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Ito, Takashi; Higemoto, Wataru; Koda, Akihiro*; Nakamura, Jumpei*; Shimomura, Koichiro*
Interactions (Internet), 245(1), p.25_1 - 25_7, 2024/12
Fujihara, Masayoshi; Okabe, Hirotaka*; Koda, Akihiro*
Interactions (Internet), 245(1), p.13_1 - 13_6, 2024/12
Quantum states are difficult to observe experimentally. In addition, ideal model materials have not been found for some of the lattice systems in which exotic quantum states are predicted to be realized. Numerous candidates for low-dimensional quantum magnets are hidden in copper minerals, and the number of candidates is increasing every year. We succeeded to synthesize seven copper minerals by imitating the environment where they are discovered and reported their quantum states. The properties of pulsed muons are very suitable for investigating the spin state of artificial copper minerals.
Shimomura, Koichiro*; Koda, Akihiro*; Pant, A. D.*; Sunagawa, Hikaru*; Fujimori, Hiroshi*; Umegaki, Izumi*; Nakamura, Jumpei*; Fujihara, Masayoshi; Tampo, Motonobu*; Kawamura, Naritoshi*; et al.
Interactions (Internet), 245(1), p.31_1 - 31_6, 2024/12
Imaizumi, Yuya; Kamiyama, Kenji; Matsuba, Kenichi
Annals of Nuclear Energy, 206, p.110658_1 - 110658_10, 2024/10
Maruyama, Shuhei; Yamamoto, Akio*; Endo, Tomohiro*
Annals of Nuclear Energy, 205, p.110591_1 - 110591_13, 2024/09
Hirooka, Shun; Morimoto, Kyoichi; Matsumoto, Taku; Ogasawara, Masahiro*; Kato, Masato; Murakami, Tatsutoshi
Journal of Nuclear Materials, 598, p.155188_1 - 155188_9, 2024/09
no abstracts in English
Nakanishi, Takahiro; Sakuma, Kazuyuki; Oyama, Takuya; Hagiwara, Hiroki; Suzuki, Takashi
Environmental Pollution, 355, p.124213_1 - 124213_7, 2024/08
This study investigated the transport behavior of I by riverbank surveys conducted from 2013 to 2015 in a watershed where the
I/
Cs activity ratio is low in the mountainous area and high in the plain as of 2011. Until 2015, the
I/
Cs activity ratio of the levee crown in the studied watershed was similar to that of the surrounding area in 2011. However, the
I/
Cs ratios of the surface riverbank sediments were all low, indicating that radionuclides transported from the mountainous area were deposited on the riverbank in the plain. The vertical distribution of the
I/
Cs ratio in the riverbank sediments indicated that some
I and
Cs deposited during the accident remained in the lower layers, but most were eroded immediately after the accident. Based on the
I/
Cs ratios of sediments deposited on the riverbank, which remained constant until 2015 after the accident, the amount of
I discharged to the ocean was determined from the previously evaluated
Cs discharge. It was calculated that 1.8
10
Bq and 1.2
10
Bq of
I were discharged with sediment from the studied watershed and the contaminated river watersheds (Abukuma River and Fukushima coastal rivers, including the study river), respectively. The results of this study indicate that the continuous
I discharge from the river contribute little to their amount in the seafloor sediments along the Fukushima coast.
Qin, T. Y.*; Hu, F. F.*; Xu, P. G.; Zhang, H.*; Zhou, L.*; Ao, N.*; Su, Y. H.; Shobu, Takahisa; Wu, S. C.*
International Journal of Fatigue, 185, p.108336_1 - 108336_13, 2024/08
Kawai, Kiyoshi*; Sogabe, Tomochika*; Nakagawa, Hiroshi; Yamada, Takeshi*; Koseki, Shigenobu*
Journal of Food Engineering, 375, p.112066_1 - 112066_9, 2024/08
The purpose of this study was to clarify effect of glycerol and glucose on the mechanical glass transition and dynamical transition of freeze-dried bacteria at various water activity (aw)-conditions. From the water sorption isotherm, it was noted that the water content at each aw and monolayer water content were higher in the order of glycerol, glucose, non-added samples. Effect of temperature on the mean square displacement (MSD) of atoms in the samples was investigated by incoherent elastic neutron scattering. The MSD increased gradually with an increase in temperature depending on the aw and added solute. From the linear fitting, three dynamical transition temperatures (low-, middle- and high-Tds) were determined. The Couchman-Karasz model suggested that the added solute and bacteria were not completely miscible.
