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Takasaki, Koji; Yasumune, Takashi; Yamaguchi, Yukako; Hashimoto, Makoto; Maeda, Koji; Kato, Masato
Journal of Nuclear Science and Technology, 60(11), p.1437 - 1446, 2023/11
Times Cited Count：0 Percentile：0.01(Nuclear Science & Technology)The aerodynamic radioactive median diameter (AMAD) is necessary information to assess the internal exposure. On June 6, 2017, at a plutonium handling facility in Oarai site of Japan Atomic Energy Agency (JAEA), during the inspection work of a storage container that contains nuclear fuel materials, accidental contamination occurred and five workers inhaled radioactive materials including plutonium. Some smear papers and an air sampling filter were measured with the imaging plate, and we conservatively estimated minimum AMADs for two cases, plutonium nitrate and plutonium dioxide. As a result of AMAD estimation, even excluding a giant particle of a smear sample, the minimum AMADs of plutonium nitrate from smear papers were 4.3 - 11.3 
m and those of plutonium dioxide were 5.6 - 14.1 m. Also, the minimum AMAD of plutonium nitrate from an air sampling filter was 3.0 m and that of plutonium dioxide was 3.9 m.
particle diameters using an alpha-particle imaging detectorMorishita, Yuki; Sagawa, Naoki; Takada, Chie; Momose, Takumaro; Takasaki, Koji
Radiation Protection Dosimetry, 199(13), p.1376 - 1383, 2023/08
Times Cited Count：0 Percentile：0.01(Environmental Sciences)It is very important to evaluate the diameters (activity median aerodynamic diameter) of Plutonium dioxide (PuO) particles for internal exposure dose evaluation. In this study, a method of evaluating PuO particle diameters using an alpha-particle imaging detector was developed. PuO particles with different diameters were modeled by Monte Carlo simulation, and the change in the shape of the energy spectrum for each particle diameter was evaluated. Two different patterns were modeled, namely, the case of 
PuO and the case of PuO (including isotopic composition of Pu). Multiple regression analysis was performed to determine the PuO particle diameter from the obtained parameters. The simulated diameters and the diameters obtained with the regression model were in good agreement. The advantage of using the alpha-particle imaging detector is to measure the alpha energy spectrum for individual particle, and this allows accurate measurement of particle diameter distribution.
Morishita, Yuki; Takasaki, Koji; Kitayama, Yoshiharu; Tagawa, Akihiro; Shibata, Takuya; Hoshi, Katsuya; Kaneko, Junichi*; Higuchi, Mikio*; Oura, Masatoshi*
Radiation Measurements, 160, p.106896_1 - 106896_10, 2023/01
Times Cited Count：0 Percentile：0.01(Nuclear Science & Technology)This study proposes a newly developed phoswich alpha/beta detector that can discriminate alpha and beta particles emitted from the alpha and beta contaminations in the FDNPS site. The phoswich alpha/beta detector is made up of two layers of scintillators that detect alpha and beta particles. The pulse shape discrimination (PSD) method was used to detect alpha particles in high beta particle and high gamma-ray (comparable to gamma-ray dose rate near the FDNPS reactor building) environments. Due to a 23.3% full width at half maximum (FWHM) energy resolution for alpha particles, the detector can be used to distinguish between nuclear fuel materials such as plutonium and its radon progeny (Po-214). Moreover, the detector could distinguish alpha particles from 
Cs gamma rays with a dose rate background up to 9.0 mSv/h. It is the first to demonstrate that the developed phoswich detector can be used to discriminate and measure alpha and beta particles of the actual contaminated FDNPS samples.
