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Fujimura, Yuki; Ishikawa, Norito; Kondo, Keietsu
JAEA-Technology 2024-012, 26 Pages, 2024/10
JAEA-Technology-2024-012.pdf:3.03MB
While ceramic materials exhibit high temperature strength and corrosion resistance, they are also chemically stable. Specifically, aluminum oxide (Al
O
) is recognized as one of the highly radiation resistant materials. On the other hand, the precise evaluation of irradiation damage in these materials poses a significant challenge because detecting radiation damage induced in highly radiation-resistant ceramics is difficult. The objective of this study is to evaluate irradiation-induced lattice strain using Electron BackScatter Diffraction (EBSD), a technique commonly employed for damage analysis in metals. Ion irradiation tests were conducted on AlO, a representative highly radiation-resistant ceramic, at various doses. Through lattice strain analysis using EBSD, we successfully identified irradiation-induced lattice strain in the direction parallel to the irradiation, consistent with previous XRD analysis results. Lattice strain in the direction perpendicular to the irradiation was also detected. It was observed that the lattice strain tends to increase with increasing irradiation damage. In conclusion, lattice strain analysis using EBSD proves to be an effective method for assessing the irradiation effects on ceramics.
Ogawa, Hiroaki; Ishikawa, Norito
2023-Nendo Daigaku Kenkyu Josei Gijutsu Kenkyu Hokokusho, p.123 - 134, 2024/03
Evaluation of corrosion and hydrogen embrittlement is important in the quality control of stainless steel and the development of next steel materials assuming a high-pressure hydrogen environment. Typically, a secondary ion mass spectrometer (SIMS) is used to analyze hydrogen in steel materials. The hydrogen concentration of conventional standard substance for hydrogen analysis is as small as 1wt-ppm, which has been a problem in hydrogen analysis. We use a hydrogen-implant method to create a locally higher hydrogen concentration than that of the conventional. Hydrogen concentration analysis has been evaluated using the nuclear reaction analysis (NRA) method at a tandem accelerator. We have succeeded in creating a sample with a higher hydrogen concentration of about 1,900 wt-ppm than that of the conventional in locally.
Ishikawa, Norito; Fukuda, Shoma; Nakajima, Toru; Ogawa, Hiroaki; Fujimura, Yuki; Taguchi, Tomitsugu*
Materials, 17(3), p.547_1 - 547_21, 2024/02
Times Cited Count：2 Percentile：57.76(Chemistry, Physical)Natural monoclinic zirconia (baddeleyite) was irradiated with 340-MeV Au ions, and the irradiation-induced nanostructures (i.e., ion tracks and nanohillocks) were observed using transmission electron microscopy. The diameter of the nanohillocks is approximately 10 nm, which is similar to the maximum molten region size calculated using the analytical thermal spike model. Ion tracks are imaged as strained regions that maintain their crystalline structure. The cross-sections of most of the ion tracks are imaged as parallelopiped or rectangular contrasts as large as 10 nm. These results strongly indicate that the molten region is recrystallized anisotropically, reflecting the lattice structure. Furthermore, low-density track cores are formed in the center of the ion tracks. The formation of low-density track cores can be attributed to the ejection of molten matter toward the surface.
Amekura, Hiroshi*; Chettah, A.*; Narumi, Kazumasa*; Chiba, Atsuya*; Hirano, Yoshimi*; Yamada, Keisuke*; Yamamoto, Shunya*; Leino, A. A.*; Djurabekova, F.*; Nordlund, K.*; et al.
Nature Communications (Internet), 15, p.1786_1 - 1786_10, 2024/02
Times Cited Count：2 Percentile：57.35(Multidisciplinary Sciences)Injecting high-energy heavy ions in the electronic stopping regime into solids can create cylindrical damage zones called latent ion tracks. Although these tracks form in many materials, none have ever been observed in diamond, even when irradiated with high-energy GeV uranium ions. Here we report the first observation of ion track formation in diamond irradiated with 2-9 MeV C
fullerene ions. Depending on the ion energy, the mean track length (diameter) changed from 17 (3.2) nm to 52 (7.1) nm. High resolution scanning transmission electron microscopy (HR-STEM) indicated the amorphization in the tracks, in which 
-bonding signal from graphite was detected by the electron energy loss spectroscopy (EELS).
Ishikawa, Norito
JAEA-Conf 2022-002, p.111 - 115, 2023/03
In this report, some of the research topics related to radiation damage and atomic physics researches utilizing the tandem accelerator at JAEA are introduced.
