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Journal Articles

Lanthanide and actinide ion complexes containing organic ligands investigated by surface-enhanced infrared absorption spectroscopy

Hirata, Sakiko*; Kusaka, Ryoji; Meiji, Shogo*; Tamekuni, Seita*; Okudera, Kosuke*; Hamada, Shoken*; Sakamoto, Chihiro*; Honda, Takumi*; Matsushita, Kosuke*; Muramatsu, Satoru*; et al.

Inorganic Chemistry, 62(1), p.474 - 486, 2023/01

 Times Cited Count:0 Percentile:0.01(Chemistry, Inorganic & Nuclear)

Journal Articles

Basic study on a novel single-end readout type radiation distribution sensing method using an optical fiber

Terasaka, Yuta; Watanabe, Kenichi*; Uritani, Akira*

Hoshasen (Internet), 47(3), p.89 - 96, 2022/10

Journal Articles

Design and actual performance of J-PARC 3 GeV rapid cycling synchrotron for high-intensity operation

Yamamoto, Kazami; Kinsho, Michikazu; Hayashi, Naoki; Saha, P. K.; Tamura, Fumihiko; Yamamoto, Masanobu; Tani, Norio; Takayanagi, Tomohiro; Kamiya, Junichiro; Shobuda, Yoshihiro; et al.

Journal of Nuclear Science and Technology, 59(9), p.1174 - 1205, 2022/09

 Times Cited Count:1 Percentile:71.47(Nuclear Science & Technology)

In the Japan Proton Accelerator Research Complex, the purpose of the 3 GeV rapid cycling synchrotron (RCS) is to accelerate a 1 MW, high-intensity proton beam. To achieve beam operation at a repetition rate of 25 Hz at high intensities, the RCS was elaborately designed. After starting the RCS operation, we carefully verified the validity of its design and made certain improvements to establish a reliable operation at higher power as possible. Consequently, we demonstrated beam operation at a high power, namely, 1 MW. We then summarized the design, actual performance, and improvements of the RCS to achieve a 1 MW beam.

Journal Articles

Theoretical and experimental estimation of the relative optically stimulated luminescence efficiency of an optical-fiber-based BaFBr:Eu detector for swift ions

Hirata, Yuho; Sato, Tatsuhiko; Watanabe, Kenichi*; Ogawa, Tatsuhiko; Parisi, A.*; Uritani, Akira*

Journal of Nuclear Science and Technology, 59(7), p.915 - 924, 2022/07

 Times Cited Count:3 Percentile:94.4(Nuclear Science & Technology)

The reliability of dose assessment with radiation detectors is an important feature in various fields, such as radiotherapy, radiation protection, and high-energy physics. However, many detectors irradiated by high linear energy transfer (LET) radiations exhibit decreased efficiency called the quenching effect. This quenching effect depends not only on the particle LET but strongly on the ion species and its microscopic pattern of energy deposition. Recently, a computational method for estimating the relative efficiency of luminescence detectors was proposed following analysis of microdosimetric specific energy distributions simulated using the particle and heavy ion transport code system (PHITS). This study applied the model to estimate the relative optically stimulated luminescence (OSL) efficiency of BaFBr:Eu detectors. Additionally, we measured the luminescence intensity of BaFBr:Eu detectors exposed to $$^{4}$$He, $$^{12}$$C and $$^{20}$$Ne ions to verify the calculated data. The model reproduced the experimental data in the cases of adopting a microdosimetric target diameter of approximately 30-50 nm. The calculated relative efficiency exhibit ion-species dependence in addition to LET. This result shows that the microdosimetric calculation from specific energy is a successful method for accurately understanding the results of OSL measurements with BaFBr:Eu detectors irradiated by various particles.

