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Toigawa, Tomohiro; Hotoku, Shinobu; Kumagai, Yuta; Abe, Yuma*; Oyama, Kanichi*; Fukaya, Hiroyuki; Tsubata, Yasuhiro; Ban, Yasutoshi; Kida, Takashi; Hasegawa, Satoshi*; et al.
Journal of Nuclear Science and Technology, 63(8), p.969 - 975, 2026/08
Times Cited Count：0 Percentile：0.00(Nuclear Science & Technology)The effect of temperature on hydrogen generated from radiolysis was investigated to determine the safety implications in nuclear fuel reprocessing. Radiolytic hydrogen production poses a risk due to its flammability, especially when it accumulates in confined spaces without ventilation. Herein, generation of radiolytic hydrogen from an actual nuclear fuel-derived solution is investigated. Compared to previous studies using a plutonium nitric acid solution, this study evaluates radiolytic hydrogen yield under more realistic conditions, reflecting post-irradiation fuel composition. G-values of H
are determined at multiple temperatures, and the impact of alpha, beta, and gamma radiation doses is evaluated using PHITS-based simulations. Findings from this study confirmed a reduction in hydrogen yield due to scavenging effects of high-concentration nitric acid and metal ions dissolved in the solution, and temperature dependence appeared to be minor. A weak decreasing trend of G-values with temperature under agitated conditions might be related to hydrogen consumption by palladium species.
Oguri, Kaori; Arai, Yoichi; Watanabe, So; Seko, Noriaki*; Hoshina, Hiroyuki*
Annual Research Report 2024 (Physical Science, Engineering), p.269 - 278, 2026/03
Radium-226 (
Ra) has recently attracted attention as a source for the production of Actinium-225 (
Ac), which can be used for the alpha-particle treatment of cancer. Ra is present in approximately 10,000 tons in the sea. The amount of Ra in seawater could help patients with metastatic cancer around the world. Therefore, we focused on the extraction of Ra from seawater and examined an effective process for refining Ra. Due to the low concentration of Ra in seawater, only a few ppb, it has not received much attention in terms of economic point. Therefore, we focused on adsorbents prepared by Radiation-Induced Graft Polymerization to selectively collect Ra. In this study, we performed adsorption studies with Barium (Ba), homologs element of Ra, which may coexist with Ra in seawater.
Toigawa, Tomohiro; Hotoku, Shinobu; Kumagai, Yuta; Abe, Yuma*; Oyama, Kanichi*; Fukaya, Hiroyuki; Ban, Yasutoshi; Kida, Takashi; Hasegawa, Satoshi*; Nakano, Masanao*; et al.
Journal of Nuclear Science and Technology, 63(3), p.322 - 327, 2026/03
Times Cited Count：2 Percentile：61.39(Nuclear Science & Technology)The effect of temperature on hydrogen production generated from radiolysis was investigated to determine the associated implications for nuclear fuel reprocessing safety. The hydrogen yield from radiolysis of plutonium nitric acid solution was measured at temperatures up to the boiling temperature of the solution. The results showed no notable temperature dependence even under boiling conditions. The impact of solution agitation on hydrogen production was also assessed, which revealed minor differences in the hydrogen yield between static and agitated conditions at room temperature. These findings suggest that high temperatures or boiling the solution do not considerably enhance hydrogen generation, and provide crucial information for accurately modeling hydrogen risks under severe accidents.
Watanabe, Takahiro; Kida, Fukuka; Yamasaki, Shinichi*; Yamagishi, Hiroyuki*; Ochiai, Shinya*; Matsunaka, Tetsuya*; Nara, Fumiko; Tsuchiya, Noriyoshi*
Bunseki Kagaku, 74(10-11), p.611 - 619, 2025/10
Bromine and iodine contents in geological samples can be used as useful tools to understand various environmental phenomena such as past sea-level changes, geological uplift and subsidence, as well as marine incursion to the inland due to paleo tsunami and storm surges. In this study, we measured bromine and iodine contents in possible standard materials and lake sediment samples using the WDXRF at Tono Geoscience Center and polarizing EDXRF at Tohoku University. We compared both results and confirmed that the WDXRF method for Bromine and iodine content determinations can provide the reliable results.