Iwase, Akihiro*; Fukuda, Kengo*; Saito, Yuichi*; Okamoto, Yoshihiro; Semboshi, Satoshi*; Amekura, Hiroshi*; Matsui, Toshiyuki*
Journal of Applied Physics, 132(16), p.163902_1 - 163902_10, 2022/10
Times Cited Count：0 Percentile：0.00(Physics, Applied)Amorphous SiO samples were implanted with 380 keV Fe ions at room temperature. After implantation, some of the samples were irradiated with 16 MeV Au ions. magnetic properties were investigated using a SQUID magnetometer, and the morphology of the Fe-implanted SiO samples was examined using transmission electron microscopy and X-ray absorption spectroscopy (EXAFS and XANES), which showed that the size of Fe nanoparticles was increasing The size of Fe nanoparticles increased with increasing Fe implantation amount; some of the Fe nanoparticles consisted of Fe oxides, and the valence and structure of Fe atoms became closer to that of metallic 
-Fe with increasing Fe injection amount. The magnetization-field curve of the sample implanted with a small amount of Fe was reproduced by Langevin's equation, suggesting that the Fe nanoparticles behave in a superparamagnetic manner. In addition, when a large amount of Fe was implanted, the magnetization-magnetic field curve shows a ferromagnetic state. These magnetic property results are consistent with the X-ray absorption results. Subsequent 16 MeV Au irradiation crushed the Fe nanoparticles, resulting in a decrease in magnetization.
Fe
O
/Pt heterostructuresIeda, Junichi; Okayasu, Satoru; Harii, Kazuya*; Kobata, Masaaki; Yoshii, Kenji; Fukuda, Tatsuo; Ishida, Masahiko*; Saito, Eiji
IEEE Transactions on Magnetics, 58(8), p.1301106_1 - 1301106_6, 2022/08
Times Cited Count：1 Percentile：9.40(Engineering, Electrical & Electronic)The combination of spin-driven thermoelectric (STE) devices based on spin Seebeck effect (SSE), and radioactive isotopes as heat sources, has potential as a next-generation method of power generation in applications such as power supplies for space probes. However, there has been very limited knowledge available indicating the irradiation tolerance of spin thermoelectric devices. Through analysis using a heavy ion-beam accelerator and the hard X-ray photoemission spectroscopy (HAXPES) measurements, we show that a prototypical STE device based on YFeO/Pt heterostructures has tolerance to irradiation of high-energy heavy-ion beams. We used 320 MeV gold ion beams modeling cumulative damages due to fission products emitted from the surface of spent nuclear fuels. By varying the dose level, we confirmed that the thermoelectric and magnetic properties of the SSE elements are not affected by the ion-irradiation dose up to 
ions/cm
fluence and that the SSE signal is extinguished around 
ions/cm, in which the ion tracks almost fully cover the sample surface. In addition, the HAXPES measurements were performed to understand the effects at the interface of YFeO/Pt. The HAXPES measurements suggest that the chemical reaction that diminishes the SSE signals is enhanced with the increase of the irradiation dose. We share the current understandings of the damage analysis in YFeO/Pt for developing better STE devices applicable to harsh environmental usages.
irradiated with swift heavy ions at grazing incidenceIshikawa, Norito; Fujimura, Yuki; Kondo, Keietsu; Szabo, G. L.*; Wilhelm, R. A.*; Ogawa, Hiroaki; Taguchi, Tomitsugu*
Nanotechnology, 33(23), p.235303_1 - 235303_10, 2022/06
Times Cited Count：7 Percentile：53.46(Nanoscience & Nanotechnology)A single crystal of SrTiO doped with niobium (Nb-STO) was irradiated with 200 MeV Au ions at grazing incidence. Atomic force microscopy (AFM) and scanning electron microscopy (SEM) are used to study the relation between irradiation-induced change of surface topography and corresponding material property changes. As expected, multiple hillocks as high as 5-6 nm are imaged by AFM observation. It is also found that the region in between the adjacent hillocks is slightly elevated rather than depressed. Line-like contrasts along the ion paths are found in both AFM phase images and SEM images, indicating the formation of continuous ion tracks in addition to multiple hillocks. Cross-sectional transmission electron microscopy (TEM) observation shows that the ion tracks in the near-surface region are found to be relatively large, whereas buried ion tracks in the deeper region are relatively small. The results suggest that recrystallization plays an important role in the formation of small ion tracks in the deep region, whereas formation of large ion tracks in the near-surface region is likely due to the absence of recrystallization.
