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Journal Articles

A Model intercomparison of atmospheric $$^{137}$$Cs concentrations from the Fukushima Daiichi Nuclear Power Plant accident, phase III; Simulation with an identical source term and meteorological field at 1-km resolution

Sato, Yosuke*; Sekiyama, Tsuyoshi*; Fang, S.*; Kajino, Mizuo*; Qu$'e$rel, A.*; Qu$'e$lo, D.*; Kondo, Hiroaki*; Terada, Hiroaki; Kadowaki, Masanao; Takigawa, Masayuki*; et al.

Atmospheric Environment; X (Internet), 7, p.100086_1 - 100086_12, 2020/10

The third model intercomparison project for investigating the atmospheric behavior of $$^{137}$$Cs emitted during the Fukushima Daiichi Nuclear Power Plant (FDNPP) accident (FDNPP-MIP) was conducted. A finer horizontal grid spacing (1 km) was used than in the previous FDNPP-MIP. Nine of the models used in the previous FDNPP-MIP were also used, and all models used identical source terms and meteorological fields. Our analyses indicated that most of the observed high atmospheric $$^{137}$$Cs concentrations were well simulated, and the good performance of some models improved the performance of the multi-model ensemble. The analyses also confirmed that the use of a finer grid resolution resulted in the meteorological field near FDNPP being better reproduced. The good representation of the wind field resulted in the reasonable simulation of the narrow distribution of high deposition amount to the northwest of FDNPP and the reduction of the overestimation over the area to the south of FDNPP. In contrast, the performance of the models in simulating plumes observed over the Nakadori area, the northern part of Gunma, and the Tokyo metropolitan area was slightly worse.

Journal Articles

Atmospheric-dispersion database system that can immediately provide calculation results for various source term and meteorological conditions

Terada, Hiroaki; Nagai, Haruyasu; Tanaka, Atsunori*; Tsuzuki, Katsunori; Kadowaki, Masanao

Journal of Nuclear Science and Technology, 57(6), p.745 - 754, 2020/06

 Times Cited Count:0 Percentile:100(Nuclear Science & Technology)

We have estimated source term and analyzed processes of atmospheric dispersion of radioactive materials released during the Fukushima Daiichi Nuclear Power Station (FDNPS) accident by the Worldwide version of System for Environmental Emergency Dose Information. On the basis of this experience, we developed an dispersion calculation method that can respond to various needs in a nuclear emergency and provide useful information for emergency-response planning. By this method, if a release point is known, it is possible to immediately obtain the prediction results by applying provided source term to the database of dispersion-calculation results prepared in advance. With this function, it is easy to compare results by applying various source term with monitoring data, and to find out the optimum source term, which was applied for the source term estimation of the FDNPS accident. By performing this calculation with past meteorological-analysis data, it is possible to immediately get dispersion-calculation results for various source term and meteorological conditions. This database can be used for pre-accident planning, such as optimization of a monitoring plan and understanding of events to be supposed in considering emergency countermeasures.

Journal Articles

Development of strength evaluation method of ceramic reactor for iodine-sulfur process and hydrogen production test in Japan Atomic Energy Agency

Takegami, Hiroaki; Noguchi, Hiroki; Tanaka, Nobuyuki; Iwatsuki, Jin; Kamiji, Yu; Kasahara, Seiji; Imai, Yoshiyuki; Terada, Atsuhiko; Kubo, Shinji

Nuclear Engineering and Design, 360, p.110498_1 - 110498_6, 2020/04

 Times Cited Count:1 Percentile:19.53(Nuclear Science & Technology)

Japan Atomic Energy Agency (JAEA) has been conducting R&D on the thermochemical iodine-sulfur (IS) process for nuclear-powered hydrogen production. The IS process is one of the promising candidates of heat application of the high-temperature gas-cooled reactors. JAEA fabricated main chemical reactors made of industrial structural materials and confirmed their integrity in practical corrosive environments in the IS process. Based on the results of these confirmation tests, JAEA have constructed a 100 NL/h-H$$_{2}$$-scale test facility made of industrial structural materials. In this report, we succeeded in extending the hydrogen production time from 8 hours to 31 hours by developing a stable hydrogen iodide solution transfer technology in a continuous hydrogen production test. In addition, using the fracture test data of the ceramic specimen, an equation for estimating the strength of the ceramic component was developed.

