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論文

Topological spin-orbit torque in ferrimagnetic Weyl semimetal

目黒 智成*; 小沢 耀弘*; 小林 浩二*; 荒木 康史; 野村 健太郎*

Physical Review Research (Internet), 7(2), p.L022065_1 - L022065_8, 2025/06

We theoretically find a topological spin-orbit torque (SOT) in the compensated ferrimagnetic Weyl semimetal Ti$$_{2}$$MnAl. The topological SOT arises from all the occupied states, which is free from dissipation. However, it is negligible in metallic magnets and was not reported in Weyl semimetals. We show the enhancement of the topological SOT from the mixed Berry curvature around the Weyl points in Ti$$_{2}$$MnAl. This finding provides a guiding principle for designing highly efficient SOT devices using the topological nature of ferrimagnetic Weyl semimetals.

論文

Electrical mutual switching in a noncollinear-antiferromagnetic-ferromagnetic heterostructure

Yoon, J.-Y.*; 竹内 祐太朗*; 武智 涼太*; Han, J.*; 内山 友宏*; 山根 結太*; 金井 駿*; 家田 淳一; 大野 英男*; 深見 俊輔*

Nature Communications (Internet), 16, p.1171_1 - 1171_8, 2025/02

 被引用回数:0 パーセンタイル:0.00(Multidisciplinary Sciences)

Spin-orbit torque (SOT) provides a promising mechanism for electrically encoding information in magnetic states. Unlike existing schemes, where the SOT is passively determined by the material and device structures, an active manipulation of the intrinsic SOT polarity would allow for flexibly programmable SOT devices. Achieving this requires electrical control of the current-induced spin polarization of the spin source. Here we demonstrate a proof-of-concept current-programmed SOT device. Using a noncollinear-anti-ferromagnetic/nonmagnetic/ferromagnetic Mn$$_3$$Sn/Mo/CoFeB hetero-structure at zero magnetic eld, we show current-induced switching in the CoFeB layer due to the spin current polarized by the magnetic structure of the Mn$$_3$$Sn; by properly tuning the driving current, the spin current from the CoFeB further reverses the magnetic orientation of the Mn$$_3$$Sn, which determines the polarity of the subsequent switching of the CoFeB. This scheme of mutual switching can be achieved in a spin-valve-like simple protocol because each magnetic layer serves as a reversible spin source and target magnetic electrode. It yields intriguing proof-of-concept functionalities for unconventional logic and neuromorphic computing.

論文

Possible field-induced quantum state in a rhombic lattice antiferromagnet KCoPO$$_{4}$$$$cdot$$H$$_{2}$$O

藤原 理賀; 萩原 雅人; 幸田 章宏*; 中村 惇平*; 松尾 晶*; 金道 浩一*; 石角 元志*

Physical Review Materials (Internet), 9(1), p.014406_1 - 014406_9, 2025/01

 被引用回数:1 パーセンタイル:0.00(Materials Science, Multidisciplinary)

We reported the magnetic behavior of a rhombic lattice quantum antiferromagnet KCoPO$$_{4}$$$$cdot$$H$$_{2}$$O. The rhombic lattice model is equivalent to a model of a square lattice with two different diagonal components, and competing exchange interactions potentially produce exotic quantum states. This compound is well characterized by the $$J$$$$_{rm{eff}}$$ = 1/2 state. The magnetic structure of KCoPO$$_{4}$$$$cdot$$H$$_{2}$$O is identified as an incommensurate helical structure, characterized by a magnetic modulation propagation vector $$bold{k}$$ = (0.1747(1) 0 0) with an in-plane moment rotating along the $$a$$ axis. Moreover, a magnetic field-induced phase transition is observed at approximately 1 T. The application of a magnetic field suppresses spin ordering and enhance spin fluctuations. Our experimental results suggest the presence of a quantum phase in the magnetic phase diagram of the spin-1/2 Heisenberg rhombic lattice antiferromagnet with easy-plane anisotropy.

