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and conventional superconductors under pressure郷地 順*; 住山 昭彦*; 山口 明*; 本山 岳*; 木村 憲彰*; 山本 悦嗣; 芳賀 芳範; 大貫 惇睦
JPS Conference Proceedings (Internet), 3, p.011067_1 - 011067_6, 2014/06
The Josephson critical current
between a single crystal UPt
and conventional superconductors has been measured under pressure. The observation of
well above the critical pressure 0.25 GPa, together with a Fraunhofer-like pattern in the magnetic field modulation of
indicates that the Josephson effect is allowed in the superconducting state of UPt
.
=1 zigzag spin-orbital chain大西 弘明
JPS Conference Proceedings (Internet), 3, p.014025_1 - 014025_5, 2014/06
We investigate ground-state properties of a
-orbital Hubbard model on a zigzag chain, by exploiting numerical techniques. The electron number per site is set to be two, leading to a local
=1 state. That is, the system is a Haldane system with active orbital degrees of freedom. We assume that the
level is split into the
(
) and
(
) levels due to the tetragonal crystalline electric field effect. With varying the level splitting, we observe a quantum phase transition that accompanies the change of the orbital state. We will report the detailed ground-state phase diagram and discuss the spin and orbital states. We will also discuss possible relevance of the obtained results to real compounds such as CaV
O
.
Zn
金子 耕士; Raymond, S.*; Ressouche, E.*; Lapertot, G.*; 竹内 徹也*; 広瀬 雄介*; 本多 史憲*; 大貫 惇睦
JPS Conference Proceedings (Internet), 3, p.011061_1 - 011061_5, 2014/06
YbCo
Zn
has a heavy-fermion ground state with an enormously large Sommerfeld coefficient of 8 J/molK
, and that is sensitive to external fields. Whereas pressure induces antiferromagnetic order, magnetic field induces metamagnetic transitions around 0.5 T, and new ordered state appears above 6 T for
. In order to get insights into electronic states and its magnetic field response, neutron scattering experiments on single crystalline samples were carried. In a field-induced phase, magnetic reflections were successfully observed, which has a different propagation vector to that of pressure induced phase. Inelastic neutron scattering probes a crystal-field excitation at a low excitation energy which overlaps to quasielastic response. The results suggest degenerated energy scale, and that leads to variety of external response in YbCo
Zn
.
松田 康弘*; Her, J.-L.*; 道村 真司*; 稲見 俊哉; 海老原 孝雄*; 網塚 浩*
JPS Conference Proceedings (Internet), 3, p.011044_1 - 011044_6, 2014/06
CeRh
Si
の放射光X線吸収実験を32Tまでのパルス強磁場下で行った。Ceの価数は5Kで3+よりわずかに大きく、20T以上の磁場印加に伴い減少する。磁場誘起の価数変化は磁化過程のメタ磁性転移に対応している。この現象は我々の以前に行ったCeRu
Si
の結果に似ており、Ce系重い電子系化合物に共通の現象と思われる。
La
B
studied by resonant X-ray diffraction松村 武*; 道村 真司*; 稲見 俊哉; 大坪 亨*; 谷田 博司*; 伊賀 文俊*; 世良 正文*
JPS Conference Proceedings (Internet), 3, p.014008_1 - 014008_6, 2014/06
Ce
La
B
の1.5K以下の
型反強八極子秩序相(AFO)を磁場中共鳴X線回折法で研究し、AFO相の磁場誘起の多極子を同定した。
4重項結晶場基底状態における
型AFO相に対する平均場近似では、
と
が最も誘起される反強四極子と予想される。しかし、この予想に反して、主な誘起モーメントは
型反強四極子と分かった。
Sr
CuO
佐藤 研太朗*; 松浦 直人*; 藤田 全基*; 梶本 亮一; Ji, S.*; 池内 和彦*; 中村 充孝; 稲村 泰弘; 新井 正敏; 榎木 勝徳*; et al.
