting films

Kirihara, Akihiro*; Kondo, Koichi*; Ishida, Masahiko*; Ihara, Kazuki*; Iwasaki, Yuma*; Someya, Hiroko*; Matsuba, Asuka*; Uchida, Kenichi*; Saito, Eiji; Yamamoto, Naoharu*; et al.

Scientific Reports (Internet), 6, p.23114_1 - 23114_7, 2016/03

 Times Cited Count:49 Percentile:91.65(Multidisciplinary Sciences)

Heat-flow sensing is expected to be an important technological component of smart thermal management in the future. Conventionally, the thermoelectric (TE) conversion technique, which is based on the Seebeck effect, has been used to measure a heat flow by converting the flow into electric voltage. However, for ubiquitous heat-flow visualization, thin and flexible sensors with extremely low thermal resistance are highly desired. Recently, another type of TE effect, the longitudinal spin Seebeck effect (LSSE), has aroused great interest because the LSSE potentially offers favourable features for TE applications such as simple thin-film device structures. Here we demonstrate an LSSE-based flexible TE sheet that is especially suitable for a heat-flow sensing application. This TE sheet contained a Ni$$_{0.2}$$Zn$$_{0.3}$$Fe$$_{2.5}$$O$$_4$$ film which was formed on a flexible plastic sheet using a spray-coating method known as ferrite plating. The experimental results suggest that the ferrite-plated film, which has a columnar crystal structure aligned perpendicular to the film plane, functions as a unique one-dimensional spin- current conductor suitable for bendable LSSE-based sensors. This newly developed thin TE sheet may be attached to differently shaped heat sources without obstructing an innate heat flux, paving the way to versatile heat-flow measurements and management.

Journal Articles

J-PARC transmutation experimental facility programme

Sasa, Toshinobu; Takei, Hayanori; Saito, Shigeru; Obayashi, Hironari; Nishihara, Kenji; Sugawara, Takanori; Iwamoto, Hiroki; Yamaguchi, Kazushi; Tsujimoto, Kazufumi; Oigawa, Hiroyuki

NEA/CSNI/R(2015)2 (Internet), p.85 - 91, 2015/06

Nuclear transmutation got much interested as an effective option of nuclear waste management. Japan Atomic Energy Agency (JAEA) proposes the transmutation of minor actinides (MA) by accelerator-driven system (ADS) using lead-bismuth alloy (Pb-Bi). To obtain the data for ADS design, JAEA plans to build a Transmutation Experimental Facility (TEF) in the J-PARC project. TEF consists of two buildings, an ADS target test facility (TEF-T) with 400MeV-250kW Pb-Bi target, and a Transmutation Physics Experimental Facility (TEF-P), which set up a fast critical assembly driven by low power proton beam with MA fuel. In TEF-T, irradiation test for materials, and engineering tests for Pb-Bi target operation will be performed. Various research plans such as nuclear data measurements have been proposed and layout of the experimental hall are underway. In the presentation, roadmap to establish the ADS transmutor and latest design activities for TEF construction will be summarized.

208 (Records 1-20 displayed on this page)