論文

Single-layer spin-orbit-torque magnetization switching due to spin berry curvature generated by minute spontaneous atomic displacement in a Weyl oxide

堀内 皓斗*; 荒木 康史; 若林 勇希*; 家田 淳一; 山ノ内 路彦*; 他7名*

Advanced Materials, p.2416091_1 - 2416091_9, 2025/00

 被引用回数:0

Spin Berry curvature characterizes the band topology as the spin counterpart of Berry curvature and is crucial in generating novel spintronics functionalities. By breaking the crystalline inversion symmetry, the spin Berry curvature is expected to be significantly enhanced; this enhancement will increase the intrinsic spin Hall effect in ferromagnetic materials and, thus, the spin-orbit torques (SOTs). However, this intriguing approach is not applied to devices; generally, the spin Hall effect in ferromagnet/heavy-metal bilayer is used for SOT magnetization switching. Here, SOT-induced partial magnetization switching is demonstrated in a single layer of a single-crystalline Weyl oxide SrRuO$$_{3}$$ (SRO) with a small current density of $$approx 3.1 times 10^6 {rm A} {rm cm}^{-2}$$. Detailed analysis of the crystal structure in the seemingly perfect periodic lattice of the SRO film reveals barely discernible oxygen octahedral rotations with angles of $$approx 5^circ$$ near the interface with a substrate. Tight-binding calculations indicate that a large spin Hall conductivity is induced around small gaps generated at band crossings by the synergy of inherent spin-orbit coupling and band inversion due to the rotations, causing magnetization reversal. The results indicate that a minute atomic displacement in single-crystal films can induce strong intrinsic SOTs that are useful for spin-orbitronics devices.

論文

Interfacial Dzyaloshinskii-Moriya interaction in nonmagnetic/noncollinear-antiferromagnetic bilayers

山根 結太*; 荒木 康史; 深見 俊輔*

Physical Review B, 111(14), p.144412_1 - 144412_9, 2025/00

 被引用回数:0 パーセンタイル:0.00(Materials Science, Multidisciplinary)

We study the Dzyaloshinskii-Moriya interaction (DMI) appearing at the interface of a nonmagnetic/noncollinear-antiferromagnetic bilayer. The DMI is an antisymmetric exchange interaction between neighboring magnetic spins, arising in the absence of an inversion center between the spins, the explicit expression of which is dictated by system symmetry. We formulate the interfacial DMI for different crystalline orientations of the noncollinear antiferromagnet with a stacked-kagome lattice structure. From this formulation, we show that, when the kagome planes are perpendicular to the sample film plane, the DMI serves as a uniaxial magnetic anisotropy for the antiferromagnetic order parameter. Our findings reveal an important physical manifestation of a DMI, shedding light on microscopic mechanisms of the magnetic anisotropy in noncollinear antiferromagnets.

論文

ナノ構造磁性体における創発インダクタンス

家田 淳一

日本磁気学会研究会資料, 250, p.1 - 5, 2024/10

近年スピントロニクスの効果を利用することで、らせん磁性金属薄膜がインダクタとして機能することが指摘された。従来のコイルインダクタの原理である電流誘起磁場による電磁誘導ではなく、磁化と電流の相互作用に基づくスピントルク(STT)とスピン起電力(SMF)の連続作用の結果として薄膜素子断面積に反比例する特徴的なインダクタンスがもたらされる。この仕組みは、提案者の永長により「創発インダクタ」(emergent inductor)と命名され、横内らによってらせん磁性体Gd$$_3$$Ru$$_4$$Al$$_{12}$$を用いた実験で実証された。本稿では、簡略化したモデルでその基礎的な振る舞いを確認したのち、当該研究におけるスピン軌道相互作用が果たす役割を中心にこれまでの研究動向を概観する。

論文

Chiral gauge field in fully spin-polarized magnetic Weyl semimetal with magnetic domain walls

小沢 耀弘*; 荒木 康史; 野村 健太郎*

Journal of the Physical Society of Japan, 93(9), p.094704_1 - 094704_9, 2024/09

 被引用回数:0 パーセンタイル:0.00(Physics, Multidisciplinary)

