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Journal Articles

Feasibility study on burnable poison credit concept to HTGR fuel fabrication from core specification perspective

Fukaya, Yuji; Ueta, Shohei; Goto, Minoru; Ohashi, Hirofumi

Annals of Nuclear Energy, 151( ), p.107937_1 - 107937_9, 2021/02

Feasibility study on Burnable Poison (BP) credit concept to High Temperature Gas-cooled Reactor (HTGR) fuel fabrication has been performed. By mixing BP into fuel material in the first place of fuel fabrication, criticality safety is ensured in the all fuel fabrication process even with high enrichment fuel such as 14 wt% used in commercial HTGR. However, the poison effect also prevents the criticality even in the HTGR core, and it may shorten cycle length and achievable burn-up of the core. Therefore, the effect is evaluated by whole core burn-up calculation. As a BP, boron, gadolinium, erbium, and hafnium are investigated. As a result, it is found that boron and gadolinium suit this concept and the 14 wt% fuel can be fabricated in the plant fabricating 9.9 wt% High Temperature engineering Test Reactor (HTTR) fuel. With the boron and gadolinium, the commercial HTGR fuel can be fabricated with the safety measure as same as Light Water Reactor (LWR) fuel facility to treat the fuel with the enrichment up to 5 wt%. Especially, gadolinium is significantly suitable to this concept due to the dependency to spectrum, and more enhanced safety measure is feasible as well.

Journal Articles

Direct measurement of fast ortho-para conversion of molecularly chemisorbed H$$_{2}$$ on Pd(210)

Ueta, Hirokazu; Sasakawa, Yuya*; Ivanov, D.*; Ono, Satoshi*; Ogura, Shohei*; Fukutani, Katsuyuki

Physical Review B, 102(12), p.121407_1 - 121407_5, 2020/09

 Times Cited Count:0

Ortho-to-para conversion of molecularly chemisorbed H$$_{2}$$ on a Pd(210) surface at a surface temperature of 50 K is reported. A combination of a pulsed molecular beam, photo-stimulated desorption and resonance-enhanced multiphoton ionization techniques was used for probing the change in the rotational states of molecularly chemisorbed H$$_{2}$$ on the surface. Our result shows that fast ortho-para conversion of chemisorbed H$$_{2}$$ occurs. The conversion time was experimentally determined to be about 2 s, which is in good agreement with a previous theoretical calculation. This agreement supports that the ortho-para conversion mechanism of the molecularly chemisorbed H$$_{2}$$ on Pd(210) is the two-step process based on the hyperfine-Coulomb excitation.

Journal Articles

Research and development on high burnup HTGR fuels in JAEA

Ueta, Shohei; Mizuta, Naoki; Sasaki, Koei; Sakaba, Nariaki; Ohashi, Hirofumi; Yan, X. L.

Mechanical Engineering Journal (Internet), 7(3), p.19-00571_1 - 19-00571_12, 2020/06

JAEA has been progressing to design HTGR fuels for not only small-type practical HTGRs but also VHTR proposed in GIF which can be utilized for various purposes with high-temperature heat at 750 to 950 $$^{circ}$$C. To increase economy of these HTGRs, JAEA has been upgrading the design method for the HTGR fuel, which can maintain their integrities at the burnup of three to four times higher than that of the conventional HTTR fuel. Design principles and specifications of various concepts of the high burnup HTGR fuels designed by JAEA are reported. As the latest results on post-irradiation examinations of the high burnup HTGR fuel progressing in a framework of international collaboration with Kazakhstan, irradiation shrinkage rate of the fuel compact as a function of fast neutron fluence was obtained at around 100 GWd/t. Furthermore, the future R&Ds needed for the high burnup HTGR fuel are described based on these experimental results.

Journal Articles

VHTR technology development in Japan; Progress of R&D activities for GIF VHTR system

Shibata, Taiju; Sato, Hiroyuki; Ueta, Shohei; Takegami, Hiroaki; Takada, Shoji; Kunitomi, Kazuhiko

2018 GIF Symposium Proceedings (Internet), p.99 - 106, 2020/05

no abstracts in English

Journal Articles

Study on plutonium burner high temperature gas-cooled reactor in Japan; Introduction scenario, reactor safety and fabrication tests of the 3S-TRISO fuel

Ueta, Shohei; Mizuta, Naoki; Fukaya, Yuji; Goto, Minoru; Tachibana, Yukio; Honda, Masaki*; Saiki, Yohei*; Takahashi, Masashi*; Ohira, Koichi*; Nakano, Masaaki*; et al.