Journal Articles

Refinement of source term and atmospheric dispersion simulations of radionuclides during the Fukushima Daiichi Nuclear Power Station accident

Terada, Hiroaki; Nagai, Haruyasu; Tsuzuki, Katsunori; Furuno, Akiko; Kadowaki, Masanao; Kakefuda, Toyokazu*

Journal of Environmental Radioactivity, 213, p.106104_1 - 106104_13, 2020/03

 Times Cited Count:4 Percentile:6.48(Environmental Sciences)

In order to assess the radiological dose to the public resulting from the Fukushima Daiichi Nuclear Power Station accident in Japan, the spatial and temporal distribution of radioactive materials in the environment is necessary to be reconstructed by computer simulations with the atmospheric transport, dispersion and deposition model (ATDM) and source term of radioactive materials discharged into the atmosphere is essential. In this study, we carried out refinement of the source term and improvement of ATDM simulation by using an optimization method based on Bayesian inference with various measurements (air concentration, surface deposition, and fallout). We also constructed the spatiotemporal distribution of some major radionuclides in the air and on the surface (optimized dispersion database) by using the optimized release rates and ATDM simulations which is used for the comprehensive dose assessment by coupling with the behavioral pattern of evacuees from the accident.

Journal Articles

Processes affecting land-surface dynamics of $$^{129}$$I impacted by atmospheric $$^{129}$$I releases from a spent nuclear fuel reprocessing plant

Ota, Masakazu; Terada, Hiroaki; Hasegawa, Hidenao*; Kakiuchi, Hideki*

Science of the Total Environment, 704, p.135319_1 - 135319_15, 2020/02

 Times Cited Count:1 Percentile:100(Environmental Sciences)

Land-surface transfers of $$^{129}$$I are modeled and incorporated into a land-surface model (SOLVEG-II), and the model was applied to the observed transfer of $$^{129}$$I at a vegetated field impacted by atmospheric releases of $$^{129}$$I from Rokkasho reprocessing plant during 2007 to investigate the importance of each $$^{129}$$I-transfer pathway. The model calculation revealed that contamination of leaves of wild bamboo grasses was mostly caused by foliar adsorption of $$^{129}$$I (81%) induced via wet deposition of $$^{129}$$I. Wet deposition of $$^{129}$$I was the main $$^{129}$$I-input to the soil, ten-fold the dry deposition of $$^{129}$$I$$_{2}$$; however, the deposition of $$^{129}$$I during 2007 was only 2% of the model-assumed $$^{129}$$I that pre-existed in the soil; indicating the importance of long-term accumulation of $$^{129}$$I in soils. The model calculation also revealed that root uptake of $$^{129}$$I, not methylation, control the long-term turnover of soil $$^{129}$$I.

Journal Articles

Intercomparison of numerical atmospheric dispersion prediction models for emergency response to emissions of radionuclides with limited source information in the Fukushima Dai-ichi Nuclear Power Plant accident

Iwasaki, Toshiki*; Sekiyama, Tsuyoshi*; Nakajima, Teruyuki*; Watanabe, Akira*; Suzuki, Yasushi*; Kondo, Hiroaki*; Morino, Yu*; Terada, Hiroaki; Nagai, Haruyasu; Takigawa, Masayuki*; et al.