磁性ワイル半金属における磁化の変調は、運動量空間におけるワイル点位置のシフトを引き起こし、ワイルフェルミオンに対して実効的なカイラリティ依存のゲージ場として働く。本研究では、完全スピン偏極したワイル強磁性体Co$$_{3}$$Sn$$_{2}$$S$$_{2}$$において、このような磁化誘起カイラルゲージ場の効果を取り扱う。磁化と結合した積層カゴメ格子上で定義したCo$$_{3}$$Sn$$_{2}$$S$$_{2}$$の強束縛模型を用いて、運動量空間におけるワイル点の位置(カイラルゲージ場に相当)の磁化方向依存性を計算した。これを用いて、磁壁構造が存在する場合に、カイラルゲージ場の空間構造から生じるカイラル磁場を評価した。その結果磁壁存在下では、ワイルフェルミオンに対してランダウ量子化を強く引き起こすほどの、数百テスラという巨大なカイラル磁場が生じることが導出された。このような巨大カイラル磁場は、従来の磁性体スピントロニクスにおけるスピン起電力に相当する、磁壁の運動による電荷ポンピングを誘起することも予想される。

論文

スピン軌道相互作用による創発インダクタンス

家田 淳一; 荒木 康史; 山根 結太*

固体物理, 59(8), p.403 - 410, 2024/08

In recent years, "emergent inductors" using current-induced magnetization dynamics in magnetic nanostructures have been discovered, opening the way to power control in the nanoscale, which was previously impossible. We review the spin-orbit interaction phenomenon for emergent inductors.

論文

Room-temperature flexible manipulation of the quantum-metric structure in a topological chiral antiferromagnet

Han, J.*; 内村 友宏*; 荒木 康史; Yoon, J.-Y.*; 竹内 祐太郎*; 山根 結太*; 金井 駿*; 家田 淳一; 大野 英男*; 深見 俊輔*

Nature Physics, 20(7), p.1110 - 1117, 2024/07

 被引用回数:15 パーセンタイル:96.56(Physics, Multidisciplinary)

量子状態の幾何学的構造を特徴づける基礎的な量として、「量子計量」と「ベリー曲率」が存在する。ベリー曲率は、凝縮系において多種の重要な現象に寄与することが知られている。一方、量子計量も新たなトポロジカル物理現象の起源となることが予想されているが、特に常温常圧下においては、その効果はほとんど探索されていない。本研究では、トポロジカルカイラル反強磁性体Mn$$_{3}$$Snと白金の接合系を用い、界面でのナノスピン構造を介して、電子系の量子計量構造の制御に成功した。ベリー曲率ではなく量子計量特有の効果として、時間反転反対称でかつ電子散乱に対して頑強な、二次非線形ホール効果を測定した。更に、界面スピン構造は弱磁場及び界面スピン軌道相互作用によって急峻に変調されるため、量子計量構造も鋭敏に制御可能であることを示した。本研究成果により、量子状態に内在する量子計量構造を活用したトポロジカル物理現象が室温環境下でも可能になり、且つ応用面においても非線形素子を構築する助けとなることが期待される。

論文

Non-Hermitian Casimir effect of magnons

仲田 光樹; 鈴木 渓

npj Spintronics (Internet), 2, p.11_1 - 11_6, 2024/06

量子場の真空ゆらぎによって創発されるカシミア効果は、古典力学には対応物が存在しないという意味において、真に量子力学的な効果である。本研究では、従来の「散逸のないエルミート系」におけるマグノンカシミア効果を「散逸のある非エルミート系」に拡張する。そして「例外点に誘起される非エルミートカシミア振動」をはじめとする、従来のエルミート系にはない、非エルミート系に固有のマグノン・カシミア量子物性を明らかにする。本研究は、カシミア効果を制御・デザインする「カシミア・エンジニアリング」の基礎学理の構築に大きく貢献することが期待される。

論文

Tuning of spin-orbit coupling in chiral molecule-incorporated two-dimensional organic-inorganic hybrid perovskite copper halides with ferromagnetic exchange interactions