Nuclear Engineering and Design, 357, p.110419_1 - 110419_10, 2020/02

 Times Cited Count:1 Percentile:21.8(Nuclear Science & Technology)

The concept of a plutonium (Pu) burner HTGR is proposed to incarnate highly-effective Pu utilization by its inherent safety features. The security and safety fuel (3S-TRISO fuel) employs the coated fuel particle with a fuel kernel made of plutonium dioxide (PuO$$_{2}$$) and yttria stabilized zirconia (YSZ) as an inert matrix. This paper presents feasibility study of Pu burner HTGR and R&D on the 3S-TRISO fuel.

JAEA Reports

Code-B-2.5.2 for stress calculation for SiC-TRISO fuel particle

Aihara, Jun; Goto, Minoru; Ueta, Shohei; Tachibana, Yukio

JAEA-Data/Code 2019-018, 22 Pages, 2020/01

JAEA-Data-Code-2019-018.pdf:1.39MB

Concept of Pu-burner high temperature gas-cooled reactor (HTGR) was proposed for purpose of more safely reducing amount of recovered Pu. In Pu-burner HTGR concept, coated fuel particle (CFP), with ZrC coated yttria stabilized zirconia (YSZ) containing PuO$$_{2}$$ (PuO$$_{2}$$-YSZ) small particle and with tri-structural isotropic (TRISO) coating, is employed for very high burn-up and high nuclear proliferation resistance. ZrC layer is oxygen getter. On the other hand, we have developed Code-B-2.5.2 for prediction of pressure vessel failure probabilities of SiC-tri-isotropic (TRISO) coated fuel particles for HTGRs under operation by modification of an existing code, Code-B-2. The main purpose of modification is preparation of applying code for CFPs of Pu-burner HTGR. In this report, basic formulae are described.

Journal Articles

Development of fabrication and inspection technologies for oxidation-resistant fuel element for high-temperature gas-cooled reactors

Aihara, Jun; Yasuda, Atsushi*; Ueta, Shohei; Ogawa, Hiroaki; Honda, Masaki*; Ohira, Koichi*; Tachibana, Yukio

Nippon Genshiryoku Gakkai Wabun Rombunshi, 18(4), p.237 - 245, 2019/12

Development of fabrication and inspection technologies of oxidation resistant fuel element for improvement of safety of high temperature gas-cooled reactors (HTGRs) in severe oxidation accident was carried out. Simulated coated fuel particles (CFPs), alumina particles, were over-coated with mixed powder of Si, C and small amount of resin to form over-coated particles, and over-coated particles were molded and hot-pressed to sinter simulated oxidation resistant fuel elements with SiC/C mixed matrix. Simulated oxidation resistant fuel elements with matrix whose Si/C mole ratio is 1.00 were fabricated. Failure fraction of CFPs in fuel elements is one of very important inspection subjects of HTGR fuel. It is essential that CFPs are extracted from fuel elements without additional failure. Development of method for extraction of CFPs was carried out. Desolation of SiC by KOH method or pressurized acidolysis method should be applied to extraction of CFPs.

Journal Articles

Microstructures of ZrC coated kernels for fuel of Pu-burner high temperature gas-cooled reactor in Japan

Aihara, Jun; Ueta, Shohei; Honda, Masaki*; Mizuta, Naoki; Goto, Minoru; Tachibana, Yukio; Okamoto, Koji*

Journal of Nuclear Materials, 522, p.32 - 40, 2019/08

In order to realize Pu-burner high temperature gas-cooled reactor (HTGR), coated fuel particles (CFPs) with PuO$$_{2}$$-yittria stabilized zirconia (YSZ) fuel kernel coated with ZrC is employed for high nuclear proliferation resistance and very high burn-up. Japan Atomic Energy Agency (JAEA) have carried out ZrC coatings of particles which simulated PuO$$_{2}$$-YSZ kernels (CeO$$_{2}$$-YSZ particles or commercially available YSZ particles). Ce was used as simulating element of Pu. In this manuscript, microstructures of ZrC coated CeO$$_{2}$$-YSZ or YSZ particles were reported.

Journal Articles

Research and development on high burnup HTGR fuels in JAEA

Ueta, Shohei; Mizuta, Naoki; Sasaki, Koei; Sakaba, Nariaki; Ohashi, Hirofumi; Yan, X. L.

