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論文

Anharmonic Pr guest modes in Pr(Os$$_{1-x}$$Ru$$_x$$)$$_4$$Sb$$_{12}$$ investigated by inelastic X-ray scattering

筒井 智嗣; 金子 耕士; 宮崎 亮一*; 東中 隆二*; 青木 勇二*; 小林 理気*; 脇本 秀一; Baron, A. Q. R.*; 菅原 仁*; 佐藤 英行*

JPS Conference Proceedings (Internet), 3, p.011060_1 - 011060_5, 2014/06

https://doi.org/10.7566/JPSCP.3.011060

We have investigated the Ru/Os concentration dependence of the Pr guest mode in Pr(Os$$_{1-x}$$Ru$$_x$$)$$_4$$Sb$$_{12}$$ and its variation with temperature. The Pr guest mode at 3.2 meV in PrOs$$_4$$Sb$$_{12}$$ at the N point linearly shifts to a higher energy with the substitution of Ru into the Os site. The energy of the Pr guest mode decreases with decreasing temperature for all compositions, indicating the presence of an anharmonic potential at the Pr site. The slope of the temperature dependence of the guest mode energy is steeper for pure PrOs$$_4$$Sb$$_{12}$$ than for the other Pr(Os$$_{1-x}$$Ru$$_x$$)$$_4$$Sb$$_{12}$$ compounds we measured. The present results imply the importance of the transition metal in determining anharmonicity in Pr(Os$$_{1-x}$$Ru$$_x$$)$$_4$$Sb$$_{12}$$.

論文

Single-crystal growth and de Haas-van Alphen effect study of ThRu$$_2$$Si$$_2$$

松本 裕司*; 芳賀 芳範; 立岩 尚之; 青木 晴善*; 木村 憲彰*; 松田 達磨*; 山本 悦嗣; Fisk, Z.; 山上 浩志*

JPS Conference Proceedings (Internet), 3, p.011096_1 - 011096_5, 2014/06

https://doi.org/10.7566/JPSCP.3.011096

Electronic differences between heavy Fermion CeRu$$_2$$Si$$_2$$ and isoelectronic nonmagnetic ThRu$$_2$$Si$$_2$$ have been investigated. We succeeded in observing the de Haas-van Alphen oscillation in a high quality single crystal of ThRu$$_2$$Si$$_2$$. The mean free path of conduction carriers has been estimated as 6400 ${AA}$, indicating the high quality of the present sample.

論文

DC magnetization study on heavy-electron superconductor UBe$$_{13}$$

清水 悠晴*; 芳賀 芳範; 柳澤 達也*; 網塚 浩*; 青木 大*; Brison, J.-P.*; Braithwaite, D.*

JPS Conference Proceedings (Internet), 3, p.015009_1 - 015009_6, 2014/06

https://doi.org/10.7566/JPSCP.3.015009

Static DC magnetization measurements were performed in order to investigate magnetic response of the unconventional superconducting state of UBe$$_{13}$$. An unusual anomaly was observed inside the superconducting mixed state corresponding either to a peculiarity of superconducting diamagnetism or the anomalous vortex core structures.

論文

Unique Fermi surface and emergence of charge density wave in EuGa$$_4$$ and EuAl$$_4$$

仲村 愛*; 平仲 裕一*; 辺土 正人*; 仲間 隆男*; 三浦 泰直*; 堤 泰樹*; 森 晶宣*; 石田 一裕*; 三田村 勝哉*; 広瀬 雄介*; et al.

JPS Conference Proceedings (Internet), 3, p.011012_1 - 011012_6, 2014/06

https://doi.org/10.7566/JPSCP.3.011012

Two europium compounds with the same structure EuGa$$_4$$ and EuAl$$_4$$ have been investigated. The Fermi surfaces revealed experimentally show a peculiar feature: flat Fermi surface sheets appear parallel to the tetragonal [110] planes. Reflecting this, a charge density wave transition due to the nesting of Fermi surface sheets has been observed in EuAl$$_4$$.