JPS Conference Proceedings (Internet), 3, p.017010_1 - 017010_6, 2014/06
We studied the temperature dependence of spin excitation in the underdoped La
Sr
CuO
in a wide energy range. At low temperature, a clear magnetic signal emerging from incommensurate (IC) (0.5
0.09, 0.5) positions was observed. The low-energy (
10 meV) IC signal was confirmed at 200K, while the IC signal gradually merges upon warming and turns into a single commensurate peak centered at (0.5, 0.5) at 300 K. The overall spectral shape above
60 meV measured at 5 K and 350 K was almost the same, meaning the weak thermal effect on the high-energy dispersion relation. This weak change in the high-energy dispersion is consistent with the localized spin picture, whereas the robust IC structure against the temperature would be difficult to explain within a simple stripe model.
and Cu
Ag
CrO
studied by inelastic neutron scattering梶本 亮一; 中島 健次; 河村 聖子; 稲村 泰弘; 奥田 哲治*; 富安 啓輔*
JPS Conference Proceedings (Internet), 3, p.014018_1 - 014018_5, 2014/06
Two-dimensional triangular-lattice Heisenberg antiferromagnet (TLHA) is one of the simplest examples of the geometrical frustration, where nontrivial spin states are expected due to the frustration. CuCrO
is one of the TLHAs where the
= 3/2 spins of Cr
ions form the triangular-lattice. The spins show a three-dimensional ordering with a proper screw structure below
= 24 K. To find nontrivial spin fluctuations in addition to the conventional spin wave, we have studied the magnetic excitations by inelastic neutron scattering using the chopper spectrometer AMATERAS at J-PARC. We found that the excitation spectrum shows an additional diffusive quasielastic component at temperatures (
's) slightly below
and
. This diffuse scattering shows the different
dependence from that of the spin wave excitations, as well as a characteristic
dependence. We argue the origin of the diffuse scattering in terms of the
-vortex and spin molecules.
O
樹神 克明; 井川 直樹; 社本 真一; 池田 一貴*; 大下 英敏*; 金子 直勝*; 大友 季哉*; 鈴谷 賢太郎; 星川 晃範*; 石垣 徹*
JPS Conference Proceedings (Internet), 3, p.013012_1 - 013012_6, 2014/06
LiMn
O
has a cubic spinel structure with a single Mn site whose valence is +3.5. Below about 260 K, the compound exhibits a charge ordering and has inequivalent Mn sites with valences of +3 and +4. However, even in the cubic phase without the charge ordering, temperature dependence of the electrical conductivity is non-metallic. We have performed PDF (atomic pair distribution function) analysis on powder neutron diffraction data of LiMn
O
obtained above 300 K where the compound has cubic structure. The local structure determined by PDF analysis has an orthorhombic lattice distortion and includes the inequivalent Mn sites with valences of +3 and +4 up to, at least, about 450 K. These results indicate that valence electrons are localized at Mn sites with short range periodicity, resulting in the non-metallic electrical conductivity. It can be regarded as a glass state of valence electrons whereas a charge ordering can be regarded as a crystallization of valence electrons.
Al
藤森 伸一; 川崎 郁斗*; 保井 晃*; 竹田 幸治; 岡根 哲夫; 斎藤 祐児; 藤森 淳; 山上 浩志; 芳賀 芳範; 山本 悦嗣; et al.
JPS Conference Proceedings (Internet), 3, p.011072_1 - 011072_5, 2014/06
この講演では、軟X線放射光を利用した角度分解光電子分光実験の結果についてレビューをする。特に強磁性と超伝導が共存するURhGe及び反強磁性と超伝導が共存するURhGeに対する結果について、バンド計算との比較を行って、これらの化合物におけるU 5f電子状態について議論する。
-US
立岩 尚之; 芳賀 芳範; 山本 悦嗣; Fisk, Z.