Proceedings of 27th International Conference on Nuclear Engineering (ICONE-27) (Internet), 8 Pages, 2019/05

JAEA has been progressing to design HTGR fuels for not only small-type practical HTGRs but also VHTR proposed in GIF which can be utilized for various purposes with high-temperature heat at 750 to 950 $$^{circ}$$C. To increase economy of these HTGRs, JAEA has been upgrading the design method for the HTGR fuel, which can maintain their integrities at the burnup of three to four times higher than that of the conventional HTTR fuel. Design principles and specifications of various concepts of the high burnup HTGR fuels designed by JAEA are reported. As the latest results on post-irradiation examinations of the high burnup HTGR fuel progressing in a framework of international collaboration with Kazakhstan, irradiation shrinkage rate of the fuel compact as a function of fast neutron fluence was obtained at around 100 GWd/thm. Furthermore, the future R&Ds needed for the high burnup HTGR fuel are described based on these experimental results.

Journal Articles

Study of SiC-matrix fuel element for HTGR

Mizuta, Naoki; Aoki, Takeshi; Ueta, Shohei; Ohashi, Hirofumi; Yan, X. L.

Proceedings of 27th International Conference on Nuclear Engineering (ICONE-27) (Internet), 5 Pages, 2019/05

Enhancement of safety and cooling performance of fuel elements are desired for a commercial High Temperature Gas-cooled Reactor (HTGR). Applying sleeveless fuel elements and dual side directly cooling structures with oxidation resistant SiC-matrix fuel compact has a possibility of improving safety and cooling performance at the pin-in-block type HTGR. The irradiated effective thermal conductivity of a fuel compact is an important physical property for core thermal design of the pin-in-block type HTGR. In order to discuss the irradiated effective thermal conductivity of the SiC-matrix fuel compact which could improve the cooling performance of the reactor, the maximum fuel temperature during normal operation of the pin-in-block type HTGR with dual side directly cooling structures are analytically evaluated. From these results, the desired irradiated thermal conductivity of SiC matrix are discussed. In addition, the suitable fabrication method of SiC-matrix fuel compact is examined from viewpoints of the sintering temperature, the purity and the mass productivity.

Journal Articles

Development of fabrication technology for oxidation-resistant fuel elements for high-temperature gas-cooled reactors

Aihara, Jun; Honda, Masaki*; Ueta, Shohei; Ogawa, Hiroaki; Ohira, Koichi*; Tachibana, Yukio

Nippon Genshiryoku Gakkai Wabun Rombunshi, 18(1), p.29 - 36, 2019/03

Japan Atomic Energy Agency carried out development of fabrication technology of oxidation resistant fuel element for improvement of safety of high temperature gas-cooled reactors in serious oxidation accident, based on precursor research in former JAEA. Dummy coated fuel particles (alumina particles) were over-coated with mixed powder of Si, C and small amount of resin to form over-coated particles, and over-coated particles were molded and hot-pressed to sinter dummy oxidation resistant fuel elements with SiC/C mixed matrix. We fabricated dummy oxidation resistant fuel elements with matrix whose Si/C mole ratio (about 0.551) is three times as large as that in precursor research. Si peak was not detected by X-ray diffraction of matrix. Better oxidation resistant was confirmed with oxidation test in 20% O$$_{2}$$ at 1673 K than that of ordinal fuel compact with ordinal graphite/carbon matrix. All dummy coated fuel particles were held in specimen after 10 h oxidation.

Journal Articles

Development of security and safety fuel for Pu-burner HTGR; Test and characterization for ZrC coating

Ueta, Shohei; Aihara, Jun; Goto, Minoru; Tachibana, Yukio; Okamoto, Koji*

Mechanical Engineering Journal (Internet), 5(5), p.18-00084_1 - 18-00084_9, 2018/10

To develop the security and safety fuel (3S-TRISO fuel) for Pu-burner high temperature gas-cooled reactor (HTGR), R&D on zirconium carbide (ZrC) directly coated on yttria stabilized zirconia (YSZ) has been started in the Japanese fiscal year 2015. As results of the direct coating test of ZrC on the dummy YSZ particle, ZrC layers with 18 - 21 microns of thicknesses have been obtained with 0.1 kg of particle loading weight. No deterioration of YSZ exposed by source gases of ZrC bromide process was observed by Scanning Transmission Electron Microscope (STEM).