論文

Transport properties of UT$$_2$$Zn$$_{20}$$ (T: Co, Ir)

広瀬 雄介*; 竹内 徹也*; 吉内 伸吾*; 山本 悦嗣; 芳賀 芳範; 摂待 力生*; 大貫 惇睦

JPS Conference Proceedings (Internet), 3, p.011056_1 - 011056_6, 2014/06

https://doi.org/10.7566/JPSCP.3.011056

Transport properties of UT$$_2$$Zn$$_{20}$$ (T: Co, Ir) have been investigated by measuring Hall effect. Overall behavior is explained by the skew scattering on the impurity model at high temperatures and the periodic Anderson model at low temperatures. Rather complicated behavior was observed in UIr$$_2$$Zn$$_{20}$$ with ferromagnetic instability, implying the electronic modification under magnetic field.

論文

Local structural analysis by using atomic pair distribution function on mixed valence compound LiMn$$_2$$O$$_4$$

樹神 克明; 井川 直樹; 社本 真一; 池田 一貴*; 大下 英敏*; 金子 直勝*; 大友 季哉*; 鈴谷 賢太郎; 星川 晃範*; 石垣 徹*

JPS Conference Proceedings (Internet), 3, p.013012_1 - 013012_6, 2014/06

https://doi.org/10.7566/JPSCP.3.013012

LiMn$$_2$$O$$_4$$ has a cubic spinel structure with a single Mn site whose valence is +3.5. Below about 260 K, the compound exhibits a charge ordering and has inequivalent Mn sites with valences of +3 and +4. However, even in the cubic phase without the charge ordering, temperature dependence of the electrical conductivity is non-metallic. We have performed PDF (atomic pair distribution function) analysis on powder neutron diffraction data of LiMn$$_2$$O$$_4$$ obtained above 300 K where the compound has cubic structure. The local structure determined by PDF analysis has an orthorhombic lattice distortion and includes the inequivalent Mn sites with valences of +3 and +4 up to, at least, about 450 K. These results indicate that valence electrons are localized at Mn sites with short range periodicity, resulting in the non-metallic electrical conductivity. It can be regarded as a glass state of valence electrons whereas a charge ordering can be regarded as a crystallization of valence electrons.

論文

Angle resolved photoelectron spectroscopy study of heavy fermion superconductor UPd$$_{2}$$Al$$_{3}$$

藤森 伸一; 川崎 郁斗*; 保井 晃*; 竹田 幸治; 岡根 哲夫; 斎藤 祐児; 藤森 淳; 山上 浩志; 芳賀 芳範; 山本 悦嗣; et al.

JPS Conference Proceedings (Internet), 3, p.011072_1 - 011072_5, 2014/06

https://doi.org/10.7566/JPSCP.3.011072

この講演では、軟X線放射光を利用した角度分解光電子分光実験の結果についてレビューをする。特に強磁性と超伝導が共存するURhGe及び反強磁性と超伝導が共存するURhGeに対する結果について、バンド計算との比較を行って、これらの化合物におけるU 5f電子状態について議論する。

論文

Drastic change in ferromagnetic ground state associated with pressure-induced metal-insulator transition in $$beta$$-US$$_2$$

立岩 尚之; 芳賀 芳範; 山本 悦嗣; Fisk, Z.

JPS Conference Proceedings (Internet), 3, p.011086_1 - 011086_7, 2014/06

https://doi.org/10.7566/JPSCP.3.011086

$$beta$$-US$$_2$$は常圧で非磁性の半導体である。圧力を加えると、0.5GPaで非常に弱い強磁性状態が誘起される。この強磁性状態は「誘起磁性」状態と理解される。本研究では、$$beta$$-US$$_2$$の高圧下磁化測定を絶縁体金属転移する5GPaを越え行った。金属状態へと転移すると、自発磁化の値は、0.04から0.4$${mu}_{rm B}$$/Uへと増大する。強磁性状態は、伝導キャリアの増大とともに安定化すると思われる。

論文

Analysis of magnetization behavior in magnetic semiconductor $$beta$$-US$$_{2}$$

山本 悦嗣; 立岩 尚之; 芳賀 芳範; 池田 修悟*; 酒井 宏典; 大貫 惇睦; Fisk, Z.

