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Journal Articles

Oxygen reduction activity and interfacial structures of La$$_{0.8}$$Sr$$_{0.2}$$CoO$$_{3}$$ at initial electrochemical process in an alkaline solution

Matsuzaki, Akira*; Hirayama, Masaaki*; Oguchi, Shoya*; Komo, Mamoru*; Ikezawa, Atsunori*; Suzuki, Kota*; Tamura, Kazuhisa; Arai, Hajime*; Kanno, Ryoji*

Electrochemistry (Internet), 90(10), p.107001_1 - 107001_8, 2022/10

 Times Cited Count:0 Percentile:0.01(Electrochemistry)

Oxygen reduction and evolution reactions (ORR and OER) of perovskite-type La$$_{0.8}$$Sr$$_{0.2}$$CoO$$_{3}$$ were characterized using two-dimensional model electrodes with different reaction planes. Synthesized by pulsed laser deposition, these thin and flat electrodes can reveal the reaction plane dependence of the ORR activity. From steady-state polarization measurements in KOH (aq.), the ORR activity was the highest on the (001) film during the first ORR/OER cycle, and it decreased significantly during the second cycle. In-situ synchrotron X-ray diffraction clarified crystal structure changes in the bulk and surface regions of La$$_{0.8}$$Sr$$_{0.2}$$CoO$$_{3}$$, and these changes are associated with forming oxygen defects during the initial electrochemical process. Furthermore, the La$$_{0.8}$$Sr$$_{0.2}$$CoO$$_{3}$$ surface partially decomposed upon reacting. Therefore, the interfacial structures formed in the electrochemical reaction field is important for enhancing ORR and OER activities.

JAEA Reports

Report on activities of "Technical Committee on Mine Closure Activities of the Tono Mine"

Tsurudome, Koji; Suzuki, Hajime; Aoki, Katsunori

JAEA-Review 2021-031, 186 Pages, 2021/12

JAEA-Review-2021-031.pdf:11.79MB

Tono Geoscience Center, Japan Atomic Energy Agency has been conducting mine closure activities at Tono Mine based on "Plan for closure activities of the Tono Mine" since FY2010. The closure activities of the Tono Mine are carried out in accordance with the Mining Act, the Mine Safety Act and the Industrial Safety and Health Act. In particular, in order to examine the technologies applied to the closure activities of the Tono mine, also the surrounding environmental monitoring, "Technical Committee on Mine Closure Activities of the Tono Mine" was organized at Tono Geoscience Center in FY2013 and the results in the previous fiscal year and the plan for the current fiscal year have been reported and discussed at the annual meeting. As a result, it has been confirmed that the closure activities are making progress as planned and that the environment around the mine meets the legally required standards from the monitoring results. This document is a compilation of meeting materials of all eight committee meetings held between FY2013 and FY2019.

JAEA Reports

Database for corrosion under irradiation conditions (Contract research)

Sato, Tomonori; Hata, Kuniki; Kaji, Yoshiyuki; Ueno, Fumiyoshi; Inoue, Hiroyuki*; Taguchi, Mitsumasa*; Seito, Hajime*; Tada, Eiji*; Abe, Hiroshi*; Akiyama, Eiji*; et al.

JAEA-Review 2021-001, 123 Pages, 2021/06

JAEA-Review-2021-001.pdf:10.33MB

In the implement of the decommissioning of Fukushima Daiichi Nuclear Power Station (1F), there are many problems to be solved. Specially, the mitigation of the aging degradation by the corrosion of the structural materials is important to implement the decommissioning safely and continuously. However, there are limited data for the environmental factors of corrosion in 1F, and the condition of 1F is continuously changing. So, the literature data for the water radiolysis and the corrosion under irradiation are listed as the database of corrosion under irradiation in this report. And the new obtained radiolysis and corrosion data, which have not been reported in the literature and will be required in the decommissioning of 1F, are reported.

Journal Articles

Thermally altered subsurface material of asteroid (162173) Ryugu

Kitazato, Kohei*; Milliken, R. E.*; Iwata, Takahiro*; Abe, Masanao*; Otake, Makiko*; Matsuura, Shuji*; Takagi, Yasuhiko*; Nakamura, Tomoki*; Hiroi, Takahiro*; Matsuoka, Moe*; et al.