Iwamoto, Osamu; Koura, Hiroyuki; Endo, Shunsuke; Kimura, Atsushi; Nakayama, Shinsuke; Araki, Shohei; Nishio, Katsuhisa; Otsuka, Naohiko*; Minato, Futoshi*; Watanabe, Yukinobu*; et al.
Kaku Deta Nyusu (Internet), (142), p.18 - 30, 2025/10
no abstracts in English
Arai, Yoichi; Goto, Yasuhiro; Watanabe, So; Agou, Tomohiro*; Arai, Tsuyoshi*; Katsuki, Kenta*; Fukumoto, Hiroki*; Hoshina, Hiroyuki*; Seko, Noriaki*
Progress in Nuclear Science and Technology (Internet), 8, p.329 - 332, 2025/09
Kato, Hiroyuki S.*; Muroyama, Mizuho*; Kobayakawa, Nano*; Muneyasu, Riku*; Tsuda, Yasutaka; Murase, Natsumi*; Watanabe, Seiya*; Yamada, Takashi*; Kanematsu, Yusuke*; Tachikawa, Masanori*; et al.
Journal of Physical Chemistry Letters (Internet), 15(43), p.10769 - 10776, 2024/10
Times Cited Count：2 Percentile：20.65(Chemistry, Physical)Arai, Yoichi; Watanabe, So; Watanabe, Masayuki; Arai, Tsuyoshi*; Katsuki, Kenta*; Agou, Tomohiro*; Fujikawa, Hisaharu*; Takeda, Keisuke*; Fukumoto, Hiroki*; Hoshina, Hiroyuki*; et al.
Nuclear Instruments and Methods in Physics Research B, 554, p.165448_1 - 165448_10, 2024/09
Times Cited Count：0 Percentile：0.00(Instruments & Instrumentation)Nemoto, Takahiro; Fujiwara, Yusuke; Arakawa, Ryoki; Choyama, Yuya; Nagasumi, Satoru; Hasegawa, Toshinari; Yokoyama, Keisuke; Watanabe, Masashi; Onishi, Takashi; Kawamoto, Taiki; et al.
JAEA-Technology 2024-003, 17 Pages, 2024/06
JAEA-Technology-2024-003.pdf:1.91MB
In order to investigate the cause of the increase in differential pressure in the primary helium circulator filter that occurred during the RS-14 cycle, a clogged filter was investigated. As a result of the investigation, deposits caused by silicone oil were confirmed on the surface of the filter element. These results revealed that the cause of filter clogging was silicone oil mixed into the primary system due to performance deterioration of the charcoal filter in the gas circulator of primary helium purification system. As a measure to prevent the recurrence of this event, in addition to the conventional management based on operating hours for replacing of charcoal filter in the gas circulator of primary helium purification system, we have established a new replacement plan for every three years.
Holm-Janas, S.*; Akaki, Mitsuru*; Fogh, E.*; Kihara, Takumi*; Le, M. D.*; Forino, P. C.*; Nikitin, S. E.*; Fennell, T.*; Painganoor, A.*; Vaknin, D.*; et al.
Physical Review B, 109(17), p.174413_1 - 174413_11, 2024/05
Times Cited Count：6 Percentile：52.19(Materials Science, Multidisciplinary)
CoSiYamauchi, Hiroki; Sari, D. P.*; Yasui, Yukio*; Sakakura, Terutoshi*; Kimura, Hiroyuki*; Nakao, Akiko*; Ohara, Takashi; Honda, Takashi*; Kodama, Katsuaki; Igawa, Naoki; et al.