JPS Conference Proceedings (Internet), 3, p.011095_1 - 011095_4, 2014/06

https://doi.org/10.7566/JPSCP.3.011095

$$beta$$-US$$_2$$ is a paramagnetic semiconductor. Chemical substitution of the sulfur site or application of hydrostatic pressure induces ferromagnetic ordering, indicating that $$beta$$-US$$_2$$ is located near the ferromagnetic instability. Application of magnetic field leads to a huge negative magnetoresistance in $$beta$$-US$$_2$$ and this behavior is discussed based on the magnetic polaron. In the present study, we study the magnetic, transport and thermal properties of $$beta$$-US$$_2$$ in detail to clarify the anomalous behavior. Magnetization measurements at low temperature can roughly be explained by a ferromagnetic cluster behavior where the number of the cluster is equal to the number of carrier estimated from Hall effect measurements, consistent with the magnetic polaron model.

論文

Hybrid density functional study on plutonium dioxide

中村 博樹; 町田 昌彦

JPS Conference Proceedings (Internet), 3, p.017034_1 - 017034_4, 2014/06

https://doi.org/10.7566/JPSCP.3.017034

核燃料開発においては、より精密で信頼性の高い物性値を計算可能とする数値シミュレーション技術の開発が求められている。本発表では上記課題に対して、第一原理計算手法の一つであるハイブリッド密度汎関数法に基づく、二酸化プルトニウムの物性値評価の結果を報告する。なお、課題解決にあたっては、ハイブリッド法を採用することにより、従来、強相関効果を取り入れた手法でしか再現できなかった電子状態を得ることに成功した。この解決により、二酸化プルトニウムを含む酸化物核燃料の物性評価をより精度よく推算できるようになることが期待される。

論文

Valence state in Ce-based heavy fermion compounds at high magnetic fields

松田 康弘*; Her, J.-L.*; 道村 真司*; 稲見 俊哉; 海老原 孝雄*; 網塚 浩*

JPS Conference Proceedings (Internet), 3, p.011044_1 - 011044_6, 2014/06

https://doi.org/10.7566/JPSCP.3.011044

CeRh$$_2$$Si$$_2$$の放射光X線吸収実験を32Tまでのパルス強磁場下で行った。Ceの価数は5Kで3+よりわずかに大きく、20T以上の磁場印加に伴い減少する。磁場誘起の価数変化は磁化過程のメタ磁性転移に対応している。この現象は我々の以前に行ったCeRu$$_2$$Si$$_2$$の結果に似ており、Ce系重い電子系化合物に共通の現象と思われる。

論文

Effects of Co substitution on the magnetic excitation in heavy fermion compound PrFe$$_{4}$$P$$_{12}$$

Hao, L.*; 岩佐 和晃*; 小林 広樹*; 中島 健次; 河村 聖子; 菊地 龍弥; Chen, D.*; Liu, Y.*; Liu, Z.*; Li, S.*; et al.

JPS Conference Proceedings (Internet), 3, p.011088_1 - 011088_6, 2014/06

https://doi.org/10.7566/JPSCP.3.011088

PrFe$$_{4}$$P$$_{12}$$の重い電子系状態と非磁気秩序状態におけるd電子ドープの効果を調べるために、Pr(Fe$$_{1-x}$$Co$$_{x}$$)$$_{4}$$P$$_{12}$$に対して、比熱、及び、中性子非弾性散乱測定を行った。その結果、Co置換がPrイオンの持つ4f電子の秩序化をもたらし、重い電子系状態と磁気秩序を抑える働きがあることがわかった。

論文

Low-energy spin fluctuations in CuCrO$$_{2}$$ and Cu$$_{0.85}$$Ag$$_{0.15}$$CrO$$_{2}$$ studied by inelastic neutron scattering

