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Journal Articles

Evaluation of thermal neutron scattering law of nuclear-grade isotropic graphite

Nakayama, Shinsuke; Iwamoto, Osamu; Kimura, Atsushi

EPJ Web of Conferences, 294, p.07001_1 - 07001_6, 2024/04

Graphite is a candidate of moderator in innovative nuclear reactors such as molten salt reactors. Scattering of thermal neutrons by the moderator material has a significant impact on the reactor core design. To contribute to the development of innovative nuclear reactors, an evaluation method of thermal neutron scattering law for reactor grade graphite was studied. The inelastic scattering component due to lattice vibration was evaluated based on the phonon density of states computed with first-principles lattice dynamics simulations. The simulations were performed for ideal crystalline graphite. The coherent elastic scattering component due to crystal structure was evaluated based on neutron transmission and scattering experiments recently performed in the J-PARC/MLF facility. In comparison with the neutron transmission experiments, it was found that the quantification of small-angle neutron scattering due to structures larger than crystal, such as pores in graphite, is important. Based on the above methods, thermal neutron scattering law data for reactor-grade graphite at room temperature were evaluated.

Journal Articles

Linearization of thermal neutron scattering cross section to optimize the number of energy grid points

Tada, Kenichi

Proceedings of 12th International Conference on Nuclear Criticality Safety (ICNC2023) (Internet), 8 Pages, 2023/10

The number of energy grids of the thermal neutron scattering law data has a large impact on the data size of a cross section file of continuous energy Monte Carlo calculation codes. The optimization of the number of energy grids is an effective way to reduce the data size. This study developed the linearization method of the thermal neutron scattering cross section to optimize the number of energy grids and the linearization function was implemented in the nuclear data processing code FRENDY. The linearization process which is used in the resonance reconstruction and the Doppler broadening was adopted. The criticality benchmarks which use ZrH as the moderator were calculated to estimate the impact of the difference of the energy grids on neutronics calculations. The calculation results indicate that the linearization of the thermal neutron scattering cross section improves the prediction accuracy of neutronics calculations.

Journal Articles

Preliminary analyses of modified STACY core configuration using serpent with JENDL-5

Kawaguchi, Maho*; Shiba, Shigeki*; Iwahashi, Daiki*; Okawa, Tsuyoshi*; Gunji, Satoshi; Izawa, Kazuhiko; Suyama, Kenya

Proceedings of 12th International Conference on Nuclear Criticality Safety (ICNC2023) (Internet), 8 Pages, 2023/10

The Nuclear Regulation Authority (NRA) has been working on an experimental approach for evaluating the criticality of fuel debris produced by the Fukushima Daiichi Nuclear Power Plant (FDNP) accident since 2014, collaborating with the Japan Atomic Energy Agency (JAEA). As part of the approach, JAEA has modified the STAtic experiment Critical facilitY (STACY) for critical experiments to evaluate characteriscs of pseudo-fuel debris. As the preliminary analyses, we verified critical characteristics with major nuclear data libraries for the proposed core configuration patterns. The three-dimensional continuous-energy Monte Carlo neutron and photon transport code, SERPENT-V2.2.0 was used with the latest JENDL, JENDL-5. As a result, larger multiplication factors of JENDL-5 across the modified STACY core configuration patterns were evaluated in comparison to the other libraries. And, $$^{1}$$H scattering and $$^{238}$$U fission sensitivity coefficients of JENDL-5 were different from those of the other libraries. Comparing among analyses with those libraries, the updated S($$alpha$$, $$beta$$) of JENDL-5 might affect the result of critical characteristics in the critical analyses for the modified STACY core configuration.

Journal Articles

Inelasticity effect on neutron scattering intensities of the null-H$$_{2}$$O

Kameda, Yasuo*; Sasaki, Motoya*; Usuki, Takeshi*; Otomo, Toshiya*; Ito, Keiji*; Suzuya, Kentaro; Fukunaga, Toshiharu*

Journal of Neutron Research, 11(3), p.153 - 163, 2003/09

We describe results of time-of-flight (TOF) neutron diffraction of the liquid water null-H$$_{2}$$O in order to investigate the effect of both the scattering angle and the neutron flight path ratio to the observed self-scattering intensities. An empirical inelasticity correction procedure is proposed using the self-scattering intensity observed for the null-H$$_{2}$$O.