Nature Astronomy (Internet), 5(3), p.246 - 250, 2021/03

 Times Cited Count:30 Percentile:96.87(Astronomy & Astrophysics)

Here we report observations of Ryugu's subsurface material by the Near-Infrared Spectrometer (NIRS3) on the Hayabusa2 spacecraft. Reflectance spectra of excavated material exhibit a hydroxyl (OH) absorption feature that is slightly stronger and peak-shifted compared with that observed for the surface, indicating that space weathering and/or radiative heating have caused subtle spectral changes in the uppermost surface. However, the strength and shape of the OH feature still suggests that the subsurface material experienced heating above 300 $$^{circ}$$C, similar to the surface. In contrast, thermophysical modeling indicates that radiative heating does not increase the temperature above 200 $$^{circ}$$C at the estimated excavation depth of 1 m, even if the semimajor axis is reduced to 0.344 au. This supports the hypothesis that primary thermal alteration occurred due to radiogenic and/or impact heating on Ryugu's parent body.

Journal Articles

Vertical distributions of Iodine-129 and iodide in the Chukchi Sea and Bering Sea

Miwa, Kazuji; Obata, Hajime*; Suzuki, Takashi

Journal of Nuclear Science and Technology, 57(5), p.537 - 545, 2020/05

 Times Cited Count:2 Percentile:21.95(Nuclear Science & Technology)

This study investigated the vertical distribution of Iodine-129 ($$^{129}$$I) which is mainly produced by European nuclear reprocessing plants in the Chukchi Sea and Bering Sea. $$^{129}$$I was found to be distributed almost uniformly in fallout level, and an increasing in $$^{129}$$I concentration levels caused by high $$^{129}$$I water inflow from the Atlantic Ocean was not observed. Additionally, we revealed the vertical distribution of iodide, one chemical form of iodine, from the Bering Shelf area to the Chukchi Sea for the first time. The increasing tendency of iodide near sea bottom was observed.

Journal Articles

$$omega N$$ scattering length from $$omega$$ photoproduction on the proton near the reaction threshold

Ishikawa, Takatsugu*; Fujimura, Hisako*; Fukasawa, Hiroshi*; Hashimoto, Ryo*; He, Q.*; Honda, Yuki*; Hosaka, Atsushi; Iwata, Takahiro*; Kaida, Shun*; Kasagi, Jirota*; et al.

Physical Review C, 101(5), p.052201_1 - 052201_6, 2020/05

Journal Articles

Corrosion monitoring in humidity-controlled environment simulating gamma ray irradiation

Omori, Atsushi*; Akiyama, Eiji*; Abe, Hiroshi*; Hata, Kuniki; Sato, Tomonori; Kaji, Yoshiyuki; Inoue, Hiroyuki*; Taguchi, Mitsumasa*; Seito, Hajime*; Tada, Eiji*; et al.

Zairyo To Kankyo, 69(4), p.107 - 111, 2020/04

To evaluate the effect of oxidants, which are formed by radiolysis of water under gamma ray irradiation, on the corrosion of a carbon steel in humid environment, ozone was introduced as a model oxidant in to humidity-controlled air at 50$$^{circ}$$C in a thermo-hygrostat chamber. Corrosion monitoring was performed by using an Atmospheric Corrosion Monitor-type (ACM) sensor consisting of a carbon steel anode and an Ag cathode. The output current of the ACM sensor was increased with the increase in relative humidity and it was obviously increased with the increase in the introduced ozone concentration at each relative humidity. The results indicate that ozone accelerates the corrosion of the carbon steel. The effect of ozone on the corrosion acceleration is attributed to the fast reduction reaction and fast dissolution reaction in to water compared to that of oxygen.

JAEA Reports

Decommissioning activities and R&D of nuclear facilities in the second midterm plan

Terunuma, Akihiro; Mimura, Ryuji; Nagashima, Hisao; Aoyagi, Yoshitaka; Hirokawa, Katsunori*; Uta, Masato; Ishimori, Yuu; Kuwabara, Jun; Okamoto, Hisato; Kimura, Yasuhisa; et al.

JAEA-Review 2016-008, 98 Pages, 2016/07

JAEA-Review-2016-008.pdf:11.73MB

Japan Atomic Energy Agency formulated the plan to achieve the medium-term target in the period of April 2010 to March 2015(hereinafter referred to as "the second medium-term plan"). JAEA determined the plan for the business operations of each year (hereinafter referred to as "the year plan"). This report is that the Sector of Decommissioning and Radioactive Waste Management has summarized the results of the decommissioning technology development and decommissioning of nuclear facilities which were carried out in the second medium-term plan.