梶本 亮一; 中島 健次; 河村 聖子; 稲村 泰弘; 奥田 哲治*; 富安 啓輔*

JPS Conference Proceedings (Internet), 3, p.014018_1 - 014018_5, 2014/06

https://doi.org/10.7566/JPSCP.3.014018

Two-dimensional triangular-lattice Heisenberg antiferromagnet (TLHA) is one of the simplest examples of the geometrical frustration, where nontrivial spin states are expected due to the frustration. CuCrO$$_{2}$$ is one of the TLHAs where the $$S$$ = 3/2 spins of Cr$$^{3+}$$ ions form the triangular-lattice. The spins show a three-dimensional ordering with a proper screw structure below $$T_N$$ = 24 K. To find nontrivial spin fluctuations in addition to the conventional spin wave, we have studied the magnetic excitations by inelastic neutron scattering using the chopper spectrometer AMATERAS at J-PARC. We found that the excitation spectrum shows an additional diffusive quasielastic component at temperatures ($$T$$'s) slightly below $$T_N$$ and $$T > T_N$$. This diffuse scattering shows the different $$T$$ dependence from that of the spin wave excitations, as well as a characteristic $$Q$$ dependence. We argue the origin of the diffuse scattering in terms of the $$Z_2$$-vortex and spin molecules.

論文

Ground state of $$S$$=1 zigzag spin-orbital chain

大西 弘明

JPS Conference Proceedings (Internet), 3, p.014025_1 - 014025_5, 2014/06

https://doi.org/10.7566/JPSCP.3.014025

We investigate ground-state properties of a $$t_{rm 2g}$$-orbital Hubbard model on a zigzag chain, by exploiting numerical techniques. The electron number per site is set to be two, leading to a local $$S$$=1 state. That is, the system is a Haldane system with active orbital degrees of freedom. We assume that the $$t_{rm 2g}$$ level is split into the $$a_{rm 1g}$$ ($$xy$$) and $$e_{rm g}$$ ($$yz,zx$$) levels due to the tetragonal crystalline electric field effect. With varying the level splitting, we observe a quantum phase transition that accompanies the change of the orbital state. We will report the detailed ground-state phase diagram and discuss the spin and orbital states. We will also discuss possible relevance of the obtained results to real compounds such as CaV$$_{2}$$O$$_{4}$$.

論文

Field-induced order in heavy-fermion compound YbCo$$_2$$Zn$$_{20}$$

金子 耕士; Raymond, S.*; Ressouche, E.*; Lapertot, G.*; 竹内 徹也*; 広瀬 雄介*; 本多 史憲*; 大貫 惇睦

JPS Conference Proceedings (Internet), 3, p.011061_1 - 011061_5, 2014/06

https://doi.org/10.7566/JPSCP.3.011061

YbCo$$_2$$Zn$$_{20}$$ has a heavy-fermion ground state with an enormously large Sommerfeld coefficient of 8 J/molK$$^2$$, and that is sensitive to external fields. Whereas pressure induces antiferromagnetic order, magnetic field induces metamagnetic transitions around 0.5 T, and new ordered state appears above 6 T for $$B{parallel}{langle}111{rangle}$$. In order to get insights into electronic states and its magnetic field response, neutron scattering experiments on single crystalline samples were carried. In a field-induced phase, magnetic reflections were successfully observed, which has a different propagation vector to that of pressure induced phase. Inelastic neutron scattering probes a crystal-field excitation at a low excitation energy which overlaps to quasielastic response. The results suggest degenerated energy scale, and that leads to variety of external response in YbCo$$_2$$Zn$$_{20}$$.

論文

X-ray magnetic circular dichroism study of Ce$$_{0.5}$$Gd$$_{0.5}$$Ni

岡根 哲夫; 竹田 幸治; 矢野 一雄*; 藤森 淳; 山上 浩志; 西村 克彦*; 石川 義和*; 佐藤 清雄*

JPS Conference Proceedings (Internet), 3, p.011028_1 - 011028_6, 2014/06

https://doi.org/10.7566/JPSCP.3.011028

(Ce$$_{x}$$Gd$$_{1-x}$$)Ni is an interesting material to study the magnetic properties of Ce 4$$f$$ electrons under the strong influence of other magnetic elements. Previous soft X-ray magnetic circular dichroism (XMCD) study of Ce$$_{0.2}$$Gd$$_{0.8}$$Ni at the Gd $$M_{4,5}$$, Ni $$L_{2,3}$$, and Ce $$M_{4,5}$$ absorption edges has revealed that, while the Gd 4$$f$$ and Ni 3$$d$$ magnetic moments show a saturation at around 2 T, the Ce 4$$f$$ magnetic moment takes a maximum at around 2 T and then shows a linear decrease with magnetic, which can be interpreted as a spin flip behavior. Present study provides the results of similar XMCD study for Ce$$_{0.5}$$Gd$$_{0.5}$$Ni to investigate the stoichiometry dependence of the magnetic properties of Gd 4$$f$$, Ni 3$$d$$, and Ce 4$$f$$ electrons, especially focusing on the spin flip behavior of Ce 4$$f$$ electrons.