Matsuoka, Amane; Yasumune, Takashi; Kojima, Nobuhiro; Miyauchi, Hideaki; Takasaki, Koji; Hashimoto, Makoto
JAEA-Review 2021-055, 11 Pages, 2021/12
JAEA-Review-2021-055.pdf:1.12MB
The dose limit for the eye lens was lowered on April 1 2021, and a 3 mm dose equivalent was added to the calculation. The guidelines require that lens dosimeters be worn and managed when there is a risk of exceeding control standards. In this report, in order to examine future management methods, we investigated whether work that might exceed the equivalent dose limit was performed in the past. As a result of the investigation, the exposure dose for all works after fiscal year 2008 was sufficiently low compared to the equivalent dose limit. For this reason, it is considered that there is no need for additional management of wearing a personal dosimeter near the eyes for the work that is normally performed. In the future, as in the past, the basic management method will be to wear a dosimeter only on the basic part of the trunk under uniform exposure conditions, and to wear a dosimeter on the basic part of the trunk and the maximum dose part under nonuniform exposure conditions. When performing work with a high exposure dose to the eye lens, a dosimeter should be worn near the eye to measure the 3 mm dose equivalent.
Takasaki, Koji; Yasumune, Takashi; Hashimoto, Makoto; Maeda, Koji; Kato, Masato; Yoshizawa, Michio; Momose, Takumaro
JAEA-Review 2019-003, 48 Pages, 2019/03
JAEA-Review-2019-003.pdf:3.81MB
June 6, 2017, at Plutonium Fuel Research Facility in Oarai Research and Development Center of JAEA, when five workers were inspecting storage containers containing plutonium and uranium, resin bags in a storage container ruptured, and radioactive dust spread. Though they were wearing a half face mask respirator, they inhaled radioactive materials. In the evaluation of the internal exposure dose, the aerodynamic radioactive median diameter (AMAD) is an important parameter. We measured 14 smear samples and a dust filter paper with imaging plates, and estimated the AMAD by image analysis. As a result of estimating the AMAD, from the 14 smear samples, the AMADs are 4.3 to 11 m or more in the case of nitrate plutonium, and the AMADs are 5.6 to 14 m or more in the case of the oxidized plutonium. Also, from the dust filter paper, the AMAD is 3.0 m or more in the case of nitrate plutonium, and the AMAD is 3.9 m or more in the case of the oxidized plutonium.
Nakamura, Keisuke; Morishita, Yuki; Takasaki, Koji; Maehata, Keisuke*; Sugimoto, Tetsuya*; Kiguchi, Yu*; Iyomoto, Naoko*; Mitsuda, Kazuhisa*
Journal of Low Temperature Physics, 193(3-4), p.314 - 320, 2018/11
Times Cited Count：0 Percentile：0(Physics, Applied)
I concentrations in the air using data measured by monitoring posts applied by determination of passing-through time of plume using noble gas countsYamada, Junya; Hashimoto, Makoto; Seya, Natsumi; Haba, Risa; Muto, Yasunobu; Shimizu, Takehiko; Takasaki, Koji; Yokoyama, Sumi*; Shimo, Michikuni*
Hoken Butsuri, 52(1), p.5 - 12, 2017/03
The purpose of this study is to improve a quick method for estimation of I concentrations in the air using data measured by monitoring posts in case that a nuclear disaster occurs. In this method, I concentrations were estimated by multiplying I count rates of cloud-shine measured with NaI (Tl) detector by concentration conversion factor. A previous study suggested that it was difficult to determine passing-through time of plume from temporal change of I count rates or dose rate. Our study applies the method for estimating passing-through time of plume from temporal change of noble gas counts. The I concentrations in the air at Oarai center, Japan Atomic Energy Agency resulting from the accident at the Fukushima Daiichi Nuclear Power Plant were estimated by proposal technique. The result of comparison of this method with sampling method for I concentrations in the air were within factor 3.
I concentrations in the air from pulse-height distribution observed by NaI(Tl) detector in monitoring postsYamada, Junya; Hashimoto, Makoto; Seya, Natsumi; Haba, Risa; Muto, Yasunobu; Shimizu, Takehiko; Takasaki, Koji; Yokoyama, Sumi*; Shimo, Michikuni*
Radioisotopes, 65(10), p.403 - 408, 2016/10
The purpose of this study is to develop a quick method for estimation of I concentrations in the air using data measured by monitoring posts. In this method, I concentrations were estimated by multiplying I count rates at the full-energy peak measured with a NaI(Tl) detector by a concentration conversion factor. The concentration conversion factor for monitoring posts in JAEA Oarai Center was calculated with an EGS5 Monte Carlo code. As a result, the concentration conversion factor for an infinite-air-source was 25.7 Bq/m
/cps.