Journal Articles

First demonstration of a novel single-end readout type position-sensitive optical fiber radiation sensor based on wavelength-resolved photon counting

Terasaka, Yuta; Watanabe, Kenichi*; Uritani, Akira*

Nuclear Instruments and Methods in Physics Research A, 1034, p.166793_1 - 166793_6, 2022/07

 Times Cited Count:0 Percentile:0.02(Instruments & Instrumentation)

Journal Articles

Feasibility study of the one-dimensional radiation distribution sensing method using an optical fiber sensor based on wavelength spectrum unfolding

Terasaka, Yuta; Watanabe, Kenichi*; Uritani, Akira*; Yamazaki, Atsushi*; Sato, Yuki; Torii, Tatsuo; Wakaida, Ikuo

Journal of Nuclear Engineering and Radiation Science, 7(4), p.042002_1 - 042002_7, 2021/10

For the application in the measurement of the high dose rate hot spots inside the Fukushima Daiichi Nuclear Power Station (FDNPS) buildings, we propose a novel one-dimensional radiation distribution sensing method using an optical fiber sensor based on wavelength spectrum unfolding. The proposed method estimates the incident position of radiation to the fiber by the unfolding of the wavelength spectrum output from the fiber edge using the fact that the attenuation length of light along the fiber depends on the wavelength. Because this method measures the integrated light intensity, this method can avoid the problem of counting loss and signal pile-up, which occurs in the radiation detector with pulse counting mode under high dose rate field. Through basic experiments using the ultraviolet light source and $$^{90}$$Sr/$$^{90}$$Y radioactive point source, basic properties of source position detection were confirmed.

Journal Articles

Deexcitation dynamics of muonic atoms revealed by high-precision spectroscopy of electronic $$K$$ X rays

Okumura, Takuma*; Azuma, Toshiyuki*; Bennet, D. A.*; Caradonna, P.*; Chiu, I. H.*; Doriese, W. B.*; Durkin, M. S.*; Fowler, J. W.*; Gard, J. D.*; Hashimoto, Tadashi; et al.

Physical Review Letters, 127(5), p.053001_1 - 053001_7, 2021/07

 Times Cited Count:3 Percentile:45.66(Physics, Multidisciplinary)

We observed electronic $$K$$X rays emitted from muonic iron atoms using a superconducting transition-edge-type sensor microcalorimeter. The energy resolution of 5.2 eV in FWHM allowed us to observe the asymmetric broad profile of the electronic characteristic $$K$$$$alpha$$ and $$K$$$$beta$$ X rays together with the hypersatellite $$K$$$$alpha$$ X rays around 6 keV. This signature reflects the time-dependent screening of the nuclear charge by the negative muon and the $$L$$-shell electrons, accompanied by electron side-feeding. Assisted by a simulation, this data clearly reveals the electronic $$K$$- and $$L$$-shell hole production and their temporal evolution during the muon cascade process.

Journal Articles

Evaluation of a one-dimensional position-sensitive quartz optical fiber sensor based on the time-of-flight method for high radiation dose rate applications

Terasaka, Yuta; Watanabe, Kenichi*; Uritani, Akira*

Nuclear Instruments and Methods in Physics Research A, 996, p.165151_1 - 165151_8, 2021/04

 Times Cited Count:1 Percentile:32.08(Instruments & Instrumentation)

For the measurement of radiation distribution inside the Fukushima Daiichi Nuclear Power Station (FDNPS) buildings, the evaluation of a small-diameter quartz optical fiber as a one-dimensional position-sensitive sensor was conducted. The sensor determines the incident position of radiation into the fiber using the time-of-flight information of emitted Cerenkov photons in the optical fiber. Compared with the conventional sensor using the plastic scintillating fiber, the quartz optical fiber has much higher position resolution, which may be the result of the improvement of timing characteristics caused by the prompt emission mechanism of the Cerenkov radiation. Additionally, the response of position-sensitive quartz optical fiber sensor under high radiation field was evaluated, and good count rate linearity was confirmed using the 10 m long quartz optical fiber with a diameter of 0.4 mm up to the dose rate at least 20 mSv/h, and the radiation tolerance property up to the accumulated dose of 1 kGy was evaluated.

Journal Articles

Status of LBE study and experimental plan at JAEA

Saito, Shigeru; Wan, T.*; Okubo, Nariaki; Obayashi, Hironari; Watanabe, Nao; Ohdaira, Naoya*; Kinoshita, Hidetaka; Yamaki, Kenichi*; Kita, Satoshi*; Yoshimoto, Hidemitsu*; et al.