Atmospheric Environment, 214, p.116830_1 - 116830_11, 2019/10

 Times Cited Count:1 Percentile:100(Environmental Sciences)

The utilization of numerical atmospheric dispersion prediction (NDP) models for accidental discharge of radioactive substances was recommended by a working group of the Meteorological Society of Japan. This paper is to validate the recommendation through NDP model intercomparison in the accidental release from the Fukushima Dai-ichi Nuclear Power Plant in 2011. Emission intensity is assumed to be constant during the whole forecast period for the worst-case scenario unless time sequence of emission is available. We expect to utilize forecasts of surface air contaminations for preventions of inhalations of radioactive substances, and column-integrated amounts for mitigation of radiation exposure associated with wet deposition. Although NDP forecasts have ensemble spread, they commonly figure out relative risk in space and time. They are of great benefit to disseminating effective warnings to public without failure. The multi-model ensemble technique may be effective to improve the reliability.

JAEA Reports

Activities on predictions of atmospheric dispersion of radionuclides for nuclear tests by North Korea

Ishizaki, Shuhei; Hayakawa, Tsuyoshi; Tsuzuki, Katsunori; Terada, Hiroaki; Togawa, Orihiko

JAEA-Technology 2018-007, 43 Pages, 2018/10

JAEA-Technology-2018-007.pdf:5.67MB

When North Korea has carried out a nuclear test, by a request from Nuclear Regulation Authority (NRA), Nuclear Emergency Assistance and Training Center (NEAT) predicts atmospheric dispersion of radionuclides by WSPEEDI-II system in cooperation with Nuclear Science and Engineering Center (NSEC), and submits the predicted results to NRA as the activity to assist responses by the Japanese Government. This report explains frameworks of the Japanese Government and Japan Atomic Energy Agency (JAEA) to cope with nuclear tests by North Korea, and describes a series of activities by NEAT regarding predictions of atmospheric dispersion of radionuclides in response to the 5th and 6th nuclear tests carried out by North Korea in September 2016 and September 2017. Future plans and issues to be solved for responses to nuclear tests are also described in this report, together with an outline of a computer program system used in the predictions.

Journal Articles

Model intercomparison of atmospheric $$^{137}$$Cs from the Fukushima Daiichi Nuclear Power Plant accident; Simulations based on identical input data

Sato, Yosuke*; Takigawa, Masayuki*; Sekiyama, Tsuyoshi*; Kajino, Mizuo*; Terada, Hiroaki; Nagai, Haruyasu; Kondo, Hiroaki*; Uchida, Junya*; Goto, Daisuke*; Qu$'e$lo, D.*; et al.

Journal of Geophysical Research; Atmospheres, 123(20), p.11748 - 11765, 2018/10

 Times Cited Count:8 Percentile:32.79(Meteorology & Atmospheric Sciences)

A model intercomparison of the atmospheric dispersion of $$^{137}$$Cs emitted following the Fukushima Daiichi Nuclear Power Plant accident was conducted by 12 models to understand the behavior of $$^{137}$$Cs in the atmosphere. The same meteorological data, horizontal grid resolution, and an emission inventory were applied to all the models to focus on the model variability originating from the processes included in each model. The multi-model ensemble captured 40% of the observed $$^{137}$$Cs events, and the figure-of-merit in space for the total deposition of $$^{137}$$Cs exceeded 80. Our analyses indicated that the meteorological data were most critical for reproducing the $$^{137}$$Cs events. The results also revealed that the differences among the models were originated from the deposition and diffusion processes when the meteorological field was simulated well. However, the models with strong diffusion tended to overestimate the $$^{137}$$Cs concentrations.

Journal Articles

Current R&D status of thermochemical water splitting hydrogen production iodine-sulfur process in Japan Atomic Energy Agency, 1; Hydrogen production test and component development

Takegami, Hiroaki; Noguchi, Hiroki; Tanaka, Nobuyuki; Iwatsuki, Jin; Kamiji, Yu; Kasahara, Seiji; Imai, Yoshiyuki; Terada, Atsuhiko; Kubo, Shinji

Proceedings of 9th International Topical Meeting on High Temperature Reactor Technology (HTR 2018) (USB Flash Drive), 7 Pages, 2018/10

Japan Atomic Energy Agency (JAEA) has been conducting R&D on the thermochemical iodine-sulfur (IS) process for nuclear-powered hydrogen production. The IS process is one of the promising candidates of heat application of the high-temperature gas-cooled reactors. JAEA fabricated main chemical reactors made of industrial structural materials and confirmed their integrity in practical corrosive environments in the IS process. Based on the results of these confirmation tests, JAEA have constructed a 100 NL/h-H$$_{2}$$-scale test facility made of industrial structural materials. This report will present an outline and results of hydrogen production tests and reliability improvements of operation stability and components, such as development of a strength estimation method for heat-resistant and corrosion-resistant ceramics components made of silicon carbide.