Journal Articles

Lithium intercalation and structural changes at the LiCoO$$_{2}$$ surface under high voltage battery operation

Taminato, So*; Hirayama, Masaaki*; Suzuki, Kota*; Tamura, Kazuhisa; Minato, Taketoshi*; Arai, Hajime*; Uchimoto, Yoshiharu*; Ogumi, Zempachi*; Kanno, Ryoji*

Journal of Power Sources, 307, p.599 - 603, 2016/03

 Times Cited Count:31 Percentile:72.1(Chemistry, Physical)

An epitaxial-film model electrode of LiCoO$$_{2}$$(104) was fabricated on SrRuO$$_{3}$$(100)/Nb:SrTiO$$_{3}$$(100) using pulsed laser deposition. The 50 nm thick LiCoO$$_{2}$$(104) film exhibited lithium (de-)intercalation activity with a first discharge capacity of 119 mAh g$$^{-1}$$ between 3.0 and 4.4 V, followed by a gradual capacity fading with subsequent charge-discharge cycles. In contrast, a 3.2 nm thick Li$$_{3}$$PO$$_{4}$$-coated film exhibited a higher intercalation capacity of 148 mAh g$$^{-1}$$ with superior cycle retention than the uncoated film. In situ surface X-ray diffraction measurements revealed a small lattice change at the coated surface during the (de-)intercalation processes compared to the uncoated surface. The surface modification of LiCoO$$_{2}$$ by the Li$$_{3}$$PO$$_{4}$$ coating could lead to improvement of the structural stability at the surface region during lithium (de-)intercalation at high voltage.

Journal Articles

In-vessel coils for magnetic error field correction in JT-60SA

Matsunaga, Go; Takechi, Manabu; Sakurai, Shinji; Suzuki, Yasuhiro*; Ide, Shunsuke; Urano, Hajime

Fusion Engineering and Design, 98-99, p.1113 - 1117, 2015/10

 Times Cited Count:14 Percentile:77.78(Nuclear Science & Technology)

Journal Articles

Integrated modelling of toroidal rotation with the 3D non-local drift-kinetic code and boundary models for JT-60U analyses and predictive simulations

Honda, Mitsuru; Satake, Shinsuke*; Suzuki, Yasuhiro*; Yoshida, Maiko; Hayashi, Nobuhiko; Kamiya, Kensaku; Matsuyama, Akinobu; Shinohara, Koji; Matsunaga, Go; Nakata, Motoki; et al.

Nuclear Fusion, 55(7), p.073033_1 - 073033_11, 2015/07

 Times Cited Count:6 Percentile:28.65(Physics, Fluids & Plasmas)

Journal Articles

Assessment of the accuracy of plasma shape reconstruction by the Cauchy condition surface method in JT-60SA

Miyata, Yoshiaki; Suzuki, Takahiro; Takechi, Manabu; Urano, Hajime; Ide, Shunsuke

Review of Scientific Instruments, 86(7), p.073511_1 - 073511_13, 2015/07

 Times Cited Count:5 Percentile:24.25(Instruments & Instrumentation)

It is essential for a stable plasma equilibrium control to reconstruct an accurate plasma boundary in tokamak devices. Cauchy Condition Surface (CCS) method is a numerical approach to calculate the spatial distribution of the magnetic flux outside a hypothetical plasma surface and reconstruct the plasma boundary from the magnetic measurements located outside the plasma. It is found that the optimum number of unknown parameters and shape of the CCS for minimizing errors in the reconstructed plasma shape increase in proportion to the plasma size. It is shown that the accuracy of the plasma shape reconstruction greatly improves by using the optimum number of unknown parameters. The assessment of accuracy of plasma shape reconstruction by CCS method in JT-60SA is reported.

Journal Articles

Advance in integrated modelling towards prediction and control of JT-60SA plasmas

Hayashi, Nobuhiko; Honda, Mitsuru; Shiraishi, Junya; Miyata, Yoshiaki; Wakatsuki, Takuma; Hoshino, Kazuo; Toma, Mitsunori; Suzuki, Takahiro; Urano, Hajime; Shimizu, Katsuhiro; et al.

Europhysics Conference Abstracts (Internet), 39E, p.P5.145_1 - P5.145_4, 2015/06

Journal Articles

Experimental analyses and predictive simulations of toroidal rotation driven by the neoclassical toroidal viscosity in rippled tokamaks

Honda, Mitsuru; Satake, Shinsuke*; Suzuki, Yasuhiro*; Matsunaga, Go; Shinohara, Koji; Yoshida, Maiko; Matsuyama, Akinobu; Ide, Shunsuke; Urano, Hajime

Nuclear Fusion, 54(11), p.114005_1 - 114005_14, 2014/11

 Times Cited Count:15 Percentile:59.37(Physics, Fluids & Plasmas)

Journal Articles

Integrated modeling of toroidal rotation with the 3D non-local drift-kinetic code and boundary models for JT-60U analyses and predictive simulations

Honda, Mitsuru; Satake, Shinsuke*; Suzuki, Yasuhiro*; Yoshida, Maiko; Hayashi, Nobuhiko; Kamiya, Kensaku; Matsuyama, Akinobu; Shinohara, Koji; Matsunaga, Go; Nakata, Motoki; et al.