JPS Conference Proceedings (Internet), 33, p.011041_1 - 011041_6, 2021/03

An Accelerator Driven System (ADS) for waste transmutation investigated in JAEA employs lead-bismuth eutectic (LBE) as a neutron production target material and coolant. The neutrons are to be produced via the spallation with 1.5 GeV proton beam injection. As materials irradiation data are important for ADS development, JAEA plans to construct an irradiation facility with LBE neutron production target in J-PARC. There are many technical issues on LBE for practical use. In JAEA, various R&Ds are being carried out. Concerning corrosion study, conditioning operation and functional tests of OLLOCHI started. Oxygen concentration control technology has also developing. In the large scale LBE loop experiment, the operation for steady state and transient experiments was performed by using IMMORTAL. In the area of instrument, development of ultrasonic flow meter and freeze seal valve are progressing as a key technology for the LBE loop system. Investigation of behavior of impurities in LBE, which is important for design of the irradiation facility, started. In this paper, the status of the LBE studies and experimental plan will be presented.

Journal Articles

Development of one-dimensional optical fiber type radiation distribution sensing method based on wavelength spectrum unfolding

Terasaka, Yuta; Watanabe, Kenichi*; Uritani, Akira*; Yamazaki, Atsushi*; Sato, Yuki; Torii, Tatsuo; Wakaida, Ikuo

Proceedings of International Youth Nuclear Congress 2020 (IYNC 2020) (Internet), 4 Pages, 2020/05

Journal Articles

Impact of hydrided and non-hydrided materials near transistors on neutron-induced single event upsets

Abe, Shinichiro; Sato, Tatsuhiko; Kuroda, Junya*; Manabe, Seiya*; Watanabe, Yukinobu*; Liao, W.*; Ito, Kojiro*; Hashimoto, Masanori*; Harada, Masahide; Oikawa, Kenichi; et al.

Proceedings of IEEE International Reliability Physics Symposium (IRPS 2020) (Internet), 6 Pages, 2020/04

Single event upsets (SEUs) caused by neutrons have been recognized as a serious reliability problem for microelectronic devices on the ground level. In our previous work, it was found that hydride placed in front of the memory chip has considerably impact on SEU cross sections because H ions generated via elastic scattering of neutrons with hydrogen atoms are only emitted in a forward direction. In this study, the effect of components neighboring transistors on neutron-induced SEUs was investigated for 65-nm bulk SRAMs by using PHITS. It was found that the shape of the SEU cross section around few MeV comes from the thickness and the position of components placed in front of transistors when that components do not contains hydrogen atoms. By considering components adjoin memory cells in the test board used in the simulation, measured data at J-PARC BL10 were reproduced well. In addition, it was found that the effect of components neighboring transistors on neutron-induced SERs does not negligible in terrestrial environment.

Journal Articles

Pulsed neutron imaging based crystallographic structure study of a Japanese sword made by Sukemasa in the Muromachi period

Oikawa, Kenichi; Kiyanagi, Yoshiaki*; Sato, Hirotaka*; Omae, Kazuma*; Pham, A.*; Watanabe, Kenichi*; Matsumoto, Yoshihiro*; Shinohara, Takenao; Kai, Tetsuya; Harjo, S.; et al.

Materials Research Proceedings, Vol.15, p.207 - 213, 2020/02

Journal Articles

First nuclear transmutation of $$^{237}$$Np and $$^{241}$$Am by accelerator-driven system at Kyoto University Critical Assembly

Pyeon, C. H.*; Yamanaka, Masao*; Oizumi, Akito; Fukushima, Masahiro; Chiba, Go*; Watanabe, Kenichi*; Endo, Tomohiro*; Van Rooijen, W. G.*; Hashimoto, Kengo*; Sakon, Atsushi*; et al.