Journal Articles

Impacts of anthropogenic source from the nuclear fuel reprocessing plants on global atmospheric iodine-129 cycle; A Model analysis

Kadowaki, Masanao; Katata, Genki*; Terada, Hiroaki; Suzuki, Takashi; Hasegawa, Hidenao*; Akata, Naofumi*; Kakiuchi, Hideki*

Atmospheric Environment, 184, p.278 - 291, 2018/07

 Times Cited Count:6 Percentile:38.79(Environmental Sciences)

The long-lived radioactive iodine ($$^{129}$$I) is a useful geochemical tracer in the atmospheric environment. We recently observed clear seasonal trends in air concentration and deposition of $$^{129}$$I in Japan. Using these data, we developed a global atmospheric $$^{129}$$I transport model to reveal key processes for the global atmospheric $$^{129}$$I cycle. The model generally reproduced the observed seasonal change in air concentration and deposition of $$^{129}$$I in Japan, and the global distribution of $$^{129}$$I concentration in rain as presented in past literature. Numerical experiments changing the intensity of anthropogenic and natural sources were conducted to quantify the impact of anthropogenic sources on the global $$^{129}$$I cycle. The results indicated that the atmospheric $$^{129}$$I from the anthropogenic sources was deposited in winter and can be accumulated mainly in the northern part of Eurasia. In contrast, the atmospheric $$^{129}$$I from the natural sources dominated the deposition in summer. These results suggested that the re-emission process of $$^{129}$$I from the Earth's surface may be important as a secondary impact of $$^{129}$$I in the global-scaled environment. Furthermore, although wet deposition dominated the total deposition in the Northern hemisphere, dry deposition regionally and seasonally contributed to the total deposition over arctic and northern part of Eurasia in winter, suggesting that the dry deposition may play a key role in the seasonal change of $$^{129}$$I deposition in the Northern hemisphere high latitudes.

Journal Articles

Atmospheric modeling of $$^{137}$$Cs plumes from the Fukushima Daiichi Nuclear Power Plant; Evaluation of the model intercomparison data of the Science Council of Japan

Kitayama, Kyo*; Morino, Yu*; Takigawa, Masayuki*; Nakajima, Teruyuki*; Hayami, Hiroshi*; Nagai, Haruyasu; Terada, Hiroaki; Saito, Kazuo*; Shimbori, Toshiki*; Kajino, Mizuo*; et al.

Journal of Geophysical Research; Atmospheres, 123(14), p.7754 - 7770, 2018/07

 Times Cited Count:9 Percentile:27.84(Meteorology & Atmospheric Sciences)

We compared seven atmospheric transport model results for $$^{137}$$Cs released during the Fukushima Daiichi Nuclear Power Plant accident. All the results had been submitted for a model intercomparison project of the Science Council of Japan in 2014. We assessed model performance by comparing model results with observed hourly atmospheric concentrations of $$^{137}$$Cs, focusing on nine plumes over the Tohoku and Kanto regions. The results showed that model performance for $$^{137}$$Cs concentrations was highly variable among models and plumes. We also assessed model performance for accumulated $$^{137}$$Cs deposition. Simulated areas of high deposition were consistent with the plume pathways, though the models that best simulated $$^{137}$$Cs concentrations were different from those that best simulated deposition. The ensemble mean of all models consistently reproduced $$^{137}$$Cs concentrations and deposition well, suggesting that use of a multimodel ensemble results in more effective and consistent model performance.