Seya, Natsumi; Hashimoto, Makoto; Nemoto, Koji*; Shimizu, Takehiko; Takasaki, Koji
Hoken Butsuri, 49(1), p.29 - 38, 2014/03
Evaluation of annual average of radionuclide concentration in surface air obtained from atmospheric dispersion factor is intended to determine a public dose as a primary source for the safety analysis of nuclear facilities in normal operation. Oarai Research and Development Center (ORDC) of the JAEA have used fixed 5-year meteorological statistics for derivation of atmospheric dispersion factors as average conditions. To show that the meteorological statistics for any 5-year period could be used as representative data for evaluation of average conditions, annual average (1-year average) and 5-year average of evaluated radionuclide concentrations derived from the meteorological data observed from 1991 to 2010 at ORDC were analyzed. The fluctuations of evaluated radionuclide concentrations of any 5-year averages were smaller than those of 1-year averages during 20 years, and any 5-year averages contained no rejections by the F-test (5% significance level). It means that any 5-year averages of radionuclide concentration evaluations are well representative for the safety analysis under normal condition in ORDC.
Takasaki, Koji; Yasumune, Takashi; Onishi, Takashi; Nakamura, Keisuke; Ishimi, Akihiro; Ito, Chikara; Osaka, Masahiko; Ono, Masashi*; Hatakeyama, Shuichi*; Takahashi, Hiroyuki*; et al.
JAEA-Research 2013-043, 33 Pages, 2014/01
JAEA-Research-2013-043.pdf:13.81MB
In the Fukushima Daiichi Nuclear Power Plant, it is assumed that the core fuels melted partially or wholly, and the normal technique of accounting for a fuel assembly is not applicable. Therefore, it is necessary to develop the transparent and rational technique of accounting in the process of collection and storage of fuel debris. In this research, an application of the superconducting phase Transition Edge Sensor microcalorimeter (TES microcalorimeter) is studied for the accounting of nuclear materials in the fuel debris. It is expected that the detailed information of nuclear materials and fission products in fuel debris is obtained by using a high-resolution characteristic of TES microcalorimeter. In this report, the principle of TES microcalorimeter, the measurement experiment using TES in JAEA, and the simulated calculation using the EGS5 code system are summarized.
Yamada, Junya; Seya, Natsumi; Haba, Risa; Muto, Yasunobu; Numari, Hideyuki*; Sato, Naomitsu*; Nemoto, Koji*; Takasaki, Hiroichi*; Shimizu, Takehiko; Takasaki, Koji
JAEA-Data/Code 2013-006, 100 Pages, 2013/06
JAEA-Data-Code-2013-006.pdf:12.04MB
This report presents the results of emergency radiation monitoring, including ambient 
-ray dose rate, atmospheric radioactivity, meteorological observation and estimation of internal exposure resulting from the accident at the Fukushima Daiichi Nuclear Power Plant triggered by the earthquake off the pacific coast of Tohoku on 11th March 2011, conducted by Oarai Research and Development Center (ORDC), Japan Atomic Energy Agency (JAEA) from March to May, 2011. ORDC is located in the central part of Ibaraki prefecture and approximately 130 km southwest of the Fukushima Daiichi Nuclear Power Plant. From around 15th to 21st March, 2011, the ambient -ray dose rate increased and many radioactive nuclides were detected in the atmosphere.