谷口 耕治*; Huang, P.-J.*; 佐賀山 基*; 鬼柳 亮嗣; 大石 一城*; 鬼頭 俊介*; 中村 唯我*; 宮坂 等*

Physical Review Materials (Internet), 8(2), p.024409_1 - 024409_10, 2024/02

 被引用回数:2 パーセンタイル:56.91(Materials Science, Multidisciplinary)

Leveraging the flexible material designability of organic-inorganic hybrid systems, spatial inversion symmetry breaking and spin-orbit coupling (SOC) were simultaneously controlled in a series of two-dimensional organic-inorganic hybrid perovskite (2D-OIHP) copper halides with ferromagnetic exchange interaction (FMI). In chiral molecule-incorporated 2D-OIHP copper halides, an increase in Br component over Cl component at halogen sites leads to systematic variations in magnetic phase diagrams owing to the competition between the FMI and Dzyaloshinskii-Moriya interaction induced by the SOC. The crucial role of noncentrosymmetry in the competition for the magnetic interactions was confirmed by comparing the magnetic phase diagrams of chiral and achiral 2D-OIHP copper bromides.

論文

Gyromagnetic bifurcation in a levitated ferromagnetic particle

佐藤 哲也*; 加藤 岳生*; 大上 能悟*; 松尾 衛

Physical Review B, 107(18), p.L180406_1 - L180406_6, 2023/05

 被引用回数:2 パーセンタイル:27.36(Materials Science, Multidisciplinary)

We examine the mechanical rotation of a levitated magnetic particle that is induced by ferromagnetic resonance under microwave irradiation. We show that two stable solutions appear in a certain range of parameters by bifurcation when the rotation frequency is comparable to the microwave frequency. This phenomenon originates from the coexistence of the Barnett and the Einstein-de Haas effects. We also reveal that this measurement is sensitive to the strength of the spin-rotation coupling. Our work provides a platform for accessing a microscopic relaxation process from spin to macroscopic rotation.

論文

Magnon dynamics in a Skyrmion-textured domain wall of antiferromagnets

Lee, S.*; 仲田 光樹; Tchernyshyov, O.*; Kim, S. K.*

Physical Review B, 107(18), p.184432_1 - 184432_12, 2023/05

 被引用回数:13 パーセンタイル:80.38(Materials Science, Multidisciplinary)

超対称量子力学に基づき、反強磁性スカーミオン構造を有する磁壁中のマグノンのトポロジカル量子輸送物性を明らかにする。スカーミオン型の磁気構造を有する磁壁中を伝搬するマグノンは、一種のゲージ場として作用する有効磁場を獲得する。そこで、この有効磁場中でのマグノンの反射・屈折現象を超対称量子力学に基づいて解析し、その伝搬および束縛マグノン状態を明らかにする。そして、ラウダウアー公式を用いて、磁壁のカイラリティが増加するにつれてマグノンによる熱流が減少することを明らかにする。本研究はスピンホール効果を活用した熱流の制御方法を理論的に提案する。

論文

Breaking down the magnonic Wiedemann-Franz law in the hydrodynamic regime

佐野 涼太郎*; 松尾 衛

Physical Review Letters, 130(16), p.166201_1 - 166201_7, 2023/04

 被引用回数:4 パーセンタイル:61.37(Physics, Multidisciplinary)

Recent experiments have shown an indication of a hydrodynamic magnon behavior in ultrapure ferromagnetic insulators; however, its direct observation is still lacking. Here, we derive a set of coupled hydrodynamic equations and study the thermal and spin conductivities for such a magnon fluid. We reveal the drastic breakdown of the magnonic Wiedemann-Franz law as a hallmark of the hydrodynamics regime, which will become key evidence for the experimental realization of an emergent hydrodynamic magnon behavior. Therefore, our results pave the way toward the direct observation of magnon fluids.