Journal Articles

Study on Pu-burner high temperature gas-cooled reactor in Japan; Introduction scenario

Fukaya, Yuji; Goto, Minoru; Ueta, Shohei; Tachibana, Yukio; Okamoto, Koji*

Proceedings of 9th International Topical Meeting on High Temperature Reactor Technology (HTR 2018) (USB Flash Drive), 9 Pages, 2018/10

The research on introduction scenarios of Pu-burner High Temperature Gas-cooled Reactor (HTGR) of Japan has been performed based on the "Long-term Energy Supply and Demand Outlook" released by the Ministry of Economy, Trade and Industry (METI) of Japan in 2015. In the perspective, the electricity generation capacity of nuclear power generation reduces from 50 GWe (peak around 2010) to 30 GWe in 2030. To maintain the capacity, light water reactors (LWRs) should be introduced from 2025 to 2030. After 2030, HTGRs, which are superior to LWRs from the viewpoint of safety and economy, will be introduced to fill the capacity and incinerate plutonium. We assumed introduction of U fueled HTGR as well. The Pu-burner reactor will be introduced with the priority to incinerate separated plutonium by reprocessing. Moreover, we also evaluated hydrogen generation and its effect on CO$$_{2}$$ reduction. As a result, effective plutonium incineration and CO$$_{2}$$ reduction effect are confirmed.

Journal Articles

Conceptual plant system design study of an experimental HTGR upgraded from HTTR

Ohashi, Hirofumi; Goto, Minoru; Ueta, Shohei; Sato, Hiroyuki; Fukaya, Yuji; Kasahara, Seiji; Sasaki, Koei; Mizuta, Naoki; Yan, X.; Aoki, Takeshi*

Proceedings of 9th International Topical Meeting on High Temperature Reactor Technology (HTR 2018) (USB Flash Drive), 6 Pages, 2018/10

Conceptual design study of an experimental HTGR is performed to upgrade the plant system from Japanese High Temperature engineering Test Reactor (HTTR) to a commercial HTGR. Safety systems of HTTR are upgraded to demonstrate the commercial HTGR concept, such as a passive reactor cavity cooling system, a confinement, etc. An intermediate heat exchanger (IHX) is replaced by a steam generator (SG) for a process heat supply to demonstrate the technology for a commercial use. This paper describes the conceptual design study results of the plant system of the experimental HTGR.

Journal Articles

Study on Pu-burner high temperature gas-cooled reactor in Japan; Design study of fuel and reactor core

Goto, Minoru; Aihara, Jun; Inaba, Yoshitomo; Ueta, Shohei; Fukaya, Yuji; Okamoto, Koji*

Proceedings of 9th International Topical Meeting on High Temperature Reactor Technology (HTR 2018) (USB Flash Drive), 6 Pages, 2018/10

JAEA has conducted design studies of a Pu-burner HTGR. The Pu-burner HTGR incinerates Pu by fission, and hence a high burn-up is required for the efficient incineration. In the fuel design, a thin ZrC layer, which acts as an oxygen getter and suppresses the internal pressure, was coated on the fuel kernel to prevent the CFP failure at the high burn-up. A stress analysis of the SiC layer, which acts as a pressure vessel for the CFP, was performed for with consideration of the depression effect due to the ZrC layer. As a result, the CFP failure fraction at high burn-up of 500 GWd/t satisfied the target value. In the reactor core design, an axial fuel shuffling was employed to attain the high burn-up, and the nuclear burn-up calculations with the whole core model and the fuel temperature calculations were performed. As a result, the nuclear characteristics, which are the shutdown margin and the temperature coefficient of reactivity, and the fuel temperature satisfied their target values.

Journal Articles

Study on Pu-burner high temperature gas-cooled reactor in Japan; Test and characterization for ZrC coating

Ueta, Shohei; Aihara, Jun; Mizuta, Naoki; Goto, Minoru; Fukaya, Yuji; Tachibana, Yukio; Okamoto, Koji*

Proceedings of 9th International Topical Meeting on High Temperature Reactor Technology (HTR 2018) (USB Flash Drive), 7 Pages, 2018/10

The security and safety fuel (3S-TRISO fuel) employs the coated fuel particle with a fuel kernel made of plutonium dioxide (PuO$$_{2}$$) and yttria stabilized zirconia (YSZ) as an inert matrix. Especially, a zirconium carbide (ZrC) coating is one of key technologies of the 3S-TRISO, which performs as an oxygen getter to reduce the fuel failure due to internal pressure during the irradiation. R&Ds on ZrC coating directly on the dummy CeO$$_{2}$$-YSZ kernel have been carried in the Japanese fiscal year 2017. As results of ZrC coating tests by the bromide chemical vapor deposition process, stoichiometric ZrC coatings with 3 - 18 microns of thicknesses were obtained with 0.1 kg of particle loading weight.