JPS Conference Proceedings (Internet), 3, p.011086_1 - 011086_7, 2014/06
-US
は常圧で非磁性の半導体である。圧力を加えると、0.5GPaで非常に弱い強磁性状態が誘起される。この強磁性状態は「誘起磁性」状態と理解される。本研究では、
-US
の高圧下磁化測定を絶縁体金属転移する5GPaを越え行った。金属状態へと転移すると、自発磁化の値は、0.04から0.4
/Uへと増大する。強磁性状態は、伝導キャリアの増大とともに安定化すると思われる。
-US
山本 悦嗣; 立岩 尚之; 芳賀 芳範; 池田 修悟*; 酒井 宏典; 大貫 惇睦; Fisk, Z.
JPS Conference Proceedings (Internet), 3, p.011095_1 - 011095_4, 2014/06
-US
is a paramagnetic semiconductor. Chemical substitution of the sulfur site or application of hydrostatic pressure induces ferromagnetic ordering, indicating that
-US
is located near the ferromagnetic instability. Application of magnetic field leads to a huge negative magnetoresistance in
-US
and this behavior is discussed based on the magnetic polaron. In the present study, we study the magnetic, transport and thermal properties of
-US
in detail to clarify the anomalous behavior. Magnetization measurements at low temperature can roughly be explained by a ferromagnetic cluster behavior where the number of the cluster is equal to the number of carrier estimated from Hall effect measurements, consistent with the magnetic polaron model.
中村 博樹; 町田 昌彦
JPS Conference Proceedings (Internet), 3, p.017034_1 - 017034_4, 2014/06
核燃料開発においては、より精密で信頼性の高い物性値を計算可能とする数値シミュレーション技術の開発が求められている。本発表では上記課題に対して、第一原理計算手法の一つであるハイブリッド密度汎関数法に基づく、二酸化プルトニウムの物性値評価の結果を報告する。なお、課題解決にあたっては、ハイブリッド法を採用することにより、従来、強相関効果を取り入れた手法でしか再現できなかった電子状態を得ることに成功した。この解決により、二酸化プルトニウムを含む酸化物核燃料の物性評価をより精度よく推算できるようになることが期待される。
杉本 貴則*; 森 道康; 遠山 貴己*; 前川 禎通
JPS Conference Proceedings (Internet), 3, p.014016_1 - 014016_5, 2014/06
We theoretically study a spin-spin correlation enhanced by non-magnetic impurities in a frustrated two-leg spin ladder. The frustration is introduced by the next-nearest-neighbor antiferromagnetic interaction in the leg direction in the antiferromagnetic two-leg spin ladder. The spin-spin correlation function around impurity site is calculated by the density-matrix renormalization-group method. We find that the spin-spin correlation is enhanced around impurity site with the wavenumber reflecting the frustration. As increasing the frustration, the wavenumber is shifted from commensurate to incommensurate. We discuss several experimental results on BiCu
PO
in the light of our theory.
Si
松本 裕司*; 芳賀 芳範; 立岩 尚之; 青木 晴善*; 木村 憲彰*; 松田 達磨*; 山本 悦嗣; Fisk, Z.; 山上 浩志*
JPS Conference Proceedings (Internet), 3, p.011096_1 - 011096_5, 2014/06
Electronic differences between heavy Fermion CeRu
Si
and isoelectronic nonmagnetic ThRu
Si
have been investigated. We succeeded in observing the de Haas-van Alphen oscillation in a high quality single crystal of ThRu
Si
. The mean free path of conduction carriers has been estimated as 6400
, indicating the high quality of the present sample.

清水 悠晴*; 芳賀 芳範; 柳澤 達也*; 網塚 浩*; 青木 大*; Brison, J.-P.*; Braithwaite, D.*
JPS Conference Proceedings (Internet), 3, p.015009_1 - 015009_6, 2014/06
Static DC magnetization measurements were performed in order to investigate magnetic response of the unconventional superconducting state of UBe
. An unusual anomaly was observed inside the superconducting mixed state corresponding either to a peculiarity of superconducting diamagnetism or the anomalous vortex core structures.