論文

Thermal stability of non-collinear antiferromagnetic Mn$$_3$$Sn nanodot

佐藤 佑磨*; 竹内 祐太郎*; 山根 結太*; Yoon, J.-Y.*; 金井 駿*; 家田 淳一; 大野 英男*; 深見 俊輔*

Applied Physics Letters, 122(12), p.122404_1 - 122404_5, 2023/03

 被引用回数:5 パーセンタイル:58.52(Physics, Applied)

$$D0_{19}$$-Mn$$_3$$Sn, an antiferromagnet having a non-collinear spin structure in a kagome lattice, has attracted great attention owing to various intriguing properties such as large anomalous Hall effect. Stability of magnetic state against thermal fluctuation, characterized in general by the thermal stability factor $$Delta$$, has been well studied in ferromagnetic systems but not for antiferromagnets. Here we study $$Delta$$ of the antiferromagnetic Mn$$_3$$Sn nanodots as a function of their diameter $$D$$. To obtain $$Delta$$, we measure the switching probability as a function of pulse-field amplitude and analyze the results based on a model developed by accounting for two and six-fold magnetic anisotropies in the kagome plane. We observe no significant change in $$Delta$$ down to $$D = 300$$ nm below which it decreases with $$D$$. The obtained $$D$$ dependence is well explained by a single-domain and nucleation-mediated reversal models. These findings provide a basis to understand the thermal fluctuation and reversal mechanism of antiferromagnets for device application.

論文

Magnonic Casimir effect in ferrimagnets

仲田 光樹; 鈴木 渓

Physical Review Letters, 130(9), p.096702_1 - 096702_6, 2023/03

 被引用回数:11 パーセンタイル:85.32(Physics, Multidisciplinary)

量子場の真空ゆらぎによって創発されるカシミア効果は、古典力学には対応物が存在しないという意味において真に量子力学的な効果である。しかし、カシミア効果はこれまでフォトン(光子)を舞台に研究されており、磁性体中でのカシミア効果、特にそのカシミアエネルギーの膜厚依存性については十分な理解は得られていない。そこで本研究では格子場の理論の観点から、磁性絶縁体中のスピン波を量子化したマグノンに着目し、マグノン量子場により創発されるカシミア効果「マグノン・カシミア効果」及びその膜厚依存性を明らかにする。更に反強磁性絶縁体だけでなくフェリ磁性絶縁体(例:YIG)においてもマグノン・カシミア効果が創発することを示し、スピントロニクス分野で中心的な役割を担うYIGがカシミア効果の工学的応用を目指すカシミアエンジニアリング分野にとっても絶好の舞台であることを明らかにする。本研究は、マグノン・カシミアエンジニアリングの基礎学理の構築に大きく貢献することが期待される。

論文

Two-dimensional quantum universality in the spin-1/2 triangular-lattice quantum antiferromagnet Na$$_{2}$$BaCo(PO$$_{4}$$)$$_{2}$$

Sheng, J.*; Wang, L.*; Candini, A.*; Jiang, W.*; Huang, L.*; Xi, B.*; Zhao, J.*; Ge, H.*; Zhao, N.*; Fu, Y.*; et al.

Proceedings of the National Academy of Sciences of the United States of America, 119(51), p.e2211193119_1 - e2211193119_9, 2022/12

 被引用回数:30 パーセンタイル:93.24(Multidisciplinary Sciences)

Although considerable progress has been made in the theoretical understanding of the low-dimensional frustrated quantum magnets, experimental realizations of a well-established scaling analysis are still scarce. This is particularly true for the two-dimensional antiferromagnetic triangular lattices. Owing to the small exchange strength, the newly discovered compound Na$$_{2}$$BaCo(PO$$_{4}$$)$$_{2}$$ provides a rare opportunity for clarifying the quantum criticality in an ideal triangular lattice with quantum spin S=1/2. In addition to the establishment of the complete phase diagrams, the spin Hamiltonian with a negligible interplane interaction has been determined through the spin wave dispersion in the polarized state, which is consistent with the observation of a two-dimensional quantum critical point with the Bose-Einstein condensation of diluted free bosons.