論文

Spin polarized neutron scattering study on metal-insulator crossover in uranium dichalcogenide $$beta$$-US$$_{2}$$

目時 直人; 酒井 宏典; 鈴木 通人; 山本 悦嗣; 芳賀 芳範; 松田 達磨; 池田 修悟*

JPS Conference Proceedings (Internet), 3, p.013011_1 - 013011_6, 2014/06

https://doi.org/10.7566/JPSCP.3.013011

ウランカルコゲナイドの金属からモット絶縁体までの多様な物性は多くの興味を集めている。中でもダイカルコゲナイド化合物はカルコゲンや外場(磁場・圧力)によって金属-非金属の変化を示すために興味を持たれている。この講演では、最近の中性子散乱実験の結果と5$$f$$電子の性格がこの物質の物性に関与している点を示すとともに、電子構造との関連性について議論する。

論文

Spin-spin correlation enhanced by impurities in a frustrated two-leg spin ladder

杉本 貴則*; 森 道康; 遠山 貴己*; 前川 禎通

JPS Conference Proceedings (Internet), 3, p.014016_1 - 014016_5, 2014/06

https://doi.org/10.7566/JPSCP.3.014016

We theoretically study a spin-spin correlation enhanced by non-magnetic impurities in a frustrated two-leg spin ladder. The frustration is introduced by the next-nearest-neighbor antiferromagnetic interaction in the leg direction in the antiferromagnetic two-leg spin ladder. The spin-spin correlation function around impurity site is calculated by the density-matrix renormalization-group method. We find that the spin-spin correlation is enhanced around impurity site with the wavenumber reflecting the frustration. As increasing the frustration, the wavenumber is shifted from commensurate to incommensurate. We discuss several experimental results on BiCu$$_{2}$$PO$$_{6}$$ in the light of our theory.

論文

Multipole order and fluctuation in Ce$$_{0.7}$$La$$_{0.3}$$B$$_6$$ studied by resonant X-ray diffraction

松村 武*; 道村 真司*; 稲見 俊哉; 大坪 亨*; 谷田 博司*; 伊賀 文俊*; 世良 正文*

JPS Conference Proceedings (Internet), 3, p.014008_1 - 014008_6, 2014/06

https://doi.org/10.7566/JPSCP.3.014008

Ce$$_{0.7}$$La$$_{0.3}$$B$$_6$$の1.5K以下の$$T_{beta}$$型反強八極子秩序相(AFO)を磁場中共鳴X線回折法で研究し、AFO相の磁場誘起の多極子を同定した。$$Gamma_8$$ 4重項結晶場基底状態における$$T_{beta}$$型AFO相に対する平均場近似では、$$O_{22}$$と$$O_{20}$$が最も誘起される反強四極子と予想される。しかし、この予想に反して、主な誘起モーメントは$$O_{xy}$$型反強四極子と分かった。

論文

Non-Fermi liquid behavior in nonlinear susceptibility in Pr$$_{0.05}$$La$$_{0.95}$$Pb$$_3$$

河江 達也*; 古賀 幹人*; 佐藤 由昌*; 牧山 駿*; 稲垣 祐次*; 立岩 尚之; 藤原 哲也*; 鈴木 博之*; 北井 哲夫*

JPS Conference Proceedings (Internet), 3, p.012030_1 - 012030_6, 2014/06

https://doi.org/10.7566/JPSCP.3.012030

Pr$$_{0.05}$$La$$_{0.95}$$Pb$$_3$$において非線形磁化率$${chi}_3$$の測定を行った。$${chi}_3$$は多極子の自由度が反映される。2.5K以下で$${chi}_3$$の温度依存に$$lnT$$依存が観測され非フェルミ流体的特性が明らかとなった。この結果は、四極子の伝導電子による遮蔽効果が異常な低温物性の起源であることを示唆し、Pr$$_{0.05}$$La$$_{0.95}$$Pb$$_3$$における四極子の自由度の存在を意味する。

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