P
under high pressure荒木 新吾*; 林田 みなみ*; 西海 尚人*; 眞鍋 博紀*; 池田 陽一*; 小林 達生*; 村田 惠三*; 稲田 佳彦*; Wi
niewski, P.*; 青木 大*; et al.
JPS Conference Proceedings (Internet), 3, p.011081_1 - 011081_6, 2014/06
Hall effect measurements in ferromagnet U
P
were carried out under pressure up to 4.3 GPa. The Hall resistivity at paramagnetic state is dominated by the extraordinary Hall effect due to the skew scattering. The Curie temperature decreases with increasing pressure and disappears at Pc = 4.1 GPa. The clear first-order metamagnetic transition from the paramagnetic state to the strongly ferromagnetic state appears around Pc at low temperature.
investigated by de Haas-van Alphen effect and high pressure resistivity measurements松本 裕司; 芳賀 芳範; 立岩 尚之; 山本 悦嗣; 木村 憲彰*; 青木 晴善*; Fisk, Z.
JPS Conference Proceedings (Internet), 3, p.011097_1 - 011097_5, 2014/06
Single crystal samples of a new uranium compound URhIn
with the well-known tetragonal HoCoGa
-type structure have been grown by the indium flux method. Although this compound is isostructural to a Ga-analogue URhGa
, the unit cell volume is significantly larger in URhIn
. In contrast to non-magnetic behavior in the isostructural URhGa
, URhIn
has a magnetic ground state with a magnetic transition at 98 K, indicating a drastic difference in electronic states between these compounds.
筒井 健二; 遠山 貴己*; 前川 禎通
JPS Conference Proceedings (Internet), 3, p.017008_1 - 017008_6, 2014/06
銅酸化物高温超伝導物質における不純物置換効果の研究がこれまで世界中で数多く研究されている。Ni不純物置換に対してキャリアがNi不純物近傍へ局在化するといった興味深い現象が実験及び理論的研究により明らかになってきている。本研究ではクラスター計算によって、不純物濃度に比べてホール濃度が高い場合の電子状態を議論し、共鳴非弾性X線散乱スペクトルの予見を行った。
久保 勝規
JPS Conference Proceedings (Internet), 3, p.011023_1 - 011023_6, 2014/06
We study ferromagnetic states in the periodic Anderson model by using the Gutzwiller method. We find three ferromagnetic states: a weakly polarized state, a half-metallic state, and a ferromagnetic state with an almost completely polarized f-electron state. Between these ferromagnetic states, the structure of the Fermi surface is different. In the paramagnetic state, a large Fermi-surface is realized. The topology of the Fermi surface in the weakly polarized state is the same as in the paramagnetic state. In the half-metallic state, the Fermi surface for the majority spin disappears. In the ferromagnetic state with large f-electron polarization, a small Fermi-surface is realized. Then, the phase transitions between these ferromagnetic states accompany change in the Fermi-surface topology, called Lifshitz transitions.
永井 佑紀; 中村 博樹; 町田 昌彦
JPS Conference Proceedings (Internet), 3, p.015013_1 - 015013_6, 2014/06
トポロジカル絶縁体と呼ばれる端のみで電流を運ぶ熱電変換効率の高いと予想される物質群が、原子力分野をはじめとして、さまざまな産業への応用も期待され盛んに研究されている。一方、トポロジカル絶縁体BiSeに銅を導入することによって作製された超伝導体CuxBiSeは、端のみで電流を流すという特異な物性を持ち、かつ超伝導ともなるため、従来にない新しいデバイスとして期待されており、その物性の詳細を明らかにすることが求められている。本講演では、以前構築に成功したトポロジカル超伝導体の有効理論をさらに発展させることにより、表面の効果を扱えるようになったことを報告する。具体的には、トポロジカル絶縁体の表面に生成される表面束縛状態の情報を用いて、それが超伝導となったときに物性にどのような影響を与えるかを記述する方程式を導出した。