200 MeV ion irradiationPogrebnjak, A. D.*; Bagdasaryan, A. A.*; Horodeck, P.*; Tarelnyk, V.*; Buranich, V. V.*; Amekura, Hiroshi*; Okubo, Nariaki; Ishikawa, Norito; Beresnev, V. M.*
Materials Letters, 303, p.130548_1 - 130548_4, 2021/11
Times Cited Count：25 Percentile：79.76(Materials Science, Multidisciplinary)Positron annihilation spectroscopy (PAS) of ion-irradiated (TiZrHfNbV)N nitride which is a high-entropy alloy-based material indicates that the vacancy-defects are the dominant defects type. Although the specimens are irradiated up to 5
10
ions/cm
no amorphization or intermetallic phase formation is detected after the irradiation, demonstrating the radiation tolerance of the high-entropy alloys.
single crystal by ion irradiation; A Molecular dynamics studySasajima, Yasushi*; Kaminaga, Ryuichi*; Ishikawa, Norito; Iwase, Akihiro*
Quantum Beam Science (Internet), 5(4), p.32_1 - 32_14, 2021/11
The nano-pore formation process that occurs by supplying a thermal spike to single crystal CeO has been simulated using a molecular dynamics method. As the initial condition, high thermal energy was supplied to the atoms in a nano-cylinder placed at the center of a fluorite structure. A nano-pore was generated abruptly at around 0.3 ps after the irradiation. It grew to its maximum size at 0.5 ps, and successively it shrank during the time to 1.0 ps. The nano-pore size increased with increasing effective stopping power.
ZnSnS
thin films induced by 200 MeV Xe swift heavy ions irradiationKhoualed, M.*; Boutebakh, F. Z.*; Chettah, A.*; Amekura, Hiroshi*; Ishikawa, Norito; Ghemid, S.*; Attaf, N.*; Aida, M. S.*
Journal of Materials Science; Materials in Electronics, 32(20), p.25516 - 25527, 2021/10
Times Cited Count：4 Percentile：27.19(Engineering, Electrical & Electronic)CuZnSnS (CZTS) thin films deposited on glass substrate using spray pyrolysis technique were irradiated by 200 MeV Xe ions at different fluences. The effect of high-density electronic excitations on the properties of CZTS thin films has been examined using UV-visible spectrophotometry for optical properties, X-ray diffraction and Raman spectroscopy for structural properties. A pronounced blue-shift in the transmittance spectra edges and bandgap widening up to 2.05 eV were observed by the irradiation.
Sueyoshi, Tetsuro*; Enokihata, Ryusei*; Yamaguchi, Hiroshi*; Fujiyoshi, Takanori*; Okuno, Yasuki*; Ishikawa, Norito
IEEE Transactions on Applied Superconductivity, 31(5), p.8000305_1 - 8000305_5, 2021/08
Angular behaviors of critical current density Jc at 77 K, 1 T were investigated in YBCO films with columnar defects (CDs) tilted at small angles to the ab-plane before and after the additional introduction of CDs at different angles, where CDs were installed by heavy-ion irradiations. The enhanced Jc at 
by the initial irradiation at 
i=
85
relative to the c-axis was reduced by the additional irradiation at i=75, whereas the Jc was increased at the intermediate angle between the two irradiation angles. The addition of CDs at i=0 also lowered the Jc around , which were enhanced by the initial irradiation angles of i=80.
Ishikawa, Norito; Taguchi, Tomitsugu*; Okubo, Nariaki
Shototsu, 18(3), p.43 - 55, 2021/05
Radiation damage mechanism in ceramics irradiated with swift heavy ions has been studied by using transmission electron microscopy (TEM). We introduce how the mechanisms are unveiled by our recent TEM studies.
superconductorsSueyoshi, Tetsuro*; Enokihata, Ryusei*; Hidaka, Yuka*; Irie, Masahiro*; Fujiyoshi, Takanori*; Okuno, Yasuki*; Ishikawa, Norito
Physica C, 582, p.1353824_1 - 1353824_5, 2021/03
Times Cited Count：3 Percentile：17.11(Physics, Applied)We investigated the combined effect of flux pinning by three-directional columnar defects (CDs) in a wide field-angular range of YBaCuOy thin films, where CDs parallel to the 
-axis and CDs crossing at (=45, 60 and 80) relative to the c-axis were installed by 200 MeV Xe-ion irradiations. The three-directional CDs with 
60 form a field angular curve of critical current density Jc with a broad peak centered at magnetic field (B) parallel to the -axis, whereas the Jc shows no peaks around the crossing angles of . When the crossing angle is expanded to =80, a drastic change in the field- angular behavior of Jc is induced: there is not a large enhancement of 
around B//c. We also demonstrated that the combined configuration consisting of CDs at = 0, 45, 60 and 80 provides a uniform enhancement of over a wide angular-region.
