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Journal Articles

Construction of a Compton camera-equipped robotic system capable of moving autonomously towards the radiation source

Sato, Yuki; Kakuto, Takeshi*; Tanaka, Takayuki*; Shimano, Hiroyuki*

European Physical Journal; Special Topics, 235(4), p.949 - 958, 2026/04

 Times Cited Count:0 Percentile:0.00(Physics, Multidisciplinary)

JAEA Reports

Development of mesh generation method in a fast reactor fuel assembly

Kikuchi, Norihiro; Imai, Yasutomo*; Yoshikawa, Ryuji; Tanaka, Masaaki; Ohshima, Hiroyuki

JAEA-Data/Code 2025-018, 96 Pages, 2026/03

JAEA-Data-Code-2025-018.pdf:5.54MB

In the Japan Atomic Energy Agency, a detailed thermal-hydraulic analysis code named SPIRAL based on the finite element method (FEM) is being developed to evaluate the detailed thermal-hydraulic properties of fuel assemblies (FAs) in sodium-cooled fast reactors (FBRs). Because the quality of the computational grid (elements) used in the calculations has a significant impact on the prediction accuracy, the allocation of high-quality elements in the wire-spacer-type FA pin bundle region is an important issue for numerical analysis. Although a commercial mesh generation program (mesher) with CAD data of FA's geometric shape can be considered as one measure, it is an extremely complicated task to perform element division of complex FA region. Therefore, to efficiently allocate high-quality elements, we developed a mesher that automatically performs element division in the FA region using the FA's geometric shape (design information) and meshing parameters as input conditions. This report describes the details of the mesher's various meshing models and their usage. To regularly allocate the computational grid for the complex FA region, the mesher first divides the region into multiple blocks using a multi-block method, then generates boundary-fitted curvilinear coordinate grids for each block region, and finally integrates them into a single FA mesh system. In addition, a combination of hexahedral elements and prism-shaped elements is arranged to maintain element continuity between adjacent block regions. Element division for both the normal FAs surrounded by a hexagonal cross-section tube and the irregular FAs, inside which a duct is installed to promote the discharge of molten fuel, is possible. The development of this mesher has made it possible to accurately and efficiently perform element division of complex FA region on various conditions.

JAEA Reports

Development of computer program for detailed thermal-hydraulic analysis in a fast reactor fuel assembly, 3; Implementation and validation of hybrid-type k-$$varepsilon$$/k$$_{theta}$$-$$varepsilon$$$$_{theta}$$ model

Kikuchi, Norihiro; Imai, Yasutomo*; Yoshikawa, Ryuji; Tanaka, Masaaki; Ohshima, Hiroyuki

JAEA-Data/Code 2025-017, 133 Pages, 2026/03

JAEA-Data-Code-2025-017.pdf:3.9MB

In a core design of sodium-cooled fast reactors (SFRs), it is necessary to confirm the integrity of fuel assemblies (FAs) in the core over a wide range of operating conditions. To evaluate the velocity and temperature distributions within the FAs in detail, we have been developing a detailed FA thermal-hydraulic analysis code named SPIRAL. In our previous works, we implemented numerical methods for fluid mechanics at isothermal conditions and turbulence models. Subsequently, we implemented turbulent heat transfer models for the evaluation of temperature distribution within the FAs, and validated them through experimental analyses mainly under high flow rate conditions. The thermal-hydraulics within the FAs varies depending on the operating conditions. Furthermore, the local Reynolds (Re) number within the FAs varies widely due to the influence of wire spacers spirally wound around the fuel rod. For this reason, it has been shown that standard and low Re number k-$$varepsilon$$/k$$_{theta}$$-$$varepsilon$$$$_{theta}$$ models have difficulty reproducing the thermal-hydraulics in the laminar-turbulent transition region. Therefore, to reproduce the thermal-hydraulics over a wide Re number range, we developed a hybrid k-$$varepsilon$$/k$$_{theta}$$-$$varepsilon$$$$_{theta}$$ model that combines the standard k-$$varepsilon$$/k$$_{theta}$$-$$varepsilon$$$$_{theta}$$ model with the advantages of the low Re number k-$$varepsilon$$/k$$_{theta}$$-$$varepsilon$$$$_{theta}$$ model. This paper describes the governing equations, constitutive equations derived from various turbulence models, their formularizations by the finite element method, their numerical treatment, and the treatment of boundary conditions. We also report the results of analyses conducted to validate the hybrid k-$$varepsilon$$/k$$_{theta}$$-$$varepsilon$$$$_{theta}$$ model for predicting pressure drop and temperature distribution.