JAEA Reports

THRUSH: A code for calculating thermal neutron scattering kernel

*

JAERI-M 8927, 26 Pages, 1980/06

JAERI-M-8927.pdf:0.63MB

no abstracts in English

Journal Articles

Neutron scattering study of the anharmonic lattice vibrations in calcium fluoride

Journal of the Physical Society of Japan, 35(1), p.204 - 212, 1973/01

 Times Cited Count:3

no abstracts in English

Journal Articles

Dispersion relations of the normal vibrations in strontium titanate

; ; *

J.Phys.,C, 6(21), p.3021 - 3023, 1973/00

no abstracts in English

JAEA Reports

Theoretical Calculation for Thermal Neutron Scattering Kernel

JAERI 1095, 34 Pages, 1965/12

JAERI-1095.pdf:2.09MB

no abstracts in English

JAEA Reports

Survey and Problems in the Study of Thermal Neutron Scattering

JAERI 1086, 115 Pages, 1965/10

JAERI-1086.pdf:5.28MB

no abstracts in English

Oral presentation

Development of nuclear data processing system FRENDY, 2; Scattering cross section generation in the thermal energy range

Tada, Kenichi; Nagaya, Yasunobu

no journal, , 

JAEA has been developed the nuclear data processing system FRENDY (FRom Evaluated Nuclear Data librarY to any application). In this presentation, verification of scattering cross section generation in the thermal energy range is described.

Oral presentation

Development of nuclear data processing system FRENDY

Tada, Kenichi

no journal, , 

In JAEA, the nuclear data processing system FRENDY (FRom Evaluated Nuclear Data librarY to any application) has been developed. In this presentation, the overview and verification of FRENDY is described.

Oral presentation

Generation of thermal neutron scattering cross section from evaluated nuclear data

Tada, Kenichi

no journal, , 

The nuclear data processing is very important to generate cross section libraries for neutronics calculation codes. Though many researchers want to generate cross section libraries by themselves, only few researchers can generate them. This presentation explains the processing flow and method of the nuclear data processing from evaluated nuclear data file into the cross section library. This presentation also explains how to generate cross section library from experimental data or analytical results of thermal neutron scattering.

Oral presentation

Development of a Monte Carlo Solver Solomon for criticality safety analysis, 3; Implementation of thermal neutron scattering models

Nagaya, Yasunobu

no journal, , 

In order to build a criticality characteristics database for fuel debris, a Monte Carlo Solver Solomon has been under development. Thermal neutron scattering models have been implemented into Solomon to extend the applicability area to thermal reactor systems. The implementation has been verified with the inter-code comparison of effective multiplication factors for simple geometries.

Oral presentation

Investigation of the impact of difference between open nuclear data processing codes on neutron transport calculations, 3; Difference of nuclear data processing method

Tada, Kenichi; Ikehara, Tadashi; Ono, Michitaka*; Tojo, Masayuki*

no journal, , 

JAEA develops a nuclear data processing code FRENDY. We can comparison and verification of conventional nuclear data processing code using FRENDY. In this presentation, we focus on the thermal scattering law data. We found some problems of NJOY to process the thermal scattering law data as follows, (1) The generation of input file is complex and we found some inputting error in the official ACE library, (2) The maximum energy of ACE file is not identical to the inputted maximum energy, (3) If user uses iwt=2 option in ACER module, MCNP6.1 cannot treat this generated ACE file appropriately and the calculation will not completed This presentation explains the overview of these problems.

Oral presentation

Theoretical study of thermal neutron scattering by light and heavy water with molecular dynamics simulation

Ichihara, Akira; Abe, Yutaka*

no journal, , 

Light and heavy water are being used as moderators in fission reactors. Reliable data of thermal neutron scattering in these materials is essential to the analysis of reactor cores. In this study we tried to evaluate angular distribution and energy spectrum of emitted neutrons employing the information obtained from molecular dynamics simulations. The simulations have been performed for light and heavy water. The thermal neutron scattering has been evaluated by using the fluctuation-dissipation theorem of statistical mechanics, where the trajectory data for hydrogen, deuterium and oxygen atoms were utilized. In calculation, incoherent scattering was assumed to be dominant in light water, while both the coherent and incoherent scattering contributions were considered in heavy water.