Journal Articles

Electrochemical reaction mechanisms under various charge-discharge operating conditions for Li$$_{1.2}$$Ni$$_{0.13}$$Mn$$_{0.54}$$Co$$_{0.13}$$O$$_{2}$$ in a lithium-ion battery

Konishi, Hiroaki*; Hirano, Tatsumi*; Takamatsu, Daiko*; Gunji, Akira*; Feng, X.*; Furutsuki, Sho*; Okumura, Takafumi*; Terada, Shohei*; Tamura, Kazuhisa

Journal of Solid State Chemistry, 262, p.294 - 300, 2018/06

 Times Cited Count:5 Percentile:39.08(Chemistry, Inorganic & Nuclear)

The potential in each state of charge (SOC) during charging of Li$$_{1.2}$$Ni$$_{0.13}$$Mn$$_{0.54}$$Co$$_{0.13}$$O$$_{2}$$ is higher than that during discharging. To clarify the effect of chargedischarge operating conditions on the electrochemical reaction, Li$$_{1.2}$$Ni$$_{0.13}$$Mn$$_{0.54}$$Co$$_{0.13}$$O$$_{2}$$ was charged and discharged under various charge-discharge operating ranges, and OCP, crystal structure, and oxidation states of the ransition metals were evaluated by electrochemical measurement, XRD, and XAFS. These results indicate that OCP, lattice parameters, and oxidation states of the transition metals of Li$$_{1.2}$$Ni$$_{0.13}$$Mn$$_{0.54}$$Co$$_{0.13}$$O$$_{2}$$ in each SOC are not constant. The XRD results indicate that two phases, namely, LiNi$$_{0.33}$$Mn$$_{0.33}$$Co$$_{0.33}$$O$$_{2}$$-like and Li$$_{2}$$MnO$$_{3}$$-like, exist in Li$$_{1.2}$$Ni$$_{0.13}$$Mn$$_{0.54}$$Co$$_{0.13}$$O$$_{2}$$.

Journal Articles

Mechanisms responsible for two possible electrochemical reactions in Li$$_{1.2}$$Ni$$_{0.13}$$Mn$$_{0.54}$$Co$$_{0.13}$$O$$_{2}$$ used for lithium ion batteries

Konishi, Hiroaki*; Hirano, Tatsumi*; Takamatsu, Daiko*; Gunji, Akira*; Feng, X.*; Furutsuki, Sho*; Okumura, Takafumi*; Terada, Shohei*; Tamura, Kazuhisa

Journal of Solid State Chemistry, 258, p.225 - 231, 2018/02

 Times Cited Count:6 Percentile:32.16(Chemistry, Inorganic & Nuclear)

Li$$_{1.2}$$Ni$$_{0.13}$$Mn$$_{0.54}$$Co$$_{0.13}$$O$$_{2}$$ is known as one of the cathode electrode material for Li ion batteries and its structure during charge and discharge process was investigated using electrochemical method and X-ray diffraction. It was found that in the charge process the structure changes in the order of Li$$_{2}$$MnO$$_{3}$$, LiNi$$_{0.33}$$Mn$$_{0.33}$$Co$$_{0.33}$$O$$_{2}$$, and Li$$_{2}$$MnO$$_{3}$$. On the other hand, in the discharge process, the structure changes in the order of Li$$_{2}$$MnO$$_{3}$$ and LiNi$$_{0.33}$$Mn$$_{0.33}$$Co$$_{0.33}$$O$$_{2}$$.

JAEA Reports

Development of a calculation method for atmospheric dispersion database that can immediately provide calculation results for any source term and period from hindcast to short-term forecast (Joint research)

Terada, Hiroaki; Tsuzuki, Katsunori; Kadowaki, Masanao; Nagai, Haruyasu; Tanaka, Atsunori*

JAEA-Data/Code 2017-013, 31 Pages, 2018/01

JAEA-Data-Code-2017-013.pdf:9.52MB

We developed an atmospheric dispersion calculation method that can respond to various needs for dispersion prediction in nuclear emergency and prepare database of information useful for planning of emergency response. In this method, it is possible to immediately get the prediction results for provided source term by creating a database of dispersion calculation results without specifying radionuclides, release rate and period except release point. By performing this calculation steadily along with meteorological data update, it is possible to immediately get calculation results for any source term and period from hindcast to short-term forecast. This function can be used for pre-accident planning such as optimization of monitoring plan and understanding events to be supposed for emergency response. Spatiotemporal distribution of radioactive materials reproduced by source term estimated inversely from monitoring based on this method is useful as a supplement to monitoring.