Nakamura, Keisuke; Maeda, Makoto*; Yasumune, Takashi*; Maehata, Keisuke*; Ishibashi, Kenji*; Tanaka, Keiichi*; Umeno, Takahiro*; Takasaki, Koji; Momose, Takumaro
Radiation Protection Dosimetry, 146(1-3), p.88 - 91, 2011/07
Times Cited Count：1 Percentile：10.73(Environmental Sciences)A Transition Edge Sensor (TES) microcalorimeter has been developed for use as an energy dispersive X-ray spectrometer. A TES microcalorimeter is a thermal detector used to measure the energy of an incident photon with increase in temperature. In this work, a TES microcalorimeter with a 5m Au absorber was developed for use in measuring LX rays emitted from transuranium elements. Furthermore, as a cooling system a dilution refrigerator utilizing a Gifford-McMahon refrigerator was used, which needs no liquid helium. The performance of the TES microcalorimeter was evaluated by measuring the LX rays emitted by an 
Am source. This system proved effective in the measurement of the LX rays because the full width at half maximum of the L
X ray was about 80 eV.
Takasaki, Koji; Sagawa, Naoki; Kurosawa, Shigeyuki; Mizuniwa, Harumi
Journal of Nuclear Science and Technology, 48(6), p.911 - 918, 2011/06
Times Cited Count：12 Percentile：66.82(Nuclear Science & Technology)An autoradiographical method using an imaging plate (IP) was developed to analyze the plutonium contamination in the plutonium handling facility and was applied to the monitoring of the workplace in a practical uranium-plutonium mixed oxide (MOX) fuel fabrication facility. A good relationship between the photo stimulated luminescence (PSL) intensities of IP and radioactivities measured by a radiation counter was obtained by the least-square fitting, taking the fading effect into consideration. The 
-radioactivities of plutonium contamination were derived from the PSL image in this IP method, and their relative errors were evaluated from exposure time.
Takashima, Hideki; Takasaki, Koji; Shimizu, Takehiko; Kurihara, Ryoichi
Genshiryoku eye, 57(5), p.72 - 76, 2011/05
no abstracts in English
Sagawa, Naoki; Yamazaki, Takumi; Kurosawa, Shigeyuki*; Izaki, Kenji; Mizuniwa, Harumi; Takasaki, Koji
JAEA-Technology 2010-051, 35 Pages, 2011/03
JAEA-Technology-2010-051.pdf:1.83MB
The image analysis method using a imaging plate (IP) is recent technique, and this method can get the information of radioactivity distribution by the unit of Photo Simulated Luminescence (PSL). We have investigated the PSL images obtained by measuring some plutonium samples which are radiation protection samples in order to apply imaging plate to the radiation protection at the MOX fuel facility. Plutonium spots were extracted from the PSL image extracted by the threshold, in which about 99% of the back ground was excluded, and identified by the additional requirement that the spot size is more than 40 pixels. The average background is subtracted from PSL strength of the spot area identified as Pu, and the radioactivity of the Pu spot was evaluated by multiplying the conversion calculation that is in consideration of fading.
Takasaki, Koji; Kobayashi, Hirohide; Suzuki, Hideki; Ushigome, Sadaharu*
Journal of Nuclear Science and Technology, 47(3), p.255 - 261, 2010/03
Times Cited Count：3 Percentile：24.08(Nuclear Science & Technology)The wide-range krypton-85 detector was developed for monitoring of krypton-85 gas, which was discharged from the stack of a nuclear fuel reprocessing plant and varied largely in concentration. The detector combined a current-mode-operated plastic scintillation counter with a gated photomultiplier. The discrimination voltage of gated photomultiplier was determined, and the effects of temperature and humidity were examined on the background measurement. The detector was calibrated by krypton-85 gas and the decision threshold was estimated. These examinations showed that the wide-range krypton-85 detector worked in the measurement range as wide as 10
-10
Bq/cm in linearity and the decision threshold of krypton-85 concentration was 1.3
10 Bq/cm for 10-minute measurement. The parallel measurement was made between this detector and a GM counter in the reprocessing laboratory. Both concentrations showed a good agreement with each other.