論文

Observation of domain structure in non-collinear antiferromagnetic Mn$$_3$$Sn thin films by magneto-optical Kerr effect

内村 友宏*; Yoon, J.-Y.*; 佐藤 佑磨*; 竹内 祐太郎*; 金井 駿*; 武智 涼太*; 岸 桂輔*; 山根 結太*; DuttaGupta, S.*; 家田 淳一; et al.

Applied Physics Letters, 120(17), p.172405_1 - 172405_5, 2022/04

 被引用回数:24 パーセンタイル:88.93(Physics, Applied)

We perform a hysteresis-loop measurement and domain imaging for $$(1100)$$-oriented $$D0_{19}$$-Mn$$_{3+x}$$Sn$$_{1-x}$$ $$(-0.11 le x le 0.14)$$ thin films using magneto-optical Kerr effect (MOKE) and compare it with the anomalous Hall effect (AHE) measurement. We obtain a large Kerr rotation angle of 10 mdeg., comparable with bulk single-crystal Mn$$_3$$Sn. The composition $$x$$ dependence of AHE and MOKE shows a similar trend, suggesting the same origin, i.e., the non-vanishing Berry curvature in the momentum space. Magnetic domain observation at the saturated state shows that x dependence of AHE and MOKE is explained by an amount of reversible area that crucially depends on the crystalline structure of the film. Furthermore, in-depth observation of the reversal process reveals that the reversal starts with nucleation of sub-micrometer-scale domains dispersed in the film, followed by a domain expansion, where the domain wall preferentially propagates along the $$[11bar{2}0]$$ direction. Our study provides a basic understanding of the spatial evolution of the reversal of chiral-spin structure in non-collinear antiferromagnetic thin films.

論文

Mn L$$_{2,3}$$-edge EXAFS and magnetic EXAFS studies on the halfmetallic ferromagnet Co$$_{2}$$MnSi

向後 純也*; 藤原 秀紀*; 関山 明*; 斎藤 祐児; 梅津 理恵*; 二木 かおり*

Journal of the Physical Society of Japan, 91(3), p.034702_1 - 034702_12, 2022/03

 被引用回数:0 パーセンタイル:0.00(Physics, Multidisciplinary)

We report magnetic circular dichroism in extended X-ray absorption fine structure (EXAFS) in a prototypical halfmetallic ferromagnet, Co$$_{2}$$MnSi. The EXAFS oscillations at the Mn L$$_{2,3}$$ edges are analyzed to obtain parameters used in the analysis of the magnetic EXAFS (MEXAFS). Theoretical calculations of MEXAFS spectra in Co$$_{2}$$MnSi show that the linear-path scatterings have larger contributions than the multiple triangular-path scatterings. Furthermore, the period of the oscillations in the MEXAFS spectra is shorter than that in the EXAFS spectra indicating that the far site contributions from the second to the fourth nearest neighbor Co and the third nearest Si atoms can strongly influence the MEXAFS oscillations, while the Mn atoms, despite the large magnetic moment, can have little contributions due to the interference of the spin components.

論文

Magnetic sensitivity distribution of Hall devices in antiferromagnetic switching experiments

Schreiber, F.*; Meer, H.*; Schmitt, C.*; Ramos, R.*; 齊藤 英治; Baldrati, L.*; Kl$"a$ui, M.*

Physical Review Applied (Internet), 16(6), p.064023_1 - 064023_9, 2021/12

 被引用回数:4 パーセンタイル:24.33(Physics, Applied)

We analyze the complex impact of the local magnetic spin texture on the transverse Hall-type voltage in device structures utilized to measure magnetoresistance effects. We find a highly localized and asymmetric magnetic sensitivity in the eight-terminal geometries that are frequently used in current-induced switching experiments, for instance, to probe antiferromagnetic materials. Using current-induced switching of antiferromagnetic NiO/Pt as an example, we estimate the change in the spin Hall magnetoresistance signal associated with switching events based on the domain-switching patterns observed via direct imaging. This estimate correlates with the actual electrical data after subtraction of a nonmagnetic contribution. Here, the consistency of the correlation across three measurement geometries with fundamentally different switching patterns strongly indicates a magnetic origin of the measured and analyzed electrical signals.

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