Journal Articles

Improvement of atmospheric dispersion simulation using an advanced meteorological data assimilation method to reconstruct the spatiotemporal distribution of radioactive materials released during the Fukushima Daiichi Nuclear Power Station accident

Kadowaki, Masanao; Nagai, Haruyasu; Terada, Hiroaki; Katata, Genki*; Akari, Shusaku*

Energy Procedia, 131, p.208 - 215, 2017/12

BB2016-0128.pdf:1.61MB

 Times Cited Count:3 Percentile:4.44

When radioactive materials are released into the atmosphere due to nuclear accidents, numerical simulations that can reproduce temporal and spatial distribution of radioactive materials are useful to provide the information for emergency responses and radiological dose assessment. In this study, we attempt to improve the atmospheric dispersion simulation using an advanced meteorological data assimilation method and reconstruct the spatiotemporal distribution of radioactive materials released due to the Fukushima Daiichi Nuclear Power Station (FDNPS) accident. The atmospheric dispersion simulations were carried out by the Lagrangian particle dispersion model GEARN developed by Japan Atomic Energy Agency. To obtain meteorological fields for GEARN calculation, we used the Weather Research and Forecasting model WRF with meteorological data assimilation using four-dimensional variational method (4D-Var). GEARN calculations of the surface deposition and air concentration of radionuclides were compared with measurements. In the area close to FDNPS, the spatial distribution of the deposition of Cs-137 and I-131 simulated by GEARN agreed with the measured one. The accuracy of modeled deposition in northwest and south directions from FDNPS was particularly improved. This results were mainly attributed to the better reproducibility of wind field by using the meteorological data assimilation with 4D-Var. The improvement of the accuracy of modeled deposition distribution of Cs-137 in the East Japan area was also apparent under the meteorological fields modified by 4D-Var. The information of atmospheric dispersion processes reconstructed in this study is used for updating the existing assessment of radiological dose resulting from the FDNPS accident based on atmospheric simulations by our previous studies. It can also provide useful suggestions to make emergency response plans for nuclear facilities in Japan.

Journal Articles

Magnetic Bragg dip and Bragg edge in neutron transmission spectra of typical spin superstructures

Mamiya, Hiroaki*; Oba, Yojiro; Terada, Noriki*; Watanabe, Norimichi*; Hiroi, Kosuke; Shinohara, Takenao; Oikawa, Kenichi

Scientific Reports (Internet), 7(1), p.15516_1 - 15516_8, 2017/11

 Times Cited Count:1 Percentile:88.91(Multidisciplinary Sciences)

no abstracts in English

Journal Articles

Updating source term and atmospheric dispersion simulations for the dose reconstruction in Fukushima Daiichi Nuclear Power Station accident

Nagai, Haruyasu; Terada, Hiroaki; Tsuzuki, Katsunori; Katata, Genki; Ota, Masakazu; Furuno, Akiko; Akari, Shusaku

EPJ Web of Conferences, 153, p.08012_1 - 08012_7, 2017/09

 Times Cited Count:2 Percentile:9.06

In order to assess the radiological dose to the public resulting from the Fukushima Daiichi Nuclear Power Station (FDNPS) accident in Japan, the spatiotemporal distribution of radioactive materials in the environment are reconstructed by computer simulations. In this study, by refining the source term of radioactive materials and modifying the atmospheric dispersion model (ATDM), the atmospheric dispersion simulation of radioactive materials is improved. Then, a database of spatiotemporal distribution of radioactive materials in the air and on the ground surface is developed from the output of the simulation. This database is used in other studies for the dose assessment by coupling with the behavioral pattern of evacuees from the FDNPS accident. The ATDM simulation was improved to use a new meteorological model and sophisticated deposition scheme. Although the improved ATDM simulations reproduced well the $$^{137}$$Cs deposition pattern in the eastern Japan scale, the reproducibility of deposition pattern was decreased in the vicinity of FDNPS. This result indicated the necessity of further refinement of the source term by optimization to the improved ATDM simulations.