Journal Articles

Development of HCl-free solid-phase extraction combined with ICP-MS/MS for rapid assessment of difficult-to-measure radionuclides, 4; Rapid determination of $$^{107}$$Pd in concrete rubble

Ota, Yuki; Do, V.-K.; Banjarnahor, I. M.; Iwahashi, Hiroyuki; Furuse, Takahiro; Tanaka, Kosuke

Journal of Radioanalytical and Nuclear Chemistry, 335(1), p.939 - 948, 2026/02

 Times Cited Count:0 Percentile:0.00(Chemistry, Analytical)

JAEA Reports

Analysis of deposits inside "X-6 penetration" for the Unit 2 primary containment vessel at Fukushima Daiichi Nuclear Power Station

Yoneyama, Kai; Nitta, Ayako; Tanaka, Yasuyuki; Kodaka, Noriyasu; Kikuchi, Riku; Sakano, Takuma; Furuse, Takahiro; Sato, Soichi; Sambongi, Mitsuru; Tanaka, Kosuke

JAEA-Technology 2025-008, 44 Pages, 2025/12

JAEA-Technology-2025-008.pdf:4.3MB

At the TEPCO's Fukushima Daiichi Nuclear Power Station (1F), an investigation inside the reactors has been carried out. In order to safely carry out the decommissioning work such as fuel debris retrieval and building demolition, it is important to estimate the contamination in primary containment vessel for control the decommissioning planning and the worker radiation exposure levels. Therefore, the analysis of the deposit inside the penetration for the 1F Unit 2 primary containment vessel ("X-6 penetration") was performed to clarify the components and activity. The smears from the deposit were used for the analysis. Non-destructive analysis such as gamma-ray spectrometry, X-ray Fluorescence (XRF) and Scanning Electron Microscope-Energy dispersive X-ray spectroscopy (SEM-EDX) for the smear-samples were performed to determine the gamma-nuclides and the morphology of elements in the deposit. Furthermore, in order to evaluate the nuclides and nuclide composition of the deposit in detail, the smear-samples were dissolved and the quantitative analysis of gamma-nuclides, Sr-90, alpha-nuclides in the dissolved solution were conducted. The results (non-destructive analysis and quantitative analysis) were compared with the results of samples collected at different locations in the X-6 penetration in 2020. In the gamma-ray spectrometry as non-destructive analysis where the smears were analyzed directly, Co-60, Sb-125, Cs-134, Cs-137, Eu-154, Eu-155 and Am-241 were detected. In XRF results, Fe originating from construction material was detected as a major element and small amount of U and Zr originating from the fuel and fuel cladding were also detected. In SEM-EDX results, O and Fe were found as a major element of the deposit and U particles coexisting with Fe, Si, Cr, Ni and Zr were also found. These results were consistent with the SEM-EDX results of the samples collected in 2020. In radioactivity analysis, quantitative values for gamma-nuclides (Co-60, Sb-125, Cs-134, Cs-137, Eu-154, Eu-155), Sr-90, Pu-238, Pu-239+240, Am-241, Cm-244, U-235 and U-238 were obtained. Using the results, the ratios of radioactivity based on Cs-137 and U-238 were calculated. Both sets of the ratios were compared to the calculated value of the Unit 2 fuel composition from ORIGEN.