Journal Articles

Investigation of irradiated properties of extended burnup TRISO fuel

Shaimerdenov, A.*; Gizatulin, S.*; Kenzhin, Y.*; Dyussambayev, D.*; Ueta, Shohei; Aihara, Jun; Shibata, Taiju

Proceedings of 9th International Topical Meeting on High Temperature Reactor Technology (HTR 2018) (USB Flash Drive), 6 Pages, 2018/10

The Institute of Nuclear Physics of the Republic of Kazakhstan (INP) conducts an irradiation test and post-irradiation examinations (PIEs) of the high-temperature gas-cooled reactor (HTGR) fuel and materials to develop the extend burnup fuel up to 100 GWd/t-U collaboratively with the Japan Atomic Energy Agency (JAEA) under projects in a frame of the International Science and Technology Centre (ISTC). Cylindrical fuel compact specimens consisting of newly-designed TRISO (tri-structural isotropic) coated fuel particles and a matrix made of graphite material were manufactured in Japan. An irradiation test of the fuel specimens using a helium-gas swept capsule designed and constructed in the INP has been performed up to 100 GWd/t-U in the WWR-K research reactor by April 2015. In the next stage, PIEs with the irradiated fuel specimens have been started in February 2017 as a new ISTC project. Several PIE technologies by non-destructive and destructive techniques with irradiated fuel compacts were developed by the INP. This report presents the developed technologies and interim results of the PIE for high burning TRISO fuel.

JAEA Reports

Excellent feature of Japanese HTGR technologies

Nishihara, Tetsuo; Yan, X.; Tachibana, Yukio; Shibata, Taiju; Ohashi, Hirofumi; Kubo, Shinji; Inaba, Yoshitomo; Nakagawa, Shigeaki; Goto, Minoru; Ueta, Shohei; et al.

JAEA-Technology 2018-004, 182 Pages, 2018/07

JAEA-Technology-2018-004.pdf:18.14MB

Research and development on High Temperature Gas-cooled Reactor (HTGR) in Japan started since late 1960s. Japan Atomic Energy Agency (JAEA) in cooperation with Japanese industries has researched and developed system design, fuel, graphite, metallic material, reactor engineering, high temperature components, high temperature irradiation and post irradiation test of fuel and graphite, high temperature heat application and so on. Construction of the first Japanese HTGR, High Temperature engineering Test Reactor (HTTR), started in 1990. HTTR achieved first criticality in 1998. After that, various test operations have been carried out to establish the Japanese HTGR technologies and to verify the inherent safety features of HTGR. This report presents several system design of HTGR, the world-highest-level Japanese HTGR technologies, JAEA's knowledge obtained from construction, operation and management of HTTR and heat application technologies for HTGR.

JAEA Reports

Comparison between HTFP code and minory changed FORNAX-A code

Aihara, Jun; Ueta, Shohei; Goto, Minoru; Inaba, Yoshitomo; Shibata, Taiju; Ohashi, Hirofumi

JAEA-Technology 2018-002, 70 Pages, 2018/06

JAEA-Technology-2018-002.pdf:1.46MB

HTFP code is code for calculation of additional release amount of fission product (FP) from fuel rod in high temperature gas-cooled reactor (HTGR) after stop of fission. Minory changed Fornax-A code also can calculate that. Therefore, release behavior of Cs calculated with HTFP code was compared with that calculated with minory modified FORNAX-A code in this report. Release constants of Cs evaluated with minory modified FORNAX-A code are rather different from default values for HTFP code.

Journal Articles

Development of security and safety fuel for Pu-burner HTGR, 2; Design study of fuel and reactor core

Goto, Minoru; Ueta, Shohei; Aihara, Jun; Inaba, Yoshitomo; Fukaya, Yuji; Tachibana, Yukio; Okamoto, Koji*

Proceedings of 25th International Conference on Nuclear Engineering (ICONE-25) (CD-ROM), 6 Pages, 2017/07

A PuO$$_{2}$$-YSZ fuel kernel with a ZrC coating, which enhances safety, security and safeguard, namely: 3S-TRISO fuel, was proposed to introduce to the plutonium-burner HTGR. In this study, the efficiency of the ZrC coating as the free-oxygen getter was examined based on a thermochemical calculation. A preliminary study on the feasibility of the 3S-TRISO fuel was conducted focusing on the internal pressure. Additionally, a nuclear feasibility of the reactor core was studied. As a result, all the amount of the free-oxygen is captured by a thin ZrC coating under 1600$$^{circ}$$C and coating ZrC on the fuel kernel should be very effective method to suppress the internal pressure. The internal pressure of the 3S-TRISO fuel at 500 GWd/t is lower than that of UO$$_{2}$$ kernel TRISO fuel whose feasibility had been already confirmed and the 3S-TRISO fuel should be feasible. The fuel shuffling allows to achieve 500 GWd/t. The temperature coefficient of reactivity is negative during the operation period and thus the nuclear feasibility of the reactor core should be achievable.

134 (Records 1-20 displayed on this page)