Journal Articles

Development of the Eulerian atmospheric transport model GEARN-FDM; Validation against the European tracer experiment

Kadowaki, Masanao; Katata, Genki; Terada, Hiroaki; Nagai, Haruyasu

Atmospheric Pollution Research, 8(2), p.394 - 402, 2017/03

 Times Cited Count:2 Percentile:91.88(Environmental Sciences)

We developed a dispersion model based on the finite difference method, GEARN-FDM, for long-range dispersion, which solves the advection-diffusion equation using numerical schemes with low artificial diffusion. The advection and diffusion terms are modeled using a fully mass conservative scheme and the Crank-Nicolson method, respectively. GEARN-FDM was validated using the dataset from the European Tracer Experiment. In the entire domain throughout the simulation period of the observed dataset, GEARN-FDM showed high performance with factors of 2 and 5 of 39% and 78%, respectively. While testing the sensitivity of the horizontal diffusivity with this model, the simulated horizontal diffusivity was distributed heterogeneously in the model domain. High diffusivity was primarily seen over the coastal and mountainous regions. Therefore, for the long-range simulations of radionuclides, we need to consider to the transport caused by horizontal diffusion.

Journal Articles

Impacts of C-uptake by plants on the spatial distribution of $$^{14}$$C accumulated in vegetation around a nuclear facility; Application of a sophisticated land surface $$^{14}$$C model to the Rokkasho reprocessing plant, Japan

Ota, Masakazu; Katata, Genki; Nagai, Haruyasu; Terada, Hiroaki

Journal of Environmental Radioactivity, 162-163, p.189 - 204, 2016/10

 Times Cited Count:4 Percentile:75.06(Environmental Sciences)

Impacts of plant C uptake on ($$^{14}$$C) distributions around a nuclear facility were investigated by a land surface $$^{14}$$C model (SOLVEG-II). The simulation combined the SOLVEG-II with a mesoscale model and an dispersion model was applied to $$^{14}$$CO$$_{2}$$ transfer at test operations of the Rokkasho reprocessing plant (RRP) in 2007. The calculated $$^{14}$$C-specific activities in rice grains agreed with the observations. Numerical experiment of chronic $$^{14}$$CO$$_{2}$$ release from the RRP showed that $$^{14}$$C-specific activities of rice plants at harvest differed from the annual mean ones in the air, which was attributed to seasonal variations in atmospheric $$^{14}$$CO$$_{2}$$ and plant growth. $$^{14}$$C accumulation in plant significantly increased when $$^{14}$$CO$$_{2}$$ releases were limited during daytime, compared with the results observed during nighttime, due to extensive $$^{14}$$CO$$_{2}$$ uptake by daytime photosynthesis. These results indicated that plant growth and photosynthesis should be considered in predictions of ingestion dose of $$^{14}$$C for long-term chronic and short-term diurnal releases of $$^{14}$$CO$$_{2}$$, respectively.

Journal Articles

Utilization of $$^{134}$$Cs/$$^{137}$$Cs in the environment to identify the reactor units that caused atmospheric releases during the Fukushima Daiichi accident

Chino, Masamichi; Terada, Hiroaki; Nagai, Haruyasu; Katata, Genki; Mikami, Satoshi; Torii, Tatsuo; Saito, Kimiaki; Nishizawa, Yukiyasu

Scientific Reports (Internet), 6, p.31376_1 - 31376_14, 2016/08

 Times Cited Count:22 Percentile:3.08(Multidisciplinary Sciences)

154 (Records 1-20 displayed on this page)