Amekura, Hiroshi*; Toulemonde, M.*; Narumi, Kazumasa*; Li, R.*; Chiba, Atsuya*; Hirano, Yoshimi*; Yamada, Keisuke*; Yamamoto, Shunya*; Ishikawa, Norito; Okubo, Nariaki; et al.
Scientific Reports (Internet), 11(1), p.185_1 - 185_11, 2021/01
Times Cited Count：15 Percentile：69.32(Multidisciplinary Sciences)We report the track formation of 10 nm in diameter in silicon irradiated with 6 MeV C, i.e., much lower energy than the previously reported energy threshold.
Ishikawa, Norito; Taguchi, Tomitsugu*; Ogawa, Hiroaki
Quantum Beam Science (Internet), 4(4), p.43_1 - 43_14, 2020/12
Amorphizable ceramics were irradiated with 200 MeV Au ions, and the as-irradiated samples were observed by transmission electron microscopy (TEM). The ion track diameter and hillock diameter are similar for all the amorphizable ceramics. For SrTiO and niobium-doped STO, 200 MeV Au ion irradiation and TEM observation were also performed. The ion track diameters in these materials are found to be markedly smaller than the hillock diameters. The ion tracks in these materials exhibit inhomogeneity, which is similar to that reported for non-amorphizable ceramics. On the other hand, the hillocks appear to be amorphous, and the amorphous feature is in contrast to the crystalline feature of hillocks observed in non-amorphizable ceramics. No marked difference is recognized between the nanostructures in STO and those in Nb-STO.
Amekura, Hiroshi*; Li, R.*; Okubo, Nariaki; Ishikawa, Norito; Chen, F.*
Quantum Beam Science (Internet), 4(4), p.39_1 - 39_11, 2020/12
Evolution of depth profiles of the refractive index in YAl
O (YAG) crystals were studied under 200 MeV Xe ion irradiation. The index changes were observed at three different depth regions; (i) a plateau near the surface between 0 and 3 
m in depth, which can be ascribed to the electronic stopping Se, (ii) a broad peak at 6 m in depth, and (iii) a sharp dip at 13 m in depth, which is attributed to the nuclear stopping Sn peak.
Tsuchida, Hidetsugu*; Kai, Takeshi; Kitajima, Kensei*; Matsuya, Yusuke; Majima, Takuya*; Saito, Manabu*
European Physical Journal D, 74(10), p.212_1 - 212_7, 2020/10
Times Cited Count：5 Percentile：33.43(Optics)Fundamental study of interaction between biomolecules and heavy ions in water is very important to predict an initial stage of radiation biological effects. A heavy ion irradiation experiment into droplet target assumed as a biological system in a vacuum was performed to measure production yields of cations and anions for glycine, which was ejected from the droplet target to the vacuum. However, the production mechanisms have been unknown. The PHITS code adapting ion track structure mode was used to analyze the production mechanisms from the dose evaluation at the surface between the vacuum and the water. It is found that induction yields of ionization and excitation, and dissociative electron attachment involved in the secondary electrons were correlated with the production yields of cations and anions of the glycine. The results provide us newly scientific insights to predict an initial stage of radiation biological effects.
by using Poisson distribution functionYamamoto, Yuki*; Ishikawa, Norito; Hori, Fuminobu*; Iwase, Akihiro*
Quantum Beam Science (Internet), 4(3), p.26_1 - 26_13, 2020/09
The lattice constant and the magnetic state of CeO are modified by the irradiation with 200 MeV Xe ions. Under the assumption that these modifications are induced in the narrow one-dimensional region (the ion track) along the ion beam path, the dependence of the lattice constant and the saturation magnetization of CeO on the Xe ion fluence can be analyzed by using the Poisson distribution function. The analysis reveals that the lattice constant inside the ion track, which is larger than outside the ion track is not affected by the overlapping of the ion track. The present result implies that the Poisson distribution function is useful for describing the effect of ion track overlapping on the ion irradiation induced ferromagnetic state in CeO.
Okayasu, Satoru; Harii, Kazuya*; Kobata, Masaaki; Yoshii, Kenji; Fukuda, Tatsuo; Ishida, Masahiko*; Ieda, Junichi; Saito, Eiji
Journal of Applied Physics, 128(8), p.083902_1 - 083902_7, 2020/08
Times Cited Count：3 Percentile：14.27(Physics, Applied)