Journal of Nuclear Science and Technology, 56(8), p.684 - 689, 2019/08

 Times Cited Count:12 Percentile:86.85(Nuclear Science & Technology)

This study demonstrates, for the first time, the principle of nuclear transmutation of minor actinide (MA) by the accelerator-driven system (ADS) through the injection of high-energy neutrons into the subcritical core at the Kyoto University Critical Assembly. The main objective of the experiments is to confirm fission reactions of neptunium-237 ($$^{237}$$Np) and americium-241 ($$^{241}$$Am), and capture reactions of $$^{237}$$Np. Subcritical irradiation of $$^{237}$$Np and $$^{241}$$Am foils is conducted in a hard spectrum core with the use of the back-to-back fission chamber that obtains simultaneously two signals from specially installed test ($$^{237}$$Np or $$^{241}$$Am) and reference (uranium-235) foils. The first nuclear transmutation of $$^{237}$$Np and $$^{241}$$Am by ADS soundly implemented by combining the subcritical core and the 100 MeV proton accelerator, and the use of a lead-bismuth target, is conclusively demonstrated through the experimental results of fission and capture reaction events.

JAEA Reports

Annual report for research on geosphere stability for long-term isolation of radioactive waste in fiscal year 2016

Ishimaru, Tsuneari; Yasue, Kenichi*; Asamori, Koichi; Kokubu, Yoko; Niwa, Masakazu; Watanabe, Takahiro; Yokoyama, Tatsunori; Fujita, Natsuko; Saiga, Atsushi; Shimizu, Mayuko; et al.

JAEA-Research 2018-008, 83 Pages, 2018/12

JAEA-Research-2018-008.pdf:11.43MB

This annual report documents the progress of research and development (R&D) in the 2nd fiscal year during the JAEA 3rd Mid- and Long-term Plan (fiscal years 2015-2021) to provide the scientific base for assessing geosphere stability for long-term isolation of the high-level radioactive waste. The planned framework is structured into the following categories: (1) Development and systematization of investigation techniques, (2) Development of models for long-term estimation and effective assessment, (3) Development of dating techniques. In this paper, the current status of R&D activities with previous scientific and technological progress is summarized.

Journal Articles

Magnetic Bragg dip and Bragg edge in neutron transmission spectra of typical spin superstructures

Mamiya, Hiroaki*; Oba, Yojiro; Terada, Noriki*; Watanabe, Norimichi*; Hiroi, Kosuke; Shinohara, Takenao; Oikawa, Kenichi

Scientific Reports (Internet), 7(1), p.15516_1 - 15516_8, 2017/11

 Times Cited Count:1 Percentile:6.72(Multidisciplinary Sciences)

no abstracts in English

Journal Articles

The Applicability of SiC-SiC fuel cladding to conventional PWR power plant

Furumoto, Kenichiro*; Watanabe, Seiichi*; Yamamoto, Teruhisa*; Teshima, Hideyuki*; Yamashita, Shinichiro; Saito, Hiroaki; Shirasu, Noriko

Proceedings of 2017 Water Reactor Fuel Performance Meeting (WRFPM 2017) (USB Flash Drive), 10 Pages, 2017/09

Since 2015, Mitsubishi Nuclear Fuel (MNF) has joined in a Japanese R&D project of ATF founded by the Ministry of Economy, Trade and Industry (METI) as a subcontractor to Japan Atomic Energy Agency (JAEA) which is the prime contractor to METI. In this program, MNF plans to evaluate an influence of Silicon Carbide (SiC) composite cladding upon fuel rod behavior in current pressurized water reactors (PWR). This paper reports the evaluation result of the applicability of fuel rod with SiC composite cladding for a conventional PWR. For the applicability evaluations of SiC composite to conventional PWR, both of analytical evaluations and out-of-pile tests for SiC composite were conducted. Analytical evaluations were performed by Mitsubishi's own fuel rod design code and the fuel rod behavior evaluation code developed by JAEA. These codes were modified to evaluate the behavior of the fuel rod with SiC composite cladding. As out-of-pile tests, thermal diffusivity measurement and autoclave corrosion test for SiC composite samples were performed. Test apparatus were developed for evaluation of performance of SiC composite under the condition simulated design basis accident (DBA).