He, X.*; Kagi, Hiroyuki*; Komatsu, Kazuki*; Iizuka, Riko*; Okajima, Hajime*; Hattori, Takanori; Sano, Asami; Machida, Shinichi*; Abe, Jun*; Goto, Hirotada*; et al.
Journal of Molecular Structure, 1310, p.138271_1 - 138271_8, 2024/08
High-pressure responses of the O-DF hydrogen bonds in deuterated magnesium hydroxyfluoride were investigated using neutron powder diffraction and Raman spectroscopy. The Rietveld analysis at ambient conditions revealed a chemical formula of Mg(OD)
F
and hydroxyl group/fluorine disorder (OD/F disorder) in the crystal structure, which gave rise to two hydrogen-bonding configurations. The Rietveld analysis showed the hydrogen-bonding geometries remains up to 9.8 GPa, indicating no pressure-induced strengthening of hydrogen bonds. The Raman spectra at ambient conditions showed three hydroxyl stretching bands at 2613, 2694, and 2718 cm
. The high frequencies of the O-D stretching modes indicated that the hydroxyls should be involved in weak or none hydrogen-bonding interactions. Up to 20.2 GPa, the mode initially centered at 2694 cm
displayed a pressure-induced blue shift, revealing no strengthening of hydrogen bonds under compression. We discuss the existence of hydrogen bonds and the causes of the blue-shifting hydroxyls at ambient and at high pressures.
Ueki, Taro
Progress in Nuclear Energy, 173, p.105236_1 - 105236_10, 2024/08
The theme of this paper is how to efficiently analyse extreme realizations of neutron effective multiplication factor (keff) over random media replicas modelled by incomplete randomized Weierstrass function (IRWF). To this end, a new bounded amplification (BA) technique is applied to IRWF. Numerical results indicate that the BA-applied IRWF reduces a required number of random media replicas at least by an order of magnitude. To validate this efficiency gain, generalized extreme value (GEV) analysis is applied to a data set of keff values obtained without applying BA. It turns out that the extreme values of these keff values follow the Weibull distribution. Therefore, the theory of GEV guarantees the existence of the upper limit of these keff values, and the actually computed upper limit is indeed smaller than the top two keff values obtained from an order-of magnitude reduced number of BA-applied IRWF random media replicas. This means that the efficiency gain via BA has been confirmed by GEV analysis.
Abe, Satoshi; Shibamoto, Yasuteru
Annals of Nuclear Energy, 202, p.110461_1 - 110461_16, 2024/07
Times Cited Count:0 Percentile:0.05Murmiliuk, A.*; Iwase, Hiroki*; Kang, J.-J.*; Mohanakumar, S.*; Appavou, M.-S.*; Wood, K.*; Almsy, L.*; Len, A.*; Schw
rzer, K.*; Allgaier, J.*; et al.
Journal of Colloid and Interface Science, 665, p.801 - 813, 2024/07
The complexity of protein structure limits our ability to predict and tune the properties of the formed nanoparticles. The goal of our research is to elucidate the key triggers of the morphological transition in protein/PE complexes, evaluate their encapsulation efficacy, and assess particle stability by the systematic study of complexes formed by block copolymers with proteins and ionic drugs. We demonstrated that copolymers consisting of PE and neutral hydrophilic block co-assemble with insulin at pH values close to the protein isoelectric point. The insulin arrangement within the particle is controlled by electrostatic forces between protein molecules, and the morphology of the formed particles can be tuned by varying pH and ionic strength.