Maehata, Keisuke*; Nakamura, Keisuke*; Yasumune, Takashi*; Ishibashi, Kenji*; Takasaki, Koji; Tanaka, Keiichi*; Odawara, Akikazu*; Nagata, Atsushi*
Journal of Nuclear Science and Technology, 47(3), p.308 - 313, 2010/03
Times Cited Count：5 Percentile：35.74(Nuclear Science & Technology)A phase transition edge sensor (TES) microcalorimeter was developed for the energy dispersive measurement of LX-ray photons emitted from transuranium elements. The phase transition temperature of the TES was designed to be 200 mK by using bilayer structure of Au of 120 nm thick and Ti of 50 nm thick. The Au layer of 5.0 m thick was deposited on the Au/Ti bilayer for absorption efficiency of 50% and counting rate of 100 counts per second in the detection of LX-ray photons with the energy from 10 to 20 keV. The TES microcalorimeter was operated for the detection of LX-ray photons emitted from Am, 
Pu and Pu sources. The decay time constant of 180 s of detection signal pulses allowed the TES microcalorimeter operating with the counting rate higher than 100 counts per second. The energy resolution was obtained to be 50 eV of FWHM value for a peak corresponding to 
Np L
X-ray of 17.75 keV.
Horikoshi, Yoshinori; Nemoto, Norio; Kurosawa, Shigeyuki*; Takasaki, Koji; Mizuniwa, Harumi
JAEA-Testing 2008-003, 29 Pages, 2008/04
JAEA-Testing-2008-003.pdf:1.65MB
In the Plutonium Fuel Technical Development Center, protective clothing suitable for sweltering radiation work was examined. Since it worried about the influence of wet protective clothing with sweat on detection of MOX powder contamination, Detection situations, the diffusion of contamination, and the osmosis and penetrability to wet protective clothing were examined about the present fabric and other new fabrics. As a result of examination, it was confirmed that the influence of detection on alpha ray in the wet condition of new fabrics was smaller than the current fabric. This report compiled the result of examination and points in the fabric selection suitable for protective clothing.
Takasaki, Koji; Sagawa, Naoki; Kurosawa, Shigeyuki*; Shioya, Satoshi; Suzuki, Kazunori; Horikoshi, Yoshinori; Mizuniwa, Harumi
JAEA-Technology 2008-028, 73 Pages, 2008/03
JAEA-Technology-2008-028.pdf:5.88MB
Recently, an imaging plate (IP) was developed. Pu analysis by an IP was studied in the JAEA Cooperative Research Scheme on the Nuclear Fuel Cycle, and the availability about detection of Pu and discrimination with radon progenies was shown. In order to apply these results to the radiation control, this research aims at evaluation of radioactivity, discrimination with radon progenies, and evaluation of AMAD by an IP. In the conventional autoradiography (ARG) by a ZnS and Polaroid film, Contamination of Pu can only be grasped by viewing. Since the digital data of the radiation and location is obtained by an IP, Pu can be detected quantitatively and radioactivity can be evaluated. As a result of this research, the image of alpha emitter on an IP is the same as that of the conventional ARG, and can be applied also to the ARG of beta and emitter. In measurement of Pu, the function of Image J (image-analysis software) was very available. Pu radioactivity was evaluated by an IP.
Kurihara, Osamu; Takada, Chie; Takasaki, Koji; Ito, Kimio; Momose, Takumaro; Miyabe, Kenjiro
Radiation Protection Dosimetry, 127(1-4), p.411 - 414, 2007/11
Times Cited Count：7 Percentile：47.34(Environmental Sciences)Practical action levels for beginning chelation therapy to remove plutonium in the body are now under discussion in Japan since there has been no experience in administrating agents to a subject in accidental intake in Japan although a first commercial reprocessing plant is about to start operation. Recently, International Commission on Radiological Protection (ICRP) proposed some medical intervention levels for chelation therapy on ICRP Publication 96. These levels are determined based on internal dose however common monitoring methods such as lung counting or excreta analysis are not necessarily suitable in terms of both sensitivity and promptness. As an alternative, the authors paid attention to nose swabs and introduced the practical action levels.