Journal Articles

Speciation of cesium in a radiocesium-bearing microparticle emitted from Unit 1 during the Fukushima nuclear accident by XANES spectroscopy using transition edge sensor

Takahashi, Yoshio*; Miura, Hikaru*; Yamada, Shinya*; Sekizawa, Oki*; Nitta, Kiyofumi*; Hashimoto, Tadashi*; Yomogida, Takumi; Yamaguchi, Akiko; Okada, Shinji*; Itai, Takaaki*; et al.

Journal of Hazardous Materials, 495, p.139031_1 - 139031_19, 2025/09

 Times Cited Count:1 Percentile:40.80(Engineering, Environmental)

In this presentation, we analyzed the chemical state of cesium in radiocesium-bearing microparticles (CsMPs) released during the 2011 Fukushima Daiichi Nuclear Power Plant accident using high-resolution X-ray absorption spectroscopy (XANES) and micro X-ray fluorescence ($$mu$$-XRF). The results identified two forms of cesium: one dissolved in glass and the other enriched on the surfaces of internal voids. The latter is considered to have originally existed as a gas and became concentrated during the cooling and solidification of the molten glass. These findings are crucial for understanding the formation process of CsMPs during the accident, as well as for future decommissioning and safety assessments.

Journal Articles

Development of proton exchange membranes for HI concentration in thermochemical water-splitting IS process

Tanaka, Nobuyuki; Sawada, Shinichi*; Koshikawa, Hiroshi*; Yamaki, Tetsuya*

Material Stage, 25(6), p.76 - 80, 2025/09

A thermochemical water-splitting iodine-sulfur process enables us to provide the Carbon-free hydrogen (H$$_{2}$$) at high-efficiency levels, and it uses high-temperature heat sources, including high-temperature gas-cooled reactors, solar heat, and more. The cation exchange membranes (CEMs) for the HI mediated electro-electrodialysis (EED) were developed using a radiation grafted polymerization method in order to improve the process efficiency of the IS process. High proton (H$$^{+}$$) conductivity and selectivity are required for the performance of CEMs to reduce the consumption energy for EED. The H$$^{+}$$ conductivity of the radiation grafted CEMs were successfully improved by controlling the grafting amount, comparing with that of Nafion. Moreover, the H$$^{+}$$ selectivity and water transport of the developed CEMs was improved by introducing the crosslinker. Currently, the further improvement of the membrane performance is underway by using the ion-track grafting technic.

Journal Articles

Validation study on SFR core bowing codes using Joyo ex-core experiment data; Multiple duct bowing benchmark

Wozniak, N.*; Ohgama, Kazuya; Doda, Norihiro; Ota, Hirokazu*; Shemon, E.*; Feng, B.*; Uwaba, Tomoyuki; Futagami, Satoshi; Tanaka, Masaaki; Yamano, Hidemasa; et al.

Progress in Nuclear Science and Technology (Internet), 8, p.165 - 170, 2025/09

To enhance the accuracy of the safety evaluations for sodium-cooled fast reactors, it is necessary to develop a method that can realistically evaluate the reactivity changes induced by core deformation. In this context, Japan and the United States jointly conducted a benchmark analysis of thermal bowing experiments using multiple ducts from a Joyo-type fuel assembly. The aim was to confirm the validity of the core bowing analysis codes. Comparisons of analysis and experimental results demonstrated that the codes used by both countries were able to reasonably predict the thermal bowing of a row of assemblies in multiple duct configuration.

Journal Articles

Validation study on SFR core bowing codes using Joyo ex-core experiment data; Single duct bowing benchmark

Ohgama, Kazuya; Doda, Norihiro; Ota, Hirokazu*; Wozniak, N.*; Uwaba, Tomoyuki; Futagami, Satoshi; Tanaka, Masaaki; Yamano, Hidemasa; Ogata, Takanari*; Shemon, E.*; et al.

Progress in Nuclear Science and Technology (Internet), 8, p.160 - 164, 2025/09

To enhance the accuracy of the safety evaluations for sodium-cooled fast reactors, it is necessary to develop a method that can realistically evaluate the reactivity changes induced by core deformation. In this context, Japan and the United States jointly conducted a benchmark analysis of thermal bowing experiments using a single duct from a Joyo-type fuel assembly. The aim was to confirm the validity of the core bowing analysis codes. Comparisons of analysis and experimental results demonstrated that the codes used by both countries were able to reasonably predict the axial distribution of horizontal duct displacement caused by thermal bowing as well as the contact load on the duct pad.