Nakamichi, Shinya; Sunaoshi, Takeo*; Hirooka, Shun; Vauchy, R.; Murakami, Tatsutoshi
Journal of Nuclear Materials, 595, p.155072_1 - 155072_11, 2024/07
Sato, Yuki; Terasaka, Yuta; Oura, Masatoshi*
Journal of Nuclear Science and Technology, 61(7), p.856 - 870, 2024/07
Frazer, D.*; Saleh, T. A.*; Matsumoto, Taku; Hirooka, Shun; Kato, Masato; McClellan, K.*; White, J. T.*
Nuclear Engineering and Design, 423, p.113136_1 - 113136_7, 2024/07
Nanoindentation based techniques can be employed on minute volumes of material to measure mechanical properties, including Young's modulus, hardness, and creep stress exponents. In this study, (U,Ce)O solid solutions samples are used to develop elevated temperature nanoindentation and nanoindentation creep testing methods for use on mixed oxide fuels. Nanoindentation testing was performed on 3 separate (Ux-1,Cex)O
compounds ranging from x equals 0.1 to 0.3 at up to 800
C: their Young's modulus, hardness, and creep stress exponents were evaluated. The Young's modulus decreases in the expected linear manner while the hardness decreases in the expected exponential manner. The nanoindentation creep experiments at 800
C give stress exponent values, n=4.7-6.9, that suggests dislocation motion as the deformation mechanism.
Johnson, M.*; Emura, Yuki; Clavier, R.*; Matsuba, Kenichi; Kamiyama, Kenji; Brayer, C.*; Journeau, C.*
Nuclear Engineering and Design, 423, p.113165_1 - 113165_14, 2024/07
Experimental investigation of two interactions between molten jets and sodium, pertaining to severe accidents in a sodium-cooled fast reactor, have been undertaken at the JAEA's MELT facility. X-ray imaging and debris analysis reveal rapid formation of a crust at the melt coolant-interface, instigating thermal fragmentation events. Heat transfer calculations at the jet-coolant interface, supported by particle tracking velocimetry characterisation of the jet velocity, imply the formation of a solid crust within milliseconds of contact with the coolant. A mechanism for enhanced thermal fragmentation is proposed, inspired by observations from the X-ray imaging of coolant entrainment into the jet.
Ito, Fumiaki*; Lee, J.; Hironaka, Kota; Takahashi, Tone; Suzuki, Satoshi*; Mochimaru, Takanori*; Hori, Junichi*; Terada, Kazushi*; Koizumi, Mitsuo
Nuclear Instruments and Methods in Physics Research A, 1064, p.169465_1 - 169465_9, 2024/07
Nakahara, Masaumi; Watanabe, So; Kimura, Shuya; Sasaki, Misa*; Inagaki, Hiromitsu*; Moriguchi, Tetsuji*
Progress in Nuclear Energy, 172, p.105195_1 - 105195_8, 2024/07
A novel removal technique with ultrafine bubbles has been proposed for decommissioning of nuclear facilities. The performance of removal technology with ultrafine bubbles was evaluated in the removal experiments with non-radioactive materials, simulated contaminants precipitated Co oxides. To investigate the influence of difference in the chemical forms, the decontamination experiments were carried out with the fuel pin end plugs contaminated radioactive materials in a hot cell.
Shimazaki, Yosuke; Jidaisho, Tatsuya; Ishii, Toshiaki; Inoi, Hiroyuki; Iigaki, Kazuhiko
JAEA-Technology 2024-005, 23 Pages, 2024/06
HTTR has newly assumed Beyond Design Basis Accident (BDBA) as part of conformity assessment with the new regulatory standards and has established measures to prevent the spread of BDBA. Among these measures, to prevent the spread of BDBA caused by cooling water leaks from spent fuel storage pool, the Oarai Research Institute's fire engine was selected as an equipment to prevent the spread of BDBA, and required performances such as pumping water performance were determined. After all required performances were confirmed by inspections, the fire engine passed the operator's pre-use inspection and contributed to the restart of the HTTR operations.