Physical Review Research (Internet), 6(1), p.013144_1 - 013144_9, 2024/02
Oikawa, Kenichi; Sato, Hirotaka*; Watanabe, Kenichi*; Su, Y. H.; Shinohara, Takenao; Kai, Tetsuya; Kiyanagi, Yoshiaki*; Hasemi, Hiroyuki
Journal of Physics; Conference Series, 2605, p.012013_1 - 012013_6, 2023/10
Shobuda, Yoshihiro; Harada, Hiroyuki; Saha, P. K.; Takayanagi, Tomohiro; Tamura, Fumihiko; Togashi, Tomohito; Watanabe, Yasuhiro; Yamamoto, Kazami; Yamamoto, Masanobu
Proceedings of 68th ICFA Advanced Beam Dynamics Workshop on High Intensity and High Brightness Hadron Beams (HB2023) (Internet), p.162 - 169, 2023/10
At the 3-GeV Rapid Cycling Synchrotron (RCS) within the Japan Proton Accelerator Research Complex (J-PARC), kicker impedance causes beam instability. A 1-MW beam with a large emittance can be delivered to the Material and Life Science Experimental Facility (MLF) by suppressing beam instabilities without the need for a transverse feedback system - simply by turning off the sextuple magnets. However, we require other high-intensity and high-quality beams with smaller emittances for the Main Ring (MR). To address this, we proposed a scheme for suppressing the kicker impedance using a diode stack and resistors, which effectively reduces beam instability. Importantly, these devices have a negligible effect on the extracted beam from the RCS.
Watanabe, Nao; Yamashita, Susumu; Uesawa, Shinichiro; Nishihara, Kenji; Yoshida, Hiroyuki
Proceedings of 20th International Topical Meeting on Nuclear Reactor Thermal Hydraulics (NURETH-20) (Internet), p.3522 - 3534, 2023/08
Accelerator-driven system (ADS), the coolant of which is lead-bismuth eutectic (LBE), has been designed by Japan Atomic Energy Agency. Estimating corrosion rate at the wall surface of LBE channel is an important issue in considering safety and the life of the entire structure. The corrosion rate depends on state of oxygen layers forming at the material surface. Therefore, this study aims to develop a method to evaluate the corrosion rate in ADS for the design study by estimation of the oxide layer growth and dissolution (OLGD) rates by means of numerical analysis. The OLGD rates, mass transfer rates of oxygen and iron between the material and LBE and advection-diffusion rates of them in LBE depend on each other. Therefore, in order to estimate OLGD rates, the three numerical analysis models should be coupled. For the advection-diffusion calculation, to use CFD code should be reasonable approach to analyze complex flow in ADS, while for the OLGD and the mass transfer calculation, to use some correlation equations should be reasonable because their scales are much smaller than the advection-diffusion. The present work has developed the analysis method of OLGD rates by using JUPITER code, which is CFD code developed in JAEA. In terms of the correlation equations of OLGD and mass transfer rates, existing models used in a previous study were used with modified.
Nemoto, Takahiro; Arakawa, Ryoki; Kawakami, Satoru; Nagasumi, Satoru; Yokoyama, Keisuke; Watanabe, Masashi; Onishi, Takashi; Kawamoto, Taiki; Furusawa, Takayuki; Inoi, Hiroyuki; et al.
JAEA-Technology 2023-005, 33 Pages, 2023/05
JAEA-Technology-2023-005.pdf:5.25MB
During shut down of the HTTR (High Temperature engineering Test Reactor) RS-14 cycle, an increasing trend of filter differential pressure for the helium gas circulator was observed. In order to investigate this phenomenon, the blower of the primary helium purification system was disassembled and inspected. As a result, it is clear that the silicon oil mist entered into the primary coolant due to the deterioration of the charcoal filter performance. The replacement and further investigation of the filter are planning to prevent the reoccurrence of the same phenomenon in the future.
Shobuda, Yoshihiro; Harada, Hiroyuki; Saha, P. K.; Takayanagi, Tomohiro; Tamura, Fumihiko; Togashi, Tomohito; Watanabe, Yasuhiro; Yamamoto, Kazami; Yamamoto, Masanobu
Physical Review Accelerators and Beams (Internet), 26(5), p.053501_1 - 053501_45, 2023/05
Times Cited Count：1 Percentile：14.99(Physics, Nuclear)At the Rapid Cycling Synchrotron (RCS) in Japan Proton Accelerator Research Complex (J-PARC), theoretical predictions have indicated that the kicker-impedance would excite the beam-instability. A 1 MW beam with large emittance can be delivered to the Material and Life Science Experimental Facility (MLF) through suppression of the beam instabilities by choosing the appropriate machine parameters. However, we require other high-intensity and high-quality smaller emittance beams (than the 1 MW beam) for the Main Ring (MR). Hence, we proposed a scheme for suppressing the kicker-impedance by using prototype diodes and resistors, thereby demonstrating the effect on the kicker impedance reduction. However, the J-PARC RCS must be operated with a repetition rate of 25 Hz, which urged us to consider special diodes that are tolerant to heating. After developments, we have demonstrated that the special diodes with resistors can suppress the beam instability by reducing the kicker impedance. Enhanced durability of the prototype diodes and resistors for the 25 Hz operation was also realized. Moreover, the new diodes and the resistors have negligible effect on the extracted beam from the RCS. From a simulation point of view, the scheme can be employed for at least 5 MW beam operation within the stipulated specifications.