JAEA Reports

Annual report for research on geosphere stability for long-term isolation of radioactive waste in fiscal year 2015

Ishimaru, Tsuneari; Umeda, Koji*; Yasue, Kenichi; Kokubu, Yoko; Niwa, Masakazu; Asamori, Koichi; Watanabe, Takahiro; Yokoyama, Tatsunori; Fujita, Natsuko; Shimizu, Mayuko; et al.

JAEA-Research 2016-023, 91 Pages, 2017/02

JAEA-Research-2016-023.pdf:13.33MB

This annual report documents the progress of research and development (R&D) in the 1st fiscal year during the JAEA 3rd Mid- and Long-term Plan (fiscal years 2015-2021) to provide the scientific base for assessing geosphere stability for long-term isolation of the high-level radioactive waste. The planned framework is structured into the following categories: (1) Development and systematization of investigation techniques, (2) Development of models for long-term estimation and effective assessment, (3) Development of dating techniques. In this paper, the current status of R&D activities with previous scientific and technological progress is summarized.

JAEA Reports

Research plan on geosphere stability for long-term isolation of radioactive waste (Scientific programme for fiscal year 2016)

Ishimaru, Tsuneari; Yasue, Kenichi; Kokubu, Yoko; Niwa, Masakazu; Asamori, Koichi; Watanabe, Takahiro; Yokoyama, Tatsunori; Fujita, Natsuko; Shimizu, Mayuko; Hama, Yuki

JAEA-Review 2016-016, 44 Pages, 2016/08

JAEA-Review-2016-016.pdf:2.28MB

This report is a plan of research and development (R&D) on geosphere stability for long-term isolation of high-level radioactive waste (HLW) in JAEA, in fiscal year 2016. The objectives and contents in fiscal year 2016 are described in detail based on the outline of 7 years plan (fiscal years 2015-2021). Background of this research is clarified with the necessity and the significance for site investigation and safety assessment, and the past progress in this report. In addition, the plan framework is structured into the following categories: (1) Development and systematization of investigation techniques, (2) Development of models for long-term estimation and effective assessment, (3) Development of dating techniques.

Journal Articles

Towards a novel laser-driven method of exotic nuclei extraction-acceleration for fundamental physics and technology

Nishiuchi, Mamiko*; Sakaki, Hironao*; Esirkepov, T. Zh.*; Nishio, Katsuhisa; Pikuz, T. A.*; Faenov, A. Ya.*; Skobelev, I. Yu.*; Orlandi, R.; Pirozhkov, A. S.*; Sagisaka, Akito*; et al.

Plasma Physics Reports, 42(4), p.327 - 337, 2016/04

 Times Cited Count:12 Percentile:60.9(Physics, Fluids & Plasmas)

A combination of a petawatt laser and nuclear physics techniques can crucially facilitate the measurement of exotic nuclei properties. With numerical simulations and laser-driven experiments we show prospects for the Laser-driven Exotic Nuclei extraction-acceleration method proposed in [M. Nishiuchi et al., Phys. Plasmas 22, 033107 (2015)]: a femtosecond petawatt laser, irradiating a target bombarded by an external ion beam, extracts from the target and accelerates to few GeV highly charged short-lived heavy exotic nuclei created in the target via nuclear reactions.

Journal Articles

Influence of linear energy transfer on the scintillation decay behavior in a lithium glass scintillator

Koshimizu, Masanori*; Iwamatsu, Kazuhiro*; Taguchi, Mitsumasa; Kurashima, Satoshi; Kimura, Atsushi; Yanagida, Takayuki*; Fujimoto, Yutaka*; Watanabe, Kenichi*; Asai, Keisuke*

Journal of Luminescence, 169(Part B), p.678 - 681, 2016/01

We analyzed the effects of linear energy transfer (LET) on the scintillation properties of a Li glass scintillator, GS20. The scintillation time profiles were measured by using pulsed ion beams having different LETs. The rise in the scintillation time profiles was faster for higher LET, whereas the decay part was not significantly different for largely different LETs. The LET effects in the rise was ascribed to the effects of excited states interaction during the energy transfer process from the host glass to the luminescent centers, Ce$$^{3+}$$ ions. Supposing that the light yield decreases with LET, the fast rise at high LET was explained in terms of the competition between the energy transfer and the quenching due to the excited states interaction.

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