Journal Articles

Core deformation reactivity with neutronics-thermal hydraulics-structural mechanics coupled analysis for FFTF LOFWOS Test #13

Doda, Norihiro; Kato, Shinya; Uwaba, Tomoyuki; Tanaka, Masaaki; Nakamine, Yoshiaki*; Igawa, Kenichi*; Iida, Masaki*

Proceedings of 21st International Topical Meeting on Nuclear Reactor Thermal Hydraulics (NURETH-21) (Internet), 14 Pages, 2025/08

Accurate evaluation of reactivity feedback due to core deformation during power increases in sodium-cooled fast reactors requires comprehensive modeling of the interactions among neutronics, thermal-hydraulics, and core mechanics. To accurately consider these interactions, JAEA has developed an evaluation method that combines multiple analysis codes that model these phenomena in detail. In this study, the evaluation method was applied to the core analysis of the FFTF LOFWOS Test #13, and the analysis results of net reactivity were compared with the test results. The sensitivity analysis results of the core structural design parameters showed that the core bowing behavior has a significant effect on the temporal variation of net reactivity.

Journal Articles

U(VI) adsorption on mudstone in the presence of carbonate; Batch experiments, modeling, cryo-TRLFS and PARAFAC analysis

Mei, H.; Aoyagi, Noboru; Saito, Takumi*; Tanaka, Kazuya; Sugiura, Yuki; Tachi, Yukio

Applied Clay Science, 276, p.107944_1 - 107944_8, 2025/07

 Times Cited Count:2 Percentile:50.74(Chemistry, Physical)

Journal Articles

Surface and interfacial aggregation states in thin films of a polystyrene/polyrotaxane blend

Taguchi, Miki*; Miyata, Noboru*; Miyazaki, Tsukasa*; Aoki, Hiroyuki; Ozawa, Satoru*; Hasegawa, Ryuichi*; Morimitsu, Yuma*; Kawaguchi, Daisuke*; Yamamoto, Satoru*; Tanaka, Keiji*

Polymer Journal, 57(7), p.737 - 743, 2025/07

 Times Cited Count:0 Percentile:0.00(Polymer Science)

Journal Articles

Neutron reflectometry study on the interfacial layer of epoxy resin to improve adhesion strength

Liu, Y.*; Miyata, Noboru*; Miyazaki, Tsukasa*; Shundo, Atsuomi*; Kawaguchi, Daisuke*; Tanaka, Keiji*; Aoki, Hiroyuki

ACS Applied Materials & Interfaces, 17(25), p.37311 - 37318, 2025/06

Journal Articles

Experimental studies on spatial resolution of a delay-line current-biased kinetic inductance detector

Vu, TheDang*; Shishido, Hiroaki*; Aizawa, Kazuya; Oku, Takayuki; Oikawa, Kenichi; Harada, Masahide; Kojima, Kenji M*; Miyajima, Shigeyuki*; Soyama, Kazuhiko; Koyama, Tomio*; et al.

Nuclear Instruments and Methods in Physics Research A, 1075, p.170425_1 - 170425_9, 2025/06

 Times Cited Count:0 Percentile:0.00(Instruments & Instrumentation)

Journal Articles

Development of HCl-free solid-phase extraction combined with ICP-MS/MS for rapid assessment of difficult-to-measure radionuclides, 3; Measurement of $$^{79}$$Se concentration in concrete rubble

Banjarnahor, I. M.; Do, V.-K.; Furuse, Takahiro; Ota, Yuki; Tanaka, Kosuke

Journal of Radioanalytical and Nuclear Chemistry, 334(7), p.4997 - 5006, 2025/05

 Times Cited Count:2 Percentile:80.51(Chemistry, Analytical)

Journal Articles

Competition between mass-symmetric and asymmetric fission modes in $$^{258}$$Md produced in the $$^{4}$$He + $$^{254}$$Es reaction

Nishio, Katsuhisa; Hirose, Kentaro; Makii, Hiroyuki; Orlandi, R.; Kean, K. R.*; Tsukada, Kazuaki; Toyoshima, Atsushi*; Asai, Masato; Sato, Tetsuya; Chiera, N. M.*; et al.