Nagata, Shuhei*; Ogawa, Yusuke*; Suzuki, Satoru*; Inoue, Hiroyuki*; Watanabe, Yutaka*; Yamamoto, Masahiro*; Abe, Hiroshi*; Mitsui, Seiichiro
NUMO-TR-22-02, p.21 - 22, 2023/03
no abstracts in English
Watanabe, Masao; Kihara, Takumi*; Nojiri, Hiroyuki*
Quantum Beam Science (Internet), 7(1), p.1_1 - 1_10, 2023/03
A pulsed magnet system has been developed as a new user-friendly sample environment equipment at the Materials and Life Science Experimental Facility in Japan Proton Accelerator Research Complex. It comprises a vacuum chamber, a 4 K closed-cycle refrigerator for samples, and a nitrogen bath made of a stainless-steel tube with a miniature solenoidal coil. The coil is cooled by liquid nitrogen supplied by an automatic liquid nitrogen supply system, and the sample is cooled by a refrigerator. This combination facilitates the automatic high magnetic field diffraction measurement for the user's operation. A relatively large scattering angle is up to 42 degrees, which is significantly wider than the previous setup. Neutron diffraction experiments were performed on a multiferroic TbMnO
and the field dependence of the diffraction peaks was clearly observed. The new pulsed magnet system was established for a practical high magnetic field diffraction for the user program.
Sn in concrete rubbleDo, V.-K.; Furuse, Takahiro; Ota, Yuki; Iwahashi, Hiroyuki; Hirosawa, Takashi; Watanabe, Masahisa; Sato, Soichi
Journal of Radioanalytical and Nuclear Chemistry, 331(12), p.5631 - 5640, 2022/12
Times Cited Count：6 Percentile：52.54(Chemistry, Analytical)Sn is one of the long-lived fission products that might have been released into the environment after the Fukushima nuclear accident in Japan in 2011. The presence of radionuclides must be monitored for the proper treatment of wastes obtained from decommissioning accident-related nuclear facilities and the surrounding environment. In the work, we propose a reliable method for verifying the presence of Sn in construction materials by combining the HCl-free solid phase extraction on TEVA resin and a selective measurement by inductively coupled plasma tandem mass spectrometry (ICP-MS/MS). The method has been optimized and characterized step by step. More than 95% of chemical recovery was achieved for Sn from typical concrete matrixes. The interference caused by an isobar Te and possible polyatomic interferences from matrixes were effectively suppressed by the developed chemical separation and the tandem MS/MS configuration. The total decontamination factor for the Te interference was of the order of 10
. The estimated method detection limit for Sn in concrete as measured at m/z = 160 was 12.1 pg g
, which is equivalent to 6.1 mBq g.
Yamamoto, Kazami; Kinsho, Michikazu; Hayashi, Naoki; Saha, P. K.; Tamura, Fumihiko; Yamamoto, Masanobu; Tani, Norio; Takayanagi, Tomohiro; Kamiya, Junichiro; Shobuda, Yoshihiro; et al.
Journal of Nuclear Science and Technology, 59(9), p.1174 - 1205, 2022/09
Times Cited Count：10 Percentile：71.75(Nuclear Science & Technology)In the Japan Proton Accelerator Research Complex, the purpose of the 3 GeV rapid cycling synchrotron (RCS) is to accelerate a 1 MW, high-intensity proton beam. To achieve beam operation at a repetition rate of 25 Hz at high intensities, the RCS was elaborately designed. After starting the RCS operation, we carefully verified the validity of its design and made certain improvements to establish a reliable operation at higher power as possible. Consequently, we demonstrated beam operation at a high power, namely, 1 MW. We then summarized the design, actual performance, and improvements of the RCS to achieve a 1 MW beam.