Proceedings of 25th IAEA Fusion Energy Conference (FEC 2014) (CD-ROM), 8 Pages, 2014/10

Journal Articles

Analysis of JT-60SA scenarios on the basis of JET and JT-60U discharges

Garcia, J.*; Hayashi, Nobuhiko; Giruzzi, G.*; Schneider, M.*; Joffrin, E.*; Ide, Shunsuke; Sakamoto, Yoshiteru; Suzuki, Takahiro; Urano, Hajime; JT-60 Team; et al.

Europhysics Conference Abstracts (Internet), 38F, p.P1.029_1 - P1.029_4, 2014/06

Journal Articles

High power laser developments with femtosecond to nanosecond pulse durations for laser shock science and engineering

Kiriyama, Hiromitsu; Mori, Michiaki; Suzuki, Masayuki*; Daito, Izuru*; Okada, Hajime; Ochi, Yoshihiro; Tanaka, Momoko; Sato, Masatoshi*; Tamaoki, Yoshinori*; Yoshii, Takehiro*; et al.

Reza Kenkyu, 42(6), p.441 - 447, 2014/06

We describe three specific high power laser systems that are being developed in our laboratory for many applications in high field science, nonlinear optics and material processing. We report on a femtosecond petawatt-class Ti:sapphire chirped-pulse amplification laser system that can produce a pulse energy of 20 J of 40 fs pulse duration, a picosecond high intensity Yb:YAG chirped-pulse amplification laser system that can generate a pulse energy of 100 mJ of 0.5 ps pulse duration, and a nanosecond high repetition rate Nd:YAG laser system that can provide an average power of 360 W with a pulse duration of 30 ns delivered at a 1 kHz repetition rate. We discuss the basic design aspects and present the results from our experimental investigations of these laser systems.

Journal Articles

Study of plasma equilibrium control for JT-60SA using MECS

Miyata, Yoshiaki; Suzuki, Takahiro; Ide, Shunsuke; Urano, Hajime

Plasma and Fusion Research (Internet), 9(Sp.2), p.3403045_1 - 3403045_5, 2014/05

The precise control of the plasma position is essential in safe and stable plasma operation. An MHD equilibrium control simulator has been developed in order to study the techniques of plasma equilibrium control for JT-60SA. In this study, the modules of plasma shape reconstruction, power supply, PF and FPPC coils are incorporated in order to simulate the real plasma equilibrium control. The plasma equilibrium control is simulated during Ip ramp-up within the power supply capability using MECS.

Journal Articles

Study of JT-60SA operation scenario using a plasma equilibrium control simulator

Miyata, Yoshiaki; Suzuki, Takahiro; Ide, Shunsuke; Urano, Hajime; Fujita, Takaaki

Plasma and Fusion Research (Internet), 8(Sp.1), p.2405109_1 - 2405109_6, 2013/08

The precise control of the plasma position is a key issue in safe and stable plasma operation. A plasma equilibrium control simulator has been developed in order to study the techniques of plasma equilibrium control for JT-60SA. The simulator consists of an equilibrium solver and controller. The equilibrium solver identifies the plasma equilibrium under the given coil current and unknown eddy current by iteration. The function which calculates the self-consistent $$I$$$$_{rm p}$$ with magnetic flux consumption has been incorporated in order to simulate the $$I$$$$_{rm p}$$ control. The waveforms of JT-60SA plasma operation scenario during the $$I$$$$_{rm p}$$ ramp-up and the controllability of the plasma equilibrium control using the equilibrium control simulator were reported.

Journal Articles

Data of heavy elements for light sources in EUV and XUV and for other applications

Koike, Fumihiro*; Funaba, Hisamichi*; Goto, Motoshi*; Kato, Daiji*; Kato, Takako*; Morita, Shigeru*; Murakami, Izumi*; Sakaue, Hiroyuki*; Sudo, Shigeru*; Suzuki, Chihiro*; et al.

AIP Conference Proceedings 1545, p.202 - 211, 2013/07

 Times Cited Count:4 Percentile:83.62

Atomic ionic states and transition properties of elements with atomic numbers Z ranging from 50 to 80 are discussed as these are important to the understanding of plasmas containing such heavy elements. As such, data productions and the current status of theoretical calculations in this field are discussed. Further, recent spectroscopic measurements and respective theoretical analyses for W, Gd, and Nd are provided.

176 (Records 1-20 displayed on this page)