Physical Review C, 111(4), p.044609_1 - 044609_12, 2025/04

 Times Cited Count:1 Percentile:59.26(Physics, Nuclear)

Journal Articles

Development of corrosion-stable dual-Si-layered membranes for hydrogen production via thermochemical iodine-sulfur process

Myagmarjav, O.; Tanaka, Nobuyuki; Noguchi, Hiroki; Kamiji, Yu; Ono, Masato; Nomura, Mikihiro*; Takegami, Hiroaki

Progress in Nuclear Science and Technology (Internet), 7, p.235 - 242, 2025/03

Journal Articles

Development of a method for distinguishing alpha particles from other types of radiation using a high-resolution alpha imager

Morishita, Yuki; Sagawa, Naoki; Fujisawa, Makoto; Kurosawa, Shunsuke*; Sasano, Makoto*; Hayashi, Masateru*; Tanaka, Hiroki*

Radiation Measurements, 181, p.107371_1 - 107371_5, 2025/02

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

The effects of different types of radiation on a high-resolution alpha imager developed using an electron multiplying charge-coupled device (EMCCD) camera were investigated. This imager was originally developed to visualize alpha particles from Pu oxide particles at decommissioning sites. Other types of radiation such as beta particles, gamma rays, and neutrons are also present. The purpose of this study is to investigate the effects of these background radiations on the imager and to develop a method to discriminate between alpha particles and other types of radiation. When measuring gamma rays, and neutrons, the sensor of the EMCCD camera generated high intensity signals due to gamma rays and neutrons. These radiations were identified by image processing. The image values were binarized and the findContours function was applied to count the number of alpha particle spots. The results showed that alpha and gamma (neutron) radiation can be discriminated by using differences in intensity. This method will be useful for visualizing alpha particles at decommissioning sites.

Journal Articles

Quantitative evaluation of leakage flow rate in the sealing part using graphite gland packing to mount a hydrogen separation membrane tube for HI decomposition membrane reaction

Sugimoto, Chihiro; Myagmarjav, O.; Tanaka, Nobuyuki; Noguchi, Hiroki; Takegami, Hiroaki; Kubo, Shinji

International Journal of Hydrogen Energy, 95, p.98 - 107, 2024/12

 Times Cited Count:0 Percentile:0.00(Chemistry, Physical)

Journal Articles

Developing an online composition prediction for an HI-I$$_{2}$$-H$$_{2}$$O system using deep neural network

Tanaka, Nobuyuki; Takegami, Hiroaki; Noguchi, Hiroki; Kamiji, Yu; Myagmarjav, O.; Ono, Masato; Sugimoto, Chihiro

Chemical Engineering Science, 299, p.120479_1 - 120479_11, 2024/11

 Times Cited Count:0 Percentile:0.00(Engineering, Chemical)

We developed a deep neural network method to predict the composition of the iodine-sulfur process of thermochemical water-splitting hydrogen production using measurable properties. Unlike conventional titration analysis, this approach allows a quick understanding of fluid composition, providing essential information for controlling operating conditions. This study focused on the HI-I$$_{2}$$-H$$_{2}$$O three-component system within the IS process. Using Gibbs phase rule, the DNN model was constructed using online measurable parameters, such as temperature, pressure, and density, as input conditions. The model was trained with experimental data, and the structural parameters were tuned. Composition prediction using actual trend data demonstrated good correlation with titration analysis measurements. Furthermore, the local interpretable model-agnostic explanations method was incorporated to gain insights into the significance of input parameters for compositions from the DNN model, providing valuable information on crucial parameters for effective composition control.

1533 (Records 1-20 displayed on this page)