Oral presentation

Treatment of thermal scattering law data in FRENDY

Tada, Kenichi

no journal, , 

We have compared the processing results of FRENDY to those of NJOY for verification of FRENDY. In this presentation, we focus on the processing of thermal scattering law data. This presentation explains the problems of NJOY. This presentation also explains the implementation of input checking functions for collect nuclear data processing and the recent development of FRENDY, e.g., the development of neutron-induced multi-group cross-section file generation function.

Oral presentation

Development of nuclear data evaluation framework for innovative reactor, 6; Study of evaluation methods for thermal neutron scattering law and charged-particle emission reaction cross section

Nakayama, Shinsuke; Iwamoto, Osamu

no journal, , 

In molten salt reactors and small modular reactors (SMRs), the use of graphite and CaH$$_{2}$$ as moderators is being considered, respectively. Thermal neutron scattering law of moderator material has a large influence on the reactor core design. In addition, charged-particle emission reactions such as (n,p) and (n,a) on K-39 in molten salt and on Cu-63 in heat pipes of SMRs can produce nuclides that are problematic for waste management. Therefore, accurate data on thermal neutron scattering laws for graphite and CaH$$_{2}$$, and charged-particle emission reaction cross sections for K-39 and Cu-63 are important for the core design of these innovative reactors. Based on the above, we have been studying the evaluation method of these data. The progress to date will be presented.

Oral presentation

Effect of thermal scattering law data for H in H$$_{2}$$O of JENDL-5 at several moderator temperatures on neutronics calculation

Tada, Kenichi; Watanabe, Tomoaki; Endo, Tomohiro*; Yamamoto, Akio*

no journal, , 

The PWR pin-cell calculations using the cross section data of each evaluated nuclear data library were compared at several moderator temperatures for the verification of the thermal scattering law data for H in H$$_{2}$$O of JENDL-5. Compared with the commonly used evaluated nuclear data libraries JENDL-4.0 and ENDF-B/VII.1, the relative differences of k-infinity varied with the moderator temperature. This difference may affect the moderator temperature coefficient. However, it is difficult to judge which library is good since there are not so much experimental data for the cross section and double differential cross section measurement of high-temperature H in H$$_{2}$$O data. Additional experimental data are required to improve the prediction accuracy of the thermal scattering law data for H in H$$_{2}$$O data.

Oral presentation

Impact of $$^{9}$$Be thermal scattering law data considering crystallite size, 2; Effect on nuclear properties of A-FNS test modules

Kwon, Saerom*; Konno, Chikara; Ota, Masayuki*; Sato, Satoshi*

no journal, , 

The analyses of the beryllium benchmark experiment at JAEA/FNS and the test modules of a fusion neutron source A-FNS were performed with the thermal scattering law data of $$^{9}$$Be considering the crystallite size of beryllium produced by the European Spallation Source group. It was concluded that the overestimation of the calculated reaction rates sensitive to low energy neutrons in the beryllium benchmark experiment at JAEA/FNS decreased with increasing the crystallite size of beryllium. The effect of the $$^{9}$$Be thermal scattering law data appeared for neutron flux below 0.1 eV in the test modules of A-FNS but the effect on tritium production rate, etc. was small because the neutron flux below 0.1 eV was small.

Oral presentation

Development of nuclear data evaluation framework for innovative reactor (II), 5; Development of evaluated nuclear data files

Nakayama, Shinsuke; Iwamoto, Osamu

no journal, , 

The use of graphite and hydrogen compounds as moderators has been considered for molten salt reactors and small modular reactors. Scattering of thermal neutrons by moderators has a significant impact on reactor core design. In addition, charged-particle emission reactions on nuclides contained in molten salts and structural materials can produce nuclides that pose a problem for waste management. Therefore, accurate thermal neutron scattering law and charged-particle emission reaction cross section data for the above materials are important for the development of such innovative reactors. Based on the above, these nuclear data were evaluated and compiled as an evaluated nuclear data file in the MEXT Innovative Nuclear Research and Development Program entitled "Development of Nuclear Data Evaluation Framework for Innovative Reactor". The evaluation method of these nuclear data is outlined.

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